Laboratory study of aging of secondary organic aerosol formed from the photooxidation of aromatic hydrocarbons
Project/Area Number |
21510023
|
Research Category |
Grant-in-Aid for Scientific Research (C)
|
Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Environmental dynamic analysis
|
Research Institution | National Institute for Environmental Studies |
Principal Investigator |
SATO Kei 独立行政法人国立環境研究所, 地域環境研究センター, 主任研究員 (10282815)
|
Project Period (FY) |
2009 – 2011
|
Project Status |
Completed (Fiscal Year 2011)
|
Budget Amount *help |
¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2011: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2010: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2009: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
|
Keywords | 芳香族炭化水素 / 二次有機エアロゾル / 光化学スモッグチャンバー / エアロゾル質量分析計 / 液体クロマトグラフ質量分析計 / 含酸素有機エアロゾル / エアロゾルエイジング |
Research Abstract |
Oxygenated organic aerosol(OOA) observed in remote areas is believed to comprise aged secondary organic aerosol(SOA); however, the reaction processes relevant to SOA chemical aging have hitherto been unclear. We analyzed SOA particles formed from the photooxidation of aromatic hydrocarbons using an Aerosol mass spectrometry, liquid chromatography/mass spectrometry, and iodometric spectrophotometry. These results indicate that SOA aging proceeds mainly by formation of carboxylic acids, and that the rate of SOA aging in laboratory chambers is limited by the oxidation of ketone groups.
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Report
(4 results)
Research Products
(94 results)
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[Journal Article] AMS and LC/MS analyses of SOA from the photooxidation of benzene and 1, 3, 5-trimethylbenzene in the presence of NOx : Effects of chemical structure on SOA aging2012
Author(s)
Sato, K., Takami, A., Kato, Y., Seta, T., Fujitani, Y., Hikida, T., Shimono, A., and Imamura, T.
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Journal Title
Atmospheric Chemistry and Physics
Volume: 12(in press)
Related Report
Peer Reviewed
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[Journal Article] AMS and LC/MS analyses of SOA from the photooxidation of benzene and 1,3,5-trimethylbenzene in the presence of NOx : Effects of chemical structure on SOA aging2012
Author(s)
Sato, K., Takami, A., Kato, Y., Seta, T., Fujitani, Y., Hikida, T., Shimono, A., Imamura, T
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Journal Title
Atmos.Chem.Phys.Discuss.
Volume: VOL.12
Pages: 283-318
DOI
Related Report
Peer Reviewed
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[Journal Article] Secondary organic aerosol formation from the photooxidation of isoprene, 1,3-butadiene, and 2,3-dimethyl-1,3-butadiene under high NO_x conditions2011
Author(s)
Sato, K., Nakao, S., Clark, C.H., Qi, L., Cocker, D.R., III
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Journal Title
Atmospheric Chemistry and Physics
Volume: 11
Issue: 14
Pages: 7301-7317
DOI
Related Report
Peer Reviewed
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[Journal Article] Secondary organic aerosol formation from phenolic compounds in the absence of Nox2011
Author(s)
Nakao, S., Clark, C., Tang, P., Sato, K., Cocker, D., III
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Journal Title
Atmos.Chem.Phys
Volume: VOL.11(20)
Issue: 20
Pages: 10649-10660
DOI
Related Report
Peer Reviewed
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[Journal Article] Aerial Observation of Aerosols Transported from East Asia. Chemical Composition of Aerosols and Layered Structure of an Air Mass over the East China Sea2011
Author(s)
Hatakeyama,S., S. Hanaoka, K. Ikeda, I. Watanabe, T. Arakaki, Y. Sadanaga, H. Bandow, S. Kato, Y. Kajii, K. Sato, A. Shimizu, and A. Takami
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Journal Title
Aerosol Air Qual. Res
Volume: 11
Issue: 5
Pages: 497-507
DOI
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Peer Reviewed
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[Journal Article] Characterization of aerosol particles in the Tokyo metropolitan area using two different aerosol mass spectrometers2011
Author(s)
Xing, J.H., Takahashi, K., Yabushita, A., Kinugawa, T., Nakayama, T., Matsumi, Y., Tonokura, K., Takami, A., Imamura, T., Sato, K., Kawasaki, M., Hikida, T, Shimono, A
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Journal Title
Aerosol Science and Technology
Volume: 45
Pages: 315-326
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Peer Reviewed
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[Journal Article] Secondary organic aerosol formation from the photooxidation of isoprene, 1,3-butadiene, and 2,3-dimethyl-1,3-butadiene under high NO_x conditions2011
Author(s)
Sato, K., Nakao, S., Clark, C.H., Qi, L., Cocker, D.R, III
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Journal Title
Atmospheric Chemistry and Physics Discussions
Volume: 11
Pages: 4313-4345
Related Report
Peer Reviewed
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[Journal Article] Secondary organic aerosol formation from phenolic compounds in the absence of NOx2011
Author(s)
Nakao, S., Clark, C., Tang, P., Sato, K., Cocker, D., III
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Journal Title
Atmospheric Chemistry and Physics Discussions
Volume: 11
Pages: 2025-2055
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Peer Reviewed
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[Journal Article] Laboratory studies on optical properties of secondary organic aerosols generated during the photooxidation of toluene and the ozonolysis of α-pinene2010
Author(s)
Nakayama, T., Matsumi, Y., Sato, K., Imamura, T., Yamazaki, A., Uchiyama, A.
