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Metallo-Dielectric Janus Particles as Building Blocks for Designer Active Materials

Research Project

Project/Area Number 20K03786
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Review Section Basic Section 13010:Mathematical physics and fundamental theory of condensed matter physics-related
Research InstitutionKyoto University

Principal Investigator

Molina John  京都大学, 工学研究科, 助教 (20727581)

Project Period (FY) 2020-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2022: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2021: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2020: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
KeywordsElectro-Hydrodynamics / Active Particles / Electrophoresis / Janus Particles / Quincke Rollers / Machine Learning / Multi-Scale Simulations / Flow Inference / Fluid Dynamics / Optimal Control / Active janus particles / Induced charge / DNS / Active Matter
Outline of Research at the Start

The aim of the current research project is to examine the collective behavior of Janus particles and propose new particle designs to build next-generation active materials.

We will develop a computational framework to elucidate the nature of the interactions between Janus particles and their environment, in order to build active systems capable of performing useful work.

In particular, we will extend the state-of-the-art colloidal simulator, KAPSEL, to handle Janus particles with arbitrary shape and material properties. We will then study the single particle and collective behavior.

Outline of Final Research Achievements

The purpose of this work is to understand the mechanisms behind the rich single- and many-particle dynamics of active colloids. For this, we have developed a computational method that accounts for the electro-hydrodynamics and rigid-body dynamics of colloidal particles under AC/DC fields. We succeeded in reproducing the dynamics of metallo-dielectric Janus particles, including the velocity dependence on the electric field strength, as well as the velocity reversal at high frequencies, which are accompanied by strong field gradients near the particle surface. We have further investigated the collective dynamics of dielectric particles under DC fields, to reveal how the interplay between the hydrodynamics and electrostatics accounts for the different phases observed experimentally. Finally, we have developed Machine-Learning methods capable of inferring constitutive relations for complex flows, as well as solutions to Stokes flow problems.

Academic Significance and Societal Importance of the Research Achievements

We have developed physical models that can be used to understand the rich dynamics of active colloidal particles, which can be used as building blocks for novel materials. We have also developed Machine-Learning methods that can significantly enhance our ability to predict complex flows.

Report

(4 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • 2020 Research-status Report
  • Research Products

    (38 results)

All 2023 2022 2021 2020

All Journal Article (7 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 5 results,  Open Access: 3 results) Presentation (31 results) (of which Int'l Joint Research: 19 results,  Invited: 3 results)

  • [Journal Article] Collective Motion of Quincke Rollers with Fully Resolved Hydrodynamics2023

    • Author(s)
      Imamura Shun、Sawaki Kohei、Molina John J.、Turner Matthew S.、Yamamoto Ryoichi
    • Journal Title

      Advanced Theory and Simulations

      Volume: 6 Issue: 4 Pages: 2200683-2200683

    • DOI

      10.1002/adts.202200683

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Direct numerical simulations of isolated rigid particles; Validation of smooth profile method2023

    • Author(s)
      Uzair Muhammad、Qasim M. Danyal、Bhatti M. Aashan、Zaidi Ali Abbas、Molina John J.、Yamamoto Ryoichi、Hamid Adnan
    • Journal Title

      Powder Technology

      Volume: 418 Pages: 118280-118280

    • DOI

      10.1016/j.powtec.2023.118280

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] からみ合い高分子溶融体の流動解析手法の進展 : マルチスケールシミュレーション法と機械学習の融合2023

    • Author(s)
      Miyamoto Souta、Molina John J.、Taniguchi Takashi
    • Journal Title

      化学工学会誌

      Volume: 87 Pages: 111-113

    • Related Report
      2022 Annual Research Report
  • [Journal Article] Dynamics of microswimmers near a soft penetrable interface2022

    • Author(s)
      Feng Chao、Molina John J.、Turner Matthew S.、Yamamoto Ryoichi
    • Journal Title

      Physical Review Research

      Volume: 4 Issue: 4 Pages: 043202-043202

    • DOI

      10.1103/physrevresearch.4.043202

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Machine Learning for the Flow Prediction of Fluids with Memory Effects on the Stress2021

    • Author(s)
      TANIGUCHI Takashi、MOLINA John J.
    • Journal Title

      JAPANESE JOURNAL OF MULTIPHASE FLOW

      Volume: 35 Issue: 3 Pages: 426-436

    • DOI

      10.3811/jjmf.2021.T008

    • NAID

      130008104319

    • ISSN
      0914-2843, 1881-5790
    • Year and Date
      2021-09-15
    • Related Report
      2021 Research-status Report
    • Open Access
  • [Journal Article] Smoothed profile method for direct numerical simulations of hydrodynamically interacting particles2021

