• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Investigation of hierarchy and dimensionality on acoustic modes via inelastic X-ray scattering

Research Project

Project/Area Number 19H04408
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 80040:Quantum beam science-related
Research InstitutionJapan Synchrotron Radiation Research Institute

Principal Investigator

Tsutsui Satoshi  公益財団法人高輝度光科学研究センター, 回折・散乱推進室, 主幹研究員 (70360823)

Co-Investigator(Kenkyū-buntansha) 金子 耕士  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力科学研究所 物質科学研究センター, 研究主幹 (30370381)
久保野 敦史  静岡大学, 工学部, 教授 (70234507)
Project Period (FY) 2019-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥12,350,000 (Direct Cost: ¥9,500,000、Indirect Cost: ¥2,850,000)
Fiscal Year 2022: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2021: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Fiscal Year 2020: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Fiscal Year 2019: ¥5,330,000 (Direct Cost: ¥4,100,000、Indirect Cost: ¥1,230,000)
Keywords固体物理 / 量子ビーム / 相補利用 / 機能性材料 / 強相関電子系 / X線非弾性散乱 / 中性子非弾性散乱 / 微視的弾性率 / 運動量・周波数空間での階層性 / 非弾性散乱 / 物質の機能発現における階層性 / 量子臨界性 / 原子ダイナミクス / 量子相転移 / 液晶相転移 / 放射光メスバウアー分光 / 物質機能発現の階層構造 / 量子ビーム利用 / 物質機能の階層性 / 量子臨界現象 / ネマティック秩序 / 強弾性転移 / 液晶
Outline of Research at the Start

音響フォノンは物質の硬さや熱伝導度と密接に関わっている。一方で、音響フォノンが観測される周波数領域がその物質の硬さや熱伝導度という機能発現の大きさと1対1対応にある。このため、物質に特有な現象が音響フォノンに現れるときには、その特異現象が観測される周波数領域によって、その機能発現に特徴的な大きさを理解する事ができる。本研究では、超伝導などと密接に関わる絶対温度ゼロ度で定義される相転移現象や結晶と液体の中間の性質を持つ液晶の音響フォノンを調べることで、物質中の諸物性に関わる機能発現に特徴的な大きさの理解を目指す。

Outline of Final Research Achievements

The complementary use and/or combination between inelastic X-ray scattering and other experimental techniques, which had been planned on the application submission of this project, enabled us to deepen our understanding hierarchy in the functional manifestation of materials. In the field of strongly correlated electron systems and thermoelectric materials, we succeeded in deepening our understanding of hierarchy., which was the goal of this project. In the field of strongly correlated electron systems, we succeeded in establishing a temporal hierarchy method for valence fluctuations, although we could not reach the knowledge of dimensionality. In the field of thermoelectric materials, we were not able to establish an understanding of hierarchy, but we were able to obtain knowledge that leads to an understanding of the hierarchy of functional expression.

Academic Significance and Societal Importance of the Research Achievements

本研究は、強相関系における価数揺動等の現象観測を通じて固体物理における時間的階層構造のための手法の確立に貢献した。加えて、熱電材料分野のフォノン分散の観測を通じて、性能指数向上に必要な格子熱伝導率の低減機構に関わるフォノン励起の観測に成功した。また、その観測に基づく機能発現機構の解明に向けた知見を明らかにすることができた。

Report

(5 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Annual Research Report
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • Research Products

    (49 results)

All 2023 2022 2021 2020 2019 Other

All Int'l Joint Research (13 results) Journal Article (17 results) (of which Int'l Joint Research: 5 results,  Peer Reviewed: 17 results,  Open Access: 6 results) Presentation (19 results) (of which Int'l Joint Research: 7 results,  Invited: 4 results)

  • [Int'l Joint Research] Max-Planck-Institut(ドイツ)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] Cavendish Laboratory/ISIS Facility(英国)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] Julich Centre for Neutron Science JCNS/Institut Laue Langevin(フランス)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] University of Johannesburg(南アフリカ)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] Polish Academy of Sciences(ポーランド)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] The Chinese University of Hong Kong(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Graz University of Technology(オーストリア)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Oak Ridge National Laboratory(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] the Max Planck Institute(ドイツ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Institut Laue Langevin(フランス)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Charles University(チェコ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Rutherford Appleton Laboratory(英国)

    • Related Report
      2019 Annual Research Report
  • [Journal Article] In-situ Analysis of Organic Semiconductor Thin Film Growth by Quartz Crystal Microbalance and Grazing Incidence X-Ray Diffraction2023

