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Spectroscopic study of novel cluster structures created as chemical intermediates in supersonic molecular beams

Research Project

Project/Area Number 20550005
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionTohoku University

Principal Investigator

MIKAMI Naohiko  Tohoku University, 大学院・理学研究科, 名誉教授 (70004447)

Co-Investigator(Renkei-kenkyūsha) YOSHIYUKI Matsuda  東北大学, 大学院・理学研究科, 助教 (70400223)
Project Period (FY) 2009 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2010: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2009: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2008: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywords分子分光 / 反応中間体構造解析 / 芳香族求核置換反応中間体 / σ-complex / 分子クラスター / ベンゼン・メタノールクラスター / プロトン付加水クラスター / アセトン2量体 / 光イオン化誘起異性化反応 / C_6F_6・NH_3クラスター / フォルムアミド・水クラスター / 水素結合形態変化 / 水和メタノールクラスター / HCP分子 / 前期解離反応機構 / レーザー分光 / 気相イオン / 反応制御
Research Abstract

Spectroscopic studies on jet-cooled molecular cluster cations have been carried out for the following systems ;
1. IR and electronic spectroscopy of [C_6H_6(NH_3)_n]^+ (n=1 and 2) revealed that their stable forms are of s-complex type, in which the ammonia moiety is covalently bonded to the benzene moiety as expected as the reaction intermediate of nucleophilic substitution of aromatics. The similar structures of [Benzene-(Methanol)_n]^+ (n=2, 3) were also investigated in combination with quantum chemical calculations.
2. H-bond network structures of H^+(H_2O)_n (n=20-200) were investigated by IR spectroscopy. It was found that the spectral features of the clusters with increasing cluster size become similar to the characteristic features of water and of ice, indicating the network morphology of the large-size clusters transmutes gradually to those of the bulk systems. It was also found that the spectral feature depends on the internal energy in the species.
3.Structures of neutral and cationic clusters of acetone and of acetic acid were investigated by using IR spectroscopy based on vacuum-ultraviolet one-photon ionization detection. It was found that the keto-enol transition is generated after the ionization for many clusters, such as their dimers, whereas their neutrals are of the keto-form. The isomerization mechanism was discussed in relation to their proton affinities and the potential surface of the proton-transfer coordinate.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (56 results)

All 2010 2009 2008 Other

All Journal Article (27 results) (of which Peer Reviewed: 27 results) Presentation (28 results) Remarks (1 results)

  • [Journal Article] Infrared Spectra and Hydrogen Bond Network Structures of Large-sized Protonated Water Clusters H^+(H_2O)_n (n=20-200)2010

    • Author(s)
      K.Mizuse, N.Mikami, A.Fujii
    • Journal Title

      Angew. Chem. Mt. Ed. 49

      Pages: 10119-10122

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Catalytic Action of a Single Water Molecule in a Proton-Migration Reaction2010

    • Author(s)
      Y.Matsuda, A.Yamada, K.Hamashima, N.Mikami, A. Fujii
    • Journal Title

      Angew. Chem. Int. Ed. 49

      Pages: 4898-4901

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Infrared and Electronic Spectroscopy of Benzene- Ammonia Cluster Radical Cations [C_6H_6(NH_3)_<(1,2)>]: Observation of Isolated and Microsolvated σ-Complexes2010

    • Author(s)
      K.Mizuse, H.Hasegawa, N.Mikami, A.Fujii
    • Journal Title

      J. Phys. Chem. A114

      Pages: 11060-11069

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Catalytic Action of a Single Water Molecule in a Proton-Migration Reaction2010

    • Author(s)
      Y.Matsuda, A.Yamada, K.Hanaue, N.Mikami, A.Fujii
    • Journal Title

      Angewante Chemie International Edition

      Volume: 49 Pages: 4898-4901

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Infrared and Electronic Spectroscopy of Benzene-Ammonia Cluster Radical Cations (C_6H_6(NH_3)_<1,2^+> Observation of Isolated and Microsolvatedo-Complexes2010

