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Generation of Multicolor and Ultrashort pulse laser and development of its applications

Research Project

Project/Area Number 20245018
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Analytical chemistry
Research InstitutionKyushu University

Principal Investigator

IMASAKA Totaro  Kyushu University, 大学院・工学研究院, 主幹教授 (30127980)

Co-Investigator(Kenkyū-buntansha) IMASAKA Tomoko  九州大学, 大学院・芸術工学研究院, 教務職員 (90193721)
内村 智博  九州大学, 工学研究院, 助教 (40346820)
財津 慎一  九州大学, 工学研究院, 助教 (60423521)
Co-Investigator(Renkei-kenkyūsha) UCHIMURA Tomohiro  九州大学, 大学院, 工学研究員・助教 (40346820)
ZAITSU Shinichi  九州大学, 大学院, 工学研究員・助教 (60423521)
Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥47,580,000 (Direct Cost: ¥36,600,000、Indirect Cost: ¥10,980,000)
Fiscal Year 2010: ¥7,410,000 (Direct Cost: ¥5,700,000、Indirect Cost: ¥1,710,000)
Fiscal Year 2009: ¥15,470,000 (Direct Cost: ¥11,900,000、Indirect Cost: ¥3,570,000)
Fiscal Year 2008: ¥24,700,000 (Direct Cost: ¥19,000,000、Indirect Cost: ¥5,700,000)
Keywordsレーザー / 非線形光学 / 超短パルス光 / 誘導ラマン散乱 / 四波ラマン混合 / 多色レーザー / 質量分析 / パルス幅測定
Research Abstract

In this project, we developed novel light sources having a multifrequemcy/broadband spectrum based on a stimulated Raman effect pumped by continuous-wave (cw) and ultrashort pulse lasers. A three-primary-color emission that could be used for the generation of an extremely highly repetitive cw optical pulse train was generated through phase-matched four-wave mixing process in the dispersion-compensated high-finesse optical cavity. In addition, our newly developed molecular modulation scheme allowed for the generation of broadband deep-ultraviolet radiation that corresponded to a duration of 10 femtosecond and the demonstration of dramatic enhancement of the detection limit of explosive chemical compounds.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (52 results)

All 2011 2010 2009 2008 Other

All Journal Article (34 results) (of which Peer Reviewed: 27 results) Presentation (17 results) Remarks (1 results)

  • [Journal Article] In Situ Third-Order Interferometric Autocorrelation of a Femtosecond Deep-Ultraviolet Pulse2011

    • Author(s)
      Yuki Miyoshi, Shin-ichi Zaitsu, Totaro Imasaka
    • Journal Title

      Applied Physics B Vol.102,in press.

    • NAID

      120004951626

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] In Situ Third-Order Interferometric Autocorrelation of a Femtosecond Deep-Ultraviolet Pulse2011

    • Author(s)
      Yuki MIYOSHI, et al.
    • Journal Title

      Applied Physics B

      Volume: 102(in press)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] コヒーレントラマン散乱による超短パルス光の発生とレーザーイオン化質量分析法への応用2010

    • Author(s)
      財津慎一、今坂藤太郎
    • Journal Title

      化学工業 第61巻、10号

      Pages: 761-768

    • Related Report
      2010 Final Research Report
  • [Journal Article] Two-Color Stimulated Raman Effect for the Generation of Ultrashort Optical Pulse2010

    • Author(s)
      今坂藤太郎
    • Journal Title

      Proc.Fifth Asian Symposium on Intense Laser Science (ASILS-5) Vol.5

      Pages: 47-54

    • Related Report
      2010 Final Research Report
  • [Journal Article] A Self-Quenching Picosecond Distributed Feedback Dye Laser Pumped by a Picosecond Laser Pulse2010

