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Synthesis of novel silicon carbide nanomaterials and nanocomposites by microstructural change using quantum beam irradiation

Research Project

Project/Area Number 19K05022
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Review Section Basic Section 26020:Inorganic materials and properties-related
Research InstitutionNational Institutes for Quantum Science and Technology

Principal Investigator

Taguchi Tomitsugu  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 東海量子ビーム応用研究センター, 上席研究員 (50354832)

Co-Investigator(Kenkyū-buntansha) 山本 春也  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 先端機能材料研究部, 上席研究員 (70354941)
佐伯 盛久  国立研究開発法人量子科学技術研究開発機構, 高崎量子応用研究所 東海量子ビーム応用研究センター, 上席研究員 (30370399)
Project Period (FY) 2019-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2021: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2020: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2019: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords炭化ケイ素 / ナノ材料 / 量子ビーム照射 / 透過型電子顕微鏡 / 微構造制御 / カーボンナノチューブ / イオン照射 / 新奇カーボンナノ材料 / 照射効果 / 微細組織観察 / 二層壁厚SiCナノチューブ / ハイブリッドカーボンナノ材料 / 電子線照射 / 白金微粒子 / 量子ビーム
Outline of Research at the Start

SiC系ナノ材料にイオン、電子線及びレーザー等の多様な量子ビームを制御して照射することで、SiCナノ材料の微構造・表面改質や積極的な欠陥の導入、加えて、量子ビーム照射誘起法による金属ナノ粒子との複合化等により、新奇SiC系ナノ材料・複合材料の創製を試みる。さらに、創製された新奇SiC系ナノ材料・複合材料の電気特性、及び、電気化学特性評価を行い、それらの微構造と機能との相関関係を明らかにする。

Outline of Final Research Achievements

The synthesis of novel structured silicon carbide (SiC) and/or carbon (C) nanomaterials and nanocomposites by the irradiation with quantum beams was investigated in this study. In the result, A successful synthesis of a novel hybrid carbon nanomaterial was achieved for the first time, which consisted of one-dimensionally stacked graphene nanodisks with diameters less than 50 nm, and cylindrical multi-walled carbon nanotubes, inside an amorphous SiC nanotube by the irradiation of C-SiC nanotubes with ions beam. Polycrystalline and amorphous double-thick-walled SiC nanotubes were also synthesized for the first time. We also successfully synthesized SiC nanotubes equipped with platinum nanoparticles (PtNPs) by electron beam irradiation in an aqueous solution containing chloroplatinic acid and ethanol. The SiC nanotubes equipped with PtNPs exhibited more excellent catalysis property compared to carbon materials with PtNPs.

Academic Significance and Societal Importance of the Research Achievements

材料をナノメーターサイズにしたり、新しい構造を有する新奇ナノ材料は、これまでにない新しい機能を有する可能性や、機能の構造が期待される。そのため、量子ビームを用いてSiCやカーボン系の新奇構造ナノ材料やナノ複合材料の合成に成功したことは、学術的に意義深いと考えられる。また、本研究で合成に成功したPt微粒子担持SiCナノチューブが、標準材料であるPt微粒子担持カーボン材料よりも優れた触媒性能を持つことを明らかにしたことは、工学的にも重要な成果だと言える。

Report

(5 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • 2020 Research-status Report
  • 2019 Research-status Report
  • Research Products

    (30 results)

All 2022 2021 2020 2019 2018

All Journal Article (14 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 14 results,  Open Access: 4 results) Presentation (16 results) (of which Int'l Joint Research: 6 results)

  • [Journal Article] Surface nanostructures on Nb-doped SrTiO<sub>3</sub> irradiated with swift heavy ions at grazing incidence2022

    • Author(s)
      Ishikawa N、Fujimura Y、Kondo K、Szabo G L、Wilhelm R A、Ogawa H、Taguchi T
    • Journal Title

      Nanotechnology

      Volume: 33 Issue: 23 Pages: 235303-235303

    • DOI

      10.1088/1361-6528/ac58a5

    • Related Report
      2022 Annual Research Report 2021 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effect of anionic surfactant on dispersibility and luminescence of silicon carbide nanotubes2022

    • Author(s)
      Suzuki Tatsuya、Ishihara Jun、Taguchi Tomitsugu、Miyajima Kensuke
    • Journal Title

      Journal of Luminescence

      Volume: 245 Pages: 118771-118771

    • DOI

      10.1016/j.jlumin.2022.118771

    • Related Report
      2022 Annual Research Report 2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Structural analysis of high-energy implanted Ni atoms into Si(100) by X-ray absorption fine structure spectroscopy2022

    • Author(s)
      Entani Shiro、Sato Shin-ichiro、Honda Mitsunori、Suzuki Chihiro、Taguchi Tomitsugu、Yamamoto Shunya、Ohshima Takeshi
    • Journal Title

      Radiation Physics and Chemistry

      Volume: 199 Pages: 110369-110369

    • DOI

      10.1016/j.radphyschem.2022.110369

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen storage by earth-abundant metals, synthesis and characterization of Al3FeH3.92021

