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State selective velocity map imaging of neutral fragments produced by the photodissociation of fullerenes

Research Project

Project/Area Number 20550029
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionInstitute for Molecular Science

Principal Investigator

KATAYANAGI Hideki  Institute for Molecular Science, 光分子科学研究領域, 助教 (00399312)

Co-Investigator(Renkei-kenkyūsha) MITSUKE Koichiro  分子科学研究所, 光分子科学研究領域, 准教授 (50190682)
Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2010: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2009: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2008: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywordsフラーレン・ナノチューブ / 化学物理 / 物性実験 / 可視化 / 反応動力学 / ナノチューブ・フラーレン
Research Abstract

Fullerenes, nano-capsules, are widely regarded as media to transport energy and materials. In order to elucidate capsule opening and closing reactions, the photodissociation initiated by one-photon excitation was investigated. An experimental apparatus which enables us to observe images of spatial scattering distributions of photofragments was developed. Although imaging of neutral fragments has not been achieved yet, accurate images of ionic fragments were obtained. Knowledge on the reaction dynamics such as flow of excess energy was obtained from the images.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (35 results)

All 2010 2009 2008 Other

All Journal Article (20 results) (of which Peer Reviewed: 10 results) Presentation (14 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Mass-analyzed velocity map imaging of thermal photofragments from C_<60>2010

    • Author(s)
      片柳英樹, 片柳英樹
    • Journal Title

      J.Chem.Phys. 133

      Pages: 81101-81101

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Exclusive Detection of Photofragments from C_<60> with a Potential-Switch Mass Selector2010

    • Author(s)
      H.Katayanagi, Md. S.I.Prodhan, B.P.Kafle, C.Huang, K. Mitsuke
    • Journal Title

      UVSOR Activity Report 2009 37

      Pages: 56-56

    • Related Report
      2010 Final Research Report
  • [Journal Article] Development of a TEPICO Technique for Determination of Excess Energy Partitioning in Dissociative Photoionization2010

    • Author(s)
      H.Katayanagi, Md.S.I.Prodhan, B.P.Kafle, C.Huang, K.Mitsuke
    • Journal Title

      UVSOR Activity Report 2009 37

      Pages: 57-57

    • Related Report
      2010 Final Research Report
  • [Journal Article] Feasibility study on the mass-selected velocity map imaging of polyatomic molecules and fullerenes2010

    • Author(s)
      H.Katayanagi, B.P.Kafle, C.Huang, Md.S.I.Prodhan, H.Yagi, K.Mitsuke
    • Journal Title

      Proceedings of Pure and Applied Chemistry International Conference 2010

      Pages: 941-941

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Mass-analyzed velocity map imaging of thermal photofragments from C_<60>2010

    • Author(s)
      H.Katayanagi, K.Mitsuke
    • Journal Title

      Journal of Chemical Physics (Communication)

      Volume: 133

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Exclusive Detection of Photofragments from C_<60> with a Potential-Switch Mass Selector2010

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他3名
    • Journal Title

      UVSOR Activity Report 2009

      Volume: 37 Pages: 56-56

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Development of a TEPICO Technique for Determination of Excess Energy Partitioning in Dissociative Photoionization2010

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他3名
    • Journal Title

      UVSOR Activity Report 2009

      Volume: 37 Pages: 57-57

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Feasibility Study on the Mass-Selected Velocity Map Imaging of Polyatomic Molecules and Fullerenes2010

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他4名
    • Journal Title

      Proceedings of Pure and Applied Chemistry International Conference 2010(PACCON2010)

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoabsorption cross section of C_<70> thin films from visible to vacuum ultraviolet2009

    • Author(s)
      H.Katayanagi, K.Mitsuke, H.Yagi, K.Nakajima, K.R.Koswattage, K.Nakagawa
    • Journal Title

      J.Chem.Phys. 130

      Pages: 234510-234510

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photoabsorption cross section of C_<60> thin films from the visible to vacuum ultraviolet2009

    • Author(s)
      H.Yagi, K.Nakajima, K.R.Koswattage, K.Nakagawa, C.Huang, Md.S.I.Prodhan, B.P.Kafle, H.Katayanagi, K.Mitsuke
    • Journal Title

      Carbon 47

      Pages: 1152-1152

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ion Imaging Study of Dissociative Photoionization of C_<60>2009

