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Search for topological phase transitions in Kitaev spin liquid candidate materials

Research Project

Project/Area Number 20H02600
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 29010:Applied physical properties-related
Research InstitutionTohoku University (2021-2023)
The University of Tokyo (2020)

Principal Investigator

Mizukami Yuta  東北大学, 理学研究科, 准教授 (80734095)

Project Period (FY) 2020-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥18,460,000 (Direct Cost: ¥14,200,000、Indirect Cost: ¥4,260,000)
Fiscal Year 2022: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2021: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2020: ¥12,870,000 (Direct Cost: ¥9,900,000、Indirect Cost: ¥2,970,000)
Keywordsキタエフ模型 / 量子スピン液体 / マヨラナ粒子 / 非可換エニオン / チャーン数 / トポロジカル転移 / 比熱測定 / 磁場角度回転 / トポロジカル相 / マヨラナフェルミオン / 微小単結晶 / トポロジカル相転移 / マヨラナ励起 / フラストレーション / 長時間緩和法 / 比熱 / 磁場角度回転比熱
Outline of Research at the Start

本研究においては、複数のキタエフ量子スピン液体候補物質に対して磁場中の精密比熱測定を行い、その温度依存性から準粒子の励起を調べる。とりわけトポロジカル相を規定する励起ギャップの磁場角度依存性を明らかにする。これにより励起が変化すると期待されるトポロジカル相転移を検出し、現実の物質における詳細な相図を構築することでキタエフ量子スピン液体やその準粒子励起に対する理解を飛躍的に向上させる。

Outline of Final Research Achievements

In this study, we investigated the change of the excitation in the bulk state of Kitaev spin liquid by performing specific heat measurements under magnetic field angle rotation. In particular, in order to detect the field-angle dependence in a single crystal, a highly sensitive field-angle-resolved specific heat measurement system was developed. We found that there is finite excitation gap when the field is directed along a-axis for the Kitaev spin liquid candidate alpha-RuCl3, whereas gapless excitation is observed for magnetic field along b-axis, indicating the Dirac-type dispersion. This observation is consistent with the excitation gap predicted by the Kitaev model for the Majorana fermion, and is first experimental verification of the bulk edge correspondence in the Kitaev spin liquid.

Academic Significance and Societal Importance of the Research Achievements

本研究で対象としたキタエフ模型は、キタエフにより提案された量子スピン模型であり、この模型で期待されるマヨラナ粒子や非可換エニオンは、基礎学理として重要のみならず、トポロジカル量子計算への応用も期待されている。本研究により、キタエフ量子スピン液体状態のバルク状態が明らかとなったことにより、現実の物質においてマヨラナ粒子や非可換エニオンの性質に対する理解が大きく進んだと言える。本研究は、量子計算への応用に向けた学理の構築に寄与することが期待される。

Report

(4 results)
  • 2023 Final Research Report ( PDF )
  • 2022 Annual Research Report
  • 2021 Annual Research Report
  • 2020 Annual Research Report
  • Research Products

    (51 results)

All 2023 2022 2021 2020 Other

All Int'l Joint Research (6 results) Journal Article (12 results) (of which Int'l Joint Research: 6 results,  Peer Reviewed: 12 results,  Open Access: 10 results) Presentation (30 results) (of which Int'l Joint Research: 4 results,  Invited: 3 results) Remarks (3 results)

  • [Int'l Joint Research] Chinese Academy of Sciences(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Colorado at Boulder(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Ecole Polytechnique(フランス)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Polish Academy of Sciences(ポーランド)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Radboud University(オランダ)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Bulk evidence of anisotropic s-wave pairing with no sign change in the kagome superconductor CsV3Sb52023

    • Author(s)
      Roppongi M.、Ishihara K.、Tanaka Y.、Ogawa K.、Okada K.、Liu S.、Mukasa K.、Mizukami Y.、Uwatoko Y.、Grasset R.、Konczykowski M.、Ortiz B. R.、Wilson S. D.、Hashimoto K.、Shibauchi T.
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 667-667

    • DOI

      10.1038/s41467-023-36273-x

    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Double dome structure of the Bose-Einstein condensation in diluted S=3/2 quantum magnets2023

    • Author(s)
      Watanabe Yoshito、Miyake Atsushi、Gen Masaki、Mizukami Yuta、Hashimoto Kenichiro、Shibauchi Takasada、Ikeda Akihiko、Tokunaga Masashi、Kurumaji Takashi、Tokunaga Yusuke、Arima Taka-hisa
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 1260-1260

    • DOI

      10.1038/s41467-023-36725-4

    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Pure nematic quantum critical point accompanied by a superconducting dome2022