    • Author(s)
      Quang Do HOA, Pham LONG, Totaro IMASAKA
    • Journal Title

      Applied Physics.B Vol.101

      Pages: 571-574

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Generation of High-Order Rotational Raman Sidebands in the Deep-Ultraviolet Region Using Molecular Phase Modulation Induced by an Intensity-Modulated Optical Pulse2010

    • Author(s)
      Norifumi YASAKA, Yuichiro KIDA, Shin-ichi ZAITSU, Totaro IMASAKA
    • Journal Title

      Journal of Applied Physics Vol.108

      Pages: 56104-56104

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Gas Chromatography/Femto-second Multiphoton Ionization/Time-of-Flight Mass Spectrometry of Dioxins2010

    • Author(s)
      Yuka WATANABE-EZOE, Xing LI, Tomoko IMASAKA, Tomohiro UCHIMURA, Totaro IMASAKA
    • Journal Title

      Analytical Chemistry Vol.82

      Pages: 6519-652

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Enhancement of Molecular Ions in Mass Spectrometry Using an Ultrashort Optical Pulse in Multiphoton Ionization2010

    • Author(s)
      Takashi SHIMIZU, Yuka WATANABE-EZOE, Satoshi YAMAGUCHI, Hiroko TSUKATANI, Tomoko IMASAKA, Shin-ichi ZAITSU, Tomohiro UCHIMURA, Totaro IMASAKA
    • Journal Title

      Analytical Chemistry Vol.82

      Pages: 3441-3444

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Enhancement of Molecular Ions in Mass Spectrometry Using an Ultrashort Optical Pulse in Multiphoton Ionization2010

    • Author(s)
      Takashi SHIMIZU, et al.
    • Journal Title

      Analytical Chemistry

      Volume: 82 Pages: 3441-3444

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Gas Chromatography/Femtosecond Multiphoton Ionization/Time-of-Flight Mass Spectrometry of Dioxins2010

    • Author(s)
      Yuka WATANABE-EZOE, et al.
    • Journal Title

      Analytical Chemistry

      Volume: 82 Pages: 6519-6525

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Generation of High-Order Rotational Raman Sidebands in the Deep-Ultraviolet Region Using Molecular Phase Modulation Induced by an Intensity-Modulated Optical Pulse2010

    • Author(s)
      Norifumi YASAKA, et al.
    • Journal Title

      Journal of Applied Physics

      Volume: 108 Pages: 56104-56104

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A Self-Quenching Picosecond Distributed Feedback Dye Laser Pumped by a Picosecond Laser Pulse2010

    • Author(s)
      Quang Do HOA, et al.
    • Journal Title

      Applied Physics.B

      Volume: 101 Pages: 571-574

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Two-Color Stimulated Raman Effect for the Generation of Ultrashort Optical Pulse2010

    • Author(s)
      Totaro IMASAKA
    • Journal Title

      Proceedings of Fifth Asian Symposium on Intense Laser Science

      Volume: 5 Pages: 47-54

    • Related Report
      2010 Annual Research Report
  • [Journal Article] コヒーレントラマン散乱による超短パルス光の発生とレーザーイオン化質量分析法への応用2010

    • Author(s)
      財津慎一、今坂藤太郎
    • Journal Title

      化学工業

      Volume: 61 Pages: 761-768

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Molecular System of Hydrogens2009

    • Author(s)
      今坂藤太郎
    • Journal Title

      Science for Future Molecular Systems Vol.3

      Pages: 37-43

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] 超高速分子光パルス整形2009

    • Author(s)
      貴田祐一郎、財津慎一、今坂藤太郎
    • Journal Title

      レーザー研究 第37巻、第4号

      Pages: 304-31

    • NAID

      10024748493

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Coherent Molecular Rotations Induced by a Femtosecond Pulse Consisting of Two Orthogonally Polarized Pulses2009

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Journal Title

      Physical Review A Vol.80,No.2

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Compression of an Ultraviolet Pulse by Molecular Phase Modulation and Self-Phase Modulation2009

