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Development of spin-valley quantum devices based on graphene heterostructures

Research Project

Project/Area Number 19K15385
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 28020:Nanostructural physics-related
Research InstitutionNational Institute for Materials Science

Principal Investigator

IWASAKI Takuya  国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, 独立研究者 (50814274)

Project Period (FY) 2019-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2020: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2019: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywordsグラフェン / 六方晶窒化ホウ素 / モアレ超格子 / 量子ドット / 量子ホール効果 / 単一電子輸送 / 量子輸送 / 単電子輸送 / 量子デバイス / 単電子デバイス / バレートロニクス / デバイス物理
Outline of Research at the Start

二次元材料であるグラフェンおよび六方晶窒化ホウ素(hBN)を、ファンデルワールス転写法により結晶方位を揃えて積層させたグラフェン/hBNモアレ超格子ヘテロ構造を用いて、量子力学的自由度であるスピンとバレーを用いた基礎的な機能素子を開発する。この素子を用いて、グラフェンおよびグラフェン/hBNモアレ超格子のキャリア輸送におけるスピン・バレー依存性を評価・解析し、超低消費電力素子の実現および物性物理学におけるバレーの役割・性質のより深い理解・解明を目指す。

Outline of Final Research Achievements

We aimed to develop graphene heterostructure-based devices that control the spin and valley degrees of freedom. First, we developed a bubble-free transfer technique that allows producing high-quality heterostructures with a high yield. By this technique, graphene/hexagonal boron nitride (hBN) heterostructure and moire superlattice were fabricated, and the high quality bilayer graphene device was realized. We also fabricated the double-quantum dot device using the moire superlattice structure and observed the single-carrier transport and quantum Hall effect in the moire superlattice. Furthermore, we fabricated the twisted bilayer/bilayer graphene/hBN device and observed an insulating state due to a strong correlation.

Academic Significance and Societal Importance of the Research Achievements

本研究で開発したバブルフリー転写法は、遷移金属ダイカルコゲナイド等様々な層状物質に応用可能であるため、二次元物質研究分野の更なる発展に貢献する重要な成果である。また、モアレ超格子二重量子ドット素子の実現はこれまで困難であった磁場中のモアレ超格子量子ドット特有の単電子輸送特性の解析が可能とし、電子一個を制御する究極の低消費電力・量子情報処理技術の発展に繋がる重要な成果である。ツイスト構造に関する結果は、「折り畳んでツイスト構造を作る」という新しい設計指針を与え、急速に発達している当該分野において、高品質素子作製工程のブレークスルーとなる可能性があり、将来のデバイス応用の基礎となる成果である。

Report

(3 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • Research Products

    (27 results)

All 2021 2020 2019 Other

All Journal Article (5 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 5 results) Presentation (20 results) (of which Int'l Joint Research: 7 results,  Invited: 1 results) Remarks (1 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Room-temperature negative magnetoresistance of helium-ion-irradiated defective graphene in the strong Anderson localization regime2021

    • Author(s)
      Iwasaki Takuya、Nakamura Shu、Agbonlahor Osazuwa G.、Muruganathan Manoharan、Akabori Masashi、Morita Yoshifumi、Moriyama Satoshi、Ogawa Shinichi、Wakayama Yutaka、Mizuta Hiroshi、Nakaharai Shu
    • Journal Title

      Carbon

      Volume: 175 Pages: 87-92

    • DOI

      10.1016/j.carbon.2020.12.076

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Bubble-Free Transfer Technique for High-Quality Graphene/Hexagonal Boron Nitride van der Waals Heterostructures2020

    • Author(s)
      Iwasaki Takuya、Endo Kosuke、Watanabe Eiichiro、Tsuya Daiju、Morita Yoshifumi、Nakaharai Shu、Noguchi Yutaka、Wakayama Yutaka、Watanabe Kenji、Taniguchi Takashi、Moriyama Satoshi
    • Journal Title

      ACS Applied Materials & Interfaces

      Volume: 12 Issue: 7 Pages: 8533-8538

    • DOI

      10.1021/acsami.9b19191

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fabrication of folded bilayer-bilayer graphene/hexagonal boron nitride superlattices2020