    • Author(s)
      Ishida Kousuke、Onishi Yugo、Tsujii Masaya、Mukasa Kiyotaka、Qiu Mingwei、Saito Mikihiko、Sugimura Yuichi、Matsuura Kohei、Mizukami Yuta、Hashimoto Kenichiro、Shibauchi Takasada
    • Journal Title

      Proceedings of the National Academy of Sciences

      Volume: 119 Issue: 18

    • DOI

      10.1073/pnas.2110501119

    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Charge Transport in Ba1-xRbxFe2As2 Single Crystals2022

    • Author(s)
      Tsujii Masaya、Ishida Kousuke、Ishida Shigeyuki、Mizukami Yuta、Iyo Akira、Eisaki Hiroshi、Shibauchi Takasada
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 91 Issue: 10 Pages: 104706-104706

    • DOI

      10.7566/jpsj.91.104706

    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Strongly correlated superconductivity in a copper-based metal-organic framework with a perfect kagome lattice2021

    • Author(s)
      Takenaka T.、Ishihara K.、Roppongi M.、Miao Y.、Mizukami Y.、Makita T.、Tsurumi J.、Watanabe S.、Takeya J.、Yamashita M.、Torizuka K.、Uwatoko Y.、Sasaki T.、Huang X.、Xu W.、Zhu D.、Su N.、Cheng J.-G.、Shibauchi T.、Hashimoto K.
    • Journal Title

      Science Advances

      Volume: 7 Issue: 12

    • DOI

      10.1126/sciadv.abf3996

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Bond Directional Anapole Order in a Spin-Orbit Coupled Mott Insulator Sr2(Ir1-xRhx)O42021

    • Author(s)
      H. Murayama, K. Ishida, R. Kurihara, T. Ono, Y. Sato, Y. Kasahara, H. Watanabe, Y. Yanase, G. Cao, Y. Mizukami, T. Shibauchi, Y. Matsuda, and S. Kasahara
    • Journal Title

      Phys. Rev. X

      Volume: 11 Issue: 1 Pages: 011021-011021

    • DOI

      10.1103/physrevx.11.011021

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] High-Pressure Phase Diagrams of FeSe1-xTex: Correlation between Suppressed Nematicity and Enhanced Superconductivity2021

    • Author(s)
      K. Mukasa, K. Matsuura, M. Qiu, M. Saito, Y. Sugimura, K. Ishida, M. Otani, Y. Onishi, Y. Mizukami, K. Hashimoto, J. Gouchi, R. Kumai, Y. Uwatoko, and T. Shibauchi
    • Journal Title

      Nat. Commun.

      Volume: 12 Issue: 1 Pages: 381-381

    • DOI

      10.1038/s41467-020-20621-2

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Suppression of Anharmonic Phonons and s-Wave Superconductivity by Defects in the Filled Skutterudite LaRu4As122020

    • Author(s)
      Y. Mizukami, M. Konczykowski, O. Tanaka, J. Juraszek, Z. Henkie, T. Cichorek, and T. Shibauchi
    • Journal Title

      Phys. Rev. Res.

      Volume: 2 Issue: 4 Pages: 043428-043428

    • DOI

      10.1103/physrevresearch.2.043428

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Dichotomy Between Orbital and Magnetic Nematic Instabilities in BaFe2S32020

    • Author(s)
      S. Hosoi, T. Aoyama, K. Ishida, Y. Mizukami, K. Hashizume, S. Imaizumi, Y. Imai, K. Ohgushi, Y. Nambu, M. Kimata, S. Kimura, and T. Shibauchi
    • Journal Title

      Phys. Rev. Res.

      Volume: 2 Issue: 4 Pages: 043293-043293

    • DOI

      10.1103/physrevresearch.2.043293

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Bose-Einstein Condensation Superconductivity Induced by Disappearance of the Nematic State2020

    • Author(s)
      T. Hashimoto, Y. Ota, A. Tsuzuki, T. Nagashima, A. Fukushima, S. Kasahara, Y. Matsuda, K. Matsuura, Y. Mizukami, T. Shibauchi, S. Shin, and K. Okazaki
    • Journal Title

      Sci. Adv.

      Volume: 6 Issue: 45

    • DOI

      10.1126/sciadv.abb9052

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Non-Fermi Liquid Transport in the Vicinity of the Nematic Quantum Critical Point of Superconducting FeSe1-xSx2020

    • Author(s)
      W. K. Huang, S. Hosoi, M. Culo, S. Kasahara, Y. Sato, K. Matsuura, Y. Mizukami, M. Berben, N. E. Hussey, H. Kontani, T. Shibauchi, and Y. Matsuda
    • Journal Title

      Phys. Rev. Res.

