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Study for atmospheric aerosol transport and transformation by the laser-ionization single-particle aerosol mass spectrometer

Research Project

Project/Area Number 20710006
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Environmental dynamic analysis
Research InstitutionKyoto University

Principal Investigator

YABUSHITA Akihiro  Kyoto University, 大学院・工学研究科, 助教 (70371151)

Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2010: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2009: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2008: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordsエアロゾル / 粒子状汚染物質 / 黄砂 / 鉛 / 多環芳香族炭化水素 / 越境大気汚染 / レーザー / 環境計測装置 / 環境動態解析 / 環境計測装置開発 / 環境計測 / 浮遊粒子状物質 / 装置開発 / 都市大気 / 微小粒子状物質
Research Abstract

Using the laser-ionization single-particle aerosol mass spectrometer, observation of atmospheric aerosol particles was performed at Fukue, Nagasaki in spring. The instrument obtains chemical compositions of the individual particles with a high time resolution. During the Kosa events, particles containing lead or polycyclic aromatic hydrocarbons were increased. Many of Pb-containing particles observed during the Kosa events also contained other metals attributed to solder and coal combustion, while many of those during non-Kosa periods contained components originating from sea salt. Information about sources or transport and transformation of Asian dust particles or particulate matters including hazardous substances were obtained by the instrument.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (45 results)

All 2011 2010 2009 2008

All Journal Article (16 results) (of which Peer Reviewed: 15 results) Presentation (29 results)

  • [Journal Article] Ion formation processes in laserablation of multicomponent inorganicparticles relevant to single particlelaser analysis of atmospheric aerosolsA.2011

    • Author(s)
      Yabushita, T.Kinugawa, M.Narukawa, K.Takahashi, M.Kawasaki, Y.
    • Journal Title

      MatsumiChemistry Letters 40

      Pages: 446-448

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ion formation processes in laser ablation of multicomponent inorganic particles relevant to single particle laser analysis of atmospheric aerosols2011

    • Author(s)
      A.Yabushita, T.Kinugawa, M.Narukawa, K.Takahashi, M.Kawasaki, Y.Matsumi
    • Journal Title

      Chemistry Letters

      Volume: 40

    • NAID

      10028242259

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nitrogen dioxide conversion to nitrateand nitrite on aqueous surfactantsT.2010

    • Author(s)
      Kinugawa, S.Enami, A.Yabushita, M.Kawasaki, M.R.Hoffmann, A.J.
    • Journal Title

      Colussi Physical Chemistry Chemical Physics 13

      Pages: 5144-5149

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of aerosol particles in the Tokyo metropolitan area using two different aerosol mass spectrometers2010

    • Author(s)
      J.Xing, K.Takahashi, A.Yabushita, T.Kinugawa, T.Nakayama, Y.Matsumi, K.Tonokura, A.Takami, T.Imamura, K.Sato, M.Kawasaki, T.Hikida, A.
    • Journal Title

      ShimonoAerosol Science and Technology 45

      Pages: 315-326

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of aerosol particles in the Tokyo metropolitan area using two different aerosol mass spectrometers2010

    • Author(s)
      J.Xing, K.Takahashi, A.Yabushita, T.Kinugawa, T.Nakayama, Y.Matsumi, K.Tonokura, A.Takami, T.Imamura, K.Sato, M.Kawasaki, T.Hikida, A.Shimono
    • Journal Title

      Aerosol Science and Technology

      Volume: 45 Pages: 315-326

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nitrogen dioxide conversion to nitrate and nitrite on aqueous surfactants2010

    • Author(s)
      T.Kinugawa, S.Enami, A.Yabushita, M.Kawasaki, M.R.Hoffinann, A.J.Colussi
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 13 Pages: 5144-5149

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Internal mixing of pollutants forsubmicron particles observed durings pringtime in Japan2009

    • Author(s)
      J.Matsumoto, M.Narukawa, K.Takahashi, Y.Matsumi, A.Yabushita, A.Shimizu, I.Matsui, N.Sugimoto
    • Journal Title

      Asian Journal of Atmospheric Environment 3

      Pages: 27-41

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Optical properties and chemical compositions of iodine-containing aerosols produced from the atmospheric photolysis of methylene iodide in thepresence of ozone2009

    • Author(s)
      Y.Sakamoto, A.Yabushita, M.Kawasaki, T.Nakayama, Y.Matsumi
    • Journal Title

      Bulletin of the Chemical Society of Japan 82

      Pages: 910-913

    • Related Report
      2010 Final Research Report
  • [Journal Article] Anion-catalyzed dissolution of NO_2 onaqueous microdroplets2009

    • Author(s)
      A.Yabushita, S.Enami, Y.Sakamoto, M.Kawasaki, M.R.Hoffmann, A.J.ColussiThe
    • Journal Title