    • Author(s)
      Saitoh Hiroyuki、Sato Toyoto、Tanikami Mai、Ikeda Kazutaka、Machida Akihiko、Watanuki Tetsu、Taguchi Tomitsugu、Yamamoto Shunya、Yamaki Tetsuya、Takagi Shigeyuki、Otomo Toshiya、Orimo Shin-ichi
    • Journal Title

      Materials &amp; Design

      Volume: 208 Pages: 109953-109953

    • DOI

      10.1016/j.matdes.2021.109953

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] 高速重イオン照射したセラミックスにおける照射損傷メカニズム2021

    • Author(s)
      石川 法人、田口 富嗣、大久保 成彰
    • Journal Title

      Journal of Atomic Collision Research

      Volume: 18 Issue: 3 Pages: 43-55

    • DOI

      10.50847/collision.18.3_43

    • ISSN
      2436-1070
    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Synthesis and formation mechanism of novel double-thick-walled silicon carbide nanotubes from multiwalled carbon nanotubes2021

    • Author(s)
      Taguchi Tomitsugu、Yamamoto Shunya、Ohba Hironori
    • Journal Title

      Applied Surface Science

      Volume: 551 Pages: 149421-149421

    • DOI

      10.1016/j.apsusc.2021.149421

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Analysis of J-HBC Stripper Foil for the J-PARC RCS2021

    • Author(s)
      Yoshimoto Masahiro、Nakanoya Takamitsu、Yamazaki Yoshio、Saha Pranab、Kinsho Michikazu、Yamamoto Shunya、Okazaki Hiroyuki、Taguchi Tomitsugu、Yamada Naoto、Yamagata Ryohei
    • Journal Title

      J. Phys. Soc Conf. Proc.

      Volume: 33 Pages: 011019-011019

    • DOI

      10.7566/jpscp.33.011019

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Comprehensive Understanding of Hillocks and Ion Tracks in Ceramics Irradiated with Swift Heavy Ions2020

    • Author(s)
      Ishikawa Norito、Taguchi Tomitsugu、Ogawa Hiroaki
    • Journal Title

      Quantum Beam Science

      Volume: 4 Issue: 4 Pages: 43-43

    • DOI

      10.3390/qubs4040043

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Development of a laser-induced breakdown spectroscopy system using a ceramic micro-laser for fiber-optic remote analysis2020

    • Author(s)
      Tamura Koji、Ohba Hironori、Saeki Morihisa、Taguchi Tomitsugu、Lim Hwan Hong、Taira Takunori、Wakaida Ikuo
    • Journal Title

      Journal of Nuclear Science and Technology

      Volume: 57 Issue: 10 Pages: 1189-1198

    • DOI

      10.1080/00223131.2020.1776648

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] TEM analysis of ion tracks and hillocks produced by swift heavy ions of different velocities in Y3Fe5O122020

    • Author(s)
      Ishikawa N.、Taguchi T.、Kitamura A.、Szenes G.、Toimil-Molares M. E.、Trautmann C.
    • Journal Title

      Journal of Applied Physics

      Volume: 127 Issue: 5 Pages: 055902-055902

    • DOI

      10.1063/1.5128973

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Precipitation of Pt Nanoparticles inside Ion-Track-Etched Capillaries2020

    • Author(s)
      S. Yamamoto, H. Koshikawa, T. Taguchi, T. Yamaki
    • Journal Title

      Quantum Beam Science

      Volume: 4 Issue: 1 Pages: 8-8

    • DOI

      10.3390/qubs4010008

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Synthesis of novel hybrid carbon nanomaterials inside silicon carbide nanotubes by ion irradiation2019

    • Author(s)
      Taguchi Tomitsugu、Yamamoto Shunya、Ohba Hironori
    • Journal Title

      Acta Materialia

      Volume: 173 Pages: 153-162

    • DOI

      10.1016/j.actamat.2019.05.007

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Photoinduced gold recovery mediated by isopolymolybdate in strongly acidic HCl/NaCl solutions2019

    • Author(s)
      Nakanishi Ryuzo、Saeki Morihisa、Taguchi Tomitsugu、Ohba Hironori
    • Journal Title

      Journal of Photochemistry and Photobiology A: Chemistry

      Volume: 383 Pages: 111994-111994

    • DOI

      10.1016/j.jphotochem.2019.111994

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] In Situ Time-Resolved XAFS Studies on Laser-Induced Particle Formation of Palladium Metal in an Aqueous/EtOH Solution2018

    • Author(s)
      Saeki Morihisa、Matsumura Daiju、Yomogida Takumi、Taguchi Tomitsugu、Tsuji Takuya、Saitoh Hiroyuki、Ohba Hironori
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 123 Issue: 1 Pages: 817-824

    • DOI

      10.1021/acs.jpcc.8b09532

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Presentation] SiCナノチューブのアモルファス化照射量に及ぼす外径の影響2022

    • Author(s)
      田口富嗣、山本春也
    • Organizer
      日本顕微鏡学会 第78回学術講演会
    • Related Report
      2022 Annual Research Report
  • [Presentation] Synthesis of Polycrystalline and Amorphous Double-Thick-Walled Silicon Carbide Nanotubes2021

