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Mechanism of disappearance of magnetic moment of Ni in relation with Rare Earths, especially with heavy fermion element of Ce

Research Project

Project/Area Number 20560618
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical properties of metals
Research InstitutionNihon University

Principal Investigator

YANO Kazuo  Nihon University, 理工学部, 准教授 (20256803)

Co-Investigator(Renkei-kenkyūsha) NISHIMURA Katsuhiko  富山大学, 大学院・理工学研究部, 教授 (70218189)
Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2010: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2009: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2008: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords磁性の発現機構 / 微視的手法 / 重い電子系 / 電子・磁気物性 / ニッケル / 磁気モーメントの消失 / 希土類元素 / セリウム / CeNi / パウリ・パラ / (Ce-Gd)Ni / 磁気秩序の発現 / RKKY相互作用 / 電子状態 / 磁気的オーダー
Research Abstract

In this study, we have aimed at making clear the electronic states of CeNi, which is one of the most famous "heavy fermion" compound systems, mainly from the view point of magnetic properties. It is well-known that the CeNi has no magnetic order and the Ni in CeNi is non-magnetic. On the other hand, the GdNi, which has the same crystal-structure as that of CeNi, is revealed to be a ferri-magnet and the Ni in GdNi does retain magnetic moment stemming from 3d electrons. It follows that in (Ce_<1-X>Gd_X) Ni system, the Ni is expected to change its electronic state (of 3d) from non-magnetic state to magnetic one according to the Gd content and the study of the transformation of this (3d) electronic state does give us important clues to understand the mechanism of appearance and disappearance of magnetism. Regarding to Ce, the same thing is expected.
What we have carried out and found in these three years is summarized as follows ; (1) we have prepared 6 kinds of single crystals (Gd=0.03, 0.10, 0.15, 0.20, 0.50, 0.80), (2) we have measured magnetic properties for 6 contents of Gd and analyzed using molecular field analysis, (3) in Gd=0.03-0.20, the exchange interaction between Gd and Gd JGd-Gd i.e. RKKY interaction is considerably suppressed, (4) soft X-ray MCD measurement was carried out for Gd=0.8 at SPring-8 and some interesting results were obtained.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (21 results)

All 2011 2010 2009 2008 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results) Presentation (16 results) Remarks (1 results)

  • [Journal Article] Magnetic ordering and properties in heavy fermion (Ce1-XGdX)Ni single crystal2010

    • Author(s)
      Kazuo Yano, Katsuhiko Nishimura, Yoshikazu Isikawa, Tsuyoshi Ohta, Kiyoo Sato
    • Journal Title

      J.Phys. 200

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Onset of magnetic ordering in heavy fermion CeNi and (Ce0.97Gd0.03)Ni2010

    • Author(s)
      Kazuo Yano, Katsuhiko Nishimura, Yoshikazu Isikawa, Tsuyoshi Ohta, Kiyoo Sato
    • Journal Title

      J.Phys. 150

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic ordering and properties in heavy fermionn(Ce_<1-x>Gd_x)Ni(X=0.15 & 0.20)single crystals2010

    • Author(s)
      K.Yano, et al.
    • Journal Title

      J.Phys. : Conference Series (印刷中)

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Onset of magnetic ordering in heavy fermion CeNi and (Ce0.97Gd0.03)Ni2009

    • Author(s)
      K. Yano, et al.
    • Journal Title

      J. Phys. : Conference Series 150

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] Ce系重い電子系化合物(Ce1-XGdX)NiにおけるRKKY 相互作用の急激な減少とKondo効果2011

    • Author(s)
      矢野一雄、西村克彦、石川義和、大田剛司、佐藤清雄
    • Organizer
      日本物理学会第66回年次大会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Final Research Report
  • [Presentation] Ce系重い電子系化合物(Ce-Gd)Ni系におけるRKKY相互作用の急激な減少とKondo効果2011

    • Author(s)
      矢野一雄, 他4名
    • Organizer
      日本物理学会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] Ce系重い電子系化合物(Ce1-XGdX)NiにおけるRKKY 相互作用とKondo効果2010

    • Author(s)
      矢野一雄、田尻佑太、西村克彦、石川義和、大田剛司、佐藤清雄
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-23
    • Related Report
      2010 Final Research Report
  • [Presentation] Ce系重い電子系化合物(Ce-Gd)Ni系におけるRKKY相互作用とKonda効果2010

    • Author(s)
      矢野一雄, 他5名
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-23
    • Related Report
      2010 Annual Research Report
  • [Presentation] 重い電子系化合物(Ce1-XGdX)NiにおけるRKKY相互作用の組成依存性2010