    • Author(s)
      H.Katayanagi, C.Huang, S.I.Prodhan, H.Yagi, B.P.Kafle, K.Nakajima, K.Mitsuke
    • Journal Title

      UVSOR Activity Report 2008 36

      Pages: 48-48

    • Related Report
      2010 Final Research Report
  • [Journal Article] Velocity map imaging apparatus applicable to a study of multiple photofragmentation of C_<60>2009

    • Author(s)
      Md.S.I.Prodhan, H.Katayanagi, C.Huang, H.Yagi, B.P.Kafle, K.Mitsuke
    • Journal Title

      Chem.Phys.Lett. 469

      Pages: 19-19

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ion Imaging Study of Dissociative Photoionization of C_<60>2009

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他5名
    • Journal Title

      UVSOR Activity Report 2008 36

      Pages: 48-48

    • Related Report
      2009 Annual Research Report
  • [Journal Article] Photoabsorption cross section of C_<60> thin films from the visible to vacuum ultraviolet2009

    • Author(s)
      H.Yagi, H.Katayanagi, K.Mitsuke, 他6名
    • Journal Title

      CARBON 47

      Pages: 1152-1157

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoabsorption cross section of C_<70> thin films from visible to vacuum ultraviolet2009

    • Author(s)
      H.Yagi, H.Katayanagi K.Mitsuke, 他3名
    • Journal Title

      JOURNAL OF CHEMICAL PHYSICS 130

      Pages: 234510-234510

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Velocity Map Imaging of C_<60> Molecular Beams2008

    • Author(s)
      H.Katayanagi, C.Huang, S.I.Prodhan, H.Yagi, B.P.Kafle, K.Nakajima, K.Mitsuke
    • Journal Title

      UVSOR Activity Report 2007 35

      Pages: 64-64

    • Related Report
      2010 Final Research Report
  • [Journal Article] Total Electron Yield Spectroscopy and Electron-Signal-Triggered TOF Mass Spectrometry Developed for the Studies on Photodissociation Dynamics of Fullerenes2008

    • Author(s)
      H.Katayanagi, C.Huang, S.I.Prodhan, H.Yagi, B.P.Kafle, K.Nakajima, K.Mitsuke
    • Journal Title

      UVSOR Activity Report 2007 35

      Pages: 65-65

    • Related Report
      2010 Final Research Report
  • [Journal Article] Velocity Map Imaging of C_<60> Molecular Beams2008

    • Author(s)
      H. Katayanagi, K. Mitsuke, 他5名
    • Journal Title

      UVSOR Activity Report 2007 35

      Pages: 64-64

    • Related Report
      2008 Annual Research Report
  • [Journal Article] Total Electron Yield Spectroscopy and Electron-Signal-Triggered TOF Mass Spectrometry Developed for the Studies on Photodissociation Dynamics of Fullerenes2008

    • Author(s)
      H. Katayanagi, K. Mitsuke, 他5名
    • Journal Title

      UVSOR Activity Report 2007 35

      Pages: 65-65

    • Related Report
      2008 Annual Research Report
  • [Journal Article] Velocity map imaging apparatus applicable to a study of multiple photofragmentation of C_<60>2008

    • Author(s)
      Md S. I. Prodhan, H. Katayanagi, K. Mitsuke, 他3名
    • Journal Title

      Chem. Phys. Lett. 469

      Pages: 19-25

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] Mass-resolved velocity map imaging for photofragmentation of fullerenes2010

    • Author(s)
      H.Katayanagi, S.I.Prodhan, B.P.Kafle, C.Huang, K.Mitsuke
    • Organizer
      Pacifichem 2010
    • Place of Presentation
      ホノルル
    • Year and Date
      2010-12-17
    • Related Report
      2010 Final Research Report
  • [Presentation] Mass-resolved velocity map imaging for photofragmentation of fullerenes2010

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他3名
    • Organizer
      Pacifichem2010
    • Place of Presentation
      ハワイコンベンションセンター(ホノルル・アメリカ)
    • Year and Date
      2010-12-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] 画像観測法を用いた高次フラーレン(C_<70>)の光分解機構の解明2010

    • Author(s)
      片柳英樹,見附孝一郎
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪府
    • Year and Date
      2010-09-17
    • Related Report
      2010 Final Research Report
  • [Presentation] 画像観測法を用いた高次フラーレン(C_<70>)の光分解機構の解明2010