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Journal Title
Journal of Geophysical Research
Volume: 115
Related Report
Peer Reviewed
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[Journal Article] Mass spectrometric study of secondary organic aerosol formed from the photo-oxidation of aromatic hydrocarbons2010
Author(s)
Sato, K., Takami, A., Isozaki, T., Hikida, T., Shimono, A., Imamura, T.
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Journal Title
Atmospheric Environment 44
Pages: 1080-1087
Related Report
Peer Reviewed
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[Journal Article] Mass spectrometric study of secondary organic aerosol formed from the photo-oxidation of aromatic hydrocarbons2009
Author(s)
Sato, K., Takami, A., Isozaki, T., Hikida, T., Shimono, A., Imamura, T.
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Journal Title
Atmospheric Environment
Volume: 44(8)
Issue: 8
Pages: 1080-1087
DOI
Related Report
Peer Reviewed
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[Journal Article] Long-range transport of particulate polycyclic aromatic hydrocarbons at a remote island site at Cape Hedo in the East China Sea between 2005 and 20082009
Author(s)
Sato, K., Li, H., Tanaka, Y., Ogawa, S., Iwasaki, Y., Takami, A., Hatakeyama, S.
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Journal Title
Journal of Atmospheric Chemistry 61
Pages: 243-257
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Peer Reviewed
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[Presentation] ジエチルアミンの日中の大気寿命決定2012
Author(s)
瀬田孝将, 佐藤圭, 今村隆史, 堀添浩司, 長安弘貢, 上條孝
Organizer
第92日本化学会春季年会
Place of Presentation
慶応義塾大学日吉キャンパス(神奈川県)
Year and Date
2012-03-25
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[Presentation] On-line measurements of nitro organic compounds emitted from automobiles by proton transfer reaction mass spectrometry : Laboratory experiments and a field measurement2011
Author(s)
Inomata, S., Tanimoto, H., Fujitani, Y., Fushimi, A.Sato, K., Sekimoto, K., Yamada, H., Hori, S., Shimono, A., Hikida, T.
Organizer
American Geophysical Union Fall Meeting 2011
Place of Presentation
Moscone Convention Center (San Fransisco, USA)
Year and Date
2011-12-05
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[Presentation] Determination of refractive index of secondary organic aerosols generated during the photooxidation of toluene and the ozonolysis of alpha-pinene2011
Author(s)
Nakayama, T., Matsumi, Y., Sato, K., Imamura, T., Yamazaki, A., Uchiyama, A.
Organizer
American Association for Aerosol Research 30^<th> Annual Conference
Place of Presentation
Rosen Shingle Creek Resort & Golf Club (Orlando, USA)
Year and Date
2011-10-05
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[Presentation] Temperature dependence of secondary organic aerosol particle-phase products from isoprene dark ozonolysis and NO photooxidation2011
Author(s)
Clark, C., Nakao, S., Sato, K., Asa-Awuku, A, Cocker III, D.
Organizer
American Association for Aerosol Research 30^<th> Annual Conference
Place of Presentation
Rosen Shingle Creek Resort & Golf Club (Orlando, USA)
Year and Date
2011-10-05
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[Presentation] 長崎県福江島における有機エアロゾル・エアロゾル金属成分の観測2011
Author(s)
吉野彩子, 畠山史郎, 小川佳美, 佐藤圭, 高見昭憲, 伊礼聡, 坂本哲夫, 村野健太郎, 定永靖宗, 坂東博, 藤井正明
Organizer
第52回大気環境学会年会
Place of Presentation
長崎大学文教地区キャンパス環境科学部(長崎県)
Year and Date
2011-09-16
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[Presentation] ディーゼル車から排出されるニトロ有機化合物2011
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Organizer
第28回エアロゾル科学・技術研究討論会
Place of Presentation
大阪府立大学中百舌鳥キャンパスB3棟(大阪府)
Year and Date
2011-08-29
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[Presentation] Applications of cavity ring-down aerosol extinction spectrometer to laboratory and field studies2011
Author(s)
Nakayama, T., Matsumi, Y., Hagino, R., Kagamitani, S., Sato, K., Imamura, T., Yamazaki, A., Uchiyama, A.