    • Author(s)
      矢野一雄、田尻佑太、西村克彦、石川義和、大田剛司、佐藤清雄
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      岡山大学
    • Year and Date
      2010-03-21
    • Related Report
      2010 Final Research Report
  • [Presentation] 重い電子系物質(Ce-Gd)NiにおけるRKKY相互作用の組成依存性2010

    • Author(s)
      矢野一雄, ほか
    • Organizer
      日本物理学会
    • Place of Presentation
      岡山大学
    • Year and Date
      2010-03-21
    • Related Report
      2009 Annual Research Report
  • [Presentation] (Ce1-XGdX)Ni(X=0.50-0.90) における磁気秩序とRKKY相互作用2009

    • Author(s)
      矢野一雄、田尻佑太、西村克彦、石川義和、大田剛司、佐藤清雄
    • Organizer
      日本物理学会秋季大会
    • Place of Presentation
      熊本大学
    • Year and Date
      2009-09-25
    • Related Report
      2010 Final Research Report
  • [Presentation] (Ce_<1-x>Gd_x)Ni(X=0.50-0.90)における磁気秩序とRKKY相互作用2009

    • Author(s)
      矢野一雄, ほか
    • Organizer
      日本物理学会
    • Place of Presentation
      熊本大学
    • Year and Date
      2009-09-25
    • Related Report
      2009 Annual Research Report
  • [Presentation] 重い電子系化合物CeNiのGdによる微小置換と磁気秩序の発現2009

    • Author(s)
      矢野一雄、西村克彦、石川義和、吉岡顕人、桜井吉晴、伊藤真義、佐藤清雄
    • Organizer
      日本物理学会秋季大会
    • Place of Presentation
      岩手大学
    • Year and Date
      2009-09-21
    • Related Report
      2010 Final Research Report
  • [Presentation] Magnetic ordering and properties in heavy fermion (Ce1-XGdX)Ni(X=0.15 & 0.20) single crystal2009

    • Author(s)
      Kazuo Yano, Katsuhiko Nishimura, Yoshikazu Isikawa, Tsuyoshi Ohta, Kiyoo Sato
    • Organizer
      ICM2009 (International Conference on Magnetism 2009)
    • Place of Presentation
      Karsruhe, Germany
    • Year and Date
      2009-07-28
    • Related Report
      2010 Final Research Report
  • [Presentation] Magnetic ordering and properties in heavy fermionn(Ce_<1-x>Gd_x)Ni(X=0.15 & 0.20)single crystals2009

    • Author(s)
      矢野一雄, et al.
    • Organizer
      ICM 2009(International Conference on Magnetism)
    • Place of Presentation
      Karlsruhe(Germany)
    • Year and Date
      2009-07-27
    • Related Report
      2009 Annual Research Report
  • [Presentation] 重い電子系物質(Ce_<1-x>Gd_x)Ni(X<0.2)の磁気秩序の発現2009

    • Author(s)
      矢野一雄, 他5 名
    • Organizer
      日本物理学会
    • Place of Presentation
      立教大学
    • Year and Date
      2009-03-27
    • Related Report
      2008 Annual Research Report
  • [Presentation] 重い電子系化合物(Ce1-XGdX)Ni(X<0.20)の磁気秩序の発現2009

    • Author(s)
      矢野一雄、田尻佑太、西村克彦、石川義和、佐藤清雄
    • Organizer
      日本物理学会第64回年次大会
    • Place of Presentation
      立教大学
    • Year and Date
      2009-03-23
    • Related Report
      2010 Final Research Report
  • [Presentation] 重い電子系物質CeNiのGdによる微小置換と磁気秩序の発現2008

    • Author(s)
      矢野一雄, 他6名
    • Organizer
      日本物理学会
    • Place of Presentation
      岩手大学
    • Year and Date
      2008-09-21
    • Related Report
      2008 Annual Research Report
  • [Presentation] Onset of magnetic ordering in heavy fermion CeNi and (Ce0.97Gd0.03)Ni2008

    • Author(s)
      Kazuo Yano, Yuta Tajiri, Katsuhiko Nishimura, Yoshikazu Isikawa, Tsuyoshi Ohta, Kiyoo Sato
    • Organizer
      LT25 (Low Temperature Physics 25)
    • Place of Presentation
      Amsterdam, Holland
    • Year and Date
      2008-08-07
    • Related Report
      2010 Final Research Report
  • [Presentation] Onset of magnetic ordering in heavy fermion CeNi and (Ce0.97Gd0. 03)Ni2008

    • Author(s)
      K Yano, et al.
    • Organizer
      25^<th> International Conference on Low Temperature Physics (LT25)
    • Place of Presentation
      Amsterdam
    • Related Report
      2008 Annual Research Report
  • [Remarks] ホームページ等(現在作成中)

    • URL

      http://www.cis-trans.org./nihon-y/index.html

    • Related Report
      2010 Final Research Report

URL: 

Published: 2008-04-01   Modified: 2016-04-21  

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