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Exploration for novel superconductivity in epitaxial thin films of iron chalcogenides

Research Project

Project/Area Number 19K14651
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionThe University of Tokyo

Principal Investigator

Nabeshima Fuyuki  東京大学, 大学院総合文化研究科, 助教 (30782776)

Project Period (FY) 2019-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2020: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2019: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords鉄カルコゲナイド超伝導体 / 磁気輸送特性 / ミュオンスピン緩和 / 磁場侵入長 / 薄膜 / 鉄カルコゲナイド超伝導 / 磁性 / マイクロ波伝導度 / 鉄系超伝導体
Outline of Research at the Start

鉄カルコゲナイド超伝導体FeSeは,非常に小さいフェルミエネルギーおよび大きなスピン軌道相互作用を持つという稀有な性質をもち,これまでにない全く新しい超伝導状態が実現している可能性がある.本研究では,広い組成領域に渡って連続的な元素置換が可能である薄膜試料を作製し,様々な測定プローブ―例えば磁気輸送特性や磁場侵入長測定など―を用いた系統的な常伝導特性・超伝導特性の評価を行うことで,この物質群の超伝導の特異性・新規性を,多角的な視点から明らかにすることを目的とする.

Outline of Final Research Achievements

We found that carrier density and the superconducting transition temperature (Tc) have positive correlation from measurement of magneto-transport and magnetic penetration depth of thin films of FeSe1-xTexと FeSe1-ySy. Our results suggest that the different Tc behavior between Te- and S-substitution results from the fact that Te- and S-substitution affect Fermi surface, or carrier density, differently. This also suggests that the electronic nematicity and its fluctuations do not play the primary role on superconductivity in iron chalcogenides. Furthermore, we demonstrated for the first time that S substitution induce magnetic order in FeSe from muon spin relaxation measurements of thin films of FeSe1-ySy.

Academic Significance and Societal Importance of the Research Achievements

鉄カルコゲナイド超伝導体FeSeは超伝導転移温度Tcが低いものの,様々な方法でTcを大幅に上昇させることができ,さらなるTcの向上や実用化を目指し,超伝導メカニズム解明に向けて精力的に研究がなされている.FeSeは静水圧下でTcが4倍程度に増大するが,元素置換による格子の圧縮(化学圧力)ではTcの上昇は見られない.磁気的なゆらぎが超伝導の重要因子の一つだと考えられているが,本研究により,物理圧力と同様に化学圧力でも磁気秩序が誘起されることが明らかになった.今後この磁気秩序を詳しく調べることで物理圧力と化学圧力でのTcの違いを明らかにし,この物質のTc上昇のメカニズムを解明できる可能性がある.

Report

(3 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • Research Products

    (33 results)

All 2021 2020 2019 Other

All Int'l Joint Research (1 results) Journal Article (6 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Open Access: 3 results) Presentation (26 results) (of which Int'l Joint Research: 6 results,  Invited: 1 results)

  • [Int'l Joint Research] Paul Scherrer Institut(スイス)

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Orbital mixing at the onset of high-temperature superconductivity in FeSe1?xTex/CaF22021

    • Author(s)
      Nakayama K.、Tsubono R.、Phan G. N.、Nabeshima F.、Shikama N.、Ishikawa T.、Sakishita Y.、Ideta S.、Tanaka K.、Maeda A.、Takahashi T.、Sato T.
    • Journal Title

      Physical Review Research

      Volume: 3 Issue: 1

    • DOI

      10.1103/physrevresearch.3.l012007

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Sulfur-induced magnetism in FeSe1-xSx thin films on LaAlO3 revealed by muon spin rotation/relaxation2021

    • Author(s)
      F. Nabeshima, Y. Kawai, N. Shikama, Y. Sakishita, A. Suter, T. Prokscha, S. E. Park, S. Komiya, A. Ichinose, T. Adachi, and A. Maeda
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 18

    • DOI

      10.1103/physrevb.103.184504

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Correlation between superconducting transition temperatures and carrier densities in Te- and S-substituted FeSe thin films2020

    • Author(s)
      Fuyuki Nabeshima, Tomoya Ishikawa, Naoki Shikama, Atsutaka Maeda
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 18