Organizer
The 2011 User Meeting and Summer School on Cavity Enhanced Spectroscopy
Place of Presentation
Chernoff Hall, Queen's University (Kingston, Canada)
Year and Date
2011-06-29
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[Presentation] Study of secondary aerosol formation from the atmospheric oxidation of amines using time-of-flight aerosol mass spectrometer2011
Author(s)
Sato, K., Imamura, T., Horizoe, K., Fujii, S., Nagayasu, H., Inui, M., Kamijo, T.
Organizer
第27回化学反応討論会
Place of Presentation
東京工業大学大岡山キャンパス西9号館デジタル多目的ホール(東京都)
Year and Date
2011-06-09
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[Presentation] 大型テフロンチャンバーを用いたイソプレンや1,3-ブタジエンの酸化で生じるSOA生成機構の解明2010
Author(s)
佐藤圭, 中尾俊介, Clark, C., Qi, L., Tang, P., Cocker, D
Organizer
第16回大気化学討論会
Place of Presentation
首都大学東京南大沢キャンパス国際交流会館(東京都)
Year and Date
2010-11-19
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[Presentation] 東シナ海を越えて輸送されるエアロゾルの航空機・地上観測-2009年10月12~19日2010
Author(s)
畠山史郎, 花岡小百合, 池田圭輔, 小川佳美, 大井彩子, 渡邉泉, 高見昭憲, 清水厚, 佐藤圭, 定永靖宗, 坂東博, 浦田淳基, 加藤俊吾, 梶井克純, 新垣雄光, 畦地総太郎, 張代洲, 原和崇
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第16回大気化学討論会
Place of Presentation
首都大学東京南大沢キャンパス国際交流会館(東京都)
Year and Date
2010-11-19
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[Presentation] Secondary organic aerosol formation from the photooxidation of conjugated dienes under high NO_x conditions2010
Author(s)
Sato, K., Nakao, S., Clark, C., Qi, L., Tang, P., Cocker, D.
Organizer
American Association for Aerosol Research 29^<th> Annual Conference
Place of Presentation
Oregon Convention Center (Portland, Oregon, U.S.A)
Year and Date
2010-10-28
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[Presentation] S Chemical characterization by particle into liquid sampling directly coupled to an accurate mass time-of-flight mass spectrometer (PILS-ToF) of secondary organic aerosol (SOA)2010
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Clark, C., Nakao, S., Sato, K., Qi, L., Asa-Awuku, A., Cocker, D.R., III
Organizer
American Association for Aerosol Research 29^<th> Annual Conference
Place of Presentation
Oregon Convention Center (Portland, Oregon, U.S.A)
Year and Date
2010-10-26
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[Presentation] PAHs and n-alkanes in the aerosol transported around the East China Sea2010
Author(s)
Ogawa, Y., Sato, K., Kaneyasu, N., Takami, A., Hatakeyama, S.
Organizer
International Aerosol Concerence 2010
Place of Presentation
University of Helsinki (Helsinki, Finland)
Year and Date
2010-08-03
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[Presentation] Secondary organic aerosol formation from the photooxidation of conjugated dienes in the presence of NO2010
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Sato, K., Nakao, S., Clark, C., Qi, L., Tang, P., Cocker, D.
Organizer
第26回化学反応討論会
Place of Presentation
広島大学佐竹メモリアルホール(広島県)
Year and Date
2010-06-03
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[Presentation] Measurement of elemental carbon at CHAAMS in spring 20092010
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Takami, A., Kaneyasu, N., Osada, K., Hasegawa, S., Sato, K., Shimizu, A., Hatakeyama, S.
Organizer
Japan Geoscience Union Meeting 2010, JpGU International Symposium 2010
Place of Presentation
幕帳メッセ国際会議場(千華県)
Year and Date
2010-05-27
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[Presentation] Secondary organic aerosol formation from m-xylene photooxidation : The role of the phenolic product2009
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Nakao, S., Qi, L., Clark, C., Sato, K., Tang, P., Cocker, D.
Organizer
2009 American Geophysical Union Fall Meeting
Place of Presentation
Moscone Center(San Francisco. U.S.A.)
Year and Date
2009-12-14
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[Presentation] Measurement of optical properties of secondary organic aerosol2009
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Organizer
Fourth Japan-China-Korea Joint Conference on Meteorology
Place of Presentation
Tsukuba
Year and Date
2009-11-08
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[Presentation] LEXTRA-Aerial obaervation of aerosols and gases transported from East Asia in March-April, 20082009
Author(s)
Hatakeyama, S., Hanaoka, S., Watanabe, I., Arakaki, T., Kawana, K., Kondo, Y., Sadanaga, Y., Bandow, H., Kato, S., Kajii, Y., Sato, K., Shimizu, A., Takami, A.