      Journal of Physical Chemistry A 113

      Pages: 4844-4848

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Internal mixing of pollutants for submicron particles observed during springtime in Japan2009

    • Author(s)
      J.Matsumoto, M.Narukawa, K.Takahashi, Y.Matsumi, A.Yabushita, et al.
    • Journal Title

      Asian journal of atmospheric environment 3

      Pages: 27-41

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct emission of 12 molecule and 10 radical from the heterogeneous reactions of gaseous ozone with aqueous potassium iodide solution2009

    • Author(s)
      Y.Sakamoto, A.Yabushita, M.Kawasaki, S.Enami
    • Journal Title

      Journal of Physical Chemistry A 113

      Pages: 7707-7713

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Optical properties and chemical compositions of iodine-containing aerosols produced from the atmospheric photolysis of methylene iodide in the presence of ozone2009

    • Author(s)
      Y.Sakamoto, A.Yabushita, M.Kawasaki, T.Nakayama, Y.Matsumi
    • Journal Title

      Bulletin of the Chemical Society of Japan 82

      Pages: 910-913

    • NAID

      10025126647

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Translational and internal states of hydrogen molecules produced from the ultraviolet photodissociation of amorphous solid methanol2009

    • Author(s)
      T. Hama, M. Yokoyama, A. Yabushita, M. Kawasaki
    • Journal Title

      Journal of Chemical Physics 130

      Pages: 1645051-10

    • NAID

      120002086099

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anion-catalyzed dissolution of NO_2 on aqueous microdroplets2009

    • Author(s)
      A. Yabushita, S. Enami, Y. Sakamoto, M. Kawasaki, M. R. Hoffmann, A. J. Colussi
    • Journal Title

      Journal of Physical Chemistry A 113

      Pages: 4844-4848

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Single particle analysis of second aryorganic aerosols formed from1,4-Cyclohexadiene ozonolysis using alaser-ionization single-particle aerosolmass spectrometer2008

    • Author(s)
      M.Narukawa, Y.Matsumi, J.Matsumoto, K.Takahashi, A.Yabushita, K.Sato, T.Imamura
    • Journal Title

      Bulletin of the Chemical Society of Japan 81

      Pages: 120-126

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Direct observation of OH radicals ejected from water ice surface in the photoirradiation of nitrate adsorbed on ice at 100 K2008

    • Author(s)
      A. Yabushita, D. Iida, T. Hama, M. Kawasaki
    • Journal Title

      Journal of Physical Chemistry A 112

      Pages: 9763-9766

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] 2010年春季長崎県福江島における東アジアから輸送されたエアロゾル化学成分の単一粒子観測2010

    • Author(s)
      衣川高志、薮下彰啓、松見豊、中山智喜、川崎昌博
    • Organizer
      第16回大気化学討論会
    • Place of Presentation
      東京
    • Related Report
      2010 Final Research Report
  • [Presentation] 2010年春季に長崎県福江島で個別粒子計測した大気エアロゾルの化学特性2010

    • Author(s)
      薮下彰啓、衣川高志、中山智喜、松見豊、川崎昌博
    • Organizer
      第27回エアロゾル科学・技術研究討論会
    • Place of Presentation
      名古屋
    • Related Report
      2010 Final Research Report
  • [Presentation] Observation of nitrate-containingparticles at an urban site of Tokyo in the summer of 2008 with use of alaser-ionization single-particle aerosolmass spectrometer2010

    • Author(s)
      T.Kinugawa, A.Yabushita, T.Nakayama, J.-H.Xing, K.Takahashi, K.Tonokura, M.Kawasaki, Y.Matsumi
    • Organizer
      The 8th International Symposiumon Advanced Environmental Monitoring
    • Place of Presentation
      Sapporo
    • Related Report
      2010 Final Research Report
  • [Presentation] 2010年春季長崎県福江島におけるレーザー誘起蛍光法を用いたNO_2観測2010

    • Author(s)
      鈴木博之、中山智喜、和田龍一、松見豊、薮下彰啓
    • Organizer
      第16回大気化学討論会
    • Place of Presentation
      首都大学東京
    • Related Report
      2010 Annual Research Report
  • [Presentation] 2010年春季長崎県福江島における東アジアから輸送されたエアロゾル化学成分の単一粒子観測2010

    • Author(s)
      衣川高志、薮下彰啓、松見豊、中山智喜、川崎昌博
    • Organizer
      第16回大気化学討論会
    • Place of Presentation
      首都大学東京
    • Related Report
      2010 Annual Research Report
  • [Presentation] 2010年春季に長崎県福江島で個別粒子計測した大気エアロゾルの化学特性2010

