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Development of provenance estimation of clay and temper materials in ancient pottery using solid solution minerals

Research Project

Project/Area Number 19K13410
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 03050:Archaeology-related
Research InstitutionFukuoka University

Principal Investigator

Ichikawa Shintaro  福岡大学, 理学部, 助教 (90593195)

Project Period (FY) 2019-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2021: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2020: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2019: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords土器 / 阿玉台式土器 / 固溶体鉱物 / 起源推定 / 混和材 / X線回折分析
Outline of Research at the Start

本研究は、意図的な混和が考えられている阿玉台式土器に関して、「胎土原料である粘土」と「混和物」それぞれの地域性を“個別に”明らかにできる分析法の開発を目的とする。含有鉱物を種類ごとに同定することができる「X線回折分析」を用いて、粘土もしくは混和物に由来する鉱物を個別に解析することで、各々の地質起源の判別が可能であることを明らかにし、土器中の鉱物の分析から解析、起源推定までの一貫した土器の胎土分析の基盤を確立する。

Outline of Final Research Achievements

In order to develop provenance estimation technique of clay and temper in ancient pottery, Atamadai-type potteries from Hinoki site were compared with the other potteries originated from the same site and period using X-ray diffractometry (XRD). As the results, the temper of the Atamadi-type potteries contains biotite which is a solid solution mineral. The biotite might archaeologically characterize the origins .of the temper by affecting a shift in lattice spacing via variations in the solid-solution ratio. Thus, 14 biotite-containing rocks from different regions were analyzed by XRD to clarify the provenance dependency. The lattice spacings of the biotite 001 were classified into five groups despite the rocks have different origins. The provenance dependency of the lattice spacing should be examined using the solid-solution ratio. The elucidation of the provenance dependency may be able to permit the provenance estimation of the temper in Atamadai-type pottery by XRD.

Academic Significance and Societal Importance of the Research Achievements

本研究は、X 線回折分析による含有鉱物に基づき、粘土と混和物の地域性を別々に明らかできる新たな胎土分析法の確立を目指した。まず、桧の木遺跡から出土した阿玉台式土器の混和物が黒雲母を含むことを明らかにした。さらに、産地の異なる黒雲母含有岩石14種類中の黒雲母001面の格子面間隔を比較し、有意差のある5つのグループに分類した。すなわち、これらの岩石中から黒雲母を取り出して固溶組成を明らかにしなければ断言することはできないが、一部の黒雲母の格子面間隔には産地依存性が見られた。したがって、本研究では、土器の粘土や混和物に由来する鉱物を用いて、各々の起源を推定できる可能性を示唆することができた。

Report

(4 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • Research Products

    (45 results)

All 2022 2021 2020 2019 Other

All Journal Article (18 results) (of which Peer Reviewed: 16 results) Presentation (26 results) (of which Int'l Joint Research: 8 results,  Invited: 3 results) Remarks (1 results)

  • [Journal Article] 島根県奥出雲町で採取した砂鉄の蛍光X線分析2022

    • Author(s)
      大久保いずみ、市川慎太郎、脇田久伸、沼子千弥、米津幸太郎、横山拓史、栗崎 敏
    • Journal Title

      X線分析の進歩

      Volume: 53 Pages: 183-194

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 黒雲母の格子面間隔による阿玉台式土器の起源推定法の件検討2022

    • Author(s)
      田中ひなの、市川慎太郎、栗崎 敏
    • Journal Title

      X線分析の進歩

      Volume: 53 Pages: 165-173

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] XPSによるリチウムイオンを溶解したイオン液体界面における状態分析2022

    • Author(s)
      笠間裕真、市川慎太郎、喜多條鮎子、栗崎 敏
    • Journal Title

      X線分析の進歩

      Volume: 53 Pages: 151-163

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 棒状鉄資料の蛍光X線分析における問題点-資料表面の錆の影響-2022

    • Author(s)
      市川慎太郎、佐藤かのん、脇田久伸、栗崎 敏
    • Journal Title

      九州国立博物館「大宰府学研究」シンポジウム アジアを変えた鉄-大宰府鴻臚館の衰退と海商の時代-

      Volume: - Pages: 63-70

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Preliminary examination for revealing the provenance dependency of the lattice spacing of biotite for the provenance estimation of Atamadai-type pottery (2500?1500 BC) by XRD2021

