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Investigation of strong-field optoelectronics in solids

Research Project

Project/Area Number 19H02623
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 30020:Optical engineering and photon science-related
Research InstitutionNational Institutes for Quantum Science and Technology

Principal Investigator

Ishii Nobuhisa  国立研究開発法人量子科学技術研究開発機構, 関西光科学研究所 光量子科学研究部, 主幹研究員 (40586898)

Co-Investigator(Kenkyū-buntansha) 篠原 康  日本電信電話株式会社NTT物性科学基礎研究所, フロンティア機能物性研究部, リサーチスペシャリスト (90775024)
Project Period (FY) 2019-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥17,680,000 (Direct Cost: ¥13,600,000、Indirect Cost: ¥4,080,000)
Fiscal Year 2021: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2020: ¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2019: ¥9,230,000 (Direct Cost: ¥7,100,000、Indirect Cost: ¥2,130,000)
Keywords超高速レーザー / 高強度レーザー / 高強度場物理 / 高次高調波発生 / 半導体ブロッホ方程式 / 第一原理計算 / 高強度レーザー開発 / 高強度場物理計算 / 紫外線 / 軟X線 / 中赤外光源 / 赤外レーザー開発 / 高強度物理 / 超高速光科学 / 高強度場科学 / 限界駆動固体物性
Outline of Research at the Start

強電界下における固体内の電子のダイナミクスを実験的に計測する。実験結果に基づき、アト秒やフェムト秒の時間スケールでの電子のダイナミクスを記述可能な、理論的なモデリングとシミュレーション手法の構築を試みる。実験的アプローチとして、高強度赤外フェムト秒光源とサブサイクルプローブ光を同期させた実験系を開発し、強電界下(10 MV/cm程度)の固体における電子波束ダイナミクスを計測する。理論的なアプローチとして、半導体ブロッホ方程式に基づくモデル計算や時間依存する第一原理計算等の枠組みを構築し、実験結果を踏まえた電子の超高速ダイナミクスのシミュレーションを行う。

Outline of Final Research Achievements

Optical parametric amplifiers pumped by high-power Yb-based lasers were developed at a central wavelength of 3000 nm. These light sources have a function to generate visible-to-near-infrared ultrashort laser pulses, that can be synchronized with the long-wavelength light sources, enabling experiments such as sub-cycle and up-conversion spectroscopy.
High harmonic generation processes from organic-inorganic hybrid perovskite were investigated theoretically. From this investigation, we obtained the first result that resolves the contribution to high harmonic generation from multiple electron orbitals explicitly. The analytical method revealed that the main contribution of high harmonic generation comes from a valence band that is different from a conduction band thought to dominate the process historically.
In addition, the high harmonic spectra dependent on the time constant of the decay of the electron orbital were investigated.

Academic Significance and Societal Importance of the Research Achievements

長波長の高出力レーザー光源開発は、電波を用いる5Gの通信に続く、ポスト(ビヨンド)5Gの通信(6G)を担うために必要不可欠なものである。またアイセーフレーザー、長距離ライダー、ソフトマテリアルの非熱加工など、これから主眼になってくるであろう研究テーマを先取りし、世界に先駆けたレーザー光源開発となる成果を上げている。
また次世代太陽電池候補と考えられている有機無機ハイブリッドペロブスカイトのMAPbCl3結晶からの高次高調波発生過程の理論的研究によって、光とペロブスカイトの相互作用における素過程の研究開発への第一歩となり、エネルギー問題を解決するような成果につながると確信している。

Report

(4 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • Research Products

    (35 results)

All 2022 2021 2020 2019

All Journal Article (16 results) (of which Int'l Joint Research: 7 results,  Peer Reviewed: 16 results,  Open Access: 13 results) Presentation (19 results) (of which Int'l Joint Research: 6 results,  Invited: 5 results)

  • [Journal Article] Atomic real-space perspective of light-field-driven currents in graphene2022

    • Author(s)
      Morimoto Yuya、Shinohara Yasushi、Ishikawa Kenichi L、Hommelhoff Peter
    • Journal Title