    • Author(s)
      松原 亮介、久保野 敦史
    • Volume
      J106-C
    • Issue
      4
    • Pages
      147-153
    • DOI

      10.14923/transelej.2022JCI0024

    • ISSN
      1881-0217
    • Year and Date
      2023-04-01
    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Investigation of the phonon dispersion associated with superlattice reflections in the BiS2-based superconductor LaBiS2O0.5F0.52023

    • Author(s)
      Tamatsukuri Hiromu、Hasegawa Takumi、Sagayama Hajime、Mizumaki Masaichiro、Murakami Youichi、Kajitani Joe、Higashinaka Ryuji、Matsuda Tatsuma D.、Aoki Yuji、Tsutsui Satoshi
    • Journal Title

      Physical Review B

      Volume: 107 Issue: 2

    • DOI

      10.1103/physrevb.107.024303

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Cluster Toroidal Multipoles Formed by Electric-Quadrupole and Magnetic-Octupole Trimers: A Possible Scenario for Hidden Orders in Ca5Ir3O122023

    • Author(s)
      Hayami Satoru、Tsutsui Satoshi、Hanate Hiroki、Nagasawa Nobumoto、Yoda Yoshitaka、Matsuhira Kazuyuki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 92 Issue: 3 Pages: 033702-033702

    • DOI

      10.7566/jpsj.92.033702

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effect of incident molecular temperature on the elementary processes in thin film growth of long-chain molecules during vacuum deposition2023

    • Author(s)
      Matsubara Ryosuke、Hagihara Kiyoshi、Kubono Atsushi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 62 Issue: 1 Pages: 010907-010907

    • DOI

      10.35848/1347-4065/acb11c

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Phonon Softening in Lu(Pt1-xPdx)2In Close to a Zero-Temperature Structural Instability2022

    • Author(s)
      Gruner T.、Lucas S.、Geibel C.、Kaneko K.、Tsutsui S.、Schmalzl K.、Stockert O.
    • Journal Title

      Physical Review B

      Volume: 106 Issue: 11 Pages: 115142-115142

    • DOI

      10.1103/physrevb.106.115142

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Multigap Superconductivity in the Filled-Skutterudite Compound LaRu4As122022

    • Author(s)
      Bhattacharyya A.、Adroja D. T.、Koza M. M.、Tsutsui S.、Cichorek T.、Hillier A. D.
    • Journal Title

      Physical Review B

      Volume: 106 Issue: 13

    • DOI

      10.1103/physrevb.106.134516

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] First Observation of Superlattice Reflections in the Hidden Order at 105 K of Spin?Orbit Coupled Iridium Oxide Ca<sub>5</sub>Ir<sub>3</sub>O<sub>12</sub>2021

    • Author(s)
      Hanate Hiroki、Hasegawa Takumi、Hayami Satoru、Tsutsui Satoshi、Kawano Shoya、Matsuhira Kazuyuki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 6 Pages: 063702-063702

    • DOI

      10.7566/jpsj.90.063702

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 193Ir Synchrotron-Radiation-Based Mossbauer Spectroscopy for Ir Valence Disproportionation in Ca5Ir3O122021

    • Author(s)
      Tsutsui Satoshi、Hanate Hiroki、Yoda Yoshitaka、Matsuhira Kazuyuki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 8 Pages: 083701-083701

    • DOI

      10.7566/jpsj.90.083701

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Application of synchrotron-radiation-based Mossbauer spectroscopy to 193Ir 73?keV transition2021

    • Author(s)
      Tsutsui Satoshi、Hanate Hiroki、Yoda Yoshitaka、Masuda Ryo、Matsuhira Kazuyuki
    • Journal Title

      Hyperfine Interactions

      Volume: 242 Issue: 1

    • DOI

      10.1007/s10751-021-01743-5

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Sm valence determination of Sm-based Intermetallics using 149Sm Mossbauer and Sm LIII-edge X-ray absorption spectroscopies2021

    • Author(s)
      Tsutsui Satoshi、Higashinaka Ryuji、Nakamura Raito、Fujiwara Kosuke、Nakamura Jin、Kobayashi Yoshio、Ito Takashi U.、Yoda Yoshitaka、Kato Kazuo、Nitta Kiyofumi、Kawamura Naomi、Mizumaki Masaichiro、Matsuda Tatsuma D.、Aoki Yuji
    • Journal Title

      Hyperfine Interactions

      Volume: 242 Issue: 1 Pages: 32-32

    • DOI

      10.1007/s10751-021-01759-x

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Rare-Earth Atomic Motion in RBe13 (R: La, Pr, Sm)2020

