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Study of Topological Phase Transitions Using Operando Spin- and Angle-Resolved Photoelectron Spectroscopy

Research Project

Project/Area Number 20H00347
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Review Section Medium-sized Section 29:Applied condensed matter physics and related fields
Research InstitutionHiroshima University

Principal Investigator

Okuda Taichi  広島大学, 放射光科学研究センター, 教授 (80313120)

Project Period (FY) 2020-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥45,890,000 (Direct Cost: ¥35,300,000、Indirect Cost: ¥10,590,000)
Fiscal Year 2023: ¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2022: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2021: ¥13,260,000 (Direct Cost: ¥10,200,000、Indirect Cost: ¥3,060,000)
Fiscal Year 2020: ¥22,620,000 (Direct Cost: ¥17,400,000、Indirect Cost: ¥5,220,000)
Keywordsスピン分解光電子分光 / トポロジカル相転移 / キラリティ誘起スピン選択(CISS)効果 / オペランド電子分光 / 放射光・レーザー / スピントロニクス / スピン・角度分解光電子分光 / 外場印加下光電子分光 / マイクロビーム / カイラル誘起スピン選択効果 / オペランド分光 / キラリティ誘起スピン選択効果 / 放射光 / オペランド / トポロジカル物質 / 放射光微小ビーム
Outline of Research at the Start

トポロジカル絶縁体に代表されるトポロジカル物質は表面に存在する理論上100%スピン偏極した特殊な表面電子状態を利用することで、スピントロニクスデバイス実現のキーマテリアルとなると考えられている。実際にスピントロニクスデバイスへ応用する際には、温度や磁場、圧力といった様々な外場に対する電子状態の応答を解明することがデバイスの安定性や、機能性デバイス創世の観点から重要である。そこで本研究では我々の保持する世界最高性能のスピン・角度分解光電子分光装置に集光ミラーによりマイクロサイズに集光した放射光ビームを導入し、トポロジカル物質の電子状態を効率よく観測し、トポロジカル物質の外場応答を解明する。

Outline of Final Research Achievements

We performed spin- and angle-resolved photoelectron spectroscopy while applying external fields (pressure, electric fields, etc.) to study topological phase transitions and related phenomena. By modifying the sample holder and manipulator to create pressure or electric field gradients etc. on the sample, and focusing the excitation light to a small spot using mirrors or lens, we developed the micro-spin ARPES system that enables to efficiently observe electronic states change caused by the external fields. Using this system, we investigated the changes in electronic states of topological materials due to pressure and temperature variations, as well as the Chiral Induced Spin Selectivity effect, which generates spin-polarized current when an electric current passes through chiral materials. As a result, we discovered new physical phenomena, including changes in electronic states of topological materials caused by pressure and a spiral photoelectron pattern from chiral materials.

Academic Significance and Societal Importance of the Research Achievements

本研究では、圧力や温度によるトポロジカル相転移や電流によるCISS効果などの解明をするため、オペランド顕微スピン角度分解光電子分光装置を開発した。トポロジカル物質の研究は物性物理において主要な研究分野であるとともに、オペランド分光や顕微分光は光電子分光業界で急速にニーズが高まっていることから、本研究で得られた成果やノウハウは当該分野の発展に寄与することが予想される。また、現在スピントロニクスなどの次世代デバイス開発研究が精力的に行われているが、開発した装置は共同利用施設であるHiSORに設置され、国内外のユーザーが利用可能であり、スピントロニクス材料等の研究に広く貢献することが期待できる。

Report

(6 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Annual Research Report
  • 2021 Annual Research Report
  • 2020 Comments on the Screening Results   Annual Research Report
  • Research Products

    (50 results)

All 2024 2023 2022 2020 Other

All Int'l Joint Research (10 results) Journal Article (9 results) (of which Int'l Joint Research: 9 results,  Peer Reviewed: 9 results,  Open Access: 3 results) Presentation (30 results) (of which Int'l Joint Research: 15 results,  Invited: 4 results) Remarks (1 results)

