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Development of ultra-efficient terahertz devices by exploiting multiple exciton generation in single-walled carbon nanotubes

Research Project

Project/Area Number 19K15047
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 21060:Electron device and electronic equipment-related
Research InstitutionOsaka University

Principal Investigator

Bagsican Filchito Renee  大阪大学, レーザー科学研究所, 特任研究員 (20791982)

Project Period (FY) 2019-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2020: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2019: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywordscarbon nanotubes / terahertz emission / photocurrent / exciton dynamics / carrier dynamics / photoconductive antenna / Boltzmann equation / Terahertz devices / Carbon nanotubes / Carrier dynamics
Outline of Research at the Start

The first part is the understanding the fundamentals of ultrafast optoelectronic response in CNT and other low-dimensional materials. These understandings will then be used in the development of efficient THz devices based on these materials. This will be done by designing optimal device structures.

Outline of Final Research Achievements

We achieved the following milestones over the course of our project: (1) successful integration of carbon nanotubes (CNTs) in photoconductive antenna devices, (2) demonstrated their promising efficiencies as terahertz (THz) emitters, and (3) showed that THz emission spectroscopy is a powerful tool in unraveling quasiparticle dynamics in low dimensional materials.

Academic Significance and Societal Importance of the Research Achievements

We were able to get a clearer understanding of dynamics of free carriers and excitons in carbon nanotubes. From a scientific standpoint, this demonstrates the drastically different behavior of low-dimensional materials. It also brings us closer to their application in future optoelectronic devices.

Report

(3 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • Research Products

    (12 results)

All 2021 2020 2019 Other

All Int'l Joint Research (4 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Open Access: 2 results) Presentation (6 results) (of which Int'l Joint Research: 6 results,  Invited: 3 results)

  • [Int'l Joint Research] Rice University(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Nanyang Technological University(シンガポール)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Rice University(米国)

    • Related Report
      2019 Research-status Report
  • [Int'l Joint Research] Nanyang Technological University(シンガポール)

    • Related Report
      2019 Research-status Report
  • [Journal Article] Ultrafast Terahertz Nanoseismology of GaInN/GaN Multiple Quantum Wells2021

    • Author(s)
      Mannan Abdul、Bagsican Filchito Renee G.、Yamahara Kota、Kawayama Iwao、Murakami Hironaru、Bremers Heiko、Rossow Uwe、Hangleiter Andreas、Turchinovich Dmitry、Tonouchi Masayoshi
    • Journal Title

      Advanced Optical Materials

      Volume: n/a Issue: 15 Pages: 2100258-2100258

    • DOI

      10.1002/adom.202100258

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Terahertz Excitonics in Carbon Nanotubes: Exciton Autoionization and Multiplication2020

    • Author(s)
      Filchito Renee G. Bagsican, Michael Wais, Natsumi Komatsu, Weilu Gao, Lincoln W. Weber, Kazunori Serita, Hironaru Murakami, Karsten Held, Frank A. Hegmann, Masayoshi Tonouchi, Junichiro Kono, Iwao Kawayama, and Marco Battiato
    • Journal Title

      Nano Lett. 2020

      Volume: 20,05 Issue: 5 Pages: 3098-3105

    • DOI

      10.1021/acs.nanolett.9b05082

    • Related Report
      2020 Annual Research Report 2019 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Ultrafast Exciton Dynamics in Semiconducting Carbon Nanotubes Probed by Terahertz Emission and Photocurrent Spectroscopy2020

    • Author(s)
      Filchito Bagsican, Michael Wais, Natsumi Komatsu, Weilu Gao, Kazunori Serita, Hironaru Murakami, Karsten Held, Iwao Kawayama, Junichiro Kono, Masayoshi Tonouchi, Marco Battiato
    • Organizer
      The 81st JSAP Autumn Meeting
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Terahertz science and technology: exploring the last frontier of the electromagnetic spectrum2019

    • Author(s)
      Filchito Renee G. Bagsican, Iwao Kawayama, Hironaru Murakami, and Masayoshi Tonouchi
    • Organizer
      21st SPVM National Physics Conference, and 2019 Int’l. Conference on Advanced Functional Materials and Nanotechnology
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Probing photocarrier dyamics in semiconducting carbon nanotubes by terahertz emission spectroscopy2019

    • Author(s)
      Filchito Renee G. Bagsican, Iwao Kawayama, Michael Wais, Natsumi Komatsu, Kazunori Serita, Weilu Gao, Lincoln Weber, Marco Battiato, Hironaru Murakami, Frank A. Hegmann, Junichiro Kono and Masayoshi Tonouchi
    • Organizer
      21st SPVM National Physics Conference, and 2019 Int’l. Conference on Advanced Functional Materials and Nanotechnology
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser terahertz emission microscopy as an investigative tool for low-dimensional materials2019

    • Author(s)
      Filchito Renee G. Bagsican, Iwao Kawayama, Hironaru Murakami, and Masayoshi Tonouchi
    • Organizer
      The 1st International Conference in Science and Mathematics (ICSM 2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Terahertz Emission from a Photoconductive Antenna Switch Based on Aligned Single-Chirality Semiconducting Carbon Nanotubes2019

    • Author(s)
      F.R. Bagsican, I. Kawayama, M. Wais, N. Komatsu, K. Serita, W. Gao, L. Weber, M. Battiato, H. Murakami, F.A. Hegmann, J. Kono, and M. Tonouchi
    • Organizer
      The 21st International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures (EDISON21)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Terahertz emission from photoconductive antenna switches based on highly-aligned and chirality-enriched semiconducting carbon nanotubes2019

    • Author(s)
      F.R. Bagsican, I. Kawayama, M. Wais, N. Komatsu, K. Serita, W. Gao, L. Weber, M. Battiato, H. Murakami, F.A. Hegmann, J. Kono, and M. Tonouchi
    • Organizer
      Optical Terahertz Science & Technology Conference (OTST)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research

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Published: 2019-04-18   Modified: 2022-01-27  

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