    • Author(s)
      片柳英樹、見附孝一郎
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪大学(大阪府)
    • Year and Date
      2010-09-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] Mass-resolved velocity map imaging for photofragmentation of fullerenes2010

    • Author(s)
      H.Katayanagi, S.I.Prodhan, B.P.Kafle, C.Huang, K. Mitsuke
    • Organizer
      第26回化学反応討論会
    • Place of Presentation
      広島県
    • Year and Date
      2010-06-04
    • Related Report
      2010 Final Research Report
  • [Presentation] Mass-resolved velocity map imaging for photofragmentation of fullerenes2010

    • Author(s)
      H.Katayanagi, K.Mitsuke, 他3名
    • Organizer
      第26回化学反応討論会
    • Place of Presentation
      広島大学(広島県)
    • Year and Date
      2010-06-04
    • Related Report
      2010 Annual Research Report
  • [Presentation] 電子スタート式飛行時間型質量分析法によるフラーレンの光解離機構の解明2010

    • Author(s)
      片柳英樹,C.Huang, Md.S.I.Prodhan, B.P.Kafle,八木創,見附孝一郎
    • Organizer
      第23回日本放射光学会年会 放射光科学合同シンポジウム
    • Place of Presentation
      兵庫県
    • Year and Date
      2010-01-09
    • Related Report
      2010 Final Research Report
  • [Presentation] 電子スタート式飛行時間型質量分析法によるフラーレンの光解離機構の解明2010

    • Author(s)
      片柳英樹、見附孝一郎, 他4名
    • Organizer
      第23回日本放射光学会年会 放射光科学合同シンポジウム
    • Place of Presentation
      イーグレ姫路(兵庫県)
    • Year and Date
      2010-01-09
    • Related Report
      2009 Annual Research Report
  • [Presentation] Development of a potential switch mass selector for the photofragment ion imaging2009

    • Author(s)
      H.Katayanagi, B.P.Kafle, Md.S.I.Prodhan, C.Huang, H.Yagi, K.Nakajima, K.Mitsuke
    • Organizer
      第25回化学反応討論会
    • Place of Presentation
      埼玉県
    • Year and Date
      2009-06-02
    • Related Report
      2010 Final Research Report
  • [Presentation] Development of a potential switch mass selector for the photofragment ion imaging2009

    • Author(s)
      片柳英樹, 見附孝一郎, 他5名
    • Organizer
      第25回化学反応討論会
    • Place of Presentation
      大宮ソニックシティ(埼玉県)
    • Year and Date
      2009-06-02
    • Related Report
      2009 Annual Research Report
  • [Presentation] 画像観測法によるフラーレンの解離性光イオン化機構の解明2008

    • Author(s)
      片柳英樹,C.Huang,Md.S.I.Prodhan,八木創,B.P.Kafle,中島弘一,見附孝一郎
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡県
    • Year and Date
      2008-09-27
    • Related Report
      2010 Final Research Report
  • [Presentation] 画像観測法によるフラーレンの解離性光イオン化機構の解明2008

    • Author(s)
      片柳英樹、見附孝一郎, 他5名
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Year and Date
      2008-09-27
    • Related Report
      2008 Annual Research Report
  • [Presentation] フラーレン分子線の運動量画像観測2008

    • Author(s)
      片柳英樹,C.Huang,Md.S.I.Prodhan,八木創,B.P.Kafle,中島弘一,見附孝一郎
    • Organizer
      第24回化学反応討論会
    • Place of Presentation
      北海道
    • Year and Date
      2008-06-03
    • Related Report
      2010 Final Research Report
  • [Presentation] フラーレン分子線の運動量画像観測2008

    • Author(s)
      片柳英樹、見附孝一郎, 他5名
    • Organizer
      第24回化学反応討論会
    • Place of Presentation
      札幌
    • Year and Date
      2008-06-03
    • Related Report
      2008 Annual Research Report
  • [Patent(Industrial Property Rights)] 原子/分子ビームの3次元速度分布測定方法及び装置

    • Inventor(s)
      片柳英樹見附孝一郎
    • Related Report
      2008 Annual Research Report

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Published: 2008-04-01   Modified: 2016-04-21  

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