  • [Int'l Joint Research] SOLEIL(フランス)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Weizmann Institute of Science(イスラエル)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] 南方科技大/中国科学院(中国)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Wurzburg University/Muenster University(ドイツ)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] University of Wisconsin-Milwaukee(米国)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Munster University/Wurzburg University(ドイツ)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] SOLEIL/Universite Paris-Saclay(フランス)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] 中国科学院/南方科学技術大学/中国・電子科技大(中国)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] 南方科技大学(中国)

    • Related Report
      2021 Annual Research Report
  • [Journal Article] Laser-based angle-resolved photoemission spectroscopy with micrometer spatial resolution and detection of three-dimensional spin vector2024

    • Author(s)
      Iwata Takuma、Kousa T.、Nishioka Y.、Ohwada K.、Sumida K.、Annese E.、Kakoki M.、Kuroda Kenta、Iwasawa H.、Arita M.、Kumar S.、Kimura A.、Miyamoto K.、Okuda T.
    • Journal Title

      Scientific Reports

      Volume: 14 Issue: 1 Pages: 127-127

    • DOI

      10.1038/s41598-023-47719-z

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Spiral band structure hidden in the bulk chiral crystal NbSi22023

    • Author(s)
      Cheng Zhang, Tatsuya Shishidou, Ryoga Amano, Koji Miyamoto, Taisei Sayo, Chiho Shimada, Yusuke Kousaka, Michael Weinert, Yoshihiko Togawa, Daichi Okuda
    • Journal Title

      Physical Review B

      Volume: 108 Issue: 23 Pages: 235164-235164

    • DOI

      10.1103/physrevb.108.235164

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Exploring spin-polarization in Bi-based high-Tc cuprates2023

    • Author(s)
      Iwasawa Hideaki、Sumida Kazuki、Ishida Shigeyuki、Le Fevre Patrick、Bertran Francois、Yoshida Yoshiyuki、Eisaki Hiroshi、Santander-Syro Andras F.、Okuda Taichi
    • Journal Title

      Scientific Reports

      Volume: 13 Issue: 1 Pages: 13451-13451

    • DOI

      10.1038/s41598-023-40145-1

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Strongly anisotropic spin and orbital Rashba effect at a tellurium - noble metal interface2023

    • Author(s)
      Geldiyev B.、Uenzelmann M.、Eck P.、Kisslinger T.、Schusser J.、Figgemeier T.、Kagerer P.、Tezak N.、Krivenkov M.、Varykhalov A.、Fedorov A.、Nicolai L.、Minar J.、Miyamoto K.、Okuda T.、Shimada K.、Di Sante D.、Sangiovanni G.、Hammer L.、Schneider M. A.、Bentmann H.、Reinert F.
    • Journal Title

      Physical Review B

      Volume: 108 Issue: 12

    • DOI

      10.1103/physrevb.108.l121107

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Surface electronic structure of Re(0001): A spin-resolved photoemission study2023

    • Author(s)
      Marcel Holtmann, Peter Kruger, Koji Miyamoto, Taichi Okuda, Kenya Shimada, and Markus Donath
    • Journal Title

      Physical Review B

      Volume: 107 Issue: 16 Pages: 165420-165420

    • DOI

      10.1103/physrevb.107.165420

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Systematic study of electronic states of Ln(O,F)BiS2 by spin- and angle-resolved photoemission spectroscopy2022

    • Author(s)
      Shi-Long Wu, Koichiro Yaji, Yuichi Ota, Ayumi Harasawa, Shik Shin, Takehito Imai, Koji Miyamoto, Masanori Nagao, Satoshi Watauchi, Isao Tanaka, Xiaoping Ma, Huaixin Yang, Yongqing Cai, Lin Zhao, Xingjiang Zhou, and Taichi Okuda
    • Journal Title