    • Author(s)
      Yamamoto Ryoichi、Molina John Jairo、Nakayama Yasuya
    • Journal Title

      Soft Matter

      Volume: - Issue: 16 Pages: 4226-4253

    • DOI

      10.1039/d0sm02210a

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Dynamics of a chiral swimmer sedimenting on a flat plate2020

    • Author(s)
      Fadda Federico、Molina John Jairo、Yamamoto Ryoichi
    • Journal Title

      Physical Review E

      Volume: 101 Issue: 5 Pages: 52608-52608

    • DOI

      10.1103/physreve.101.052608

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Presentation] Direct numerical simulations of microswimmers in viscoelastic fluids2023

    • Author(s)
      Takuya Kobayashi (*), John J. Molina, Ryoichi Yamamoto
    • Organizer
      IWEAYR-16 : The 16th International Workshop for East Asian Young Rheologists
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Direct Numerical Simulation of Metallodielectric Janus Particles2023

    • Author(s)
      John J. Molina (*), Takuya Eriguchi, Ryoichi Yamamoto
    • Organizer
      APS March Meeting 2023
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Direct numerical simulations of a model microswimmer near a liquid-liquid interface2023

    • Author(s)
      Chao Feng (*), John J. Molina, Matthew S. Turner, Ryoichi Yamamoto
    • Organizer
      Active Matter Workshop 2023
    • Related Report
      2022 Annual Research Report
  • [Presentation] Applications of machine-learned constitutive relations to simulate well-entangled polymer melt flows2022

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      PPS-37 : The 37th International Conference of the Polymer Processing Society
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Flow Problems as Inference Problems2022

    • Author(s)
      Kenta Ogawa, John J. Molina (*), Takashi Taniguchi
    • Organizer
      PPS-37 : The 37th International Conference of the Polymer Processing Society
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dynamics of micro-swimmers near deformable and penetrable interfaces2022

    • Author(s)
      Chao Feng (*), John J. Molina, Matthew S. Turner, Ryoichi Yamamoto
    • Organizer
      APPC15 : The 15th Asia Pacific Physics Conference
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Microswimmers in viscoelastic fluids2022

    • Author(s)
      Takuya Kobayashi (*), John J. Molina, Ryoichi Yamamoto
    • Organizer
      APPC15 : The 15th Asia Pacific Physics Conference
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Learning to swim efficiently in a nonuniform flow field2022

    • Author(s)
      Krongtum Sankawtong (*), John J. Molina, Matthew S. Turner, Ryoichi Yamamoto
    • Organizer
      ISMC 2022 : The International Soft Matter Conference
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Machine-learned constitutive relations for simulating well-entangled polymer melts for their history-dependent flows2022

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      The Society of Rheology 93rd Annual Meeting
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Machine Learning Physics for Flowing Soft Matter2022

    • Author(s)
      John J. Molina (*), Kenta Ogawa, Souta Miyamoto, Takashi Taniguchi
    • Organizer
      25th Anniversary Symposium of German-Japanese Joint Research Project on Nonequilibrium Statistical PHysics Perspective for Future Collaboration
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Inferring hidden utilities from optimal behaviour using physics-informed neural networks2022

    • Author(s)
      John J. Molina (*), Simon K. Schnyder, Mark P. Lynch, Ryoichi Yamamoto, Matthew S. Turner
    • Organizer
      Workshop: Modelling the Covid-19 Pandemic
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 粘弾性流体中を泳動するマイクロスイマー:回転運動による速度上昇2022

    • Author(s)
      Takuya Kobayashi (*), John J. Molina, Ryoichi Yamamoto
    • Organizer
      日本物理学会 2022年秋季大会
    • Related Report
      2022 Annual Research Report
  • [Presentation] 直接数値計算による粘弾性流体中を泳動するマイクロスイマーのダイナミクス2022

    • Author(s)
      Takuya Kobayashi (*), John J. Molina, Ryoichi Yamamoto
    • Organizer
      第70回レオロジー討論会
    • Related Report
      2022 Annual Research Report
  • [Presentation] 粘弾性流体中を泳動するモデル微生物の直接数値計算2022

    • Author(s)
      Takuya Kobayashi (*), John J. Molina, Ryoichi Yamamoto
    • Organizer
      第10回ソフトマター研究会
    • Related Report
      2022 Annual Research Report
  • [Presentation] Physics Informed Machine Learning for (Inverse) Optimal Control2022

