Charge-fluctuation mechansim of high-temperature superconductivity in cuprates using resonant inelastic x-ray scattering
Project/Area Number |
19K03741
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Research Category |
Grant-in-Aid for Scientific Research (C)
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Allocation Type | Multi-year Fund |
Section | 一般 |
Review Section |
Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
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Research Institution | The University of Tokyo (2022) Waseda University (2019-2021) |
Principal Investigator |
Fujimori Atsushi 東京大学, 大学院理学系研究科(理学部), 名誉教授 (10209108)
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Co-Investigator(Kenkyū-buntansha) |
溝川 貴司 早稲田大学, 理工学術院, 教授 (90251397)
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Project Period (FY) |
2019-04-01 – 2023-03-31
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Project Status |
Completed (Fiscal Year 2022)
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Budget Amount *help |
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2021: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2020: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2019: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
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Keywords | 高温超伝導体 / 共鳴軟X線非弾性散乱 / 角度分解光電子分光 / 高温超伝導 / 非弾性X線散乱 |
Outline of Research at the Start |
銅酸化物における高温超伝導の発見以来30年以上の間、膨大な研究が行われてきたにもかかわらず高温超伝導の発現機構は未だ解明されていない。従来型超伝導体で確立してきた電子-フォノン相互作用機構では高い超伝導転移温度を説明することが困難なため、磁気的ゆらぎによる超伝導機構がされ活発に研究されてきた。一方、電荷ゆらぎによる超伝導機構は具体的な理論研究が少なく、実験的な検証はさらに遅れている。本研究では、高輝度放射光を用いた共鳴軟X線散乱実験により電荷ゆらぎのダイナミクスを直接観測し、高温超伝導発現における電荷ゆらぎの重要性を明らかにする。
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Outline of Final Research Achievements |
Charge order, charge excitation, and phonon anomalies in cuprate high-temperature superconductors were studied by resonant inelastic x-ray scattering, and new insights into the superconductivity mechanism and the nature of the enigmatic pseudogap were obtained. Critical charge fluctuations and phonon anomalies associated with the quantum phase transition between the pseudogap phase and the Fermi-liquid phase were identified in the low-energy region near the charge-order peak. At higher energies, spectral changes in the exciton peak between the pseudogap phase and the superconducting phase were observed as predicted by the excitonic charge-fluctuation mechanism of superconductivity. At even higher energies, “acoustic plasmon”, a collective charge excitation of two-dimensional electron system was first observed in hole-doped cuprates. Using angle-resolved photoemission spectroscopy, a nematic electronic structure was identified in the pseudogap phase.
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Academic Significance and Societal Importance of the Research Achievements |
発見から35年間の膨大な研究努力にもかかわらず未解決である銅酸化物高温超伝導体の超伝導発現機構と擬ギャップ形成機構を、従来主流であったスピン自由度に注目した研究から視点を変え、電荷ゆらぎに注目して解明を目指し成果を挙げた。実験手法として既に確立している角度分解光電子分光に加えて、新しい手法である共鳴非弾性X線散乱を高い分解能で利用し、電荷秩序、電荷励起、フォノン異常について新しい知見を得ることによって、電荷ゆらぎによる高温超伝導発現機構と擬ギャップ形成機構の確立に大きく近付いた。
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Report
(5 results)
Research Products
(75 results)
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[Journal Article] Selective observation of surface and bulk bands in polar WTe2 by laser-based spin- and angle-resolved photoemission spectroscopy2022
Author(s)
Yuxuan Wan, Lihai Wang, Kenta Kuroda, Peng Zhang, Keisuke Koshiishi, Masahiro Suzuki, Jaewook Kim, Ryo Noguchi, C_dric Bareille, Koichiro Yaji, Ayumi Harasawa, Shik Shin, Sang-Wook Cheong, Atsushi Fujimori, and Takeshi Kondo
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Journal Title
Phys. Rev. B
Volume: 105
Issue: 8
Pages: 085421-085421
DOI
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Peer Reviewed / Int'l Joint Research
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[Journal Article] Oxide Fermi liquid universality revealed by electron spectroscopy2020
Author(s)
Horio M.、Kramer K. P.、Wang Q.、Zaidan A.、von Arx K.、Sutter D.、Matt C. E.、Sassa Y.、Plumb N. C.、Shi M.、Hanff A.、Mahatha S. K.、Bentmann H.、Reinert F.、M.、Rossnagel K.、Rienks E.、Vecchione A.、Kawamata T.、Adachi T.、Koike Y.、Fujimori A.、Hoesch M.、Chang J. et al.
