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Design of high selective catalytic reactor and elucidation of reaction mechanism by precise diffusion control in micro space.

Research Project

Project/Area Number 19686047
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Reaction engineering/Process system
Research InstitutionKyoto University

Principal Investigator

MAKI Taisuke  Kyoto University, 地球環境学堂, 准教授 (10293987)

Project Period (FY) 2007 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥24,570,000 (Direct Cost: ¥18,900,000、Indirect Cost: ¥5,670,000)
Fiscal Year 2009: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2008: ¥8,060,000 (Direct Cost: ¥6,200,000、Indirect Cost: ¥1,860,000)
Fiscal Year 2007: ¥12,480,000 (Direct Cost: ¥9,600,000、Indirect Cost: ¥2,880,000)
Keywords新規反応場 / マイクロ化学プロセス / マイクロリアクター / ラマン分光法 / 赤外分光法 / 触媒反応器 / 反応速度論 / メタノール分解反応
Research Abstract

It is clarified that the microreactor is preferable over the packed-bed reactor in aspects of the concentration distribution of the reactants in the microspace, the distibution of temperature and active species on a catalyst. On the basis of the knowledge obtained, some methods for intentionally control of the concentration distribution in microspace were proposed.

Report

(4 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (24 results)

All 2010 2009 2008 2007 Other

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (16 results) Remarks (2 results)

  • [Journal Article] Enhancing reaction selectivity by intentional control of concentration profile in catalytic microreactor2010

    • Author(s)
      Shinji Kudo, Taisuke Maki, Hiroyuki Kono, Kazuhiro Mae
    • Journal Title

      Journal of Chemical Engineering of Japan 43

      Pages: 63-69

    • NAID

      10027152371

    • Related Report
      2009 Annual Research Report 2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Efficient Hydrogen Production from Methanol by Combining Micro Channel with Carbon Membrane Catalyst Loaded with Cu/Zn2009

    • Author(s)
      Shinji Kudo, Taisuke Maki, Noriyuki Kitao, Kazuhiro Mae
    • Journal Title

      Journal of Chemical Engineering of Japan 42

      Pages: 680-686

    • NAID

      10028156094

    • Related Report
      2009 Annual Research Report 2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Precise control of polymer particle properties using droplets in the microchannel2009

    • Author(s)
      Y.Okubo, T.Maki, F.Nakanishi, T.Hayashi, K.Mae
    • Journal Title

      Chemical Engineering Science 65

      Pages: 386-391

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Liquid-liquid extraction for efficient synthesis and separation by utilizing micro spaces.2008

    • Author(s)
      Yoshihito Okubo, Taisuke Maki,; Nobuaki Aoki, Khoo Teng Hong
    • Journal Title

      Chemical Engineering Science 63

      Pages: 4070-4077

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Process intensification by utilizing micro space2008

    • Author(s)
      Mae, K., Maki, T., Aoki, N.
    • Journal Title

      Kagaku Kogaku Ronbunshu 34

      Pages: 8-17

    • NAID

      10020122899

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A new micromixer with needle adjustment for instant mixing and heating under high pressure and high temperature2007

    • Author(s)
      Mae, K., Suzuki, A., Maki, T., Hakuta, Y., Sato, H., Arai, K.
    • Journal Title

      Journal of Chemical Engineering of Japan 40

      Pages: 1101-1107

    • NAID

      130000019089

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Presentation] Particle Size Control of Nanoparticles by a Multistage Reaction System with Series of Micromixers2010

    • Author(s)
      Tomoya Wada, Taisuke Maki, Kazuhiro Mae
    • Organizer
      The 11th International Conference on Microreaction Technology
    • Place of Presentation
      京都リサーチパーク(京都市)
    • Year and Date
      2010-03-09
    • Related Report
      2009 Annual Research Report
  • [Presentation] マイクロリアクターを用いたナノ粒子の制御と反応モデルの検討2009

    • Author(s)
      和田知也, 牧泰輔, 前一廣
    • Organizer
      第2回化学工学3支部合同北九州大会
    • Place of Presentation
      西日本総合展示場(北九州市)
    • Year and Date
      2009-10-31
    • Related Report
      2009 Annual Research Report
  • [Presentation] 多孔質FeOOHのイオン吸着特性に対する細孔構造の影響と吸着メカニズムの検討2009

    • Author(s)
      伊藤雅浩, 牧泰輔, 前一廣
    • Organizer
      第2回化学工学3支部合同北九州大会
    • Place of Presentation
      西日本総合展示場(北九州市)
    • Year and Date
      2009-10-31
    • Related Report
      2009 Annual Research Report
  • [Presentation] マイクロリアクターを用いた触媒反応場の設計(展望講演)2009

    • Author(s)
      牧泰輔
    • Organizer
      化学工学会第41秋季大会
    • Place of Presentation
      広島大学(東広島市)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Final Research Report
  • [Presentation] 金/酸化鉄触媒の低温還元処理に伴う担体構造変化とCO変性反応の活性評価2009

