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Control of photoluminescence properties in semiconductor quantum dots by using the interaction with polymers

Research Project

Project/Area Number 20540316
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics I
Research InstitutionKagawa University

Principal Investigator

NAKANISHI Shunsuke  Kagawa University, 工学部, 教授 (30155767)

Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2010: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2009: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2008: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywords量子ドット / CdSe / ZnS / 高分子 / TiO_2ナノ粒子 / 金属ナノ粒子 / Blinking / 位相緩和 / 四光波混合 / CdSe/ZnS / 四光波混合法 / 発光特性制御 / 高分子環境
Research Abstract

We have examined that photoluminescence (PL) properties of core/shell-type semiconductor quantum dots (QDs) CdSe/ZnS are improved by the interaction with the polymers in solution. Next, we have studied the PL properties (spectra, lifetime, blinking) in both macroscopic and single QD level by the interaction with metal and TiO_2 nanoparticles and found out the blinking property of single QDs can be improved by the interaction with TiO_2. Further, we have observed a novel effect of solvent molecules on femtosecond optical phase relaxation of QDs in solutions.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (40 results)

All 2011 2010 2009 2008

All Journal Article (18 results) (of which Peer Reviewed: 18 results) Presentation (22 results)

  • [Journal Article] Investigation of the confinement potential within GaNAs/GaAs multiple quantum wells2011

    • Author(s)
      K.Goshima, A.Kittaka, K.Fujii, M.Shiraga, N.Tsurumachi, S.Koshiba, S.Nakanishi, H.Akiyama, H.Itoh
    • Journal Title

      Phys.Status Solidi C 8

      Pages: 414-416

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Femtosecond Coherent Vibrational Relaxation in PVA Film detected by Coherent Anti-Stokes Raman Spectroscopy2011

    • Author(s)
      T.Kouzai, ほか
    • Journal Title

      Ultrafast Phenomena XVII (Oxford University Press)

      Pages: 251-253

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Investigation of the confinement potential within GaNAs/GaAs multiple quantum wells2011

    • Author(s)
      K.Goshima, ほか
    • Journal Title

      Phys.Status Solidi C

      Volume: 8 Pages: 414-416

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Enhancement of terahertz detection efficiency in electro-optical sampling using Fabry-Perot microcavity structure2011

    • Author(s)
      H.Shirai, ほか
    • Journal Title

      Phys.Status Solidi C

      Volume: 8 Pages: 356-358

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The nonlinear refraction sign turned to reverse by intercalating cresyl violent dye into layered titanate nanosheets2010

    • Author(s)
      C.Dou, P.Wen, X.Kong, S.Nakanishi, Q. Feng
    • Journal Title

      Opt.Commun. 284

      Pages: 1067-1071

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Femtosecond Coherent Vibrational Relaxation in PVA Film detected by Coherent Anti-Stokes Raman Spectroscopy2010

    • Author(s)
      T.Kouzai, H.Miyagawa, N.Tsurumachi, S.Koshiba, S.Nakanishi, H.Itoh
    • Journal Title

      Ultrafast Phenomena XVII (Oxford University Press)

      Pages: 251-253

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Blinking Suppression in CdSe/ZnS Single Quantum Dots by TiO_2 Nanoparticles2010

    • Author(s)
      M.Hamada, S.Nakanishi, T.Itoh, M.Ishikawa, V.Biju
    • Journal Title

      ACS Nano 4

      Pages: 4445-4454

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Blinking Suppression in CdSe/ZnS Single Quantum Dots by TiO_2 Nanoparticles2010

    • Author(s)
      M.Hamada, ほか
    • Journal Title

      ACS Nano

      Volume: 4 Pages: 4445-4454

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The nonlinear refraction sign turned to reverse by intercalating cresyl violent dye into layered titanate nanosheets2010

    • Author(s)
      Chunsheng Don, ほか
    • Journal Title

      Optics Communications

      Volume: 284 Pages: 1067-1071

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structure and magnetic properties of Gd/Fe layers grown by MBE2009

    • Author(s)
      H.Miyagawa, H.Shiraoka, M.Tani, K.Fujii, N.Takahashi, S.Koshiba, Y.Tanaka, N.Tsurumachi, S.Nakanishi, H.Itoh
    • Journal Title

      Journal of Crystal Growth 311

      Pages: 2143-2146

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Enhancement and suppression of THz emission by Fabry-Perot cavity structure with a nonlinear optical crystal2009

    • Author(s)
      H.Shirai
    • Journal Title

      Applied Optics 48

      Pages: 6934-6939

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photostimulated detection of radiation defects produced by VUV lights in BaF_22009

    • Author(s)
      O.Arimoto
    • Journal Title

      Radiation Measurements (in press)

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structure and magnetic properties of Gd/Fe layers grown by MBE2009

    • Author(s)
      H.Miyagawa
    • Journal Title

      Journal of Crystal Growth 311

      Pages: 2143-2146

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Relations between Dewetting of Polymer Thin Films and Phase-Separation of Encompassed Quantum Dots2008

