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Diffuse scattering study by X-ray and neutron diffraction measurement and phonon dispersion relation

Research Project

Project/Area Number 21540314
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics I
Research InstitutionIbaraki University

Principal Investigator

SAKUMA Takashi  茨城大学, 理工学研究科, 教授 (10114018)

Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2011: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2010: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2009: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywords中性子回折 / 原子熱振動 / 相関効果 / 散漫散乱 / フォノン分散関係 / 力定数 / 熱振動相関効果 / 格子振動 / 散漫散乱強度 / 原子熱振動の相関効果 / 熱振動の相関効果 / フォノンの分散関係
Research Abstract

The oscillatory forms of the diffuse scattering intensities were observed from ordered crystals at room temperature. The observed diffuse scattering intensities were analyzed by including the correlation effects among thermal displacements of atoms. The values of correlation effects decrease rapidly with the increase of inter-atomic distances. From the parameters of Debye-Waller temperature factor and the values of correlation effects, the inter-atomic force constants among first, second and third nearest neighboring atoms were determined. A rough estimation of phonon dispersion relation was performed from the inter-atomic force constants and crystal structure using computer simulation.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (24 results)

All 2011 2010 2009 Other

All Journal Article (10 results) (of which Peer Reviewed: 10 results) Presentation (11 results) Book (2 results) Remarks (1 results)

  • [Journal Article] Correlation effects among thermal displacements of atoms in KBr2011

    • Author(s)
      T. Sakuma, Xianglian, N. Shimizu, S. R. Mohapatra, N. Isozaki, H. Uehara, H. Takahashi, K. Basar, N. Igawa, O. Kamishima
    • Journal Title

      Solid State Ionics

      Volume: 192 Pages: 54-57

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Neutron diffraction study of diffuse scattering in Cu_2-Se superionic compounds2011

    • Author(s)
      S. A. Danilkin, M. Avdeev, T. Sakuma, R. Macquart, C. D. Ling
    • Journal Title

      J. alloys and compounds

      Volume: 509 Pages: 5460-5465

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] NEUTRON SCATTERING STUDY OF SHORT RANGE CORRELATIONS AND IONIC DIFFUSION IN COPPER SELENIDE2011

    • Author(s)
      S. A. Danilkin, M. Avdeev, T. Sakuma, R. Macquart, C. D. Ling, M. Rusinaand, Z. Izaola
    • Journal Title

      Ionics

      Volume: 17 Pages: 75-80

    • Related Report
      2011 Final Research Report 2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Estimation of inter-atomic force constants and phonon dispersion using correlation effects among thermal displacement of atoms in Ge2011

    • Author(s)
      T. SAKUMA, S. R. MOHAPATRA, N. ISOZAKI, H. UEHARA, XIANGLIAN, K. BASAR, H. TAKAHASHI, O. KAMISHIMA, N. IGAWA
    • Journal Title

      J. Non-crystalline Solid

      Volume: 357 Pages: 559-562

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Neutron diffraction study of diffuse scattering in Cu_<2-δ>Se superionic compounds2011

    • Author(s)
      S.A.Danilkin, M.Avdeev, T.Sakuma, R.Macquart, C.D.Ling
    • Journal Title

      J.alloys and compounds

      Volume: 509 Issue: 18 Pages: 5460-5465

    • DOI

      10.1016/j.jallcom.2011.02.101

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Estimation of inter-atomic force constants and phonon dispersion using correlation effects among thermal displacement of atoms in Ge2011

    • Author(s)
      T.SAKUMA, S.R.MOHAPATRA, N.ISOZAKI, H.UEHARA, XIANGLIAN, K.BASAR, H.TAKAHASHI, O.KAMISHIMA, N.IGAWA
    • Journal Title

      J.Non-crystalline Solid

      Volume: 357 Pages: 559-562

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] CORRELATION EFFECTS AMONG THERMAL DISPLACEMENTS OF ATOMS IN VSe BY DIFFUSE NEUTRON SCATTERING MEASUREMENT2010

    • Author(s)
      T. Sakuma, Xianglian, S. Siagian, K. Basar, H. Takahashi, N. Igawa, and O. Kamishima
    • Journal Title

      J. Thermal Anal. Cal.

      Volume: 99 Pages: 173-176

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] OSCILLATORY DIFFUSE X-RAY SCATTERING FROM LEAD CHALCOGENIDES2010

    • Author(s)
      Xianglian, T. Sakuma, K. Basar and H. Takahashi
    • Journal Title

      J. Thermal Anal. Cal.

      Volume: 99 Pages: 65-69

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] CORRELATION EFFECTS AMONG THERMAL DISPLACEMENTS OF ATOMS IN VSe BY DIFFUSE NEUTRON SCATTERING MEASUREMENT2010

    • Author(s)
      T.Sakuma, Xianglian, S.Siagian, K.Basar, H.Takahashi, N.Igawa, O.Kamishima
    • Journal Title

      J.Thermal Anal.Cal. 99

      Pages: 173-176

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] OSCILLATORY DIFFUSE X-RAY SCATTERING FROM LEAD CHALCOGENIDES2010

    • Author(s)
      Xianglian, T.Sakuma, K.Basar, H.Takahashi
    • Journal Title

      J.Thermal Anal.Cal. 99

      Pages: 65-69

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] Diffuse Neutron Scattering Measurements of Ag2O and Cu_2O2011