    • DOI

      10.1103/physrevb.101.184517

    • Related Report
      2020 Annual Research Report 2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Enhancement of superconducting transition temperature in electrochemically etched FeSe/LaAlO3 films2020

    • Author(s)
      Shikama Naoki、Sakishita Yuki、Nabeshima Fuyuki、Katayama Yumiko、Ueno Kazunori、Maeda Atsutaka
    • Journal Title

      Applied Physics Express

      Volume: 13 Issue: 8 Pages: 083006-083006

    • DOI

      10.35848/1882-0786/aba649

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Chemical pressure effect of the electron-doped FeSe films with an electric double-layer-transistor structure2020

    • Author(s)
      Shikama N、Sakishita Y、Nabeshima F、Maeda A
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 1590 Issue: 1 Pages: 012012-012012

    • DOI

      10.1088/1742-6596/1590/1/012012

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Transport properties of FeSe1-xSx and FeSe1-yTey epitaxial thin films under magnetic fields2019

    • Author(s)
      N. Shikama, T. Ishikawa, F. Nabeshima, A. Maeda
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 1293 Issue: 1 Pages: 012015-012015

    • DOI

      10.1088/1742-6596/1293/1/012015

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Enhancement of superconducting transition temperature in electrochemically etched FeSe/LaAlO3 films2021

    • Author(s)
      Naoki Shikama, Yuki Sakishita, Fuyuki Nabeshima, Yumiko Katayama, Kazunori Ueno, Atsutaka Maeda
    • Organizer
      American Physical Society March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Complex conductivity of the FeSe1-xTex films2021

    • Author(s)
      Hodaka Kurokawa, Sota Nakamura, Zhao Jiahui, Naoki Shikama, Yuki Sakishita, Yue Sun, Fuyuki Nabeshima, Yoshinori Imai, Haruhisa Kitano, Atsutaka Maeda
    • Organizer
      American Physical Society March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sulfur-induced magnetism in iron-chalcogenide thin films2021

    • Author(s)
      Fuyuki Nabeshima, Yuma Kawai, Naoki Shikama, Yuki Sakishita, Andreas Suter, Sang Eun Park, Tadashi Adachi, Atsutaka Maeda
    • Organizer
      American Physical Society March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 空洞共振器による鉄カルコゲナイド薄膜の複素伝導度測定2021

    • Author(s)
      趙嘉輝, 黒川穂高, 小林友輝, 崎下雄稀, 色摩直樹, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会 第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe(Se,S)薄膜における磁気秩序の歪依存性2021

    • Author(s)
      鍋島冬樹, 色摩直樹, 小林友輝, 崎下雄稀, 前田京剛
    • Organizer
      日本物理学会 第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 第一原理計算によるネマティック相と非ネマティック相におけるFe(Se,Te)のバンド分散の評価2021

    • Author(s)
      黒川穂高, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会 第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 高濃度S置換 Fe(Se,S)薄膜における磁気秩序の観測2021

    • Author(s)
      鍋島冬樹,河合優茉,色摩直樹,崎下雄稀,Andreas Suter,Thomas Prokscha,パクサンウン,小宮世紀,一瀬中,足立匡,前田京剛
    • Organizer
      2021年第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe(Se,S)薄膜における常圧下の磁気秩序2021

    • Author(s)
      鍋島冬樹,河合優茉,色摩直樹,崎下雄稀,Andreas Suter,Thomas Prokscha,パクサンウン,小宮世紀,一瀬中,足立匡,前田京剛
    • Organizer
      高温超伝導フォーラム第8回会合
    • Related Report
      2020 Annual Research Report
  • [Presentation] Complex conductivity of FeSe1-xTex (x = 0.1-0.5) film2020

    • Author(s)
      Hodaka Kurokawa, Sota Nakamura, Jiahui Zhao, Naoki Shikama, Yuki Sakishita, Yue Sun, Fuyuki Nabesima, Yoshinori Imai, Haruhisa Kitano, Atsutaka Maeda
    • Organizer
      33rd International Symposium on Superconductivity (ISS 2020)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Fe(Se,Te)薄膜の複素電気伝導度の組成依存性2020

    • Author(s)
      黒川穂高, 中村奏太, 趙嘉輝, 色摩直樹, 崎下雄斗, 孫悦, 鍋島冬樹, 北野晴久, 前田京剛
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe(Se, Te)高温超伝導薄膜の高分解能ARPES2020