    • Author(s)
      Iwasaki Takuya、Morita Yoshifumi、Nakaharai Shu、Wakayama Yutaka、Watanabe Eiichiro、Tsuya Daiju、Watanabe Kenji、Taniguchi Takashi、Moriyama Satoshi
    • Journal Title

      Applied Physics Express

      Volume: 13 Issue: 3 Pages: 035003-035003

    • DOI

      10.35848/1882-0786/ab790d

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Single-Carrier Transport in Graphene/hBN Superlattices2020

    • Author(s)
      Iwasaki Takuya、Nakaharai Shu、Wakayama Yutaka、Watanabe Kenji、Taniguchi Takashi、Morita Yoshifumi、Moriyama Satoshi
    • Journal Title

      Nano Letters

      Volume: 20 Issue: 4 Pages: 2551-2557

    • DOI

      10.1021/acs.nanolett.9b05332

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fabrication and characterization of quantum dot devices based on tetralayer graphene/hexagonal boron nitride heterostructures2019

    • Author(s)
      Iwasaki Takuya、Kato Taku、Ito Hirohito、WATANABE Kenji、Taniguchi Takashi、Wakayama Yutaka、Hatano Tsuyoshi、Moriyama Satoshi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: 2 Pages: 024001-024001

    • DOI

      10.7567/1347-4065/ab65a8

    • NAID

      210000157928

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Presentation] Observation of charge carrier localization-induced negative magnetoresistance at room temperature in helium-ion-irradiated defective graphene2020

    • Author(s)
      Takuya Iwasaki, Shu Nakamura, Osazuwa Gabriel Agbonlahor, Manoharan Muruganathan, Masashi Akabori, Yoshifumi Morita, Satoshi Moriyama, Shinichi Ogawa, Yutaka Wakayama, Hiroshi Mizuta, and Shu Nakaharai
    • Organizer
      2020 International Conference on Solid State Devices and Materials
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Quantum transport in graphene/hexagonal boron nitride superlattices2020

    • Author(s)
      Takuya Iwasaki
    • Organizer
      A3 Foresight Program, 7th International Workshop on 2D Materials
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Strong Carrier Localization in Defective Graphene Induced by Helium Ion Irradiation.2020

    • Author(s)
      Takuya Iwasaki, Shu Nakamura, Osazuwa Gabriel Agbonlahor, Manoharan Muruganathan, Masashi Akabori, Yoshifumi Morita, Satoshi Moriyama, Shinichi Ogawa, Yutaka Wakayama, Hiroshi Mizuta, and Shu Nakaharai,
    • Organizer
      MANA International Symposium 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 垂直磁場下における4 層 グラフェン単一量子ドットデバイスの電気伝導特性2020

    • Author(s)
      加藤拓, 伊藤博仁, 岩崎拓哉, 渡邊賢司, 谷口尚, 森山悟士, 羽田野剛司
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Negative magnetoresistance of helium-ion-irradiated graphene in the strong Anderson localization regime2020

    • Author(s)
      Takuya Iwasaki, Muruganathan Manoharan, Masashi Akabori, Yoshifumi Morita, Satoshi Moriyama, Shinichi Ogawa, Yutaka Wakayama, Hiroshi Mizuta, Shu Nakaharai
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] モアレ超格子二重量子ドット素子における量子ホール効果と単一キャリア輸送特性2020

    • Author(s)
      岩崎拓哉, 中払周, 若山裕, 渡邊賢司, 谷口尚, 守田佳史, 森山悟士
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 4層グラフェンを用いた量子ドットデバイスの垂直磁場依存性2020

    • Author(s)
      加藤拓, 岩崎拓哉, 渡邊賢司, 谷口尚, 森山悟士, 羽田野剛司
    • Organizer
      第75回応用物理学会東北支部学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 垂直磁場下におけるグラフェン多重量子ドットの結合状態の変化2020

    • Author(s)
      加藤拓, 岩崎拓哉, 渡邊賢司, 谷口尚, 森山悟士, 羽田野剛司
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] バブルフリー転写法による高品質ファンデルワールス積層構造の作製2020

    • Author(s)
      岩崎拓哉, 渡辺英一郎, 津谷大樹, 守田佳史, 中払周, 若山裕, 渡邊賢司, 谷口尚, 森山悟士
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] モアレ超格子二重量子ドット素子における単一キャリア輸送2020

