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Development of the method to remedy leakage from geological CO2 reservoir using CO2 reactive grout

Research Project

Project/Area Number 21360442
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Earth system and resources enginnering
Research InstitutionTohoku University

Principal Investigator

ITO Takatoshi  東北大学, 流体科学研究所, 教授 (00184664)

Co-Investigator(Renkei-kenkyūsha) SEKINE Kotaro  石油天然ガス・金属鉱物資源機構, 技術センター, 研究員 (70361194)
SATO Akira  熊本大学, 自然科学研究科, 准教授 (40305008)
TOSHA Toshiyuki  産業技術総合研究所, 地圏資源環境研究部門, 主幹研究員 (10357551)
Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥14,950,000 (Direct Cost: ¥11,500,000、Indirect Cost: ¥3,450,000)
Fiscal Year 2011: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2010: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2009: ¥6,760,000 (Direct Cost: ¥5,200,000、Indirect Cost: ¥1,560,000)
Keywords廃棄物地下保存 / 処分 / 地球温暖化ガス排出削減 / 大深度地下 / 環境技術
Research Abstract

In order to remedy CO_2 leakage through pre-existing and/or induced fractures from storage reservoirs, we studied a concept to use an aqueous solution. The solution will have a sufficiently-low viscosity for passing through even small aperture, and it will not impact formation permeability as long as the solution is left as it is. When the solution encounters dissolved CO_2, precipitation will occur due to chemical reaction. As a result, the permeability will be reduced by filling the pores and fractures in the rocks with the precipitates. We demonstrated first this idea through laboratory experiments simulating subsurface condition at 1000 m deep, i. e. 10 MPa and 40 deg. C. The results show that the present method led to a 99 %permeability reduction in a glass-bead artificial rock even its initially-high permeability of few darcy. Such reduction of permeability was reproduced successfully by the non-isothermal reactive geochemical transport program TOUGHREACT. Based upon these success, the present method was applied by numerical modeling to a 2-D caprock-aquifer system under field physical and chemical conditions. The results show that the precipitates were produced and they filled up pores around outlet of the leakage path so sufficiently that the CO_2 migration was blocked, and the condition was confirmed stable over a long time.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (8 results)

All 2011 2010 2009

All Presentation (8 results)

  • [Presentation] CO2貯留層からの漏洩修復法とそのケーススタディー2011

    • Author(s)
      谷内雄紀, 田中秀宜, 伊藤高敏, Xu, T.
    • Organizer
      資源素材学会秋季大会企画発表・一般発表(B)(C)講演資料
    • Place of Presentation
      堺
    • Year and Date
      2011-09-28
    • Related Report
      2011 Final Research Report
  • [Presentation] CO2貯留層からの漏洩修復法とそのケーススタディー2011

    • Author(s)
      谷内雄紀, 田中秀宜, 伊藤高敏, Xu, T.
    • Organizer
      資源素材学会秋季大会
    • Place of Presentation
      堺
    • Year and Date
      2011-09-28
    • Related Report
      2011 Annual Research Report
  • [Presentation] CO2地中貯留層からの原位置反応法による漏洩修復と数値シミュレーションによる検討2010

    • Author(s)
      田中秀宜, 伊藤高敏, 関根孝太郎, Xu, T.
    • Organizer
      石油技術協会春季講演会要旨集
    • Place of Presentation
      東京
    • Year and Date
      2010-06-09
    • Related Report
      2011 Final Research Report
  • [Presentation] CO2地中貯留層からの原位置反応法による漏洩修復と数値シミュレーションによる検討2010

    • Author(s)
      田中秀宜, 伊藤高敏, 関根孝太郎, ティアンフ・スー
    • Organizer
      石油技術協会春季講演会
    • Place of Presentation
      福岡
    • Year and Date
      2010-06-09
    • Related Report
      2010 Annual Research Report
  • [Presentation] Proposed Concept of In-situReaction Barrier to Remedy Leakagefrom Reservoirs of Geological CO2Storage2010

    • Author(s)
      T. Ito
    • Organizer
      Proc. of the 2nd Int. Symp. of Experiment-Integrated Comp. Chem. Multi-scale Fluids
    • Place of Presentation
      Sendai
    • Year and Date
      2010-02-24
    • Related Report
      2011 Final Research Report
  • [Presentation] Proposed Concept of In-situ Reaction Barrier to Remedy Leakage from Reservoirs of Geological CO2 Storage(招待講演)2010

    • Author(s)
      伊藤高敏
    • Organizer
      The Second International Symposium of Experiment-Integrated Computational Chemistry on Multi-scale Fluids
    • Place of Presentation
      仙台
    • Year and Date
      2010-02-24
    • Related Report
      2009 Annual Research Report
  • [Presentation] CO2地中貯留層からの漏洩修復法の検討2009

    • Author(s)
      田中秀宜, 櫻井雅徳, 関根孝太郎, 伊藤高敏
    • Organizer
      日本地球惑星科学連合2009年大会
    • Place of Presentation
      千葉
    • Year and Date
      2009-05-21
    • Related Report
      2009 Annual Research Report
  • [Presentation] CO2地中貯留層からの漏洩修復法の検討2009

    • Author(s)
      田中秀宜, 櫻井雅徳, 関根孝太郎, 伊藤高敏
    • Organizer
      日本地球惑星科学連合大会予稿集
    • Place of Presentation
      千葉
    • Year and Date
      2009-05-18
    • Related Report
      2011 Final Research Report

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Published: 2009-04-01   Modified: 2016-04-21  

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