    • Author(s)
      Tsutsui Satoshi、Shimizu Yusei、Hidaka Hiroyuki、Koriki Akinari、Murata Ryoya、Yoda Yoshitaka、Yanagisawa Tatsuya、Amitsuka Hiroshi
    • Journal Title

      JPS Conference Proceedings

      Volume: 30 Pages: 0111151-6

    • DOI

      10.7566/jpscp.30.011115

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Nature of Structural Instabilities in Superconducting Sr3Ir4Sn132020

    • Author(s)
      Kaneko Koji、Cheung Yiu Wing、Hu Yajian、Imai Masaki、Tanioku Yasuaki、Kanagawa Hibiki、Murakawa Joichi、Moriyama Kodai、Zhang Wei、Lai Kwing To、Matsuda Masaaki、Yoshimura Kazuyoshi、Tsutsui Satoshi、Goh Swee Kuan
    • Journal Title

      JPS Conf. Proc.

      Volume: 30 Pages: 011032-011032

    • DOI

      10.7566/jpscp.30.011032

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] "Study of Phonon Dispersion of Iridium Oxide Ca5Ir3O12 with Strong Spin?Orbit Interaction"2020

    • Author(s)
      "Hiroki Hanate, Takumi Hasegawa, Satoshi Tsutsui, Kazuma Nakamura, Yoshihide Yoshimoto, Naohiro Kishigami, Sho Haneta, and Kazuyuki Matsuhira"
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 5 Pages: 053601-053601

    • DOI

      10.7566/jpsj.89.053601

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Evolution of microstructure and variations in mechanical properties accompanied with diffusionless isothermal ω transformation in β-titanium alloys2020

    • Author(s)
      N.L. Okamoto, S. Kasatani, M. Luckabauer, R. Enzinger, S. Tsutsui, M. Tane, T. Ichitsubo
    • Journal Title

      Physical Review Materials

      Volume: 4 Issue: 12 Pages: 123603-123603

    • DOI

      10.1103/physrevmaterials.4.123603

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Lattice instability coupled with valence degrees of freedom in valence fluctuation compound YbPd2020

    • Author(s)
      Tsutsui Satoshi、Hasegawa Takumi、Mitsuda Akihiro、Sugishima Masaki、Oyama Kohei、Mizumaki Masaichiro、Ogita Norio、Wada Hirofumi、Udagawa Masayuki
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 24 Pages: 245150-245150

    • DOI

      10.1103/physrevb.102.245150

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Isotropic Parallel Antiferromagnetism in the Magnetic-Field-Induced Charge-Ordered State of SmRu4P12 caused by p-f hybridization2020

    • Author(s)
      T. Matsumura, S. Michimura, T. Inami, C. H. Lee, M. Matsuda, H. Nakao, M. Mizumaki, N. Kawamura, M. Tsukagoshi, S. Tsutsui, H. Sugawara, K. Fushiya, T. D. Matsuda, R. Higashinaka, and Y. Aoki
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 21 Pages: 214444-214444

    • DOI

      10.1103/physrevb.102.214444

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Electronic and atomic dynamics in Sm and Eu cage-structured intermetallics2019

    • Author(s)
      Tsutsui Satoshi、Mizumaki Masaichiro、Kobayashi Yoshio
    • Journal Title

      Hyperfine Interactions

      Volume: 240 Issue: 1

    • DOI

      10.1007/s10751-019-1634-3

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] CrMNFeCoNIとCrCoNiのX線・中性子非弾性散乱2022

    • Author(s)
      筒井智嗣、飯田一樹、梶本亮一、Mohamad Qayyum bin Mohamad Izlan、下原諒大、清水崚雅、中野希一、脇本明拓、寺本武司、松浦直人、田中克志
    • Organizer
      日本金属学会2022秋季大会
    • Related Report
      2022 Annual Research Report
  • [Presentation] 液晶蒸着薄膜における凝集構造の蒸着速度依存性2022

    • Author(s)
      水野拓海, 松原亮介, 久保野敦史
    • Organizer
      2022年日本液晶学会討論会
    • Related Report
      2022 Annual Research Report
  • [Presentation] 液晶蒸着薄膜における凝集構造の蒸着速度依存性2022

    • Author(s)
      水野拓海, 松原亮介, 久保野敦史
    • Organizer
      第83回応用物理学会秋季学術講演会
    • Related Report
      2022 Annual Research Report
  • [Presentation] CrMnFeCoNiのフォノン分散2022