    • Author(s)
      福田貴史, 工藤真二, 牧泰輔, 前一廣
    • Organizer
      化学工学会第41回秋季大会
    • Place of Presentation
      広島大学(東広島市)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Annual Research Report
  • [Presentation] マイクロリアクターを用いた触媒反応場の設計(展望講演)2009

    • Author(s)
      牧泰輔
    • Organizer
      化学工学会第41回秋季大会
    • Place of Presentation
      広島大学(東広島市)
    • Year and Date
      2009-09-16
    • Related Report
      2009 Annual Research Report
  • [Presentation] Water-gas shift reaction by Au/ferric oxide catalyst2009

    • Author(s)
      Shinji Kudo, Taisuke Maki, Takashi Fukuda, Kazuhiro Mae
    • Organizer
      8th World Congress of Chemical Engineering
    • Place of Presentation
      Montreal, CANADA
    • Year and Date
      2009-08-26
    • Related Report
      2009 Annual Research Report
  • [Presentation] Ft-irを用いた多孔質FeOOH吸着剤の水素結合評価とイオン吸着形態の検討2009

    • Author(s)
      牧泰輔, 堀口彰太, 前一廣
    • Organizer
      化学工学会第74年会
    • Place of Presentation
      横浜
    • Year and Date
      2009-03-18
    • Related Report
      2008 Annual Research Report
  • [Presentation] Control of Reaction Selectivity by designing Concentration Profile in Catalytic Microreactor2008

    • Author(s)
      Shinji Kudo, Taisuke Maki, Hiroyuki Kono, Kazuhiro Mae
    • Organizer
      International Workshop on Process Intensification 2008 (IWPI 2008)
    • Place of Presentation
      東京
    • Year and Date
      2008-11-17
    • Related Report
      2008 Annual Research Report
  • [Presentation] アセンブル型触媒マイクロリアクターを用いた水蒸気改質・CO除去2008

    • Author(s)
      牧泰輔
    • Organizer
      触媒反応工学部会若手会第3回講演会
    • Place of Presentation
      仙台
    • Year and Date
      2008-09-23
    • Related Report
      2008 Annual Research Report
  • [Presentation] Particle size control of Au nanoparticles by a multistage reaction system with series of micromixers2008

    • Author(s)
      Taisuke Maki
    • Organizer
      International Symposium on Micro Chemical Process and Synthesis
    • Place of Presentation
      Kyoto Terrsa(Kyoto)
    • Year and Date
      2008-09-12
    • Related Report
      2009 Final Research Report
  • [Presentation] Particle size control of Au nanoparticles by a multistage reaction system with series of micromixers2008

    • Author(s)
      Taisuke Maki, Tomoya Wada, Kazuhiro Mae
    • Organizer
      International Symposium on Micro Chemical Process and Synthesis(MIPS2008)
    • Place of Presentation
      京都
    • Year and Date
      2008-09-12
    • Related Report
      2008 Annual Research Report
  • [Presentation] A new preparation method of Au/fellic oxide catalyst for low temperature CO oxidation2008

    • Author(s)
      Shinji Kudo, Atsushi Inada, Taisuke Maki, Masahiro Yamada
    • Organizer
      The 20th International Symposium on Chemical Reaction Engineering (ISCRE20)
    • Place of Presentation
      京都
    • Year and Date
      2008-09-08
    • Related Report
      2008 Annual Research Report
  • [Presentation] A new methodology for independent control of the molecular weight and particle diameter of polymers2008

    • Author(s)
      Yoshihito Okubo, Taisuke Maki, Fumito Nakanishi, Tatsuya Hayashi
    • Organizer
      The 20th International Symposium on Chemical Reaction Engineering (ISCRE20)
    • Place of Presentation
      京都
    • Year and Date
      2008-09-08
    • Related Report
      2008 Annual Research Report
  • [Presentation] Steam Reforming of Dimethyl Ether by Use of Catalyst Mixture of Cu/Zn Loaded Carbon Catalyst and γ-Al2O32007

    • Author(s)
      S. Kudo, T. Maki and K. Mae
    • Organizer
      2007 AIChE Annual Meeting
    • Place of Presentation
      Salt Lake City (USA)
    • Year and Date
      2007-11-08
    • Related Report
      2007 Annual Research Report
  • [Presentation] Production Of Zirconia Nanoparticles Using A Microreactor With Same Axle Dual Pipe2007

    • Author(s)
      T. Maki, J. Kitada and K. Mae
    • Organizer
      2007 AIChE Annual Meeting
    • Place of Presentation
      Salt Lake City (USA)
    • Year and Date
      2007-11-06
    • Related Report
      2007 Annual Research Report
  • [Remarks]

    • URL

      http://www.cheme.kyoto-u.ac.jp/8koza/micro-results.html

    • Related Report
      2009 Final Research Report
  • [Remarks]

    • URL

      http://www.cheme.kyoto-u.ac.jp/8koza/micro-results.html

    • Related Report
      2009 Annual Research Report

URL: 

Published: 2007-04-01   Modified: 2023-01-13  

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