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Study on Efficient Carbon Dioxide Sequestration by Microscopic Dispersion of Alkaline Earth Oxides

Research Project

Project/Area Number 21360366
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Metal making engineering
Research InstitutionTohoku University

Principal Investigator

ARIYAMA Tatsuro  東北大学, 多元物質科学研究所, 教授 (10436165)

Co-Investigator(Kenkyū-buntansha) INOUE Ryo  東北大学, 多元物質科学研究所, 准教授 (70111309)
UEDA Shigeru  東北大学, 多元物質科学研究所, 准教授 (80359497)
Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥13,650,000 (Direct Cost: ¥10,500,000、Indirect Cost: ¥3,150,000)
Fiscal Year 2011: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2010: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2009: ¥9,230,000 (Direct Cost: ¥7,100,000、Indirect Cost: ¥2,130,000)
Keywords地球温暖化 / 二酸化炭素削減 / 二酸化炭素隔離 / 固体化学吸収 / アルカリ系化合物 / 第一原理計算 / アルカリ化合物
Research Abstract

In order to reduce the CO_2 emissions from global warming issue, the novel solid absorbent based on alkaline earth oxides material was proposed. The effects of addition of other alkaline earth metal oxides to CaO on the CO_2 adsorption energy were also investigated both theoretically and experimentally. On the basis of these results, the favorable process and materials for CO_2 reduction using BaO-TiO_2 or Li_2O-TiO_2 were studied. Moreover, the large scale ab-initio calculations were performed for an accurate estimation of adsorption energy of CO_2 on the CaO and BaO (001)surfaces.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (19 results)

All 2012 2011 2010 2009 Other

All Journal Article (7 results) (of which Peer Reviewed: 7 results) Presentation (11 results) Remarks (1 results)

  • [Journal Article] Experiment study and atomic level description of adsorption process of CO_2 on the doped alkaline earth oxides2012

    • Author(s)
      Kohei Sasaki, Koji Wakuta, Natsuki Tokuda, Rodion V. Belosluudov, Shigeru Ueda, Ryo Inoue, Yoshiyuki Kawazoe, Tatsuro Ariyama
    • Journal Title

      ISIJ Int

      Volume: vol.52, No.7(掲載決定)

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atomistic Level Description of Adsorption Process of CO_2 on the Doped Alkaline Earth Oxides by Ab-initio Calculations2012

    • Author(s)
      Kohei Sasaki, Koji Wakuta, Natsuki Tokuda, Rodion V.Belosludov, Shigeru Ueda, Ryo Inoue, Yoshiyuki Kawazoe, Tatsuro Ariyama
    • Journal Title

      ISIJ International

      Volume: 52(掲載決定)

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] CO_2Absorption and desorption abilities of Li_2O-TiO_2 compounds2011

    • Author(s)
      Shigeru Ueada, Ryo Inoue, Kohei Sasaki, Koji Wakuta, Tatsuro Ariyama
    • Journal Title

      ISIJ Int

      Volume: vol.51, No.4 Pages: 530-537

    • NAID

      10029580675

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] CO2 Absorption and Desorption Abilities of Li2O-TiO2 Compounds2011

    • Author(s)
      Shigeru Ueda, Ryo Inoue, Kohei Sasaki, Koji Wakuta, Tatsuro Ariyama
    • Journal Title

      ISIJ International

      Volume: 51 Pages: 530-537

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Thermodynamic Consideration on the Absorption Properties of Carbon Dioxide to Basic Oxide2010

    • Author(s)
      Ryo Inoue, Shigeru Ueda, Koji Wakuta, Kohei Sasaki, Tatsuro Ariyama
    • Journal Title

      ISIJ Int

      Volume: vol.50, No.11 Pages: 1532-1538

    • NAID

      10028114574

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermodynamic Consideration of the Carbon Dioxide Absorption Properties of Basic Oxide2010

    • Author(s)
      R.Inoue, S.Ueda, K.Wakuta, K.Sasaki, T.Arivama
    • Journal Title