      Physical Review B

      Volume: 106 Issue: 10

    • DOI

      10.1103/physrevb.106.104511

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Distinct Tamm and Shockley surface states on Re(0001) mixed by spin-orbit interaction2022

    • Author(s)
      Marcel Holtmann, Peter Krüger, Koji Miyamoto, Taichi Okuda, Pascal J. Grenz, Shiv Kumar, Kenya Shimada, and Markus Donath
    • Journal Title

      Physical Review B

      Volume: 105 Issue: 24

    • DOI

      10.1103/physrevb.105.l241412

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Domain Dependent Fermi Arcs Observed in a Striped Phase Dichalcogenide2022

    • Author(s)
      Takashi Mizokawa, Alexei Barinov, Viktor Kandyba, Alessio Giampietri, Ryoya Matsumoto, Yohei Okamoto, Kou Takubo, Koji Miyamoto, Taichi Okuda, Sunseng Pyon, Hiroyuki Ishii, Kazutaka Kudo, Minoru Nohara, Naurang L. Saini
    • Journal Title

      Advanced Qunatum Technologies

      Volume: 5 Issue: 9 Pages: 202300029-202300029

    • DOI

      10.1002/qute.202200029

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Experimental verification of temperature induced topological phase transition on TlBiS2 and TlBiSe22020

    • Author(s)
      Takehito Imai , Jiahua Chen, Kazuki Kato, Kenta Kuroda, Teruo Matsuda, Akio Kimura, Koji Miyamoto, Sergey V. Eremeev, and Taichi Okuda
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 12 Pages: 125151-125151

    • DOI

      10.1103/physrevb.102.125151

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 垂直磁気異方性を示すRh(001)基板上のFeCo薄膜のスピン偏極電子状態2024

    • Author(s)
      國友香里, 角田一樹A, 宮本幸治, Cheng Zhang, 桜庭裕弥, 奥田太一
    • Organizer
      日本物理学会春季大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Electronic Properties of (Bi,Pb)/Ge(111) Studied by Spin-Resolved ARPES2024

    • Author(s)
      L. Konermann, H. Abe, K. Sumida, K. Miyamoto, T. Okuda, M. Imamura, K. Takahashi, A. Takayama
    • Organizer
      日本物理学会春季大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 軟X線角度分解光電子分光を用いた反強磁性体PdCrO2における電子状態の研究2024

    • Author(s)
      岩田 拓万、白石 海人、中西 楓恋、森田 雄晴、西岡 幸美、高佐 永遠、大和田 清貴、Munisa Nurmamat、山神 光平、木村 昭夫、宮本 幸治、奥田 太一、高津 浩、黒田 健太
    • Organizer
      日本放射光学会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Preparation of Pt Thin Film on MgO (001) and Observation of Its Electronic Structure2024

    • Author(s)
      T. Asano, K. Sumida, K. Kunitomo, T. Okuda, and K. Miyamoto
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Attempt to Control the Anisotropy of Topological Surface States2024

    • Author(s)
      R. Yamamoto, K. Sumida, K. Miyamoto, and T. Okuda
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spin-polarized electronic states of FeCo thin film on Rh(001) substrate2024

    • Author(s)
      K. Kunitomo, K. Sumida, K. Miyamoto, C. Zhang, Y. Sakuraba, and T. Okuda
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ultrafast Spin-Dependent Dynamics in a Carrier-Tuned Topological Insulator2024

    • Author(s)
      K. Sumida, K. Kunitomo, M. Kakoki, K. A. Kokh, O. E. Tereshchenko, J. Reimann, J. Gudde, U. Hofer, K. Miyamoto, T. Okuda and A. Kimura
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Demonstration of phase-resolved spin-ARPES on topological surface states in Bi2Te32024

    • Author(s)
      Towa Kousa, T. Iwata, S. Kumar, A. Kimura, K. Miyamoto, T. Okuda and K. Kuroda
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Performance of laser-based SARPES with micrometer spatial and vector spin resolution at HiSOR2024