    • Author(s)
      R.Kanemoto, A.Anas, Y.Matsumoto, R.Ueji, T.Itoh, Y.Baba, S.Nakanishi, M.Ishikawa, V.Biju
    • Journal Title

      J.Phys.Chem.C 112

      Pages: 8184-8191

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photoluminescence Quenching and Intensity Fluctuations of CdSe-ZnS Quantum Dots on an Ag Nanoparticle Film2008

    • Author(s)
      Y.Matsumoto, R.Kanemoto, T.Itoh, S.Nakanishi, M.Ishikawa, V.Biju
    • Journal Title

      J.Phys.Chem.C 112

      Pages: 1345-1350

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Relations between Dewetting of Polymer Thin Films and Phase-Separation of Encompassed Quantum Dots2008

    • Author(s)
      R. Kanemoto, A. Anas, Y. Matsumoto, S. Nakanishi, V. Biju, ほか
    • Journal Title

      J. Phys. Chem. C 112

      Pages: 8184-8191

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoluminescence Quenching and Intensity Fluctuations of CdSe-ZnS Quantum Dots on an Ag Nanoparticle Film2008

    • Author(s)
      Y. Matsumoto, R. Kanemoto, T. Itoh, S. Nakanishi, V. Biju, ほか
    • Journal Title

      J. Phys. Chem. C 112

      Pages: 1345-1350

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Optimization of Well Width and N Content for Optical Properties of GaNAs/GaAs Multiple Quantum Well Grown by RF-Molecular Beam Epitaxy2008

    • Author(s)
      K. Fujii, D. Nakase, N. Tsurumachi, H. Miyagawa, H. Itoh, S. Nakanishi, H. Akiyama, S. Koshiba
    • Journal Title

      Japanese Journal of Applied Physics 47

      Pages: 2991-2993

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] 高分子におけるフェムト秒時間分解CARS分光2011

    • Author(s)
      香西貴典, ほか
    • Organizer
      日本物理学会 第66回年会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-27
    • Related Report
      2010 Annual Research Report
  • [Presentation] CdSe/ZnS単一量子ドットのBlinking特性制御2011

    • Author(s)
      濱田守彦, 鶴町徳昭, 伊藤寛, 中西俊介, 石川満, V.Biju
    • Organizer
      日本物理学会第66回年次大会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Final Research Report
  • [Presentation] コロイド状CdSe/ZnS量子ドットの位相緩和の溶媒効果2011

    • Author(s)
      香西浩嘉, 宮川勇人, 鶴町徳昭, 小柴俊, 伊藤寛, 中西俊介, V.Biju, 石川満
    • Organizer
      日本物理学会第66回年次大会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Final Research Report
  • [Presentation] CdSe/ZnS単一量子ドットにおける電子移動によるBlinking抑制2011

    • Author(s)
      濱田守彦, ほか
    • Organizer
      日本物理学会 第66回年会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] コロイド状CdSe/ZnS量子ドットの位相緩和の溶媒効果2011

    • Author(s)
      香西浩嘉, ほか
    • Organizer
      日本物理学会 第66回年会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] Blinking control of CdSe/ZnS single quantum dots by electron transfer to TiO_2 nanoparticles2010

    • Author(s)
      M.Hamada, N.Tsurumachi, S.Nakanishi, T.Itoh, M.Ishikawa, V.Biju
    • Organizer
      6th Asian Photochemistry Conference
    • Place of Presentation
      New Zealand
    • Year and Date
      2010-11-18
    • Related Report
      2010 Final Research Report
  • [Presentation] Blinking control of CdSe/ZnS single quantum dots by electron transfer to TiO_2 nanoparticles2010

    • Author(s)
      M.Hamada, ほか
    • Organizer
      6^<th> Asian Photochemistry Conference 2010
    • Place of Presentation
      Wellington, New Zealand
    • Year and Date
      2010-11-18
    • Related Report
      2010 Annual Research Report
  • [Presentation] コロイド状CdSe/ZnS量子ドットにおける位相緩和の溶媒効果2010

    • Author(s)
      香西浩嘉, 宮川勇人, 鶴町徳昭, 小柴俊, 伊藤寛, 中西俊介, V.Biju, 石川満
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-24
    • Related Report
      2010 Final Research Report
  • [Presentation] Femtosecond Coherent Vibrational Relaxation in PVA Film detected by Coherent Anti-Stokes Raman Spectroscopy2010

    • Author(s)
      T.Kouzai, ほか
    • Organizer
      17^<th> International Symposium on Ultrafast Phenomena
    • Place of Presentation
      Snowmass, Colorado, USA
    • Year and Date
      2010-07-20
    • Related Report
      2010 Annual Research Report
  • [Presentation] Effect of TiO_2 nanoparticles on Blinking of CdSe/ZnS single quantum dots2010

    • Author(s)
      M.Hamada, N.Tsurumachi, H.Itoh, S.Nakanishi, V.Biju, M.Ishikawa
    • Organizer
      The 37th International Symposium on Compound Semiconductors
    • Place of Presentation
      Takamatsu, Japan
    • Year and Date
      2010-06-04
    • Related Report
      2010 Final Research Report
  • [Presentation] Effects of TiO_2 nanoparticles on blinking of CdSe/ZnS single quantum dots2010