    • Author(s)
      Shintaro Ichikawa, Kana Miyamoto, Tsutomu Kurisaki
    • Journal Title

      Powder Diffraction

      Volume: 36 Issue: 2 Pages: 74-77

    • DOI

      10.1017/s0885715621000178

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Relationship between Rare Earth Element Patterns and Geological Features of Iron Sands Collected from Okuizumo Shimane, Japan2021

    • Author(s)
      Izumi Okubo, Shintaro Ichikawa, Hisanobu Wakita, Chiya Numako, Kotaro Yonezu, Takushi Yokoyama, Tsutomu Kurisaki
    • Journal Title

      Proceedings of the 10th International Symposium on History of Indigenous Knowledge

      Volume: 10 Pages: 42-49

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Provenance-Estimation Method for Temper in Atamadai-Type Pottery by X-ray Diffractometry: An Examination of Heavy-Liquid-separation Method for Biotite2021

    • Author(s)
      Hinano Tanaka, Shintaro Ichikawa, Tsutomu Kurisaki
    • Journal Title

      Proceedings of the 10th International Symposium on History of Indigenous Knowledge

      Volume: 10 Pages: 50-57

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of Iron Sand around Mt. Abura for Provenance Estimation of Iron Artifacts2021

    • Author(s)
      Yuta Ishikake, Shintaro Ichikawa, Tsutomu Kurisaki
    • Journal Title

      Proceedings of the 10th International Symposium on History of Indigenous Knowledge

      Volume: 10 Pages: 66-71

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 蛍光X線分析法による微少量土器試料の高精度産地同定2021

    • Author(s)
      市川慎太郎
    • Journal Title

      X線分析の進歩

      Volume: 52 Pages: 1-14

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] 蛍光X線法およびX線回折法による油山山麓周辺の砂鉄の鉱物および化学組成分析2021

    • Author(s)
      石掛雄大、市川慎太郎、栗崎 敏
    • Journal Title

      X線分析の進歩

      Volume: 52 Pages: 207-215

    • NAID

      40022637610

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] 猪ノ鼻(1)遺跡出土須恵器の胎土分析 (蛍光X線分析)2021

    • Author(s)
      市川慎太郎
    • Journal Title

      青森県埋蔵文化財報告書

      Volume: 616 Pages: 146-152

    • Related Report
      2020 Research-status Report
  • [Journal Article] Characterization of Ancient Pottery Clay by XRF Spectrometry — Sample Preparation and Calibration Curve —2020

    • Author(s)
      市川慎太郎、松本建速、中村利廣、栗崎 敏
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 69 Issue: 9 Pages: 427-438

    • DOI

      10.2116/bunsekikagaku.69.427

    • NAID

      130007938104

    • ISSN
      0525-1931
    • Year and Date
      2020-09-05
    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Provenance identification of ancient pottery from Hachijojima Island, part of Izu Islands (Tokyo, Japan), using X-ray fluorescence spectrometry2020

    • Author(s)
      Shintaro Ichikawa, Takehaya Matsumoto, Toshihiro Nakamura, Tsutomu Kurisaki
    • Journal Title

      X-Ray Spectrometry

      Volume: 49 Pages: 515-532

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Synthetic calibration reference materials for X-ray fluorescence quantitation of 22 components in ancient Japanese pottery2020

    • Author(s)
      Shintaro Ichikawa, Tsutomu Kurisaki
    • Journal Title

      Advances in X-ray Analysis

      Volume: 63 Pages: 117-124

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Mineral analysis of river sand around Mt. Tsukuba for provenance estimation of Atamadai type pottery (2500?1500 BC) from Hinoki site (Tochigi, Japan)2019

    • Author(s)
      Shintaro Ichikawa, Yuya Sakito, Tsutomu Kurisaki
    • Journal Title

      Powder Diffraction

      Volume: 34 Issue: 2 Pages: 159-163

    • DOI

      10.1017/s0885715619000290

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Provenance determination of prehistorical pottery from Oshima Island belonging to Izu islands (Tokyo, Japan) using X‐ray fluorescence spectrometry2019

    • Author(s)
      Shintaro Ichikawa, Takehaya Matsumoto, Toshihiro Nakamura, Tsutomu Kurisaki
    • Journal Title