    • Author(s)
      Taguchi Tomitsugu, Yamamoto Shunya, Ohba hironori
    • Organizer
      Materials Research Meeting 2021
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Formation of Metal Nanoparticles inside Ion-Track-Etched Polyimide Capillaries2021

    • Author(s)
      Yamamoto Shunya, Koshikawa HIroshi, Taguchi Tomitsugu, Idesaki Akira, Okazaki Hiroyuki, Yamaki Tetsuya
    • Organizer
      Materials Research Meeting 2021
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Ion Irradiation Induced Synthesis of Novel Amorphous Double-Thick-Walled Silicon Carbide Nanotubes2021

    • Author(s)
      Taguchi Tomitsugu, Yamamoto Shunya, Ohba hironori
    • Organizer
      The 9th International Symposium on Surface Science (ISSS9)
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] イオン照射によるアモルファス二層厚壁SiCナノチューブの合成とその形状変化2021

    • Author(s)
      田口富嗣、山本春也、大場弘則
    • Organizer
      日本顕微鏡学会 第77回学術講演会
    • Related Report
      2021 Research-status Report
  • [Presentation] スパッタリング法により成膜したAl-Fe薄膜中の水素2021

    • Author(s)
      山本春也、齋藤寛之、田口富嗣、内海伶那、綿貫徹、八巻徹也
    • Organizer
      日本金属学会 2021年秋期(第169回)講演大会
    • Related Report
      2021 Research-status Report
  • [Presentation] 二層厚壁SiCナノチューブの合成2020

    • Author(s)
      田口富嗣、大場弘則
    • Organizer
      日本顕微鏡学会 第76回学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] Synthesis of Precious Metal Nanoparticles inside Ion-Track-Etched Capillaries Formed in Polyimide Films2020

    • Author(s)
      山本春也、越川博、田口富嗣、出崎亮、岡崎宏之、八巻徹也
    • Organizer
      第30回日本MRS年次大会
    • Related Report
      2020 Research-status Report
  • [Presentation] The suppression of oxidative corrosion of carbon by structural change due to ion irradiation2020

    • Author(s)
      Okazaki Hiroyuki, Yamamoto Shunya, Koshikawa Hiroshi, Taguchi Tomitsugu, Idesaki Akira, Yamaki Tetsuya
    • Organizer
      第30回日本MRS年次大会
    • Related Report
      2020 Research-status Report
  • [Presentation] Synthesis of new structured hybrid carbon nanomaterials by ion irradiation of C-SiC coaxial nanotubes2019

    • Author(s)
      Taguchi Tomitsugu, Yamamoto Shunya, Oba Hironori
    • Organizer
      第29回 日本MRS年次大会
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] C-SiCナノチューブのイオン照射による新奇ハイブリッドカーボンナノ材料の創製2019

    • Author(s)
      田口 富嗣, 山本 春也, 大場 弘則
    • Organizer
      日本顕微鏡学会第75回学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] Characterization of fiber-optic LIBS analysis using Nd:YAG ceramic micro-laser2019

    • Author(s)
      Oba Hironori, Tamura Koji, Saeki Morihisa, Taguchi Tomitsugu, Hong Lim Hwan, Taira Takunori, Tagawa Akihiro, Wakaida Ikuo
    • Organizer
      The 3rd Asian Symposium on Laser Induced Breakdown Spectroscopy
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Radiation Dose Rate Effects of Microchip-Laser Induced Breakdown Spectroscopy for Remote Analysis of Severe Accident Reactor2019

    • Author(s)
      Tamura Koji, Oba Hironori, Saeki Morihisa, Taguchi Tomitsugu, Hwan Hong Lim, Taira Takunori, Tagawa Akihiro, Wakaida Ikuo
    • Organizer
      The 3rd Asian Symposium on Laser Induced Breakdown Spectroscopy
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] 白金族元素イオン溶液におけるレーザー微粒子化反応のその場・時間分解XAFS研究2019

    • Author(s)
      佐伯 盛久, 松村 大樹, 蓬田 匠, 田口 富嗣, 辻 卓也, 齋藤 寛之, 中西 隆造, 大場 弘則
    • Organizer
      日本化学会第99春季年会 2019
    • Related Report
      2019 Research-status Report
  • [Presentation] ナノ秒パルス紫外レーザー照射時のPd溶液における光誘起微粒子化の 時間分解XAFS研究2019

    • Author(s)
      佐伯 盛久, 蓬田 匠, 松村 大樹, 中西 隆造, 田口 富嗣, 辻 卓也, 齋藤 寛之, 大場 弘則
    • Organizer
      第13回分子科学討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] レーザー誘起パラジウム微粒子化反応のDXAFS研究2019

    • Author(s)
      佐伯 盛久, 松村 大樹, 蓬田 匠, 田口 富嗣, 辻 卓也, 齋藤 寛之, 中西 隆造, 大場 弘則
    • Organizer
      XAFS・X線顕微鏡分光分析分野でのIMSS, PF戦略的利用に関する研究会
    • Related Report
      2019 Research-status Report

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Published: 2019-04-18   Modified: 2024-01-30  

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