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Journal Title

      Ultrafast Phenomena XVI Vol.16

      Pages: 816-818

    • Related Report
      2010 Final Research Report
  • [Journal Article] The S1 ← SO 0-0 Transition Energies of Poly-chlorinated Dibenzofurans (PCDFs) Revisited : CIS(D) and MP2 Calculations with Correction for Correlation Energies2009

    • Author(s)
      Shoko HIROKAWA, Tomoko IMASAKA, Totaro IMASAKA
    • Journal Title

      ournal of Molecular Structure : THEOCHEM Vol.915,No.1-3

      Pages: 79-85

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Gas Chromatography/ Time-of-Flight Mass Spectrometry of Triacetone Tri-peroxide Based on Femtosecond Laser Ionization2009

    • Author(s)
      Satoshi YAMAGUCHI, Tomohiro UCHIMURA, Tomoko IMASAKA, Totaro IMASAKA
    • Journal Title

      Rapid Communications in Mass Spectrometry Vol.23,No.19

      Pages: 3101-3106

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Analysis of Highly Chlorinated Dibenzofurans Using Gas Chromato-graphy/Multiphoton Tonzation/Time-of-flight Mass Spectrometry2009

    • Author(s)
      Yuka Watanabe-Ezoe, Koretaka OHI, Tomohiro UCHIMURA, Totaro IMASAKA
    • Journal Title

      Organohalogen Compounds Vol.71

      Pages: 271-274

    • Related Report
      2010 Final Research Report
  • [Journal Article] Data Processing Technique in Gas Chromatography/ Time-of-Flight Mass Spectrometry2009

    • Author(s)
      Tomoko IMASAKA, Nami NAKAMURA, Yuji SAKODA, Satoshi YAMAGUCHI, Yuka WATANABE-EZOE, Tomohiro UCHIMURA, Totaro IMASAKA
    • Journal Title

      Analyst Vol.134,No.4

      Pages: 712-718

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Near-Ultraviolet Femtosecond Laser Ionization of Dioxins in Gas Chromatography/Time-of-Flight Mass Spectrometry2009

    • Author(s)
      Satoshi YAMAGUCHI, Fumiaki Kira, Yuki MIYOSHI, Tomohiro UCHIMURA, Yuka WATANABE-EZOE, Shin-ichi ZAITSU, Tomoko IMASAKA, Totaro IMASAKA
    • Journal Title

      Analytica Chimica Acta Vol.632,No.2

      Pages: 229-233

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Molecular System of Hydrogens2009

    • Author(s)
      Totaro IMASAK
    • Journal Title

      Science for Future Molecular Systems

      Volume: 3 Pages: 37-43

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Compression of an Ultraviolet Pulse by Molecular Phase Modulation and Self-Phase Modulation2009

    • Author(s)
      Y.Kida, S.Zaitsu, T.Imasaka,
    • Journal Title

      Ultrafast Phenomena XVI 16

      Pages: 816-818

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Coherent Molecular Rotations Induced by a Femtosecond Pulse Consisting of Two Orthogonally Polarized Pulses2009

    • Author(s)
      Y.Kida, S.Zaitsu, T.Imasaka,
    • Journal Title

      Physical Review A 80

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 超高速分子光パルス整形2009

    • Author(s)
      貴田祐一郎、財津慎一、今坂藤太郎
    • Journal Title

      レーザー研究 37

      Pages: 304-311

    • NAID

      10024748493

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Generating Short-Pulse Laser by Using a Quenched Distributed Feedback Dye Laser2008

    • Author(s)
      D.Q.HOA, V.DUONG, P.LONG, T.H.NHUNG, Totaro IMASAKA
    • Journal Title

      Journal of Korean Physical Society Vol.53

      Pages: 3823-3826

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Stimulated Rotational Raman Scattering by a Polarization-Modulated Femtosecond Pulse2008

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Journal Title

      Physical Review A Vol.77

      Pages: 63802-63802

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] 分子変調モード同期レーザーによる連続発振超高繰り返しパルス列の発生2008