    • Author(s)
      H.Hamada, ほか
    • Organizer
      The 37^<th> International Symposium on Compound Semiconductor
    • Place of Presentation
      Takamatsu, Japan
    • Year and Date
      2010-06-04
    • Related Report
      2010 Annual Research Report
  • [Presentation] Degenerate Four-wave mixing in GaNAs/GaAs multiple quantum wells2010

    • Author(s)
      A.Kittaka, ほか
    • Organizer
      The 37^<th> International Symposium on Compound Semiconductor
    • Place of Presentation
      Takamatsu, Japan
    • Year and Date
      2010-06-04
    • Related Report
      2010 Annual Research Report
  • [Presentation] Cavity polariton in one-dimensional photonic crystals with organic dye aggregates2010

    • Author(s)
      K.Ishii, ほか
    • Organizer
      The 37^<th> International Symposium on Compound Semiconductor
    • Place of Presentation
      Takamatsu, Japan
    • Year and Date
      2010-06-04
    • Related Report
      2010 Annual Research Report
  • [Presentation] ナノ粒子によるCdSe/ZnS単一量子ドットのBlinkingに対する効果2010

    • Author(s)
      濱田守彦, 鶴町徳昭, 伊藤寛, 中西俊介, V.Biju, 石川満
    • Organizer
      日本物理学会
    • Place of Presentation
      岡山大学
    • Year and Date
      2010-03-21
    • Related Report
      2010 Final Research Report
  • [Presentation] ナノ粒子によるCdSe/ZnS単一量子ドットの Blinking に対する効果2010

    • Author(s)
      濱田守彦
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      岡山大学津島キャンパス(岡山県)
    • Year and Date
      2010-03-21
    • Related Report
      2009 Annual Research Report
  • [Presentation] PVAにおける時間分解コヒーレント・アンチストークス・ラマン分光2010

    • Author(s)
      香西貴典
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      岡山大学津島キャンパス(岡山県)
    • Year and Date
      2010-03-21
    • Related Report
      2009 Annual Research Report
  • [Presentation] Population Dynamics of Excitons in GaAs/AlAs Coupled Quantum Well Systems Detected by Pump-Probe Spectroscopy2009

    • Author(s)
      S.Nakanishi, Y.Uchida, H.Tsuji, N.Fujita, K.Fujii, H.Miyagawa, N.Tsurumachi, S.Koshiba, H.Itoh, T.G.Kim
    • Organizer
      International Conference on Nonlinear Optics
    • Place of Presentation
      Honolulu, Hawaii
    • Year and Date
      2009-07-12
    • Related Report
      2010 Final Research Report
  • [Presentation] Population Dynamics of Excitons in GaAs/AlAs Coupled Quantum Well Systems Detected by Pump-Probe Spectroscopy2009

    • Author(s)
      Y.Uchida
    • Organizer
      Nonlinear Optics
    • Place of Presentation
      ヒルトンハワイアン(アメリカ)
    • Year and Date
      2009-07-12
    • Related Report
      2009 Annual Research Report
  • [Presentation] 金属微粒子との相互作用によるCdSe量子ドットの発光特性変化2009

    • Author(s)
      松本祐介, 山岡洋也, 鶴町徳昭, 伊藤寛, 中西俊介, V.Biju, 伊藤民武, 石川満
    • Organizer
      日本物理学会第64回年次大会
    • Place of Presentation
      立教大学
    • Year and Date
      2009-03-30
    • Related Report
      2010 Final Research Report 2008 Annual Research Report
  • [Presentation] 結合量子井戸におけるPump-Probe分光2009

    • Author(s)
      内田祥久, 藤田直也, 藤井健輔, 宮川勇人, 鶴町徳昭, 小柴俊, 伊藤寛, 中西俊介, T.G.Kim
    • Organizer
      日本物理学会第64回年次大会
    • Place of Presentation
      立教大学
    • Year and Date
      2009-03-28
    • Related Report
      2010 Final Research Report
  • [Presentation] CdSe半導体量子ドットの発光特性制御2009

    • Author(s)
      中西俊介, 松本祐介, 金本嶺泰, 山岡洋也, V.Biju, 伊藤民武, 石川満
    • Organizer
      レーザー学会第29回大会
    • Place of Presentation
      徳島大学
    • Year and Date
      2009-01-08
    • Related Report
      2010 Final Research Report
  • [Presentation] 溶液中での半導体量子ドットと銀粒子間の界面相互作用2008

    • Author(s)
      松本祐介, 山岡洋也, 鶴町徳昭, 小柴俊, 伊藤寛, 中西俊介, 伊藤民武, V.P.Biju, 石川満
    • Organizer
      応用物理学会中国四国支部・日本物理学会四国支部・中国支部2008年度講演会
    • Place of Presentation
      愛媛大学
    • Year and Date
      2008-08-02
    • Related Report
      2010 Final Research Report

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Published: 2008-04-01   Modified: 2020-05-15  

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