    • Author(s)
      岩崎拓哉, 中払周, 若山裕, 渡邊賢司, 谷口尚, 守田佳史, 森山悟士
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] High-quality quantum devices based on graphene/hexagonal boron nitride heterostructures fabricated by a bubble-free transfer technique2020

    • Author(s)
      T. Iwasaki, K. Endo, E. Watanabe, D. Tsuya, Y. Morita, S. Nakaharai, Y. Noguchi, Y. Wakayama, K.Watanabe, T. Taniguchi, and S. Moriyama
    • Organizer
      MANA International Symposium 2020
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] 二層グラフェン/六方晶窒化ホウ素超格子二重量子ドットにおける単キャリア輸送特性2020

    • Author(s)
      岩崎拓哉, 中払周, 若山裕, 渡邊賢司, 谷口尚, 守田佳史, 森山悟士
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] 4層グラフェン/hBNヘテロ構造を用いた量子ドットの電子輸送特性2020

    • Author(s)
      伊藤博仁, 加藤拓, 岩崎拓哉, 渡邊賢司, 谷口尚, 森山悟士, 羽田野剛司
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] 折り重ね二層/二層グラフェン素子の作製とキャリア輸送特性2020

    • Author(s)
      岩崎拓哉, 中払周, 若山裕, 渡邊賢司, 谷口尚, 守田佳史, 森山悟士
    • Organizer
      第67回春季応用物理学会学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] 二層グラフェン/hBN超格子における単キャリア輸送特性.2020

    • Author(s)
      岩崎拓哉, 中払周, 若山裕, 渡邊賢司, 谷口尚, 守田佳史, 森山悟士
    • Organizer
      第67回春季応用物理学会学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] バブルフリー転写法による高品質グラフェン/hBN素子の作製2020

    • Author(s)
      岩崎拓哉, 遠藤滉亮, 渡辺英一郎, 津谷大樹, 守田佳史, 中払周, 野口裕, 若山裕, 渡邊賢司, 谷口 尚, 森山悟士,
    • Organizer
      第67回春季応用物理学会学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] 4 層グラフェン/hBN構造を持つ量子ドットの電気伝導特性2020

    • Author(s)
      加藤拓, 伊藤博仁, 岩崎拓哉, 渡邊賢司, 谷口尚, 森山悟士, 羽田野剛司
    • Organizer
      第67回春季応用物理学会学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] Quantum Transports in hBN/Graphene Superlattices2019

    • Author(s)
      T. Iwasaki, K. Komatsu, K. Endo, S. Nakaharai, Y. Noguchi, Y. Wakayama, E. Watanabe, D. Tsuya, K.Watanabe, T. Taniguchi, Y. Morita, and S. Moriyama
    • Organizer
      International Conference of Strongly Correlated Electron Systems (SCES 2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Valley Hall Effects in Graphene/hBN Superlattices2019

    • Author(s)
      T. Iwasaki, K. Komatsu, K. Endo, E.Watanabe, D. Tsuya, K.Watanabe, T. Taniguchi, Y. Noguchi, Y. Wakayama, Y. Morita, and S. Moriyama
    • Organizer
      The 11th annual Recent Progress in Graphene and Two-dimensional Materials Research Conference (RPGR2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Valley Hall Effect in Graphene/Hexagonal Boron Nitride Superlattices2019

    • Author(s)
      T. Iwasaki
    • Organizer
      The 2019 Frontiers in Quantum Materials and Devices workshop (FQMD)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Remarks] 研究者総覧SAMURAI

    • URL

      https://samurai.nims.go.jp/profiles/iwasaki_takuya

    • Related Report
      2019 Research-status Report
  • [Patent(Industrial Property Rights)] 貼り合わせ装置、貼り合わせ方法およびそれを用いた素子の製造方法2020

    • Inventor(s)
      岩崎拓哉, 森山悟士
    • Industrial Property Rights Holder
      国立研究開発法人物質・材料研究機構
    • Industrial Property Rights Type
      特許
    • Filing Date
      2020
    • Related Report
      2019 Research-status Report

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Published: 2019-04-18   Modified: 2022-01-27  

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