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液中TEM技術によるナノスケール沸騰現象の直接観測

Research Project

Project/Area Number 20J13061
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeSingle-year Grants
Section国内
Review Section Basic Section 19020:Thermal engineering-related
Research InstitutionKyushu University

Principal Investigator

NAG SARTHAK  九州大学, 工学府, 特別研究員(DC2)

Project Period (FY) 2020-04-24 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥2,300,000 (Direct Cost: ¥2,300,000)
Fiscal Year 2021: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 2020: ¥1,200,000 (Direct Cost: ¥1,200,000)
Keywordsnanobubbles / liquid cell / TEM / nucleation / interfacial behavior / surface nanobubbles / electron microscopy / phase change / in-situ observation
Outline of Research at the Start

Bubbles and droplets exhibit exceptional phenomenon at nanoscale. To apprehend them at nanoscale, in-situ liquid cell electron microscopy is used. Nucleation parameters along with the effect of external quantitative properties are investigated to extend our insight on the novel nanoscale phenomena.

Outline of Annual Research Achievements

In summary, we used the liquid phase electron microscopy (LPEM) technique to study the surface nanobubbles and their interfacial behaviour. We devised a three-step gas nanobubble nucleation strategy using electron beam of the TEM, which helps in the on-demand nanobubble nucleation with high probability. Moreover, the electron beam parameters can be tuned to nucleate nanobubbles having different sizes and nucleation number density. In addition, we studied the interactions between two nanobubbles at high spatial resolution. Our results demonstrated that the nanobubbles can exist with and without contact line pinning. Moreover, we captured anisotropic depinning in surface nanobubbles and revealed the role of asymmetric gas distribution on pinning of surface nanobubbles. We also found that the bubble merging is strongly pinned nanobubbles is initiated by the localized region-wise gas film formation. We then proposed a plausible mechanism indicating the formation of a high-gas molecule dense region between the nanobubbles. These findings not only provide insights into the dynamic nanobubble behaviour, but also reiterates the novel applications these nanobubbles can be used for.
In addition, we also worked on the fabrication of graphene nano-scrolls with water encapsulations for its observation in TEM. We explained the dynamics of annular liquid layer adhered to the wall of graphene nano-scrolls by considering the effect of van der Waals interaction.

Research Progress Status

令和3年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

令和3年度が最終年度であるため、記入しない。

Report

(2 results)
  • 2021 Annual Research Report
  • 2020 Annual Research Report
  • Research Products

    (11 results)

All 2022 2021 2020

All Journal Article (3 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 3 results,  Open Access: 1 results) Presentation (8 results) (of which Int'l Joint Research: 2 results,  Invited: 1 results)

  • [Journal Article] Observation of Interfacial Instability of an Ultrathin Water Film2022

    • Author(s)
      Tomo Yoko、Nag Sarthak、Takamatsu Hiroshi
    • Journal Title

      Physical Review Letters

      Volume: 128 Issue: 14 Pages: 144502-144502

    • DOI

      10.1103/physrevlett.128.144502

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Mechanistic Insights into Nanobubble Merging Studied Using In Situ Liquid-Phase Electron Microscopy2021

    • Author(s)
      Nag Sarthak、Tomo Yoko、Takahashi Koji、Kohno Masamichi
    • Journal Title

      Langmuir

      Volume: 37 Issue: 2 Pages: 874-881

    • DOI

      10.1021/acs.langmuir.0c03208

    • Related Report
      2021 Annual Research Report 2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Dynamic interplay between interfacial nanobubbles: oversaturation promotes anisotropic depinning and bubble coalescence2021

    • Author(s)
      Nag Sarthak、Tomo Yoko、Teshima Hideaki、Takahashi Koji、Kohno Masamichi
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 23 Issue: 43 Pages: 24652-24660

    • DOI

      10.1039/d1cp03451k

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Effect of three-phase boundary line pinning on the interaction between interface nanobubbles2022

    • Author(s)
      Sarthak Nag, Yoko Tomo, Hideaki Teshima, Koji Takahashi, Masamichi Kohno
    • Organizer
      第 59 回日本伝熱シンポジウム
    • Related Report
      2021 Annual Research Report
  • [Presentation] Surface nanobubbles and their dynamics studied using liquid phase electron microscopy2021

    • Author(s)
      Sarthak Nag
    • Organizer
      第16.0回相変化界面研究会
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Merging of surface nanobubbles: insights using in-situ liquid phase electron microscopy2021

    • Author(s)
      Sarthak Nag, Yoko Tomo, Koji Takahashi, Masamichi Kohno
    • Organizer
      第 59 回日本伝熱シンポジウム
    • Related Report
      2021 Annual Research Report
  • [Presentation] Coalescence in surface nanobubbles initiates via gas layer formation2021

    • Author(s)
      Sarthak Nag, Yoko Tomo, Hideaki Teshima, Koji Takahashi, Masamichi Kohno
    • Organizer
      7th Micro and Nano Flows Conference
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Liquid phase electron microscopy and its applications to study nanobubbles' dynamics2021

    • Author(s)
      Sarthak Nag
    • Organizer
      Thermal Science and Engineering Next Leaders Forum (ThSENx1)
    • Related Report
      2021 Annual Research Report
  • [Presentation] Nanobubble dynamics during merging revealed using in-situ liquid cell electron microscopyナノバルブ合体挙動の液中TEM観察2020

    • Author(s)
      Sarthak Nag, Yuzen Masame, Tatsuya Ikuta, Qin-Yi Li, Koji Takahashi, Masamichi Kohno
    • Organizer
      一般社団法人 日本機械学会熱工学コンファレンス2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] In-situ electron microscopic study of effect of temperature on nanobubble generation その場TEM観察によるナノバブル生成における温度依存性の研究2020

    • Author(s)
      Sarthak Nag, Yuzen Masame, Daichi Yosho, Qin-Yi Li, Tatsuya Ikuta, Koji Takahashi, Masamichi Kohno
    • Organizer
      57th National Heat Transfer Symposium of Japan
    • Related Report
      2020 Annual Research Report
  • [Presentation] Nanobubble dynamics studied using in-situ liquid cell electron microscopy2020

    • Author(s)
      Sarthak Nag, Yuzen Masame, Tatsuya Ikuta, Qin-Yi Li, Koji Takahashi, Masamichi Kohno
    • Organizer
      Sino-Japan-UK Frontiers in Phase Change Heat Transfer and Its Applications in Energy
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research

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Published: 2020-07-07   Modified: 2024-03-26  

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