      X-Ray Spectrometry

      Volume: 48 Issue: 2 Pages: 107-125

    • DOI

      10.1002/xrs.3003

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Rare Earth Element Patterns of Iron Sand Collected at Outcrops of Kanna-Nagashi Remains in Okuizumo Region (Shimane, Japan)2019

    • Author(s)
      Shintaro Ichikawa, Ryosuke Miki, Hisanobu Wakita, Chiya Numako, Kotaro Yonezu, Takushi Yokoyama, Tsutomu Kurisaki
    • Journal Title

      Proceedings of the 9th International Symposium of History of Indigenous Knowledg

      Volume: 9 Pages: 55-62

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] 蛍光X線分析における土器に適した試料調製法2019

    • Author(s)
      市川慎太郎、栗崎 敏
    • Journal Title

      福岡大学理学集報

      Volume: 49 Pages: 17-29

    • NAID

      120006619932

    • Related Report
      2019 Research-status Report
  • [Presentation] 棒状鉄資料の蛍光X線分析における問題点-資料表面の錆の影響-2022

    • Author(s)
      市川慎太郎、佐藤かのん、脇田久伸、栗崎 敏
    • Organizer
      九州国立博物館「大宰府学研究」シンポジウム アジアを変えた鉄-大宰府鴻臚館の衰退と海商の時代-
    • Related Report
      2021 Annual Research Report
  • [Presentation] Characterization of Elements in Iron Sands around Mt. Aburayama (Fukuoka, Japan) for Provenance Estimation of Archaeological Iron Artifacts2021

    • Author(s)
      Shintaro Ichikawa, Yuta Ishikake, Yukiko Nishi, Tsutomu Kurisaki
    • Organizer
      Denver X-Ray Conference 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Relationship between Rare Earth Element Patterns and Geological Features of Iron Sands Collected from Okuizumo Shimane, Japan2021

    • Author(s)
      Izumi Okubo, Shintaro Ichikawa, Hisanobu Wakita, Chiya Numako, Kotaro Yonezu, Takushi Yokoyama, Tsutomu Kurisaki
    • Organizer
      The 10th International Symposium on History of Indigenous Knowledge
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Provenance-Estimation Method for Temper in Atamadai-Type Pottery by X-ray Diffractometry: An Examination of Heavy-Liquid-separation Method for Biotite2021

    • Author(s)
      Hinano Tanaka, Shintaro Ichikawa, Tsutomu Kurisaki
    • Organizer
      The 10th International Symposium on History of Indigenous Knowledge
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Characterization of Iron Sand around Mt. Abura for Provenance Estimation of Iron Artifacts2021

    • Author(s)
      Yuta Ishikake, Shintaro Ichikawa, Tsutomu Kurisaki
    • Organizer
      The 10th International Symposium on History of Indigenous Knowledge
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 島根県奥出雲町の土壌および河川砂から採取した砂鉄の希土類元素パターンの地質依存性2021

    • Author(s)
      大久保いずみ、市川慎太郎、脇田久伸、沼子千弥、米津幸太郎、横山拓史、栗崎 敏
    • Organizer
      第81回分析化学討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] X線回折法による阿玉台式土器に含まれる混和材の起源推定法の検討2021

    • Author(s)
      田中ひなの、市川慎太郎、栗崎 敏
    • Organizer
      第81回分析化学討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] XPSを用いたイオン液体界面における金属イオンの特性評価2021

    • Author(s)
      笠間裕真、市川慎太郎、喜多條鮎子、栗崎 敏
    • Organizer
      第81回分析化学討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 鉄製遺物の始発原料推定を目指した油山山麓周辺の砂鉄の地域性解明2021

    • Author(s)
      市川慎太郎、石掛雄大、西 幸子、栗崎 敏
    • Organizer
      日本文化財科学会第38回大会
    • Related Report
      2021 Annual Research Report
  • [Presentation] XPSを用いたイオン液体界面におけるアルカリ金属イオンの特性評価2021

    • Author(s)
      笠間裕真、市川慎太郎、喜多條鮎子、栗崎 敏
    • Organizer
      第57回X線分析討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 島根県奥出雲町で採取した砂鉄の蛍光X線分析2021

    • Author(s)
      大久保いずみ、市川慎太郎、脇田久伸、沼子千弥、米津幸太郎、横山拓史、栗崎 敏
    • Organizer
      第57回X線分析討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 黒雲母の格子面間隔による阿玉台式土器の起源推定法の検討2021