Organizer
Fourth Japan-China-Korea Joint Conference on Meteorology
Place of Presentation
Tsukuba
Year and Date
2009-11-08
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[Presentation] Mass spectroscopic study of secondary organic aerosol from the photooxidation of aromatic hydrocarbons2009
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Sato, K., Takami, A., Isozaki, T., Hikida, T., Shimono, A., Imamura, T.
Organizer
American Association for Aerosol Research 28^<th> Annual Conference
Place of Presentation
Hyatt Regency Minneapolis(Minneapolis, USA)
Year and Date
2009-10-28
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[Presentation] Could secondary organic aerosols act as brown carbon?: Laboratory studies of aerosol absorption2009
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Nakayama, T., Matsumi, Y., Yamazaki, A., Uchiyama, A., Sato, K., Imamura, T.
Organizer
IGAC-SPARC Joint Workshop
Place of Presentation
Shiran Kaikan(Kyoto)
Year and Date
2009-10-25
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Uchida, R., Fukuda, S., Nakagawa, K., Xing, J.-H., Sato, K., Imamura, T., Hikida, T., Shimono, A.
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IGAC-SPARC Joint Workshop
Place of Presentation
Shiran Kaikan(Kyoto)
Year and Date
2009-10-25
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[Presentation] Secondary organic aerosol formation in ozone-isoprene reaction system2009
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Uchida, R., Fukuda, S., Nakagawa, K., Xing, J.-H., Sato, K., Imamura, T., Hikida, T., Shimono, A.
Organizer
International Workshop on Chemistry in the Earth's Atmosphere
Place of Presentation
Tokyo Tech Front, Tokyo Institute of Technology(Tokyo)
Year and Date
2009-09-08
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[Presentation] Effect of enhanced UV radiation on photochemical ozone and aerosol formation2009
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Fukuda, S., Uchida, R., Nakagawa, K., Sato, K., Imamura, T.
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International Workshop on Chemistry in the Earth's Atmosphere
Place of Presentation
Tokyo Tech Front, Tokyo Institute of Technology(Tokyo)
Year and Date
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[Presentation] LEXTRA航空機観測におけるエアロゾル化学成分2009
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Organizer
第28回エアロゾル科学・技術研究討論会
Place of Presentation
岡山大学津島キャンパス自然科学研究科棟
Year and Date
2009-08-19
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[Presentation] Aerial obaervation of aerosols and gases transported from East Asia in March-April, 20082009
Author(s)
Hanaoka, S., Hatakeyama, S., Watanabe, I., Arakaki, T., Kawana, K., Kondo, Y., Sadanaga, Y., Bandow, H., Kato, S., Kajii, Y., Sato, K., Shimizu, A., Takami, A.
Organizer
18^<th> International Conference Nucleation and Atmospheric Aerosols
Place of Presentation
Hotel Pyramida(Prague, Czech Republic)
Year and Date
2009-08-11
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[Presentation] Secondary organic aerosol formation in the isoprene ozonolysis2009
Author(s)
Uchida, R., Fukuda, S., Nakagawa, K., Xing, J., Sato, K., Imamura, T., Hikida, T., Shimono, A.
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第25回化学反応討論会
Place of Presentation
大宮ソニックシティ(埼玉県)
Year and Date
2009-06-01
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[Presentation] 二種類のエアロゾル質量分析計による2008年夏季東京都心のエアロゾル観測2009
Author(s)
シンジャワ, 高橋けんし, 薮下彰啓, 衣川高志, 中山智喜, 松見豊, 戸野倉賢一, 川崎昌博, 高見昭憲, 佐藤圭, 今村隆史, 疋田利秀, 下野彰夫
Organizer
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Place of Presentation
幕張メッセ国際会議場(千葉県)
Year and Date
2009-05-20
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[Presentation] 2008年春に東シナ海域で行った航空機観測LEXTRA2009
Author(s)
高見昭憲, 佐藤圭, 清水厚, 大原利眞, 加藤俊吾, 梶井克純, 定永靖宗, 坂東博, 川名華織, 竹川暢之, 近藤豊, 新垣雄光, 花岡小百合, 渡邉泉, 畠山史郎
Organizer
日本地球惑星科学連合2009年大会
Place of Presentation
幕張メッセ国際会議場(千葉県)
Year and Date
2009-05-20
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[Presentation] 二種類の質量分析計による大気エアロゾルの観測2009
Author(s)
シンジャワ, 高橋けんし, 藪下彰啓, 衣川高志, 中山智喜, 松見豊, 戸野倉賢一, 川崎昌博, 高見昭憲, 佐藤圭, 今村隆史, 疋田利秀, 下野彰夫
Organizer
第57回質量分析総合討論会
Place of Presentation
大阪国際交流センター(大阪府)
Year and Date
2009-05-15
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