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Study of Magnetic Field Induced Electronic Phase Transitions by X-ray scattering with Pulsed Fields and XFELs

Research Project

Project/Area Number 19H00647
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Review Section Medium-sized Section 13:Condensed matter physics and related fields
Research InstitutionTohoku University

Principal Investigator

NOJIRI HIROYUKI  東北大学, 金属材料研究所, 教授 (80189399)

Co-Investigator(Kenkyū-buntansha) 桑原 慶太郎  茨城大学, 理工学研究科(理学野), 教授 (90315747)
Project Period (FY) 2019-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥44,980,000 (Direct Cost: ¥34,600,000、Indirect Cost: ¥10,380,000)
Fiscal Year 2022: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2021: ¥14,300,000 (Direct Cost: ¥11,000,000、Indirect Cost: ¥3,300,000)
Fiscal Year 2020: ¥14,820,000 (Direct Cost: ¥11,400,000、Indirect Cost: ¥3,420,000)
Fiscal Year 2019: ¥10,400,000 (Direct Cost: ¥8,000,000、Indirect Cost: ¥2,400,000)
Keywords強磁場 / X線自由電子レーザー / 電子相転移 / X線散乱 / 極端条件 / X線自由電子レーザー / X線散乱 / 超強磁場 / 磁場誘起相転移 / 超伝導
Outline of Research at the Start

熱揺らぎを抑制した超低温における強磁場誘起相転移では, 本質的に量子ゆらぎが相転移を支配し, 強電子相関により電子状態が激変する電子相転移が引き起こされる. そこでは, 物質のもつ多自由度相関により対称性の破れが支配され, しばしば非自明な秩序状態が現れる. 強磁場下で全ての電子が押し込められ, 身動き出来ずせめぎ合う時に, “多体電子系がどのように対称性を破り, 秩序化するのか?”は, 物性研究の核心であり, 電子相転移の普遍性と多様性の理解は物質科学の最重要な課題の1つである. 本研究では, 未踏の70T 超領域の超強磁場XFEL 散乱手法を開拓し, 電子相転移の研究へ応用する.

Outline of Final Research Achievements

We have established an X-ray diffraction method with high accuracy and high sensitivity under ultra-low temperature and ultra-strong magnetic field. This made it possible to determine structural changes in magnetic field-induced phase transitions without thermal broadening. Using this, we clarified the commonalities between magnetic field-induced charge density waves in yttrium-based high-temperature superconductors and lanthanum-based high-temperature superconductors, and obtained results that strongly suggest the existence of a underlying universal electronic state. Furthermore, in semimetal graphite, we found that the density-wave transition associated with the one-dimensionalization of the electron system under an ultra-strong magnetic field is accompanied by non-monotonic modulation of the lattice, indicating the possibility of locking the modulation wavenumber with the lattice.

Academic Significance and Societal Importance of the Research Achievements

強磁場は電子の運動とスピンに大きな影響を与え、新しい状態が強磁場下で誘起されることは、多くの物質で見出されてきた。そのような新しい電子相の理解には、電子構造、とりわけ、結晶格子と結合したバンド構造の周期性や対称性の変化をX線で直接決定することが欠かせない。そのような実験はこれまで困難であったが、本研究によって、小型パルス磁場発生装置とX線自由電子レーザーを組みあわせた手法が確立した。これにより、強磁場中の電子状態の理解が格段に進展することが期待される。このような学術的な進展は、磁場による物質制御法の開拓とそれを用いた機能性材料の開発などに役立てられることが期待される。

Report

(6 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Annual Research Report
  • 2020 Annual Research Report
  • 2019 Comments on the Screening Results   Annual Research Report
  • Research Products

    (27 results)

All 2023 2022 2021 2020 2019 Other

All Int'l Joint Research (12 results) Journal Article (6 results) (of which Int'l Joint Research: 5 results,  Peer Reviewed: 6 results,  Open Access: 3 results) Presentation (9 results) (of which Int'l Joint Research: 5 results,  Invited: 4 results)

  • [Int'l Joint Research] SLAC National Accelerator Laboratory(米国)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] POSTECH(韓国)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] SLAC National Accelerator Laboratory(米国)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] POSTECH(韓国)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] Stanford国立研究所/Stanford大学/Rice大学(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Postec-PAL(韓国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] PSI/チューリッヒ大学(スイス)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] ヘルムホルツ研究機構ベルリン/マックスプランク固体物理研究所/ヘルムホルツ研究機構ドレスデン(ドイツ)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Stanford 国立研究所/Stanford大学/Rice大学(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] PSI/チューリッヒ大学(スイス)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] ヘルムホルツ研究機構ベルリン/マックスプランク固体物理研究所(ドイツ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Postech-PAL(韓国)

    • Related Report
      2019 Annual Research Report
  • [Journal Article] Enhanced charge density wave with mobile superconducting vortices in La1.885Sr0.115CuO42023

    • Author(s)
      Wen J.-J.、He W.、Jang H.、Nojiri H.、Matsuzawa S.、Song S.、Chollet M.、Zhu D.、Liu Y.-J.、Fujita M.、Jiang J. M.、Rotundu C. R.、Kao C.-C.、Jiang H.-C.、Lee J.-S.、Lee Y. S.
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 733-733