    • Author(s)
      財津慎一、今坂藤太郎
    • Journal Title

      レーザー研究 第36巻

      Pages: 433-439

    • NAID

      10021106200

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Generation of Intense 11-fs Ultraviolet Pulses Using Phase Modulation by Two Types of Coherent Molecular Motions2008

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Journal Title

      Optics Express Vol.16

      Pages: 13492-13498

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Generation of Intense 11-fs Ultraviolet Pulses Using Phase Modulation by Two Types of Coherent Molecular Motions2008

    • Author(s)
      Yuichiro Kida, Shin-ichi Zaitsu, Totaro Imasaka
    • Journal Title

      Optics Express 16

      Pages: 13492-13498

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 分子変調モード同期レーザーによる連続発振光繰り返しパルス列の発生2008

    • Author(s)
      財津慎一, 今坂藤太郎
    • Journal Title

      レーザー研究 36

      Pages: 433-439

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Stimulated Rotational Raman Scattering by a Polarization-Modulated Femtosecond Pulse2008

    • Author(s)
      Yuichiro Kida, Shin-ichi Zaitsu, Totaro Imasaka
    • Journal Title

      Physical Review A 77

      Pages: 63802-63802

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] 光ビート励起分子位相変調を用いて発生させた深紫外超短パルス光の測定2011

    • Author(s)
      八坂訓史、財津慎一、今坂藤太郎
    • Organizer
      レーザー学会学術講演会第31回年次大会
    • Place of Presentation
      電気通信大学
    • Year and Date
      2011-01-10
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] 分散補償光共振器を用いた三原色連続発振ラマンレーザー2010

    • Author(s)
      高林順平、財津慎一、今坂藤太郎
    • Organizer
      第71回応用物理学会学術講演会
    • Place of Presentation
      長崎大学
    • Year and Date
      2010-09-16
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Pesticides Analysis Using Gas Chromatography/Multiphoton Ionization/Mass Spectrometry with a Femtosecond laser2010

    • Author(s)
      Adan Li, Tomohiro Uchimura, Totaro Imasaka
    • Organizer
      日本分析化学会第59年会
    • Place of Presentation
      東北大学
    • Year and Date
      2010-09-15
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Generation of High-Order Raman Emissions in the Deep Ultraviolet Region Using Molecular Phase Modulation2010

    • Author(s)
      八坂訓史, 貴田祐一郎, 財津慎一, 今坂藤太郎
    • Organizer
      The 6th Asian Conference on Ultrafast phenomena
    • Place of Presentation
      National Taiwan University, Taipei
    • Year and Date
      2010-01-12
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] The generation of an Ultrashort Optical Pulse Train at the World-Fastest Repetition Rate2010

    • Author(s)
      今坂藤太郎
    • Organizer
      The 6th Asian Conference on Ultrafast phenomena
    • Place of Presentation
      National Taiwan University, Taipei
    • Year and Date
      2010-01-11
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] 光ビート励起分子位相変調による深紫外高次誘導ラマン光の発生2009

    • Author(s)
      八坂訓史、財津慎一、今坂藤太郎
    • Organizer
      第70回応用物理学会学術講演会
    • Place of Presentation
      富山大学
    • Year and Date
      2009-09-08
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] 中空キャピラリー導波路を用いた紫外超短パルス励起高次誘導ラマン散乱光の発生2009

    • Author(s)
      繹迦野卓,財津慎一,今坂藤太郎
    • Organizer
      第70回応用物理学会学術講演会
    • Place of Presentation
      富山大学
    • Year and Date
      2009-09-08
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] 位相整合四光波混合により発生した連続発振ラマンサイドバンドのフーリエ合成2009

    • Author(s)
      財津慎一、井崎博大、今坂藤太郎
    • Organizer
      第56回応用物理学関連連合講演会
    • Place of Presentation
      筑波大学
    • Year and Date
      2009-03-30
    • Related Report
      2010 Final Research Report 2008 Annual Research Report
  • [Presentation] 二色誘導ラマン散乱によるコヒーレント分子運動誘起2008