    • Author(s)
      薮下彰聲、衣川高志、中山智喜、松見豊、川崎昌博
    • Organizer
      第27回エアロゾル科学・技術研究討論会
    • Place of Presentation
      名古屋大学
    • Related Report
      2010 Annual Research Report
  • [Presentation] Observation of nitrate-containing particles at an urban site of Tokyo in the summer of 2008 with use of a laser-ionization single-particle aerosol mass spectrometer2010

    • Author(s)
      T.Kinugawa, A.Yabushita, T.Nakayama, J.Xing, K.Takahashi, K.Tonokura, M.Kawasaki, Y.Matsumi
    • Organizer
      The 8th International Symposium on Advanced Environmental Monitoring
    • Place of Presentation
      北海道大学
    • Related Report
      2010 Annual Research Report
  • [Presentation] Internal mixing states of atmospheric aerosols studied by a laser ionization single-particle mass spectrometer during spring time in Okinawa.2009

    • Author(s)
      Y.Matsumi,A.Yabushita, T.Kumazawa, J.Matsumoto, M.Narukawa, T.Nakayama, K.Tkahashi
    • Organizer
      Japan Fourth Japan-China-Korea Joint Conferenceon Meteorology
    • Place of Presentation
      Tsukuba, Japan
    • Related Report
      2010 Final Research Report
  • [Presentation] 2008年夏季東京都心におけるエアロゾル中の硝酸塩の生成2009

    • Author(s)
      衣川高志、薮下彰啓、松見豊、中山智喜、シンジャワ、高橋けんし、戸野倉賢一、川崎昌博
    • Organizer
      第15回大気化学討論会
    • Place of Presentation
      つくば
    • Related Report
      2010 Final Research Report
  • [Presentation] Observation of nitrate-containing particles at an urban site of Tokyo in the summer of 2008 with use oflaser-ionization single-particle aerosolmass spectrometry2009

    • Author(s)
      T.kinugawa, A.Yabushita, Y.Matsumi, T.Nakayama, J.-H.Xing, K.Takahashi, K.Tonokura, M.Kawasaki
    • Organizer
      Workshop on Chemistry in the Earth ' s Atmosphere - Crosscutting Aspects of Molecular Science and Atmospheric Chemistry -
    • Place of Presentation
      Tokyo
    • Related Report
      2010 Final Research Report
  • [Presentation] レーザーイオン化個別粒子質量分析計による2008年夏季東京都心のエアロゾル観測2009

    • Author(s)
      衣川高志、薮下彰啓、川崎昌博、中山智喜、松見豊、シンジャワ、高橋けんし、戸野倉賢一
    • Organizer
      日本地球惑星科学連合2009年大会
    • Place of Presentation
      千葉
    • Related Report
      2010 Final Research Report
  • [Presentation] 二種類の質量分析計による大気エアロゾル観測2009

    • Author(s)
      シンジャワ、高橋けんし、薮下彰啓、衣川高志、中山智喜、松見豊、戸野倉賢一、川崎昌博、高見昭憲、佐藤圭、今村隆史、疋田利秀、下野彰夫
    • Organizer
      第57回質量分析総合討論会
    • Place of Presentation
      大阪
    • Related Report
      2010 Final Research Report
  • [Presentation] 二種類の質量分析計による大気エアロゾル観測2009

    • Author(s)
      シンジャワ、高橋けんし、薮下彰啓, 他10名
    • Organizer
      第57回質量分析総合討論会
    • Place of Presentation
      大阪国際交流センター
    • Related Report
      2009 Annual Research Report
  • [Presentation] レーザーテオン化個別粒子質量分析計による2008年夏季東京都心のエアロゾル観測2009

    • Author(s)
      衣川高志、薮下彰啓、川崎昌博, 他5名
    • Organizer
      日本地球惑星科学連合2009年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Related Report
      2009 Annual Research Report
  • [Presentation] 夏季東京都心におけるエアロソル光学特性と化学特性の同時観測2009

    • Author(s)
      中山智喜、萩野理恵、松見豊、薮下彰啓, 他11名
    • Organizer
      日本気象学会2009年度春季大会
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2009 Annual Research Report
  • [Presentation] Optical properties and chemical compositions of iodine-containing aerosols produced from the atmospheric photolysis of methylene iodide2009

    • Author(s)
      坂本陽介、薮下彰啓、川崎昌博、中山智喜、松見豊
    • Organizer
      第25回化学反応討論会
    • Place of Presentation
      大宮ソニックシティ
    • Related Report
      2009 Annual Research Report
  • [Presentation] Observation of nitrate-containing particles at an urban site of Tokyo in the summer of 2008 with use of laser-ionization single-particle aerosol mass spectrometry2009

    • Author(s)
      T.kinugawa, A.Yabushita, Y.Matsumi, T.Nakayama, J.-H.Xing, K.Takahashi, K.Tonokura, N.Kawasaki
    • Organizer
      Workshop on Chemistry in the Earth's Atmosphere
    • Place of Presentation
      東京工業大学
    • Related Report
      2009 Annual Research Report
  • [Presentation] Optical properties and chemical compositions of iodine-containing aerosols produced from the atmospheric photolysis of methylene iodide2009

    • Author(s)
      Y.Sakamotoa, A.Yabushita, M.Kawasaki, T.Nakayama, Y.
    • Organizer
      Workshop on Chemistry in the Earth's Atmosphere
    • Place of Presentation
      東京工業大学
    • Related Report
      2009 Annual Research Report
  • [Presentation] 2008年夏季東京都心におけるエアロゾル中の硝酸塩の生成2009

    • Author(s)
      衣川高志, 薮下彰啓, 松見豊, 中山智喜, シンジャワ, 高橋けんし, 戸野倉賢一, 川崎昌博
    • Organizer
      第15回大気化学討論会
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2009 Annual Research Report
  • [Presentation] INTERNAL MIXING STATES OF ATMOSPHERIC AEROSOLS STUDIED BY ALASER IONIZATION SINGLE-PARTICLE MASS SPECTROMETER DURINGSPRING TIME IN OKINAWA, JAPAN2009

    • Author(s)
      Y.MATSUMI, A.YABUSHITA, et al.
    • Organizer
      Fourth Japan-China-Korea Joint Conference on Meteorology
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2009 Annual Research Report
  • [Presentation] 黄砂飛来時の東京におけるレーザーイオン化個別粒子質量分析計による大気エアロゾルの個別粒子分析2008

    • Author(s)
      戸野倉賢一、薮下彰啓、中山智喜、松見豊
    • Organizer
      第56回質量分析総合討論会
    • Place of Presentation
      つくば
    • Year and Date
      2008-05-06
    • Related Report
      2010 Final Research Report
  • [Presentation] 沖縄辺戸岬におけるエアロゾル中の硝酸塩と主要化学種の関係2008

    • Author(s)
      薮下彰啓、衣川高志、川崎昌博、熊澤俊哉、中山智喜、松見豊、松本淳
    • Organizer
      第14回大気化学討論会
    • Place of Presentation
      横浜
    • Related Report
      2010 Final Research Report
  • [Presentation] 大気エアロゾル単一粒子質量分析装置の開発2008

    • Author(s)
      熊澤俊哉、薮下彰啓、中山智喜、松見豊、松本淳
    • Organizer
      第14回大気化学討論会
    • Place of Presentation
      横浜
    • Related Report
      2010 Final Research Report
  • [Presentation] レーザーイオン化個別粒子質量分析計による大気エアロゾルの内部混合状態解明-沖縄辺戸岬での春季観測2008

    • Author(s)
      熊澤俊哉、松見豊、中山智喜、薮下彰啓、松本淳
    • Organizer
      第25回エアロゾル科学・技術研究討論会
    • Place of Presentation
      金沢
    • Related Report
      2010 Final Research Report
  • [Presentation] 黄砂飛来時の東京におけるレーザーイオン化個別粒子質量分析計による大気エアロゾルの個別粒子分析2008

    • Author(s)
      戸野倉賢一、薮下彰啓、中山智喜、松見豊
    • Organizer
      第56回質量分析総合討論会
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2008 Annual Research Report
  • [Presentation] メンブレン導入光イオン化飛行時間質量分析装置の開発2008

    • Author(s)
      戸野倉賢一、菅野望、長島理香、平野恭司、薮下彰啓、川崎昌博
    • Organizer
      第56回質量分析総合討論会
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2008 Annual Research Report
  • [Presentation] Formation of nitrate in aqueous aerosol microdroplets exposed to gaseous NO_22008

    • Author(s)
      薮下彰啓、江波進一、坂本陽介、川崎昌博、M.R.Hoffmann、A.J、Colussi
    • Organizer
      日本地球惑星科学連合2008年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Related Report
      2008 Annual Research Report
  • [Presentation] レーザーイオン化個別粒子質量分析計による大気エアロゾルの内部混合状態解明-沖縄辺戸岬での春季観測2008

    • Author(s)
      熊澤俊哉、松見豊、中山智喜、薮下彰啓、松本淳
    • Organizer
      第25回エアロゾル科学・技術研究討論会
    • Place of Presentation
      金沢大学角間キャンパス自然科学本館
    • Related Report
      2008 Annual Research Report
  • [Presentation] 沖縄辺戸岬におけるエアロゾル中の硝酸塩と主要化学種の関係2008

    • Author(s)
      薮下彰啓、衣川高志、熊澤俊哉、中山智喜、松見豊、松本淳、川崎昌博
    • Organizer
      第14回大気化学討論会
    • Place of Presentation
      海洋研究開発機構・横浜研究所
    • Related Report
      2008 Annual Research Report

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Published: 2008-04-01   Modified: 2016-04-21  

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