Development of the read-out system for the quantum mechanical amplitude and phase information using the frequency and time resolved spectroscopy

• Project/Area Number: 19684014
• Research Category: Grant-in-Aid for Young Scientists (A)
• Allocation Type: Single-year Grants
• Research Field: 原子・分子・量子エレクトロニクス・プラズマ
• Research Institution: Institute for Molecular Science
• Principal Investigator: KATSUKI Hiroyuki Institute for Molecular Science, 光分子科学研究領域, 助教 (10390642)
• Project Period (FY): 2007 – 2009
• Project Status: Completed (Fiscal Year 2009)
• Budget Amount: ¥20,800,000 (Direct Cost: ¥16,000,000、Indirect Cost: ¥4,800,000); Fiscal Year 2009: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000); Fiscal Year 2008: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000); Fiscal Year 2007: ¥11,700,000 (Direct Cost: ¥9,000,000、Indirect Cost: ¥2,700,000)
• Keywords: コヒーレント制御 / 超高速分光 / 量子干渉 / フェムト秒分光法 / 波束ダイナミクス / パルス波形整形

Research Abstract

I have succeeded to prepare the experimental setup for the wave packet interferometry experiment within the low temperature solid para-hydrogen crystal. The phase-stabilized double pulses of 600nm and 800nm fs laser pulses were prepared by a home-built Michelson interferometer. The dynamics of the created wave packets were probed by another fs probe pulse. The frequency resolved signal was detected by a CCD detector. We observed an extraordinary long lifetime of the signal fringe contrast, more than 60% even after 500ps from the initial wave packet preparation.