    • Author(s)
      貴田祐一郎、財津慎一、今坂藤太郎
    • Organizer
      第69回応用物理学会秋季学術講演会
    • Place of Presentation
      中部大学
    • Year and Date
      2008-09-04
    • Related Report
      2010 Final Research Report 2008 Annual Research Report
  • [Presentation] 位相同期連続発振多波長レーザーによる高繰り返し超短パルス列の発生2008

    • Author(s)
      井崎博大、財津慎一、今坂藤太郎
    • Organizer
      第69回応用物理学会秋季学術講演会
    • Place of Presentation
      中部大学
    • Year and Date
      2008-09-02
    • Related Report
      2010 Final Research Report 2008 Annual Research Report
  • [Presentation] 中空キャピラリー導波路を用いた超短パルス励起紫外ラマン光発生2008

    • Author(s)
      繹迦野卓、財津慎一、今坂藤太郎
    • Organizer
      第69回応用物理学会秋季学術講演会
    • Place of Presentation
      中部大学
    • Year and Date
      2008-09-02
    • Related Report
      2010 Final Research Report 2008 Annual Research Report
  • [Presentation] Compression of an Ultraviolet Pulse by Molecular Phase Modulation and Self-Phase Modulation2008

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Organizer
      Conference on Ultrafast Phenomena 2008
    • Place of Presentation
      Stresa Convention Centre, Italy
    • Year and Date
      2008-06-10
    • Related Report
      2010 Final Research Report
  • [Presentation] Compression of an Ultraviolet Pulse by Molecular Phase Modulation and Self-Phase Modulation2008

    • Author(s)
      Yuichiro Kida, et al.
    • Organizer
      Conference on Ultrafast Phenomena 2008
    • Place of Presentation
      Stresa Convention Centre
    • Year and Date
      2008-06-10
    • Related Report
      2008 Annual Research Report
  • [Presentation] Continuous-wave phase-matched generation of Raman sidebands in a dispersion-managed optical cavity2008

    • Author(s)
      Shin-ichi Zautsu, Hirotomo Izaki, Totaro Imasaka
    • Organizer
      Conference on Lasers and Electro-Optics 2008
    • Place of Presentation
      San Jose McEnery Convention Center, California
    • Year and Date
      2008-05-08
    • Related Report
      2010 Final Research Report
  • [Presentation] Generation of a 12-fs Ultraviolet Optical Pulse Using Two Types of Coherent Molecular Rotations2008

    • Author(s)
      貴田祐一郎, 財津慎一, 今坂藤太郎
    • Organizer
      Conference on Lasers and Electro-Optics 2008
    • Place of Presentation
      San Jose McEnery Convention Center, California
    • Year and Date
      2008-05-08
    • Related Report
      2010 Final Research Report
  • [Presentation] Generation of a 12-fs Ultraviolet Optical Pulse Using Two Types of Coherent Molecular Rotations2008

    • Author(s)
      Yuichiro Kida, et al.
    • Organizer
      Conference on Lasers and Electro-Optics 2008
    • Place of Presentation
      San Jose McEnery Convention Center
    • Year and Date
      2008-05-08
    • Related Report
      2008 Annual Research Report
  • [Presentation] Continuous-wave phase-matched generation of Raman sidebands in a dispersion-managed optical cavity2008

    • Author(s)
      Shin-ichi Zautsu, et al.
    • Organizer
      Conference on Lasers and Electro-Optics 2008
    • Place of Presentation
      San Jose McEnery Convention Center
    • Year and Date
      2008-05-08
    • Related Report
      2008 Annual Research Report
  • [Remarks] ホームページ等

    • Related Report
      2010 Final Research Report

URL: 

Published: 2008-04-01   Modified: 2017-10-13  

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