    • DOI

      10.1038/s41467-023-36203-x

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Automated Pulsed Magnet System for Neutron Diffraction Experiments at the Materials and Life Science Experimental Facility in J-PARC2023

    • Author(s)
      Watanabe, M, Kihara, T, Nojiri, H
    • Journal Title

      QUANTUM BEAM SCIENCE

      Volume: 7 Issue: 1 Pages: 1-1

    • DOI

      10.3390/qubs7010001

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Characterization of photoinduced normal state through charge density wave in superconducting YBa2Cu3O6.672022

    • Author(s)
      Hoyoung Jang 他16名 Hiroyuki Nojiri他4名
    • Journal Title

      SCIENCE ADVANCES

      Volume: 8 Issue: 6

    • DOI

      10.1126/sciadv.abk0832

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Element-specific field-induced spin reorientation and tetracritical point in MnCr2S42021

    • Author(s)
      Yamamoto, S: Suwa, H: Kihara, T: Nomura, T: Kotani, Y: Nakamura: Skourski, Y: Zherlitsyn, S: Prodan, L: Tsurkan, V: Nojiri, H: Loidl, A: Wosnitza, J
    • Journal Title

      PHYSICAL REVIEW B

      Volume: 103 Issue: 2

    • DOI

      10.1103/physrevb.103.l020408

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Successive Phase Transitions in R3Ir4Sn13 (R: La and Ce) Investigated Using Neutron and X-ray Diffraction2020

    • Author(s)
      Seiya Nakazato, Kazuaki Iwasa,, Daisuke Hashimoto, Mami Shiozawa, Keitaro Kuwahara, Hironori Nakao, Hajime Sagayama, Motoyuki Ishikado, Takashi Ohhara, Akiko Nakao, Koji Munakata, and Ryoji Kiyanagi
    • Journal Title

      JPS Conf. Proc.

      Volume: 30

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Terahertz Faraday and Kerr Rotation Spectroscopy of Bi1-xSbx Films in High Magnetic Fields up to 30 Tesla2019

    • Author(s)
      X. Li, K. Yoshioka, M. Xie, T. Hagiwara, G. T. Noe II, W. Lee, N. Marquez Peraca, W. Gao, T. Hagiwara, H. S. Orjan, L-W. Nien, T. Nagao, M. Kitajima, H. Nojiri, X. Li, C-K. Shih, A. H. MacDonald, I. Katayama, J. Takeda, G. A. Fiete, and J. Kono
    • Journal Title

      Phys. Rev. B

      Volume: 100 Issue: 11 Pages: 115145-115145

    • DOI

      10.1103/physrevb.100.115145

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] High Magnetic Field X-ray Experiments with XFEL and Synchrotron Radiation2022

    • Author(s)
      Hiroyuki Nojiri
    • Organizer
      15th Asia-Pacific Physics Conference
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] X-ray diffractions and spectroscopies in low reduced temperatures2022

    • Author(s)
      Hiroyuki Nojiri
    • Organizer
      Sciences in Cornell High Magnetic Field Beam Line
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 超強磁場X線回折装置の開発と酸化物超伝導体への応用2021

    • Author(s)
      野尻浩之
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2021 Annual Research Report 2020 Annual Research Report
  • [Presentation] X-ray and high magnetic fieldsProbing extreme states of correlated electrons systems2021

    • Author(s)
      Hiroyuki Nojiri
    • Organizer
      Symposium on the Helmholtz International Beamline for Extreme Fields at the European XFEL
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Applications to Magnetic Field Induced Phase Transitions-2021

    • Author(s)
      Hiroyuki Nojiri
    • Organizer
      SACLA User Meeting 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 近藤半金属物質Ce3Ir4Sn13における逐次相転移2020

    • Author(s)
      中里晟也, 岩佐和晃, 橋本大輔, 塩澤真未, 桑原慶太郎, 中尾裕則, 佐賀山基, 石角元志, 大原高志, 中尾朗子, 宗像孝司C, 鬼柳亮嗣, F. Damay, J.-M. Mignot
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] XFELを利用した超強磁場X線回折による磁場誘起相転移の探索2019

    • Author(s)
      野尻浩之
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Progress in High Magnetic Field XFEL Experiments2019

    • Author(s)
      H. Nojiri
    • Organizer
      14Th ASIA-PACIFIC PHYSICS CONFERENCE
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Successive phase transitions in R3Ir4Sn13 (R: La and Ce) investigated using neutron and X-ray diffraction2019

    • Author(s)
      Seiya Nakazato, Kazuaki Iwasa, Daisuke Hashimoto, Mami Shiozawa, Keitaro Kuwahara, Hironori Nakao, Hajime Sagayama, Motoyuki Ishikado, Takashi Ohhara, Akiko Nakao, Koji Munakata, and Ryoji Kiyanagi
    • Organizer
      International Conference on Strongly Correlated Electron Systems 2019
    • Related Report
      2019 Annual Research Report

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Published: 2019-04-18   Modified: 2024-01-30  

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