    • Author(s)
      筒井智嗣、飯田一樹、梶本亮一、寺本武司、松浦直人、J. Du、尾方成信、田中克志
    • Organizer
      日本金属学会2023年春季大会
    • Related Report
      2022 Annual Research Report
  • [Presentation] 高エントロピー合金のX線・中性子非弾性散乱2022

    • Author(s)
      筒井智嗣、飯田一樹、梶本亮一、松浦直人、寺本武司、Mohamad Qayyumbin Mohamad Izlan、下原諒大、田中克志
    • Organizer
      日本物理学会第76回年会
    • Related Report
      2021 Annual Research Report
  • [Presentation] Application of Synchrotron-Radiation-Based Mossbauer Spectroscopy to 193Ir 73 KeV Transition2021

    • Author(s)
      S. Tsutsui, H. Hanate, Y. Yoda, and K. Matsuhira
    • Organizer
      International Conference on the Application of the Mossbauer Effect
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sm Valence Determination of Sm-Based Intermetallics using 149Sm Mossbauer and Sm LIII-edge X-ray Absorption Spectroscopies2021

    • Author(s)
      S. Tsutsui, R. Higashinaka, R. Nakamura, K. Fujiwara, J. Nakamura, Y. Kobayashi, T. U. Ito, Y. Yoda, K. Kato, K. Nitta, M. Mizumaki, T. D. Matsuda, and Y. Aoki
    • Organizer
      International Conference on the Application of the Mossbauer Effect
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 放射光実験の横断利用による原子ダイナミクスの研究2021

    • Author(s)
      筒井智嗣
    • Organizer
      第7回 大型実験施設とスーパーコンピュータとの連携シンポジウム
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Ca5Ir3O12の193Ir放射光メスバウアー分光2021

    • Author(s)
      筒井智嗣、花手洋樹、依田芳卓、松平和之
    • Organizer
      日本物理学会第75回年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Microscopic Mechanism of Thermal Insulation in Si-Ge and Heavy-Element-Doped Heusler Alloys2020

    • Author(s)
      S. Tsutsui
    • Organizer
      The 5th International Symposium of Quantum Beam Science at Ibaraki University
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] RAl2 (R = La, Ce, Pr, Nd, Dy)のX線非弾性散乱2020

    • Author(s)
      筒井智嗣、金子耕士、Alfred Baron、海老原孝雄
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Electronic and Atomic Dynamics in Sm and Eu Cage-Structured Intermetallic2019

    • Author(s)
      S. Tsutsui
    • Organizer
      Mediterranean Conference on the Applications of the Mossbauer Effect
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 核共鳴非弾性散乱法の薄膜試料への応用2019

    • Author(s)
      筒井智嗣
    • Organizer
      フォノンエンジニアリング研究グループ 第3回研究会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Magnetic Properties and Lattica Dynamics in Type-I Clathrate Eu8Ga16Ge30 through 151Eu Mossbauer Effect and Magnetic Circular Dichroism2019

    • Author(s)
      S. Tsutsui, Y. Kobayashi, M. Mizumaki, N. Kawamura, M. K. Kubo, Y. Yoda, T. Onimaru, M. A. Avila, and T. Takabatake
    • Organizer
      International Conference on the Application of the Mossbauer Effect
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Rare-Earth Atomic Motion in RBe13 (R: rare-earth)2019

    • Author(s)
      S. Tsutsui, Y. Shimizu, H. Hidaka, A. Kohriki, R. Murata, Y. Yoda, T. Yanagisawa, and H. Amitsuka
    • Organizer
      International Conference on Strongly Correlated Electron Systems
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Application of nuclear resonant inelastic scattering to thin films2019

    • Author(s)
      Satoshi Tsutsui
    • Organizer
      PCOS(相変化研究会)2019
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] In-situ viscoelasticity measurement in the formation of vapor-deposited thin liquid crystal films2019

    • Author(s)
      Ryota TAKAHASHI, Ryosuke MATSUBARA, and Atsushi KUBONO
    • Organizer
      10th International Conference on Molecular Electrnoics and Bioelectronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 液晶蒸着薄膜形成過程におけるin-situ粘弾性解析2019

    • Author(s)
      高橋亮太、松原亮介、久保野敦史
    • Organizer
      2019年日本液晶学会討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 蒸着法により作製した液晶薄膜形成過程における粘弾性変化2019

    • Author(s)
      高橋亮太、松原亮介、久保野敦史
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report

URL: 

Published: 2019-04-18   Modified: 2024-01-30  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi