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Elucidation of competition between magnetism and conductivity in actinide chalcogenide compounds

Research Project

Project/Area Number 20740210
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Condensed matter physics II
Research InstitutionUniversity of Hyogo

Principal Investigator

SHUGO Ikeda  University of Hyogo, 大学院・物質理学研究科, 助教 (80414580)

Project Period (FY) 2008 – 2011
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2010: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2009: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2008: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywords巨大磁気抵抗 / 金属絶縁体転移 / 5f電子 / カルコゲナイド化合物 / β-US_2 / USeS / 磁気ポーラロン / EuFe_2As_2 / カルコゲナイド元素
Research Abstract

We studied the physical properties of UXS (X:S, Se, Te) with an orthorhombic crystal structure by measuring its magnetization, magnetic susceptibility, specific heat, and electrical resistivity under magnetic field and pressure. The insulating resistivity of β-US_2 markedly changes to a metallic one under a high pressure of 8 GPa similarly to that of the semimetallic Ising-type ferromagnet UTeS with a Curie temperature TC=87 K.A resistivity anomaly was also observed in the temperature dependence of the resistivity under pressure, most likely corresponding to ferromagnetic ordering. From these experimental results, it was concluded that β-US_2 is in the vicinity of ferromagnetic ordering at ambient pressure. Furthermore, we found that the easy-axis magnetization at low fields for H // [001] consists of a linear magnetization based on the 5f-CEF scheme and a ferromagnetic-like magnetization with a saturated moment of 0.042α_β/U. The latter magnetization was analyzed on the basis of the ferromagnetic cluster and discussed from the viewpoint of the magnetic polaron.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (22 results)

All 2010 2009 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results) Presentation (17 results) Remarks (1 results)

  • [Journal Article] Neutron scattering study on U-dichalcogenides2010

    • Author(s)
      N.Metoki, K.Kaneko, S.Ikeda, H.Sakai, E.Yamamoto, Y.Haga, Y, Homma, Y.Shiokawa.
    • Journal Title

      IOP Conf.Series ; Materials Science and Engineering 9

      Pages: 12088-12088

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Neutron scattering study on U-dichalcogenides2010

    • Author(s)
      N.Metoki, K.Kaneko, S.ikeda, et.al
    • Journal Title

      IOP Conf.Series ; Materials Science and Engineering

      Volume: 9

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Possible Existence of Magnetic Polaron in Nearly Ferromagnetic Semiconductor β-US_22009

    • Author(s)
      S.ikeda, H.Sakai, N.Tateiwa, T.D.Matusda, D.Aoki, Y.Homma, E.Yamamoto, A.Nakamura, Y.Shiokwa, Y.Ota, K.Sugiyama, M.Hagiwara, K.Kindo, K.Matsubayashi, M.Hedo, Y.Uwatoko, Y.Haga, Y.Onuki.
    • Journal Title

      J.Phys.Soc.Jpn. 78

      Pages: 114704-114704

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Possible Existence of Magnetic Polaron in Nearly Ferromagnetic Semiconductor β-US_22009

    • Author(s)
      池田修悟
    • Journal Title

      J.Phys.Soc.Jpn 78

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] 複合極限環境下^<57>Fe及び^<151>Eu核共鳴前方散乱によるEuFe_2As_2の電子状態研究2010

    • Author(s)
      池田修悟, 等
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学(大阪府)
    • Year and Date
      2010-09-23
    • Related Report
      2010 Annual Research Report
  • [Presentation] ウランカルコゲナイド化合物β-US_2の圧力誘起強磁性2010

    • Author(s)
      立岩尚之, 芳賀芳範, 池田修悟, 等
    • Organizer
      日本物理学会
    • Place of Presentation
      岡山大学(岡山県)
    • Year and Date
      2010-03-21
    • Related Report
      2010 Annual Research Report
  • [Presentation] 複合極限環境下^<57>Fe及び^<151>Eu核共鳴前方散乱によるEuFe_2As_2の電子状態研究2010

    • Author(s)
      池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] ウランカルコゲナイド化合物β-US_2の圧力誘起強磁性2010

    • Author(s)
      立岩尚之, 芳賀芳範, 池田修悟, 等
    • Organizer
      日本物理学会春季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] AFe_2As)2(A=Sr,Eu)の^<57>Fe核共鳴非弾性散乱による格子振動II2010

    • Author(s)
      小林寿夫, 池田修悟, 等
    • Organizer
      日本物理学会春季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] 複合極限環境下^<151>Eu核共鳴前方散乱によるEuFe_2As_2の電子状態研究2010

    • Author(s)
      池田修悟, 等
    • Organizer
      日本物理学会春季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] 複合極限環境下^<57>Fe核共鳴前方散乱実験によるEuFe_2As_2の電子状態の研究2009

    • Author(s)
      池田修悟
    • Organizer
      日本物理学会
    • Place of Presentation
      熊本大学
    • Year and Date
      2009-09-26
    • Related Report
      2009 Annual Research Report
  • [Presentation] 単結晶試料によるFe系層状物質EuFe_2As_2のメスバウアー効果測定2009

    • Author(s)
      池田修悟
    • Organizer
      日本物理学会春季大会
    • Place of Presentation
      東京池袋
    • Year and Date
      2009-03-30
    • Related Report
      2008 Annual Research Report
  • [Presentation] 複合極限環境下^<57>Fe核共鳴前方散乱実験によるEuFe_2As_2の電子状態の研究2009

    • Author(s)
      池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] ウランカルコゲナイドにおける結晶場励起の磁場依存性2009

    • Author(s)
      山本悦嗣, 芳賀芳範, 立岩尚之, 菅井孝志, 池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] ウランカルコゲナイド化合物US_2の圧力誘起秩序相の研究2009

    • Author(s)
      立岩尚之, 芳賀芳範, 山本悦嗣, 池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] EuFe_2As_2の^<57>Fe核共鳴非弾性散乱による格子振動2009

    • Author(s)
      小林寿夫, 池田修悟, 依田芳卓
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] US_2の強磁場磁性22009

    • Author(s)
      杉山清寛, 広瀬雄介, 中村太一, 戸田雅敏, 山本悦嗣, 芳賀芳範, 池田修悟
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] ウランカルコゲナイドの物性2009

    • Author(s)
      山本悦嗣, 目時直人, 池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] US_2の強磁場磁性2009

    • Author(s)
      杉山清寛, 太田有基, 広瀬雄介, 芳賀芳範, 池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] ウランカルコゲナイドにおける5f遍歴-局在クロスオーバーを伴う金属-非金属転移2009

    • Author(s)
      目時直人, 池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Presentation] 単結晶試料によるFe系層状物質EuFe_2As_2のメスバウアー効果測定2009

    • Author(s)
      池田修悟, 等
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2010 Final Research Report
  • [Remarks] ホームページ等

    • Related Report
      2010 Final Research Report

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Published: 2008-04-01   Modified: 2020-05-15  

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