      New Journal of Physics

      Volume: 24 Issue: 3 Pages: 033051-033051

    • DOI

      10.1088/1367-2630/ac5c18

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Generation and compression of an intense infrared white light continuum in YAG irradiated by picosecond pulses2021

    • Author(s)
      Ishii Nobuhisa、Maruyama Momoko、Nagashima Keisuke、Ochi Yoshihiro、Itakura Ryuji
    • Journal Title

      Optics Express

      Volume: 29 Issue: 11 Pages: 17069-17076

    • DOI

      10.1364/oe.423671

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Broadband operation of a synchronously pumped optical parametric oscillator with a spatially dispersed beam2021

    • Author(s)
      Nagashima Keisuke、Itakura Ryuji、Ishii Nobuhisa
    • Journal Title

      Optics Letters

      Volume: 46 Issue: 17 Pages: 4414-4417

    • DOI

      10.1364/ol.435039

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-harmonic generation in GaAs beyond the perturbative regime2021

    • Author(s)
      Peiyu Xia, Tomohiro Tamaya, Changsu Kim, Faming Lu, Teruto Kanai, Nobuhisa Ishii, Jiro Itatani, Hidefumi Akiyama, and Takeo Kato
    • Journal Title

      Physical Review B

      Volume: 104 Issue: 12

    • DOI

      10.1103/physrevb.104.l121202

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Generation of wavelength-tunable few-cycle pulses in the mid-infrared at repetition rates up to 10 kHz2021

    • Author(s)
      Sanari Yasuyuki、Sekiguchi Fumiya、Nakagawa Kotaro、Ishii Nobuhisa、Kanemitsu Yoshihiko、Hirori Hideki
    • Journal Title

      Optics Letters

      Volume: 46 Issue: 20 Pages: 5280-5283

    • DOI

      10.1364/ol.440228

    • NAID

      120007181736

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Attosecond electronic dynamics of core-excited states of N2O in the soft x-ray region2021

    • Author(s)
      Nariyuki Saito, Nicolas Douguet, Hiroki Sannohe, Nobuhisa Ishii, Teruto Kanai, Yi Wu, Andrew Chew, Seunghwoi Han, Barry I. Schneider, Jeppe Olsen, Luca Argenti, Zenghu Chang, and Jiro Itatani
    • Journal Title

      Phys. Rev. Res.

      Volume: 3 Issue: 4 Pages: 043222-043222

    • DOI

      10.1103/physrevresearch.3.043222

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Semiclassical description of electron dynamics in extended systems under intense laser fields2021

    • Author(s)
      Tani Mizuki、Otobe Tomohito、Shinohara Yasushi、Ishikawa Kenichi L.
    • Journal Title

      Physical Review B

      Volume: 104 Issue: 7 Pages: 075157-075157

    • DOI

      10.1103/physrevb.104.075157

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Asymmetric single-cycle control of valence electron motion in polar chemical bonds2021

    • Author(s)
      Morimoto Yuya、Shinohara Yasushi、Tani Mizuki、Chen Bo-Han、Ishikawa Kenichi L.、Baum Peter
    • Journal Title

      Optica

      Volume: 8 Issue: 3 Pages: 382-382

    • DOI

      10.1364/optica.414213

    • Related Report
      2021 Annual Research Report 2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Detecting electron-phonon coupling during photoinduced phase transition2021

    • Author(s)
      Suzuki Takeshi、Shinohara Yasushi、Lu Yangfan、Watanabe Mari、Xu Jiadi、Ishikawa Kenichi L.、Takagi Hide、Nohara Minoru、Katayama Naoyuki、Sawa Hiroshi、Fujisawa Masami、Kanai Teruto、Itatani Jiro、Mizokawa Takashi、Shin Shik、Okazaki Kozo
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 12 Pages: 1-10

    • DOI

      10.1103/physrevb.103.l121105

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Time-domain spectroscopy of optical parametric amplification for phase-stable terahertz-to-midinfrared pulses2021

    • Author(s)
      Natsuki Kanda, Nobuhisa Ishii, Jiro Itatani, Ryusuke Matsunaga
    • Journal Title

      arXiv:2005.03538

      Volume: 2005 Issue: 3 Pages: 03538-03538

    • DOI

      10.1364/oe.413200

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Role of virtual band population for high harmonic generation in solids2020