      Volume: 2 Issue: 3 Pages: 033367-033367

    • DOI

      10.1103/physrevresearch.2.033367

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Divergent Nematic Susceptibility near the Pseudogap Critical Point in a Cuprate Superconductor2020

    • Author(s)
      Kousuke Ishida, Suguru Hosoi, Yuki Teramoto, Tomohiro Usui, Yuta Mizukami, Kenji Itaka, Yuji Matsuda, Takao Watanabe, and Takasada Shibauchi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 6 Pages: 064707-064707

    • DOI

      10.7566/jpsj.89.064707

    • NAID

      40022254195

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Presentation] 少数キャリア半金属 CeX における強相関電子状態2023

    • Author(s)
      新井陽介, 黒田健太, 野本拓也, 筒井智嗣, 田中宏明, Yuyang Dong, 岩田拓万, 片山和郷, 水上雄太, 平井大悟郎, 辛埴, 久保田正人, 芳賀芳範, 鈴木博之, 宮坂茂樹, 田島節子, 有田亮太郎, 近藤猛
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] 磁場角度分解抵抗測定を用いた正方晶Fe(Se,S)におけるネマティック超伝導状態の検証2023

    • Author(s)
      近藤玲央名, 石原滉大, 松浦康平, 水上雄太, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] 不純物効果を用いたFe(Se,S)の超伝導ギャップ構造の研究2023

    • Author(s)
      永島拓也, 石原滉大, 小林雅之, 六本木雅生, 松浦康平, 水上雄太, Romain Grasset, Marcin Konczykowski, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] 18%S置換FeSeの超伝導状態における異常なスピン揺らぎ2023

    • Author(s)
      Z.-Y.Yu, 中村昂矢, 猪股和也, 御栗丈虎, 沈暁玲, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会2023年春季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] FeSe系超伝導体におけるマルチバンドBCS-BECクロスオーバー2022

    • Author(s)
      水上雄太
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
    • Invited
  • [Presentation] カゴメ格子系超伝導体CsV3Sb5における超伝導対称性2022

    • Author(s)
      六本木雅生, 石原滉大, 田中優之介, 小河弘樹, 岡田昂, 劉蘇鵬, 向笠清隆, 水上雄太, 上床美也, R. Grasset, M. Konczykowski, Brenden R. Ortiz, Stephen D. Wilson, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] カゴメ格子超伝導体CsV3Sb5におけるネマティック感受率測定2022

    • Author(s)
      大西朝登, 影山遥一, 六本木雅生, 水上雄太, Brenden R. Ortiz, Stephen D. Wilson, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] 極低温磁場角度分解比熱測定によるキタエフ候補物質 α-RuCl3におけるマヨラナ励起の検証2022

    • Author(s)
      今村薫平, 水上雄太, 吉田悠生, 橋本顕一郎, 栗田伸之, 田中秀数, 藤本聡, 山田昌彦, 松田祐司, E.-G. Moon, 芝内孝禎
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] Kitaev候補物質Na2Co2TeO6における磁場中比熱の角度依存性2022

    • Author(s)
      Shengjie Fang, 水上雄太, 今村薫平, 難波隆一, 石原滉大, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] NMRから見たS置換FeSe系の超伝導状態での異常なスピン揺らぎ2022

    • Author(s)
      Z.-Y.Yu, 中村昂矢, 猪股和也, 御栗丈虎, 沈暁玲, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会2022年秋季大会
    • Related Report
      2022 Annual Research Report 2021 Annual Research Report
  • [Presentation] Fe(Se,S)における不純物効果と超伝導ギャップ構造2022

    • Author(s)
      石原滉大, 小林雅之, 六本木雅生, 松浦康平, 水上雄太, M. Konczykowski, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会2022年秋季大会
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  • [Presentation] 比熱測定から見るキタエフ量子スピン液体のマヨラナ励起2021

    • Author(s)
      水上雄太
    • Organizer
      ワークショップ(4)「超伝導物質、トポロジカル物質」 SCTM2020
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    • Invited
  • [Presentation] 強相関超伝導体の電子対形成に関する実験研究2021

    • Author(s)
      水上雄太
    • Organizer
      日本物理学会第76回年次大会
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  • [Presentation] Bond directional anapole state in a spin-orbit coupled Mott insulator Sr2(Ir1-xRhx)O42021