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Journal Title
Physical Review B
Volume: 102
Issue: 24
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Presentation] Nodal metallic behavior of underdoped triple-layer cuprate Bi22232023
Author(s)
S. Ideta, T. Yoshida, K. Tanaka, W. O. Wang, B. Moritz, T. P. Devereaux, T. K. Lee, C. Y. Mou, S. Adachi, N. Sakaki, S. Yamaguchi, T. Watanabe, T. Noji, S. Uchida, S. Ishida, and A. Fujimori
Organizer
15th International Conference on Electronic Spectroscopy and Structure
Related Report
Int'l Joint Research
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[Presentation] Doping dependence of the energy gap in the triple-layer cuprate Bi22232022
Author(s)
S. Ideta, K. Tanaka, T. Yoshida, S. Adachi, S. Yamaguchi, N. Sasaki, T. Watanabe, T. Noji, S. Ishida, S. Uchida, and A. Fujimori
Organizer
International Workshop on Correlation and Angle-Resolved Photoemission Spectroscopy
Related Report
Int'l Joint Research
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[Presentation] Acoustic plasmons in electron- and holedoped cuprates studied by resonant inelastic xray scattering at the oxygen K edge2022
Author(s)
N. Moritsuna, A. Matsumoto, J. Okamoto, A. Singh, H. Y. Huang, J.-H. Li, A. Takahashi, T. Konno, H. Sato, Y. Koike, T. Adachi, T. Mizokawa, C. T. Chen, D. J. Huang, and A. Fujimori
Organizer
29-th International Conference on Low Temperature Physics
Related Report
Int'l Joint Research
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[Presentation] Hybridization of the electronic structure in triplelayer high-Tc cuprate Bi2223 observed by ARPES2021
Author(s)
S. Ideta, S. Johnston, T. Yoshida, K. Tanaka, M.Mori, H. Anzai, A. Ino, M. Arita, H. Namatame,M. Taniguchi, S. Ishida, K. Takashima, K. M. Kojima,T. P. Devereaux, S. Uchida, and A. Fujimori
Organizer
26th Hiroshima International Symposium on Synchrotron Radiation
Related Report
Int'l Joint Research
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[Presentation] 共鳴非弾性 X 線散乱によるPr1.3-xLa0.7CexCuO4 の電荷励起・ 電荷秩序の解明2020
Author(s)
森綱尚輝, 松本篤彦, 溝川貴司, 藤森淳, 岡本淳, A. Singh, H. Y. Huang, D. J. Huang, J. H. Li, 足立匡, 高橋晶, 今野巧也, 佐藤秀孝, 小池洋二
Organizer
日本物理学会2020 年秋季大会
Related Report
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[Presentation] 共鳴非弾性X 線散乱を用いたPr1.3-xLa0.7CexCuO4 のフォ ノン解析2020
Author(s)
松本篤彦, 森綱尚輝, 溝川貴司, 藤森淳, 岡本淳, A. Singh, H. Y. Huang, D. J. Huang, J. H. Li, 足立 匡, 高橋晶, 今野巧也, 佐藤秀孝, 小池洋二
Organizer
日本物理学会第76 回年次大会
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[Presentation] 角度分解光電子分光による三層系銅酸化物 高温超伝導体Bi2Sr2Ca2Cu3O10+d のホールドープ 依存性2019
Author(s)
出田真一郎, 吉田鉄平, 藤森淳, 足立伸太郎, 山口隼平, 佐々木菜絵, 渡辺孝夫, 野地尚, 石田茂之, 内田慎一, 田中清尚
Organizer
日 本物理学会2019年秋季大会
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