    • Author(s)
      Sanari Yasuyuki、Hirori Hideki、Aharen Tomoko、Tahara Hirokazu、Shinohara Yasushi、Ishikawa Kenichi L.、Otobe Tomohito、Xia Peiyu、Ishii Nobuhisa、Itatani Jiro、Sato Shunsuke A.、Kanemitsu Yoshihiko
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 4 Pages: 041125-041125

    • DOI

      10.1103/physrevb.102.041125

    • NAID

      120006876570

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] High-order harmonic generation from hybrid organic-inorganic perovskite thin films2019

    • Author(s)
      Hirori Hideki、Xia Peiyu、Shinohara Yasushi、Otobe Tomohito、Sanari Yasuyuki、Tahara Hirokazu、Ishii Nobuhisa、Itatani Jiro、Ishikawa Kenichi L.、Aharen Tomoko、Ozaki Masashi、Wakamiya Atsushi、Kanemitsu Yoshihiko
    • Journal Title

      APL Materials

      Volume: 7 Issue: 4 Pages: 041107-041107

    • DOI

      10.1063/1.5090935

    • NAID

      120006712768

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Optical parametric amplification of carrier-envelope phase-stabilized mid-infrared pulses generated by intra-pulse difference frequency generation2019

    • Author(s)
      Ishii Nobuhisa, Xia Peiyu, Kanai Teruto, Itatani Jiro
    • Journal Title

      Optics Express

      Volume: 27 Issue: 8 Pages: 11447-11447

    • DOI

      10.1364/oe.27.011447

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ultrafast Unbalanced Electron Distributions in Quasicrystalline 30° Twisted Bilayer Graphene2019

    • Author(s)
      Takeshi Suzuki*, Takushi Iimori, Sung Joon Ahn, Yuhao Zhao, Mari Watanabe, Jiadi Xu, Masami Fujisawa, Teruto Kanai, Nobuhisa Ishii, Jiro Itatani, Kento Suwa, Hirokazu Fukidome, Satoru Tanaka, Joung Real Ahn, Kozo Okazaki, Shik Shin, Fumio Komori*, Iwao Matsuda*
    • Journal Title

      ACS Nano

      Volume: 13 Issue: 10 Pages: 11981-11987

    • DOI

      10.1021/acsnano.9b06091

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Resonant-Like Field Enhancement by Nanoscale Grating-Coupled Propagating Surface Plasmons and Localized Surface Plasmons in the Mid-Infrared Range: Implications for Ultrafast Plasmonic Electron Sources2019

    • Author(s)
      Mizuno Tomoya、Takeuchi Kengo、Kaneshima Keisuke、Ishii Nobuhisa、Kanai Teruto、Itatani Jiro
    • Journal Title

      ACS Applied Nano Materials

      Volume: 2 Issue: 11 Pages: 7067-7073

    • DOI

      10.1021/acsanm.9b01597

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Real-time observation of electronic, vibrational, and rotational dynamics in nitric oxide with attosecond soft x-ray pulses at 400 eV2019

    • Author(s)
      Saito Nariyuki、Sannohe Hiroki、Ishii Nobuhisa、Kanai Teruto、Kosugi Nobuhiro、Wu Yi、Chew Andrew、Han Seunghwoi、Chang Zenghu、Itatani Jiro
    • Journal Title

      Optica

      Volume: 6 Issue: 12 Pages: 1542-1546

    • DOI

      10.1364/optica.6.001542

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Ybレーザーを用いた高強度極短赤外光源フロントエンド開発2022

    • Author(s)
      石井 順久、圓山 桃子、永島 圭介、越智 義浩、板倉 隆二
    • Organizer
      第69回応用物理学会春季学術講演会
    • Related Report
      2021 Annual Research Report
  • [Presentation] ピコ秒光源を用いた高強度赤外フェムト秒白色光発生とそのパルス圧縮2022

    • Author(s)
      石井 順久、圓山 桃子、永島 圭介、越智 義浩、板倉 隆二
    • Organizer
      レーザー学会学術講演会第42回年次大会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 極性固体中価電子の非対称単一サイクルコントロール2021

    • Author(s)
      森本裕也、篠原康、谷水城、 Bo-Han Chen、 石川顕一、Peter Baum
    • Organizer
      日本物理学会 2021年秋季大会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 線形偏光電場による高次高調波角度依存性の時空間対称性による記述2021

    • Author(s)
      篠原康、今坂光太郎、 芦原聡、 石川顕一
    • Organizer
      日本物理学会 2021年秋季大会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 直線偏光電場に対する高調波の角度依存性の時空間対称性による記述2021

    • Author(s)
      篠原康、今坂光太郎、芦原聡、石川顕一
    • Organizer
      第82回応用物理学会秋季学術講演会
    • Related Report
      2021 Annual Research Report
  • [Presentation] Yb:YAGレーザー励起赤外光パラメトリック増幅器開発2021

    • Author(s)
      石井 順久
    • Organizer
      4th RIKEN-RAP and QST-KPSI Joint Seminar
    • Related Report
      2020 Annual Research Report
  • [Presentation] 軟X線吸収分光による環状分子の光開環ダイナミクスの研究2020

    • Author(s)
      栗本 悠太郎、齋藤 成之、石井 順久、金井 輝人、板谷 治郎、斉田 謙一郎、武次 徹也、関川 太郎
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ハーフサイクルカットオフ近傍の光電子収量と断熱理論を用いた後方弾性散乱断面積の導出とその定量性評価2020

    • Author(s)
      水野 智也、楊 添淇、石井 順久、金井 輝人、Tolstikhin Oleg I、森下 亨、板谷 治郎
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] レーザー軟X線光源の進展とフェムト秒吸収分光への応用2020

    • Author(s)
      石井 順久
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Theoretical study on nonlinear optical absorption of crystalline solids via two-color laser from first-principles2020

    • Author(s)
      Kakeru Sasaki, Yasushi Shinohara, Kenichi L. Ishikawa
    • Organizer
      ICALEO 2020
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] A microscopic thery for selection rules of solid-state high-harmonic generation based on time-dependent Schrodinger equation2020

    • Author(s)
      Yasushi Shinohara
    • Organizer
      High-brightness Sources and Light-driven Interactions Congress
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] レーザー軟X線パルス源によるフェムト秒吸収分光2020

    • Author(s)
      石井 順久、齋藤 成之、板谷 治郎
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] High Harmonic Generation in Reflection and Transmission from Gallium Arsenide2019

    • Author(s)
      Nobuhisa Ishii, Peiyu Xia, Changsu Kim, Faming Lu, Teruto Kanai, Hidefumi Akiyama, and Jiro Itatani
    • Organizer
      Conference on Lasers and Electro-Optics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 高周波テラヘルツ帯における光パラメトリック増幅2019

    • Author(s)
      神田 夏輝、石井 順久、板谷 治郎、松永 隆佑
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 中赤外極短パルスの強電場下における固体のサブサイクル分光2019

    • Author(s)
      7.夏 沛宇、Faming Lu、石井 順久、金井 輝人、板谷 治郎
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Optical parametric amplification of CEP-locked mid-infrared pulses produced by intra-pulse difference frequency generation using multiple plate pulse compression2019

    • Author(s)
      N. Ishii, P. Xia, T. Kanai, and J. Itatani,
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Real-time ab-initio simulations for crystalline solids driven by strong laser pulse2019

    • Author(s)
      Yasushi Shinohara
    • Organizer
      The 22nd Asian Workshop on First-Principles Electronic Structure Calculations
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Theoretical study on solid-state high harmonic generation: from a one-dimensional model to an ab-initio three-dimensional approach2019

    • Author(s)
      Yasushi Shinohara
    • Organizer
      Mini-Workshop on Nonlinear Response in Laser-Matter Interaction
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Selection rules and nonlinear propagation in HHG from solids2019

    • Author(s)
      Nobuhisa Ishii
    • Organizer
      Mini-Workshop on Nonlinear Response in Laser-Matter Interaction
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2019-04-18   Modified: 2023-01-30  

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