    • Author(s)
      H. Murayama, K. Ishida, R. Kurihara, T. Ono, Y. Sato, Y. Kasahara, H. Watanabe, Y. Yanase, G. Cao, Y. Mizukami, T. Shibauchi, Y. Matsuda, and S. Kasahara
    • Organizer
      American Physical Society, March Meeting 2021
    • Related Report
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  • [Presentation] High-pressure electronic phase diagrams in FeSe1-xTex2021

    • Author(s)
      K. Mukasa, K. Matsuura, M. Qiu, M. Saito, Y. Sugimura, K. Ishida, M. Otani, Y. Onishi, Y. Mizukami, K. Hashimoto, J. Gouchi, R. Kumai, Y. Uwatoko, and T. Shibauchi
    • Organizer
      American Physical Society, March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Low-energy quasiparticle excitations in the spin-triplet superconductor UTe22021

    • Author(s)
      K. Ishihara, M. Roppongi, M. Kobayashi, Y. Mizukami, H. Sakai, Y. Haga, K. Hashimoto, and T. Shibauchi
    • Organizer
      American Physical Society, March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Low-energy quasiparticle excitations in a BiCh2-based superconductor studied by magnetic penetration depth measurements2021

    • Author(s)
      M. Roppongi, K. Ishihara, Y. Mizukami, K. Hashimoto, K. Hoshi, Y. Mizuguchi and T. Shibauchi
    • Organizer
      American Physical Society, March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] レーザー励起光電子顕微鏡を用いたSrVO3における強磁性ドメインの観察2021

    • Author(s)
      影山遥一, 児玉壮平, 水上雄太, 谷内敏之, 橋本顕一郎, Arnaud Fouchet, Andres F. Santander-Syro, 辛埴, 芝内孝禎
    • Organizer
      日本物理学会第76回年次大会
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      2020 Annual Research Report
  • [Presentation] スピントリプレット超伝導体UTe2における磁場侵入長測定2021

    • Author(s)
      石原滉大, 六本木雅生, 小林雅之, 水上雄太, 橋本顕一郎, 酒井宏典, 芳賀芳範, 芝内孝禎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Sr2Ir1-xRhxO4におけるボンド方向型アナポール秩序2021

    • Author(s)
      笠原成, 村山陽奈子, 石田浩祐, 栗原遼, 小野孝浩, 佐藤雄貴, 笠原裕一, 渡邉光, 柳瀬陽一, G. Cao, 水上雄太, 芝内孝禎, 松田祐司
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] BiCh2系超伝導体における磁場侵入長測定2021

    • Author(s)
      六本木雅生, 石原滉大, 水上雄太, 星和久, 水口佳一, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Kitaevスピン液体候補物質α-RuCl3におけるトポロジカル相転移の探索2021

    • Author(s)
      鵜飼柚希, 笠原裕一, 末次祥大, 村山陽奈子, 栗田伸之, 田中秀数, 橋本顕一郎, 水上雄太, 芝内孝禎, 松田祐司
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] キタエフスピン液体候補物質α-RuCl3における磁場中比熱の異方性2021

    • Author(s)
      原澤龍平, 田中桜平, 水上雄太, 栗田伸之, 田中秀数, 山田昌彦, 藤本聡, 笠原裕一, 松田祐司, Eun-Gook Moon, 橋本顕一郎, 芝内孝禎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] キタエフ物質α-RuCl3における電子線照射の影響2021

    • Author(s)
      今村薫平, 田中桜平, 水上雄太, 原澤龍平, 橋本顕一郎, 栗田伸之, 田中秀数, 山田昌彦, 藤本聡, 松田祐司, E.-G. Moon, M. Konczykowski, 芝内孝禎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] レーザー角度分解光電子分光によるFe(Se, S)の非ネマティック相における超伝導状態の研究2021

    • Author(s)
      長島椿, 橋本嵩広, Sahand Najafzadeh, 大内俊一郎, 鈴木剛, 福島昭子, 笠原成, 松田祐司, 松浦康平, 水上雄太, 橋本顕一郎, 芝内孝 禎, 辛埴, 岡﨑浩三
    • Organizer
      日本物理学会第76回年次大会
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      日本物理学会2020年秋季大会
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      2020 Annual Research Report
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      日本物理学会2020年秋季大会
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      日本物理学会2020年秋季大会
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    • Organizer
      日本物理学会2020年秋季大会
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    • Author(s)
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  • [Remarks]

    • URL

      https://sites.google.com/view/yutamizukamipage/home

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    • URL

      https://sites.google.com/view/yutamizukamipage/home

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    • URL

      https://sites.google.com/view/yutamizukamipage/publication

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Published: 2020-04-28   Modified: 2025-01-30  

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