Research Products

• [Journal Article] Wave Packet Interferometry with Attosecond Precision and Picometric Structure (2010)
  • Author(s): H. Katsuki, et al, 他4名
  • Journal Title: Phys. Chem. Chem. Phys 12 Pages: 5189-5198
  • Peer Reviewed
• [Journal Article] Actively tailored spatiotemporal images of quantum interference on the picometer and femtosecond scales (2009)
  • Author(s): H. Katsuki, et al, 他4名
  • Journal Title: Phys. Rev. Lett. 102 Pages: 103602-103602
  • Peer Reviewed
• [Journal Article] アト秒精度の分子波束干渉制御 (2009)
  • Author(s): 香月浩之
  • Journal Title: 応用物理 78 Pages: 136-140
  • NAID: 10024750777
  • Peer Reviewed
• [Journal Article] Actively tailored spatiotemporal images of quantum interference on the picometer and femtosecond scales (2009)
  • Author(s): H. Katsuki, et.al.
  • Journal Title: Physical Review Letters 102
  • Peer Reviewed
• [Journal Article] アト秒精度の波束干渉制御 (2008)
  • Author(s): 香月浩之, 大森賢治
  • Journal Title: レーザー研究 36 Pages: 31-36
  • NAID: 10020128980
  • Peer Reviewed
• [Journal Article] READ and WRITE Amplitude and Phase Information by Using High-Precision Molecular Wave-Packet Interferometry (2007)
  • Author(s): H. Katsuki, et al, 他3名
  • Journal Title: Phys. Rev. A 76 Pages: 13403-13403
  • Peer Reviewed
• [Journal Article] Read and write amplitude and phase information by using high-precision molecular wave-packet interferometry (2007)
  • Author(s): H. Katsuki, et. al.
  • Journal Title: Physical Review A 76
  • Peer Reviewed
• [Journal Article] Wave Packet Interferometry with Attosecond Precision and Picometric Structure
  • Author(s): H.Katsuki, et al.
  • Journal Title: Phys.Chem.Chem.Phys. (in press)
  • Peer Reviewed
• [Presentation] 分子振動波束制御の基礎と応用 (2010)
  • Author(s): 香月浩之
  • Organizer: 2009年度宇宙空間原子分子過程研究会「原子衝突におけるコヒーレント相互作用」
  • Place of Presentation: JAXA宇宙科学研究本部, 相模原
  • Year and Date: 2010-03-01
• [Presentation] 分子波束干渉制御の基礎と応用 (2010)
  • Author(s): 香月浩之
  • Organizer: 2009年度宇宙空間原子分子過程研究会「原子衝突におけるコヒーレント相互作用」
  • Place of Presentation: JAXA宇宙科学研究本部相模原キャンパス(神奈川県)
  • Year and Date: 2010-03-01
• [Presentation] Wave Packet Interferometry in Solid Parahydrogen (2009)
  • Author(s): 香月浩之, et al.
  • Organizer: JST/CREST第4回量子情報ワークショップ
  • Place of Presentation: リゾーピア熱海(静岡県)
  • Year and Date: 2009-12-08
• [Presentation] 固体パラ水素中での分子波束干渉制御 (2009)
  • Author(s): 香月浩之, 千葉寿, 大森賢治
  • Organizer: 第3回分子科学討論会
  • Place of Presentation: 名古屋大学東山キャンパス
  • Year and Date: 2009-09-21
• [Presentation] 固体パラ水素中での分子波束干渉制御 (2009)
  • Author(s): 香月浩之, et al.
  • Organizer: 第3回分子科学討論会
  • Place of Presentation: 名古屋大学(愛知県)
  • Year and Date: 2009-09-21
• [Presentation] Wave packet interferometry in a bulk solid hydrogen (2009)
  • Author(s): H. Katsuki, H. Chiba, K. Ohmori
  • Organizer: Gordon Research Conference (Quantum control of light & matter)
  • Place of Presentation: Mount Holyoke College, South Hadley, MA
  • Year and Date: 2009-08-03
• [Presentation] Wave packet interferometry in a bulk solid parahydrogen (2009)
  • Author(s): 香月浩之, et al.
  • Organizer: Gordon research conference, Quantum Control Of Light & Matter
  • Place of Presentation: Mount Holyoke College South Hadley, MA, USA
  • Year and Date: 2009-08-03
• [Presentation] 高強度赤外パルスを用いた波束干渉制御～デコヒーレンスのモデル研究 (2009)
  • Author(s): 香月浩之, 後藤悠, 千葉寿, 大森賢治
  • Place of Presentation: 日本化学会第89春季年会@日本大学船橋キャンパス
  • Year and Date: 2009-03-28
• [Presentation] 高強度赤外パルスを用いた波束干渉制御〜デコヒーレンスのモデル研究 (2009)
  • Author(s): 香月浩之, 他3名
  • Organizer: 日本化学会第89春季年会
  • Place of Presentation: 日本大学理工学部船橋キャンパス
  • Year and Date: 2009-03-28
• [Presentation] 高強度近赤外レーザー光による振動波束のコヒーレンス制御 (2008)
  • Author(s): 香月浩之, 後藤悠, J.C. Delagnes, 千葉寿, 大森賢治