    • Author(s)
      K.Mizuse, H.Hasegawa, N.Mikami, A.Fuju
    • Journal Title

      J.Phys.Chem.A

      Volume: 114 Pages: 11060-11069

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Infrared Spectra and Hydrogen Bond Network Structures of Large-sized Protonated Water Clusters H^+(H_2O)_n(n=20~200)2010

    • Author(s)
      K.Mizuse, N.Mikami, A.Fujii
    • Journal Title

      Angewante Chemie International Edition

      Volume: 49(In press)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vibrational spectroscopy of size-selected neutral and cationic clusters combined with vacuum-ultraviolet one-photon ionization detection2009

    • Author(s)
      Y.Matsda, N.Mikami, A.Fujii
    • Journal Title

      Phys. Chem. Chem. Phys. 11

      Pages: 1279-1290

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Proton switch correlated with the morphological development of the hydrogenbond network in H^+(MeOH)_m(H_2O)_1 (m=1-9): A Theoretical and Infrared Spectroscopic Study2009

    • Author(s)
      D.Bing, J-L.Kuo, K.Suhara, A.Fujii, N.Mikami
    • Journal Title

      J. Phys. Chem. A113

      Pages: 2323-2332

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Infrared spectroscopy for acetone and its dimmerbased on photoionization detection with tunable coherent vacuum-ultreviolet light2009

    • Author(s)
      Y.Matsuda, K.Ohta, N.Mikami, A.Fujii
    • Journal Title

      Chem. Phys. Lettres 471

      Pages: 50-53

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Predissociation Mechanism and Dynamics of HCP2009

    • Author(s)
      M.Namai, T.Sasaki, H.Ishikawa, H.Morikuni, N.Mikami
    • Journal Title

      J. Phys. Chem. A113

      Pages: 13081-13088

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Interpreting the Physical Background of Empirical Solvent Polarity via Photodetachment Spectroscopy of Microsolvated Aromatic Ketryl Anions2009

    • Author(s)
      T.Maeyama, Y.Yoshida, I.Yagi, N.Mikami, A.Fujii
    • Journal Title

      J. Phys. Chem. A113

      Pages: 10593-10602

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Interpretaing the Physical Background of Empirical Solvent Polarity via Photodetachment Spectroscopy_of Microsolvated Aromatic Ketyl Anions2009

    • Author(s)
      T.Maeyama, K.Yoshida, I.Yagi, N.Mikami
    • Journal Title

      J.Phys.Chem.A

      Volume: 113 Pages: 10539-10602

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Intermolecular proton-transfer in acetic acid clusters induced by vacuum-ultraviolet photoionization2009

    • Author(s)
      K.Ohta, Y.Matsuda, N.Mikami, A.Fujii
    • Journal Title

      J.Chem.Phys.

      Volume: 131 Pages: 184304-11

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vibrational spectroscopy of size-selected neutral and cationic clusters Combined with vacuum-ultraviolet one-photon ionization detection2009

    • Author(s)
      Y.Matsda, N.Mikami, A.Fujii
    • Journal Title

      Phys.Chem.Chem.Phys. 11

      Pages: 1279-1290

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Proton switch correlated with the morphological development of the hydrogen-bond network in H^+(MeOH)_m(H_2O)1 (m=1-9)2009

    • Author(s)
      D.Bing, J-L.Kuo, K.Suhara, A.Fujii, N.Mikami
    • Journal Title

      J.Phys.Chem.A 113

      Pages: 2322-2332

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Predissociation Mechanism and Dynamics of HCP2009

    • Author(s)
      M.Namai, T.Sasaki, H.Ishikawa, H.Morikuni, N.Mikami
    • Journal Title

      J.Phys.Chem.A 113

      Pages: 13081-13088

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Infrared spectroscopy for acetone and its dimmer based on photoionization detection with tunable coherent vacuum-ultreviolet light2009

    • Author(s)
      Y.Matsuda K.Ohta, N.Mikami, A.Fujii
    • Journal Title

      Chem.Phys.Lettres 471

      Pages: 50-53

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Predissociation mechanism and dynamics of HCP2009