    • Author(s)
      John J. Molina (*), Simon K. Schnyder, Matthew S. Turner, Ryoichi Yamamoto
    • Organizer
      第10回ソフトマター研究会
    • Related Report
      2022 Annual Research Report
  • [Presentation] Collective Dynamics of Quincke Rollers with Fully Resolved Hydrodynamics2022

    • Author(s)
      Shun Imamura (*), Kohei Sawaki, John J. Molina, Ryoichi Yamamoto
    • Organizer
      American Physical Society (APS) March Meeting 2022
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Application of Machine-learned constitutive relations for well-entangled polymer melt flows2022

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      American Physical Society (APS) March Meeting 2022
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Rational policy design for epidemics2022

    • Author(s)
      Simon K. Schnyder (*), John J. Molina, Ryoichi Yamamoto, Matthew S. Turner
    • Organizer
      American Physical Society (APS) March Meeting 2022
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Nash Neural Networks2022

    • Author(s)
      John J. Molina (*), Simon K. Schnyder, Matthew S. Turner, Ryoichi Yamamoto
    • Organizer
      American Physical Society (APS) March Meeting 2022
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Rational policy design for epidemics2021

    • Author(s)
      Simon K. Schnyder (*), John J. Molina, Ryoichi Yamamoto, Matthew S. Turner
    • Organizer
      27th International Conference on Computing in Economics and Finance
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Rational policy design for epidemics2021

    • Author(s)
      Simon K. Schnyder (*), John J. Molina, Ryoichi Yamamoto, Matthew S. Turner
    • Organizer
      24.5th Workshop on Economics with Heterogeneous Interacting Agents
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Learning the constitutive relation of polymer melt flows2021

    • Author(s)
      John J. Molina (*), Souta Miyamoto, Takashi Taniguchi
    • Organizer
      The 2021 International Chemical Congress of Pacific Basin Societies (Pacifichem 2021)
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] 学習された構成関係を用いた高分子液体の流動シミュレーション2021

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      化学工学会 第52回秋季大会(2021)
    • Related Report
      2021 Research-status Report
  • [Presentation] Well-entangled polymer melt flow simulations using a Machine-Learned constitutive relation2021

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      第69回レオロジー討論会
    • Related Report
      2021 Research-status Report
  • [Presentation] A Machine Learning Approach to Flow Problems2021

    • Author(s)
      John J. Molina (*), Takashi Taniguchi
    • Organizer
      第69回レオロジー討論会
    • Related Report
      2021 Research-status Report
  • [Presentation] 機械学習モデルを構成関係に代用した高分子溶融体の流動シミュレーション2021

    • Author(s)
      Souta Miyamoto (*), John J. Molina, Takashi Taniguchi
    • Organizer
      プラスチック成形加工学会第29回秋季大会
    • Related Report
      2021 Research-status Report
  • [Presentation] Gaussian Processes for Machine Learning of Fluid Flows2021

    • Author(s)
      John J. Molina (*), Takashi Taniguchi
    • Organizer
      ソフトバイオ研究会2021
    • Related Report
      2021 Research-status Report
    • Invited
  • [Presentation] Novel Soft Matter Physics through Computational and Information Science (oral)2021

    • Author(s)
      Molina John J.(*)
    • Organizer
      The Physical Society of Japan 2021 Annual Meeting (online)
    • Related Report
      2020 Research-status Report
    • Invited
  • [Presentation] Learning the Constitutive Relation of Polymer Flows with Memory: from Micro-Scale Dynamics to Macro-Scale Flow2021

    • Author(s)
      Molina John J.(*)、Seryo Naoki、Sato Takeshi, Taniguchi Takashi
    • Organizer
      SIAM Conference on Computational Science and Engineering (online)
    • Related Report
      2020 Research-status Report
    • Int'l Joint Research
  • [Presentation] Sedimenting chiral swimmers2021

    • Author(s)
      Fadda Federico(*)、Molina John J.、Yamamoto Ryoichi
    • Organizer
      Americal Physical Society (APS) March Meeting 2021 (online)
    • Related Report
      2020 Research-status Report
    • Int'l Joint Research
  • [Presentation] Direct Numerical Simulation of Induced Charge Electrophoresis of Janus Particles2020

    • Author(s)
      Eriguchi Takuya(*)、Molina John J.
    • Organizer
      68th Annual Meeting of the Society of Rheology of Japan (online)
    • Related Report
      2020 Research-status Report

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Published: 2020-04-28   Modified: 2024-01-30  

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