  • Organizer: エクストリームフォトニクスシンポジウム
  • Place of Presentation: 竹島, 蒲郡
  • Year and Date: 2008-11-11
• [Presentation] 高強度近赤外フェムト秒パルスを用いた分子振動波束の振幅位相制御 (2008)
  • Author(s): 香月浩之, 後藤悠, J.C. Delagnes, 千葉寿, 大森賢治
  • Organizer: 第2回分子科学討論会
  • Place of Presentation: 福岡国際会議場
  • Year and Date: 2008-09-25
• [Presentation] Influence of Strong Laser Pulses on the Amplitudes and Phases of Vibrational Wave Packets; Model Study of Decoherence(Invited) (2008)
  • Author(s): H. Katsuki
  • Organizer: 5th Asian Conference on Ultrafast Phenomena
  • Place of Presentation: National Univ. Singapore
  • Year and Date: 2008-01-08
• [Presentation] Influence of Strong Laser Pulses on the Amplitudes and Phases of Vibrational Wave Packets; Model Study of Decoherence (2008)
  • Author(s): Hiroyuki Katsuki
  • Organizer: 5th Asian Conference on Ultrafast Phenomena
  • Place of Presentation: National university of Singapore
  • Year and Date: 2008-01-04
• [Presentation] アト秒精度の波束干渉を用いた振動波束の制御と観測 (2007)
  • Author(s): 香月浩之
  • Organizer: 日本分光学会先端レーザー分光部会
  • Place of Presentation: 東京大学、本郷
  • Year and Date: 2007-12-07
• [Presentation] アト秒精度の波束干渉を用いた振動波束の制御と観測(Invited) (2007)
  • Author(s): 香月浩之
  • Organizer: 日本分光学会先端レーザー分光部分
  • Place of Presentation: 東京大学(本郷)
  • Year and Date: 2007-12-07
• [Presentation] アト秒精度の波束干渉を用いた振動波束の制御と観測 (2007)
  • Author(s): 香月浩之
  • Organizer: 物性研短期研究会「短波長コヒーレント光と物質中のコヒーレンスの生成・消滅」
  • Place of Presentation: 東大物性研、柏
  • Year and Date: 2007-11-27
• [Presentation] Influence of Strong Laser Pulses on the Amplitudes and Phases of Vibrational Wave Packets; Model Study of Decoherence (2007)
  • Author(s): H. Katsuki, H. goto, J.C. Delagnes, H. Chiba, K. Ohmori
  • Organizer: 6th International Symposium on Ultrafast Intense Laser Science Green Park Resort
  • Place of Presentation: Pisa, Italy
  • Year and Date: 2007-09-27
• [Presentation] 高強度フェムト秒レーザーパルスを用いた波束操作 (2007)
  • Author(s): 香月浩之, 後藤悠, J.C. Delagnes, 千葉寿, 大森賢治
  • Organizer: 第1回分子科学討論会
  • Place of Presentation: 仙台, 東北大学
  • Year and Date: 2007-09-17
• [Presentation] 高強度フェムト秒レーザーパルスを用いた波束操作(ポスター発表) (2007)
  • Author(s): 香月浩之, 他4名
  • Organizer: 第1回分子科学討論会
  • Place of Presentation: 東北大学
  • Year and Date: 2007-09-17
• [Presentation] Visualizing and Controlling Picometric Quantum Ripples in Molecules (2007)
  • Author(s): H. Katsuki, K. Ohmori
  • Organizer: 2007 CLEO Pacific Rim
  • Place of Presentation: seoul, Korea
  • Year and Date: 2007-08-27
• [Presentation] Visualizing and Controlling Picometric Quantum Ripples in Molecules(Invited) (2007)
  • Author(s): H. Katsuki, K. Ohmori
  • Organizer: 2007 CLEO Pacific Rim
  • Place of Presentation: Seoul, Korea
  • Year and Date: 2007-08-27
• [Presentation] 光分子科学の最前線と将来 (2007)
  • Author(s): Hiroyuki Katsuki
  • Organizer: 第12回日韓分子科学合同シンポジウム
  • Place of Presentation: Jejudo, Korea
  • Year and Date: 2007-07-06
• [Presentation] Visualizing and Controlling Ultrafast Vibrational Wave-Packet Interference (2007)
  • Author(s): Hiroyuki Katsuki
  • Organizer: 11th East Asian Workshop on Chemical Dynamics
  • Place of Presentation: Tokyo University of Science, Japan
  • Year and Date: 2007-05-08
• [Presentation] Visualizing and Controlling Ultrafast Vibrational Wave-Packet Interference(Invited) (2007)
  • Author(s): H. Katsuki
  • Organizer: 11th East Asian Workshop on Chemical Dynamics
  • Place of Presentation: Tokyo University of Science, Japan
  • Year and Date: 2007-05-08
• [Remarks] 第三回PCCP賞受賞(2009年)
  • URL: http://groups.ims.ac.jp/organization/ohmori_g/
• [Remarks]
  • URL: http://www.ims.ac.jp/info/2008/090317_2.html
• [Remarks]
  • URL: http://www.ims.ac.jp/topics/2007/080228.html