    • Author(s)
      田中ひなの、市川慎太郎、栗崎 敏
    • Organizer
      第57回X線分析討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 酸性条件下で合成したリンドープ酸化チタンのXRD測定による評価2021

    • Author(s)
      山本理久、山田啓二、市川慎太郎、栗崎 敏
    • Organizer
      第57回X線分析討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 蛍光X線分析法による微少量土器試料の高精度産地同定2020

    • Author(s)
      市川慎太郎
    • Organizer
      第56回X線分析討論会
    • Related Report
      2020 Research-status Report
    • Invited
  • [Presentation] Preliminary Examination for Elucidating Resource Dependency of d-spacing of Biotite for Provenance Estimation of Atamadai-Type Pottery (2500-1500 BC) with XRD2020

    • Author(s)
      Shintaro Ichikawa, Kana Miyamoto, Tsutomu Kurisaki
    • Organizer
      Denver X-Ray Conference 2020
    • Related Report
      2020 Research-status Report
    • Int'l Joint Research
  • [Presentation] 蛍光X線法およびX線回折法による油山麓周辺の砂鉄特性評価2020

    • Author(s)
      石掛雄大、市川慎太郎、栗崎 敏
    • Organizer
      第56回X線分析討論会
    • Related Report
      2020 Research-status Report
  • [Presentation] Rare Earth Element Patterns of Iron Sand Collected at Outcrops of Kanna-Nagashi Remains in Okuizumo Region (Shimane, Japan)2019

    • Author(s)
      Shintaro Ichikawa, Ryosuke Miki, Hisanobu Wakita, Chiya Numako, Kotaro Yonezu, Takushi Yokoyama, Tsutomu Kurisaki
    • Organizer
      The 9th International Symposium of History of Indigenous Knowledge 2019
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Development of Synthetic Calibration Standards for X-ray Fluorescence Determination of Japanese Ancient Pottery2019

    • Author(s)
      Shintaro Ichikawa, Tsutomu Kurisaki
    • Organizer
      Denver X-Ray Conference 2019
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Sample preparation for quantitative XRF2019

    • Author(s)
      Shintaro Ichikawa
    • Organizer
      Denver X-ray Conference 2019
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 蛍光X線法の基礎~原理と試料調製2019

    • Author(s)
      市川慎太郎
    • Organizer
      Japan Analytical & Scientific Instruments Show 2019
    • Related Report
      2019 Research-status Report
    • Invited
  • [Presentation] 蛍光X線分析による伊豆諸島八丈島出土土器の産地推定2019

    • Author(s)
      市川慎太郎、松本建速、中村利廣、栗崎 敏
    • Organizer
      第55回X線分析討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] X線と水・溶液の関わり合いー歴史と現在・未来2019

    • Author(s)
      脇田久伸、市川慎太郎、栗崎 敏
    • Organizer
      第55回X線分析討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] X線光電子分光法によるイオン液体界面のアルカリ金属イオンの溶存構造解析2019

    • Author(s)
      栗崎 敏、喜多優羽、市川慎太郎、喜多條鮎子
    • Organizer
      第55回X線分析討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] 蛍光X線法による伊豆諸島大島出土土器の産地推定2019

    • Author(s)
      市川慎太郎、松本建速、中村利廣、栗崎 敏
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Research-status Report
  • [Presentation] 紫外可視分光法とDiscrete Variational Multi Electron (DV-ME)法を用いた遷移金属水和錯体の溶存構造解析2019

    • Author(s)
      眞武徳生、市川慎太郎、山口敏男、栗崎 敏
    • Organizer
      日本分析化学会第68年会
    • Related Report
      2019 Research-status Report
  • [Presentation] 鉄製遺物の始発原料推定を目指した油山周辺の砂鉄の蛍光X線分析2019

    • Author(s)
      石掛雄大、市川慎太郎、栗崎 敏
    • Organizer
      第56回化学関連支部合同九州大会
    • Related Report
      2019 Research-status Report
  • [Remarks] 福岡大学理学部化学科物質機能化学A研究室ホームページ

    • URL

      http://www.sc.fukuoka-u.ac.jp/~ac/index.html

    • Related Report
      2021 Annual Research Report 2020 Research-status Report 2019 Research-status Report

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Published: 2019-04-18   Modified: 2023-01-30  

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