      ISIJ International

      Volume: 50 Pages: 1532-1538

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 製銑プロセスにおける低炭素・脱炭素への将来展望2009

    • Author(s)
      有山達郎
    • Journal Title

      ふぇらむ 14

      Pages: 781-789

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] B_2O_3添加によるLi_2ZrO_3の二酸化炭素吸収速度向上2011

    • Author(s)
      徳田夏樹
    • Organizer
      日本鉄鋼協会第162回秋季講演大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2011-09-20
    • Related Report
      2011 Final Research Report
  • [Presentation] B2O3添加によるLi2ZrO3の二酸化炭素吸収速度向上2011

    • Author(s)
      徳田夏樹, 植田滋, 井上亮, 有山達郎
    • Organizer
      日本鉄鋼協会秋季講演大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2011-09-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] Li_2ZrO_3のCO_2吸収脱離のCO_2分圧依存性とB_2O_3による吸収促進2011

    • Author(s)
      徳田夏樹
    • Organizer
      日本鉄鋼協会第161回春季講演大会
    • Place of Presentation
      東京都市大学
    • Year and Date
      2011-03-25
    • Related Report
      2011 Final Research Report
  • [Presentation] アルカリ系酸化物のCO_2吸収特性の熱力学2010

    • Author(s)
      有山達郎
    • Organizer
      日本学術振興会製銑第54委員会第177回研究会
    • Place of Presentation
      日本, 東京
    • Year and Date
      2010-12-10
    • Related Report
      2011 Final Research Report
  • [Presentation] 低炭素・脱炭素に基づく将来製鉄プロセスへの展望2010

    • Author(s)
      有山達郎
    • Organizer
      日本鉄鋼協会・第203、204回西山記念講座
    • Place of Presentation
      東京
    • Year and Date
      2010-11-05
    • Related Report
      2010 Annual Research Report
  • [Presentation] Li_2O-SiO_2系化合物のCO_2吸収脱離機構2010

    • Author(s)
      佐々木光平
    • Organizer
      日本鉄鋼協会第160回秋季講演大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2010-09-26
    • Related Report
      2011 Final Research Report
  • [Presentation] Li2O-SiO2系化合物のCO2吸収脱離機構2010

    • Author(s)
      佐々木光平, 植田滋, 井上亮, 有山達郎
    • Organizer
      日本鉄鋼協会第160回秋季講演大会
    • Place of Presentation
      札幌
    • Year and Date
      2010-09-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] 第一原理計算によるCO_2固体化学吸収材の設計2010

    • Author(s)
      植田滋
    • Organizer
      日本鉄鋼協会第159回春季講演大会
    • Place of Presentation
      筑波大学
    • Year and Date
      2010-03-30
    • Related Report
      2009 Annual Research Report
  • [Presentation] CO_2固体化学吸収体の熱力学的検討2010

    • Author(s)
      井上亮
    • Organizer
      日本鉄鋼協会第159回春季講演大会
    • Place of Presentation
      筑波大学
    • Year and Date
      2010-03-28
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] Li_2O-TiO_2系化合物のCO_2吸収脱離機構2010

    • Author(s)
      佐々木光平
    • Organizer
      日本鉄鋼協会第159回春季講演大会
    • Place of Presentation
      筑波大学
    • Year and Date
      2010-03-28
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] Ab initio Simulation of Chemical CO_2 Adsorption Process2010

    • Author(s)
      和久田康司
    • Organizer
      The Fourth General Meeting of ACCMS-VO(Asian Consortium on Computational Materials Science- Virtual Organization)
    • Place of Presentation
      東北大学
    • Year and Date
      2010-01-07
    • Related Report
      2009 Annual Research Report
  • [Remarks]

    • URL

      http://www.tagen.tohoku.ac.jp/modules/laboratory/index.php?laboid=54

    • Related Report
      2011 Final Research Report

URL: 

Published: 2009-04-01   Modified: 2016-04-21  

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