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Development of wide-frequency band and high-frequency tunneling magneto-dielectric effect in gradient granular structure

Research Project

Project/Area Number 19K15285
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 26020:Inorganic materials and properties-related
Research InstitutionTohoku University

Principal Investigator

Cao Yang  東北大学, 学際科学フロンティア研究所, 助教 (50804598)

Project Period (FY) 2019-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2020: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2019: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywordscomposition-gradient / broadband frequency / magneto-dielectric / Si dopant / dielectric enhanment / Composition-gradient / large enhancement / dielectric properties / nanogranular films / Dielectric properties / Magneto-dielectric / Granular nanostructure / Gradient distribution / tunnel magnetodielectric / high-frequency response
Outline of Research at the Start

In 2014, we discover a tunneling magneto-dielectric (TMD) effect in nanocomposites based on a completely new mechanism of spin-dependent quantum tunneling phenomenon. From the practical viewpoint,wide-frequency band, high-frequency TMD effect is very demanding. Here, to achieve this objective, I propose a granular-Functional Gradient Materials with wide distribution of inter-granular spacing.

Outline of Final Research Achievements

Tunnelling magneto-dielectric (TMD) effect in nanocomposites discovered by our group in 2014 features a narrow peak of the maximum dielectric variations. This limits its magnetoelectric application over a wide frequency range. From the practical viewpoint, it is highly demanded to develop the broadband TMD response. In this research, I have proposed and fabricated a composition-gradient multilayer nanogranular structure that can exhibit a broadband TMD effect up to megahertz frequency range. Additionally, I have realized the unprecedented high TMD response of up to 8.5% with small addition of Si into the conventional nanogranular films.

Academic Significance and Societal Importance of the Research Achievements

This research results may have potential in practical high-frequency band device applications in such as 5G cell phones as well as other high-frequency mobile devices.

Report

(3 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • Research Products

    (11 results)

All 2021 2020 2019

All Journal Article (3 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 3 results) Presentation (8 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results)

  • [Journal Article] Composition-graded multilayer nanogranular films enabling broadband tunneling magneto-dielectric effect: Role of the granular distribution2021

    • Author(s)
      Cao Yang、Kobayashi Nobukiyo、Ohnuma Shigehiro、Masumoto Hiroshi
    • Journal Title

      Applied Physics Letters

      Volume: 118 Issue: 3 Pages: 032901-032901

    • DOI

      10.1063/5.0027233

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Large magnetodielectric effect based on spin-dependent charge transfer in metal?insulator type Co-(BaF2) nanogranular films2020

    • Author(s)
      Kijima-Aoki Hanae、Cao Yang、Kobayashi Nobukiyo、Takahashi Saburo、Ohnuma Shigehiro、Masumoto Hiroshi
    • Journal Title

      Journal of Applied Physics

      Volume: 128 Issue: 13 Pages: 133904-133904

    • DOI

      10.1063/5.0021636

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Large tunneling magneto-dielectric enhancement in Co(Fe)-MgF2 granular films by minor addition of Si2020

    • Author(s)
      Cao Yang、Kobayashi Nobukiyo、Ohnuma Shigehiro、Masumoto Hiroshi
    • Journal Title

      Applied Physics Letters

      Volume: 117 Issue: 7 Pages: 072904-072904

    • DOI

      10.1063/5.0014137

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] スパッタリング法による Fe-F-C ナノ複相薄膜の構造と磁気-誘電特性2021

    • Author(s)
      野川健太,曹 洋, 青木 英恵, 小林 伸聖, 大沼 繁弘, 増本 博
    • Organizer
      日本セラミックス協会基礎科学討論会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Structure and dielectric properties of (CoF/FeF)-C nanocomposites2020

    • Author(s)
      Yang Cao, Nogawa Kenta, Nobukiyo Kobayashi, Shigehiro Ohnuma, and Hiroshi Masumoto
    • Organizer
      日本セラミックス協会 第33回秋季シンポジウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] トンネル効果に与える Co-BaF2 ナノグラニュラー層状膜の Co 粒子の形状と周期性の影響2020

    • Author(s)
      青木 英恵, 曹 洋, 大沼 繁弘, 小林 伸聖, 増本 博
    • Organizer
      日本金属学会2020年秋期講演大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Co-MgO 系ナノコンポジット薄膜の電気および磁気特性2020

    • Author(s)
      木村 萌,曹 洋, 青木 英恵, 大沼 繁弘, 小林 伸聖, 増本 博
    • Organizer
      日本金属学会2020年秋期講演大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe-PTFE 系ナノ複相薄膜の構造と磁気-誘電特性2020

    • Author(s)
      野川健太,曹 洋, 青木 英恵, 小林 伸聖, 大沼 繁弘, 増本 博
    • Organizer
      日本セラミックス協会東北北海道支部研究表会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Tunneling Magneto-Dielectric (TMD) effect: Recent advances and future perspectives2019

    • Author(s)
      Yang Cao
    • Organizer
      The 10th Pacific Rim International Conference on Advanced Materials and Processing (PRICM10)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Emerging Tunneling Magneto-Dielectric (TMD) Effect and Recent Progress2019

    • Author(s)
      Yang Cao
    • Organizer
      The 11th China-Japan Symposium on Ferroelectric Materials and Their Applications
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Structure and Magneto-dielectric Properties in Co-F-C Nanocomposites2019

    • Author(s)
      Yang Cao
    • Organizer
      The 13th Pacific Rim Conference of Ceramic Societies (PACRIM13)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research

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Published: 2019-04-18   Modified: 2022-01-27  

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