    • Author(s)
      中山耕輔, 坪野竜治, 大和田健太, 鍋島冬樹, 色摩直樹, 石川智也, 崎下雄稀, 前田京剛, 高橋隆, 佐藤宇史
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 低ゲート電圧で電気化学的エッチングしたFeSe薄膜におけるTczeroの増大2020

    • Author(s)
      色摩直樹, 崎下雄稀, 鍋島冬樹, 片山裕美子, 上野和紀, 前田京剛
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 高濃度S置換Fe(Se, S)薄膜における磁気秩序2020

    • Author(s)
      鍋島冬樹, 河合優茉, 色摩直樹, 崎下雄稀, A. Suter, パクサンウン, 小宮世紀, 一瀬中, 足立匡, 前田京剛
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 鉄系超伝導体FeSe0.5Te0.5における光誘起超伝導増強2020

    • Author(s)
      礒山和基, 吉川尚孝, 勝見恒太, Jeremy Wong, 色摩直樹, 崎下雄稀, 鍋島冬樹, 前田京剛, 島野亮
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 中間層最表面にCaF2を用いたFeSe1-xTexコート線材の臨界電流特性2020

    • Author(s)
      滝澤 和輝、岡田 逹典、淡路 智、色摩 直樹、鍋島 冬樹、前田 京剛、一瀬 中、中岡 晃一、和泉 輝郎
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 電子ドープFeSe/LaAlO3薄膜における超伝導特性のゲート電圧依存性2020

    • Author(s)
      色摩直樹、崎下雄稀、鍋島冬樹、片山裕美子、上野和紀、前田京剛
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe(Se,Te)薄膜の磁場侵入長の組成依存性2020

    • Author(s)
      鍋島冬樹、黒川穂高、中村奏太、色摩直樹、崎下雄稀、小林友輝、孫悦、北野晴久、前田京剛
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 電子ドープFeSe/LaAlO3薄膜における超伝導特性のゲート電圧依存性2020

    • Author(s)
      色摩直樹, 崎下雄稀, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] コプレーナ線路共振器を用いたFe(Se,Te)薄膜の磁場侵入長測定2020

    • Author(s)
      中村奏太, 黒川穂高, 崎下雄稀, 色摩直樹, 鍋島冬樹, 孫悦, 北野晴久, 前田京剛
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] FeSe1-xSx薄膜におけるスピン相関の発達2020

    • Author(s)
      足立匡, 河合優茉, 色摩直樹, 崎下雄稀, 鍋島冬樹, A. Suter, パクサンウン, 小宮世紀, 一瀬中, 前田京剛
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] Comparison between Te- and S-Substitution Effects on Superconductivity in FeSe Thin Films2019

    • Author(s)
      Fuyuki Nabeshima
    • Organizer
      Research Frontier of Advanced Spectroscopies for Correlated Electron Systems
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Comparison of Te and S substitution in FeSe thin films2019

    • Author(s)
      F. Nabeshima, T. Ishikawa, N. Shikama, S. Nakamura, H. Kurokawa and A. Maeda
    • Organizer
      Spectroscopies in Novel Superconductors (SNS 2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] 鉄カルコゲナイド超伝導薄膜の超伝導特性とその組成依存性2019

    • Author(s)
      鍋島冬樹
    • Organizer
      高温超伝導フォーラム 第7回会合
    • Related Report
      2019 Research-status Report
  • [Presentation] 超伝導体共振器を用いたFeSe1-xTex薄膜の磁場侵入長組成依存性2019

    • Author(s)
      中村奏太, 黒川穂高, 中島直哉, 石川智也, 色摩直樹, 小川亮, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2019 Research-status Report
  • [Presentation] 誘電体共振器による鉄カルコゲナイド薄膜の複素伝導度評価2019

    • Author(s)
      黒川穂高, 中島直哉, 色摩直樹, 崎下雄稀, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2019 Research-status Report
  • [Presentation] 同族元素置換したFeSeの電気二重層トランジスタ2019

    • Author(s)
      色摩直樹, 崎下雄稀, 鍋島冬樹, 前田京剛
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2019 Research-status Report

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Published: 2019-04-18   Modified: 2022-01-27  

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