    • Author(s)
      N. Namai, T. Sasaki, H. Ishikawa, H. Morikuni, and N. Mikami
    • Journal Title

      J. Phys. Chem. A (印刷中)

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental and theoretical determination of the accurate interaction energies in benzene-halomethane : the unique nature of the activated CH/π interaction of haloalkanes2008

    • Author(s)
      A.Fujii, K.Shibasaki, T.Kazama, R.Itaya, N.Mikami, S.Tsuzuki
    • Journal Title

      Phys. Chem. Chem. Phys. 10

      Pages: 2836-2843

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Observation of an Isolated Intermediate of the Nuleophilic Aromatic Substitution Reaction by Infrared Spectroscopy2008

    • Author(s)
      H.Hasegawa, K.Mizuse, M.Hachiya, Y.Matsuda, N.Mikami, A.Fujii
    • Journal Title

      Angew. Chem. Int. Ed. 47

      Pages: 6008-6010

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Size-Selected Infrared Predissociation Spectroscopy of Neutral and Cationic Formamide-Water Clusters : Stepwize Groth of Hydrated Structures and Intracluster Hydrogen Transfer Induced by Vacuum-Ultraviolet Photoionization2008

    • Author(s)
      D.Sakai, Y.Matsuda, M.Hachiya, M.Mori, A.Fujii, N.Mikami
    • Journal Title

      J. Phys. Chem. A2008 112

      Pages: 6840-6849

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Comprehensive Analysis of the Hydrogen Bond Network Morphology and OH Stretching Vibrations in Protonated Methanol-Water Mixed Clusters, H^+(MeOH)_1(H_2O)_n (n-1-8)2008

    • Author(s)
      Jer-Lai Kuo, Z.Xie, D.Bing, A.Fujii, T.Hamashima, K.Suhara, N.Mikami
    • Journal Title

      J. Phys. Chem., A2008 112

      Pages: 10125-10133

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Infrared predissociation spectroscopy of cluster cations of protic molecules, (NH_3)_n^+, n=2-4 and (CH_3OH)_n^+, n=2,32008

    • Author(s)
      M.Hachiya, Y.Matsuda, K.Suhara, N.Miakmi, Asuka Fujii
    • Journal Title

      J. Chem. Phys. 129

      Pages: 94306-94306

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Solvent Reorientation Process in the "Twisted" Intramolecular Charge-Transfer Process of Cyanophenyldisilane-(H_2O)_2 Cluster Investigated by Transient Infrared Spectroscopy2008

    • Author(s)
      M.Sugiyama, H.Ishikawa, W.Setaka, M.Kira, N.Mikami
    • Journal Title

      J. Phys. Chem., A2008 112

      Pages: 1168-1171

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dynamics of hydrogen-bonded OH stretches as revealed by single-mode infrared-ultraviolet laser double resonance spectroscopy on supersonically cooled clusters of phenol2008

    • Author(s)
      A.Doi, N.Mikami
    • Journal Title

      J. Chem. Phys. 129

      Pages: 154308-154308

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dynamics of hydrogen-bonded OH stretches as revealed by single-mode infrared-ultraviolet laser double resonance spectroscopy on supersonically cooled clusters of phenol2008

    • Author(s)
      A. Doi and N. Mikami
    • Journal Title

      J. Chem. Phys 129

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Size-selected infrared predissociation spectroscopy of neutral and cationic formamide-water clusters2008

    • Author(s)
      D. Sakai, D. Sakai, Y. Matsuda, M. Hachiya, M. Mori, A. Fujii, and N. Mikami
    • Journal Title

      J. Phys. Chem. A 112

      Pages: 6840-6849

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] ジエチルエーテルクラスターの光イオン化ダイナミクス2010

    • Author(s)
      花上謙一、松田欣之、三上直彦、藤井朱鳥
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-15
    • Related Report
      2010 Final Research Report
  • [Presentation] 大サイズプロトン付加水クラスターの赤外スペクトルにおける内部エネルギー依存性2010