    • Author(s)
      R. Sakai, T. Wada, T. Sakuma, H. Takahashi, O. Kamishima, N. Igawa, S. A. Danilkin
    • Organizer
      1st AOCNS
    • Place of Presentation
      つくば
    • Year and Date
      2011-11-21
    • Related Report
      2011 Final Research Report
  • [Presentation] Diffuse Neutron Scattering Measurements of Ag_2O and Cu_2O2011

    • Author(s)
      R.Sakai, T.Wada, T.Sakuma, H.Takahashi, O.Kamishima, N.Igawa, S.A.Danilkin
    • Organizer
      1st AOCNS
    • Place of Presentation
      つくば国際会議場
    • Year and Date
      2011-11-21
    • Related Report
      2011 Annual Research Report
  • [Presentation] Diffuse Neutron Scattering Study of Solid State Ionics2011

    • Author(s)
      T. Sakuma
    • Organizer
      ICC-IMR International Workshop
    • Place of Presentation
      仙台
    • Year and Date
      2011-11-18
    • Related Report
      2011 Final Research Report
  • [Presentation] Diffuse Neutron Scattering Study of Solid State Ionics2011

    • Author(s)
      T.Sakuma
    • Organizer
      ICC-IMR International Workshop
    • Place of Presentation
      東北大金研(招待講演)
    • Year and Date
      2011-11-18
    • Related Report
      2011 Annual Research Report
  • [Presentation] INTER-ATOMIC FORCE CONSTANTS OF Ag_2O FROM DIFFUSE NEUTRON SCATTERING MEASUREMENT2011

    • Author(s)
      T. Sakuma, T. Wada, R. Sakai, H. Uehara, Xianglian, H. Takahashi, O. Kamishima, N. Igawa, S. A. Danilkin
    • Organizer
      SSI-18
    • Place of Presentation
      Warsaw, Poland
    • Year and Date
      2011-07-04
    • Related Report
      2011 Final Research Report
  • [Presentation] INTER-ATOMIC FORCE CONSTANTS OF Ag_2O FROM DIFFUSE NEUTRON SCATTERING MEASUREMENT2011

    • Author(s)
      T.Sakuma, T.Wada, R.Sakai, H.Uehara, Xianglian, H.Takahashi, O.Kamishima, N.Igawa, S.A.Danilkin
    • Organizer
      SSI-18
    • Place of Presentation
      Warsaw, Poland(招待講演)
    • Year and Date
      2011-07-04
    • Related Report
      2011 Annual Research Report
  • [Presentation] X線・中性子回折測定と力定数2011

    • Author(s)
      佐久間隆、和田保、酒井竜太郎、高橋東之、神嶋修
    • Organizer
      第15回超イオン導電体物性研究会
    • Place of Presentation
      奈良
    • Year and Date
      2011-05-21
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] FORCE CONSTANTS OF CU CRYSTALS FROM DIFFUSE NEUTRON SCATTERING MEASUREMENT2010

    • Author(s)
      T. Sakuma
    • Organizer
      Conference on Material Science and Technology
    • Place of Presentation
      Serpong, Indonesia
    • Year and Date
      2010-10-21
    • Related Report
      2011 Final Research Report
  • [Presentation] FORCE CONSTANTS OF CU CRYSTALS FROM DIFFUSE NEUTRON SCATTERING MEASUREMENT2010

    • Author(s)
      T.Sakuma
    • Organizer
      Conference on Mterial Science and Technology(ICSMST 2011)
    • Place of Presentation
      Serpong,Indonesia
    • Year and Date
      2010-10-21
    • Related Report
      2010 Annual Research Report
  • [Presentation] ESTIMATION OF PHONON DISPERSION RELATION FROM CORRELATION EFFECTS AMONG THERMAL DISPLACEMENTS OF ATOMS2009

    • Author(s)
      T. Sakuma
    • Organizer
      6th International Discussion Meeting on Relaxations in Complex Systems
    • Place of Presentation
      Rome, Italy
    • Year and Date
      2009-09-02
    • Related Report
      2011 Final Research Report
  • [Presentation] ESTIMATION OF PHONON DISPERSION RELATION FROM CORREL ATION EFFECTS AMONG THERMAL DISPLACEMENTS OF ATOMS2009

    • Author(s)
      T.Sakuma
    • Organizer
      6th International Discussion Meeting on Relaxations in Complex Systems
    • Place of Presentation
      Rome University(Italy)
    • Year and Date
      2009-09-02
    • Related Report
      2009 Annual Research Report
  • [Book] Diffuse Neutron Scattering Study of Correlation Effects Among Thermal Displacements of Atoms2011

    • Author(s)
      T. Sakuma, Xianglian, H. Uehara and S. R. Mohapatra
    • Publisher
      Nova Science Publishers, Inc.
    • Related Report
      2011 Final Research Report
  • [Book] Diffuse Neutron Scattering Study of Correlation Effects Among Thermal Displacements of Atoms2011

    • Author(s)
      T.Sakuma, Xianglian, H.Uehara, S.R.Mohapatra
    • Publisher
      Nova Science Publishers, Inc.
    • Related Report
      2011 Annual Research Report
  • [Remarks]

    • URL

      http://info.ibaraki.ac.jp/scripts/websearch/index.htm

    • Related Report
      2009 Annual Research Report

URL: 

Published: 2009-04-01   Modified: 2020-05-15  

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