    • Author(s)
      Takuma Iwata, T. Kousa, Y. Nishioka, K. Ohwada, K. Sumida, E. Annese, M. Kakoki, K. Kuroda, H. Iwasawa, M. Arita, S. Kumar, A. Kimura, Miyamoto and T. Okuda
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Direct Observation of Spin-split Electronic Structures in Antiferromagnet NdBi by Laser-based SARPES2024

    • Author(s)
      Rikako Yamamoto, T. Motoyama, T. Iwata, T. Kosa, Y. Nishioka, K. Ideura, M. Arita, S. Ideta, K. Shimada, K. Miyamoto, T. Okuda, A. Kimura, T. Onimaru, and Kenta Kuroda
    • Organizer
      28th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spiral electronic structure of chiral crystal NbSi22023

    • Author(s)
      C. Zhang, K. Miyamoto, T. Shishidou, R. Amano, T. Sayo, C. Shimada, Y. Kousaka, M. Weinert, Y. Togawa, and T. Okuda
    • Organizer
      第36回日本放射光学会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Spiral Band Structure Hidden in the bulk Chiral Crystal NbSi22023

    • Author(s)
      Cheng Zhang, Koji Miyamoto, Tatsuya Shishidou, Ryoga Amano, Taisei Sayo, Chiho Shimada, Yusuke Kousaka, Michael Weinert, Yoshihiko Togawa, and Taichi Okuda
    • Organizer
      The 19th International Conference on Chiroptical Spectroscopy
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spiral Band Structure Hidden in the bulk Chiral Crystal NbSi22023

    • Author(s)
      C. Zhang, T. Shishidou, R. Amano, K. Miyamoto1, T. Sayo, C. Shimada, Y. Kousaka, M. Weinert, Y. Togawa, and T. Okuda
    • Organizer
      The 3rd Advanced Materials Research Grand Meeting and the 24th International Union of Materials Research Societies-International Conference in Asia
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] スピン角度分解光電子分光による酸素終端FeCo薄膜のスピン電子状態の観測2023

    • Author(s)
      國友香里, 宮本幸治, Cheng Zhang, 桜庭裕弥, 奥田太一
    • Organizer
      日本物理学会年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 軟X線角度分解光電子分光とSHG顕微鏡を用いたデラフォサイト型酸化物の電子状態の研究2023

    • Author(s)
      岩田拓万, 白石海人, 中西楓恋, 森田雄晴, 西岡幸美, 高佐永遠, 大和田清貴, Munisa Nurmamat, 山神光平, 木村昭夫, 宮本幸治, 奥田太一, 高津浩, 黒田健太
    • Organizer
      日本物理学会年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 次世代スピン分解光電子分光測定に向けたHiSORでのR&Dの現状2023

    • Author(s)
      奥田太一
    • Organizer
      ナノテラスARPESシンポジウム(ナノ集光で拓くサイエンスの新展開)
    • Related Report
      2023 Annual Research Report
  • [Presentation] Peculiar spin texture of Bi(110) observed by ESPRESSO machine2023

    • Author(s)
      Taichi Okuda
    • Organizer
      Seminar ISMO, Universite Paris-Saclay
    • Related Report
      2023 Annual Research Report
  • [Presentation] Spin- and Angle-resolved photoelectron spectroscopy and its application for chiral material2023

    • Author(s)
      Taichi Okuda
    • Organizer
      SKCM2 2023 Winter School
    • Related Report
      2023 Annual Research Report
  • [Presentation] Development of the laser based μ-SARPES machine at HiSOR2023

    • Author(s)
      Takuma Iwata, Kousa Towa, Yukimi Nishioka, Ohwada Kiyotaka, Hideaki Iwasawa, Masashi Arita, Akio Kimura, Kenta Kuroda, Koji Miyamoto, Taichi Okuda
    • Organizer
      American Physical Society March meeting
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Band structure of ferromagnetic Fe4N thin-film revealed by spin- and angle- resolved photoelectron spectroscopy2023