    • Author(s)
      水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-15
    • Related Report
      2010 Final Research Report
  • [Presentation] アセトン二量体の光イオン化誘起異性化反応2010

    • Author(s)
      花上謙一、松田欣之、保木邦仁、三上直彦、藤井朱鳥
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-15
    • Related Report
      2010 Final Research Report
  • [Presentation] [Benzene-(Methanol)_n]^+(n-2,3)赤外スペクトルの再検討~σ-complex生成の可能性~2010

    • Author(s)
      鈴木雄太、水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-14
    • Related Report
      2010 Final Research Report
  • [Presentation] ベンゼン・アルカン系におけるCH/π相互作用エネルギーの決定~相互作用エネルギーと平均分極率との相関~2010

    • Author(s)
      林聖将、朴宰佑、風間隆希、三上直彦、藤井朱鳥
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-14
    • Related Report
      2010 Final Research Report
  • [Presentation] ラジカルカチオン状態における水クラスターの水素結合ネットワーク構造2010

    • Author(s)
      水瀬賢太、松田欣之、三上直彦、藤井朱鳥
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪
    • Year and Date
      2010-09-14
    • Related Report
      2010 Final Research Report
  • [Presentation] [Benzene-(Methanol)_n]+(n=2,3)赤外スペクトルの再検討~σ-comp互ex生成の可能性~2010

    • Author(s)
      鈴木雄太、水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      分子科学会2010
    • Place of Presentation
      大阪大学、豊中
    • Related Report
      2010 Annual Research Report
  • [Presentation] ラジカルカチオン状態における水クラスターの水素結合ネットワーク構造2010

    • Author(s)
      水瀬賢太、松田欣之、三上直彦、藤井朱鳥
    • Organizer
      分子科学会2010
    • Place of Presentation
      大阪大学、豊中
    • Related Report
      2010 Annual Research Report
  • [Presentation] 大サイズプロトン付加水クラスターの赤外スペクトルにおける内部エネルギー依存性2010

    • Author(s)
      水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      分子科学会2010
    • Place of Presentation
      大阪大学、豊中
    • Related Report
      2010 Annual Research Report
  • [Presentation] ジエチルエーテルクラスターの光イオン化ダイナミクス2010

    • Author(s)
      松田欣之、花上謙一、三上直彦、藤井朱鳥
    • Organizer
      分子科学会2010
    • Place of Presentation
      大阪大学、豊中
    • Related Report
      2010 Annual Research Report
  • [Presentation] 気相クラスター新奇水素結合系の分光研究招待講演2009

    • Author(s)
      三上直彦
    • Organizer
      理研シンポジウム「動的水和構造と分子過程III」
    • Place of Presentation
      理化学研究所Spring 8、播磨
    • Year and Date
      2009-11-24
    • Related Report
      2010 Final Research Report
  • [Presentation] 招待講演「水素結合系気相分子クラスターの分光研究」2009

    • Author(s)
      三上直彦
    • Organizer
      理研シンポジウム「動的水和構造と分子過程III」
    • Place of Presentation
      理研Spring-8播磨
    • Year and Date
      2009-11-24
    • Related Report
      2009 Annual Research Report
  • [Presentation] 真空紫外1光子でイオン化されたアセトンおよびその二量体の構造2009

    • Author(s)
      花上謙一、松田欣之、太田圭亮、三上直彦、藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2009-09-23
    • Related Report
      2010 Final Research Report
  • [Presentation] 巨大サイズプロトン付加水クラスターの赤外分光2009

    • Author(s)
      水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2009-09-23
    • Related Report
      2010 Final Research Report
  • [Presentation] 巨大サイズプロトン付加水クラスターH^+(H_2O)_n(n=15-200)の赤外分光2009

    • Author(s)
      水瀬健太, 三上直彦, 藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋大学
    • Year and Date
      2009-09-23
    • Related Report
      2009 Annual Research Report
  • [Presentation] 真空紫外一光子でイオン化されたアセトンおよびその二量体の構造2009

