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Interlayer excitons in 1D-2D heterostructures and its applications

Research Project

Project/Area Number 20K15120
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 28020:Nanostructural physics-related
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

FANG NAN  国立研究開発法人理化学研究所, 開拓研究本部, 基礎科学特別研究員 (50850509)

Project Period (FY) 2020-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2021: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2020: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordscarbon nanotube / hexagonal boron nitride / tungsten diselenide / exciton / carbon nanotubes / 2D materials / heterostructure / excitons / cavity / dielectric screening
Outline of Research at the Start

Interlayer excitons will be explored in 2D-1D van der Waals heterostructures. Emission wavelength of the interlayer excitons will be modulated by choosing different 2D materials. Novel photonic devices such as excitonic transistors and photodiodes will be developed based on the interlayer excitons.

Outline of Final Research Achievements

Hexagonal boron nitride (h-BN), a two-dimensional (2D) material, is atomically flat with low defect density, which is widely used to support other 2D materials for both electronics and photonics. We expect that the advantages of h-BN can also be utilized in mixed dimensional heterostructures, and carbon nanotubes (CNTs) would provide a unique opportunity in this context. The one-dimensional nature of CNTs results in enhanced Coulomb interactions, giving rise to tightly bound excitons that show photoluminescence (PL) at room temperature. CNTs directly attached on solid-state substrates such as SiO2/Si, however, suffers from the strong substrate quenching effect, hindering applications in all-solid-state optical devices. By using h-BN as a substrate, the quenching effect is expected to be suppressed. Moreover, we also investigate the interaction between CNTs and tungsten diselenide, and find a clear exciton transfer in this system.

Academic Significance and Societal Importance of the Research Achievements

These findings indicate that h-BN is an ideal solid-state subsatrate for the CNTs photonic devices and open a new path-way for manipulating excitons in CNTs.Moreover, a strong exciton transfer between WSe2 and CNTs reveal novel excitonic physics in mixed dimensional heterostructures.

Report

(3 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • Research Products

    (3 results)

All 2021 2020

All Journal Article (2 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 2 results) Presentation (1 results)

  • [Journal Article] Deterministic transfer of optical-quality carbon nanotubes for atomically defined technology2021

    • Author(s)
      Otsuka Keigo、Fang Nan、Yamashita Daiki、Taniguchi Takashi、Watanabe Kenji、Kato Yuichiro K.
    • Journal Title

      Nature Communications

      Volume: 12 Issue: 1 Pages: 1-8

    • DOI

      10.1038/s41467-021-23413-4

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Hexagonal Boron Nitride As an Ideal Substrate for Carbon Nanotube Photonics2020

    • Author(s)
      N. Fang, K. Otsuka, A. Ishii, T. Taniguchi, K. Watanabe, K. Nagashio, and Y. K. Kato
    • Journal Title

      ACS Photonics

      Volume: 7 Issue: 7 Pages: 1773-1779

    • DOI

      10.1021/acsphotonics.0c00406

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Excitons in mixed-dimensional heterostructures2021

    • Author(s)
      Fang Nan
    • Organizer
      「物質階層原理研究」&「ヘテロ界面研究」 2021年冬合同研究会
    • Related Report
      2021 Annual Research Report

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Published: 2020-04-28   Modified: 2023-01-30  

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