    • Author(s)
      Karen Nakanishi, Kiyotaka Ohwada, Kenta Kuroda, Kazuki Sumida, Hitoshi Sato, Koji Miyamoto, Taichi Okuda, Shinji Isogami, Keisuke Masuda, Yuya Sakuraba, Akio Kimura
    • Organizer
      American Physical Society March meeting
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spiral electronic structure of chiral crystal NbSi22023

    • Author(s)
      C. Zhang, K. Miyamoto, T. Shishidou, R. Amano, T. Sayo, C. Shimada, Y. Kousaka, M. Weinert, Y. Togawa, and T. Okuda
    • Organizer
      American Physical Society March meeting
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 角度分解光電子分光によるカイラル結晶のヘリシティの可視化2023

    • Author(s)
      ZHANG Cheng ,天野凌我, 宮本幸治, 獅子堂達也, 佐用大晴, 島田千穂, 高阪勇輔, WEINERT T. Michael , 戸川欣彦, 奥田太一
    • Organizer
      日本放射光学会年会
    • Related Report
      2022 Annual Research Report
  • [Presentation] Spiral band structure hidden in the bulk chiral crystal NbSi22023

    • Author(s)
      C. Zhang, K. Miyamoto, T. Shishidou, R. Amano, T. Sayo, C. Shimada, Y. Kousaka, M.l Weinert, Y. Togawa, T. Okuda
    • Organizer
      27th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of Perpendicular Anisotropy in FeCo Alloy Films Covered with Oxygen for Development of Multi Spin Detecting Target2023

    • Author(s)
      K. Kunitomo, K. Miyamoto, T. Okuda
    • Organizer
      27th Hiroshima International Symposium on Synchrotron Radiation
    • Related Report
      2022 Annual Research Report
  • [Presentation] 次世代スピン分解光電子分光測定に向けたHiSORでのR&Dの現状ーナノテラスにおけるナノスピンARPESへの期待2023

    • Author(s)
      奥田太一
    • Organizer
      ナノテラスARPESシンポジウム「ナノ集光ビームで拓くサイエンスの新展開」
    • Related Report
      2022 Annual Research Report
    • Invited
  • [Presentation] Spin-resolved photoemission and its future prospect2023

    • Author(s)
      Taichi Okuda
    • Organizer
      6th QST International Symposium, Innovation in Science and Technology from “NanoTerasu”
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] カイラル構造を持つNbSi2の電子構造2022

    • Author(s)
      宮本幸治, 天野凌我, Chen Zhang,戸川欣彦,獅子堂達也, 奥田太一
    • Organizer
      日本物理学会分科会
    • Related Report
      2022 Annual Research Report
  • [Presentation] キラリティ誘起スピン選択のスピン分解光電子分光による観測の試み2022

    • Author(s)
      奥田太一
    • Organizer
      第26回HiSOR研究会 ~生体分子の構造機能研究におけるキラル分光の新しい可能性~
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Development of micro-focus spin-resolved photoemission spectrometer in VUV-SX region2022

    • Author(s)
      Taichi Okuda
    • Organizer
      International Chemical Congress of Pacific Basin Societies (Pacifichem 2021)
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] TlBiS2およびTlBiSe2における温度誘起トポロジカル相転移の光電子分光による研究2020

    • Author(s)
      今井健人、加藤和貴、松田旭央、Jiahua Chen、宮本幸治、木村昭夫、奥田太一
    • Organizer
      日本放射光学会
    • Related Report
      2020 Annual Research Report
  • [Remarks] 電子・スピンの運動を可視化する走査型顕微鏡の開発 -マイクロメートル領域のスピン流を精密に測定

    • URL

      https://www.hsrc.hiroshima-u.ac.jp/research/result/63.html

    • Related Report
      2023 Annual Research Report

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Published: 2020-04-28   Modified: 2025-01-30  

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