    • Author(s)
      花上謙一, 松田欣之, 太田圭亮, 三上直彦, 藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋大学
    • Year and Date
      2009-09-23
    • Related Report
      2009 Annual Research Report
  • [Presentation] アセトン・水クラスターの真空紫外光イオン化誘起プロトンマイグレーション2009

    • Author(s)
      松田欣之、山田綾子、三上直彦、藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2009-09-22
    • Related Report
      2010 Final Research Report
  • [Presentation] アセトン・水クラスターの真空紫外光イオン化誘起プロトンマイグレーション2009

    • Author(s)
      松田欣之, 山田綾子, 三上直彦, 藤井朱鳥
    • Organizer
      第3回分子科学討論会
    • Place of Presentation
      名古屋大学
    • Year and Date
      2009-09-22
    • Related Report
      2009 Annual Research Report
  • [Presentation] 水素結合の不思議招待講演2009

    • Author(s)
      三上直彦
    • Organizer
      平成21年度日本化学会化学教育協議会東北大会
    • Place of Presentation
      日大工学部、郡山
    • Year and Date
      2009-09-20
    • Related Report
      2010 Final Research Report
  • [Presentation] 招待講演「水素結合の不思議」2009

    • Author(s)
      三上直彦
    • Organizer
      平成21年度日本化学会化学教育協議会東北大会
    • Place of Presentation
      日大工学部、郡山
    • Year and Date
      2009-09-20
    • Related Report
      2009 Annual Research Report
  • [Presentation] 酢酸の水素結合クラスターの真空紫外光イオン化検出赤外解離分光2008

    • Author(s)
      太田圭亮、松田欣之、藤井朱鳥、三上直彦
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-26
    • Related Report
      2010 Final Research Report
  • [Presentation] プロトン付加水クラスターH^+(H_2O)_nにおける大規模水素結合ネットワーク構造2008

    • Author(s)
      水瀬賢太、三上直彦、藤井朱鳥
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-26
    • Related Report
      2010 Final Research Report
  • [Presentation] 気相孤立系における芳香族求核置換反応中間体の赤外分光2008

    • Author(s)
      水瀬賢太、長谷川勇人、蜂谷正樹、松田欣之、三上直彦、藤井朱鳥
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-26
    • Related Report
      2010 Final Research Report
  • [Presentation] ミクロ溶媒和負イオンの光電子脱離分光から見た"溶媒極性"の物理的背景(1)2008

    • Author(s)
      前山俊彦、吉田啓二、八木泉、藤井朱鳥、三上直彦
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-25
    • Related Report
      2010 Final Research Report
  • [Presentation] ミクロ溶媒和負イオンの光電子脱離分光から見た"溶媒極性"の物理的背景(2)2008

    • Author(s)
      吉田啓二、前山俊彦、八木泉、藤井朱鳥、三上直彦
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-25
    • Related Report
      2010 Final Research Report
  • [Presentation] プロトン付加メタノール・水混合クラスターH^+M_1W_n(n=1-8)の構造と赤外スペクトル2008

    • Author(s)
      Xie Zhi-zhong, Bing Dan, Kuo Jer-Lai、藤井朱鳥、濱島徹、須原健一郎、三上直彦
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡国際会議場
    • Year and Date
      2008-09-25
    • Related Report
      2008 Annual Research Report
  • [Presentation] プロトン付加メタノール・水混合クラスターの構造と赤外スペクトル2008

    • Author(s)
      Xie Zhi-Zhong, Bing Dan, Kuo Jer-Lai,藤井朱鳥、濱島徹、須原健一郎、三上直彦
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-24
    • Related Report
      2010 Final Research Report
  • [Presentation] プロトン性分子クラスターの光イオン化誘起クラスター内プロトン移動2008

    • Author(s)
      山田綾子、松田欣之、蜂谷正樹、三上直彦、藤井朱鳥
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-24
    • Related Report
      2010 Final Research Report
  • [Remarks] ホームページ等

    • Related Report
      2010 Final Research Report

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Published: 2008-04-01   Modified: 2016-04-21  

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