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Enhancement of sonochemical reaction by bubble-nucleation control

Research Project

Project/Area Number 21560060
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied physics, general
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

TUZIUTI Toru  独立行政法人産業技術総合研究所, 計測フロンティア研究部門, 主任研究員 (70357515)

Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2011: ¥130,000 (Direct Cost: ¥100,000、Indirect Cost: ¥30,000)
Fiscal Year 2010: ¥130,000 (Direct Cost: ¥100,000、Indirect Cost: ¥30,000)
Fiscal Year 2009: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywords音 / 超音波化学 / 気泡 / 超音波 / ソノケミカル反応 / 音響化学発光 / パルス波 / デューティサイクル / 気泡核 / 添加 / キャビテーション気泡 / アルコール / 音響発光 / 溶存気体濃度 / 脱ガス / 飽和 / 粒子 / 音圧波形 / 振動振幅 / 液面ゆれ
Research Abstract

Liquid-surface vibration amplitude and the intensity of sonochemiluminescence(SCL) with luminol were detected. It was found that the SCL intensity increases and reaches its peak and after that decreases with the applied power. The vibration amplitude of liquid surface was the order of 100 ms. It has been clarified that the amplitude more than 1/4 of sound wavelength is responsible for destruction of stable resonant standing wave structure effective for sonochemical reaction and, accordingly, the reduction in efficiency in the reaction at excess sound pressure amplitude comes from liquid surface vibration on a sonochemical reactor.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (25 results)

All 2012 2011 2010 2009 Other

All Journal Article (15 results) (of which Peer Reviewed: 11 results) Presentation (8 results) Remarks (2 results)

  • [Journal Article] 溶存気体飽和度がソノルミネッセンス強度に与える影響2012

    • Author(s)
      辻内亨
    • Journal Title

      超音波とマイクロバブルの相互作用に関するシンポジウム講演論文集

      Pages: 3-4

    • Related Report
      2011 Annual Research Report
  • [Journal Article] 洗浄に寄与するキャビテーション気泡の可視化技術2012

    • Author(s)
      辻内亨
    • Journal Title

      超音波テクノ

      Volume: 24 Pages: 6-8

    • Related Report
      2011 Annual Research Report
  • [Journal Article] Intermittent changes in the number of pulsating bubbles under ultrasound2012

    • Author(s)
      Toru Tuziuti, Kyuichi Yasui
    • Journal Title

      JAPANESE JOURNAL OF APPLIED PHYSICS

      Volume: 51 Issue: 2R Pages: 028007-028007

    • DOI

      10.1143/jjap.51.028007

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mist Separation and Sonochemiluminescence under Pulsed Ultrasound2012

    • Author(s)
      Toru Tuziuti
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY A

      Volume: 116 Issue: 14 Pages: 3593-3597

    • DOI

      10.1021/jp301205q

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of degree of gas saturation on multibubble sonoluminescence intensity2011

    • Author(s)
      辻内亨、安井久一、加藤一実
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY A

      Volume: 115 Issue: 20 Pages: 5089-5091

    • DOI

      10.1021/jp201473q

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] On the influence of degree of gas saturation on multibubble sonoluminescence intensity2011

    • Author(s)
      Toru Tuziuti, Kyuichi Yasui, Kazumi Kato
    • Journal Title

      Proceedings of Symposium on ULTRASONICS ELECTRONICS

      Volume: 32 Pages: 383-384

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] キャビテーション気泡の空間分布がソノケミカル反応効率に与える影響2010

    • Author(s)
      辻内亨
    • Journal Title

      非破壊検査

      Volume: 59 Pages: 555-561

    • NAID

      10027572861

    • Related Report
      2011 Final Research Report 2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of liquid-surface vibration on sonochemiluminescence intensity2010

    • Author(s)
      辻内亨、安井久一、小塚晃透、砥綿篤哉
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY A

      Volume: 114 Issue: 27 Pages: 7321-7325

    • DOI

      10.1021/jp101638c

    • Related Report
      2011 Final Research Report 2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] On the influence of liquid-surface vibration on sonochemiluminescence2010

    • Author(s)
      辻内亨, 安井久一, 小塚晃透, 砥綿篤哉
    • Journal Title

      Proceedings of the International Congress on Acoustics 2010

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of particle addition on sonochemiluminescence intensity under pulsed ultrasound2010

    • Author(s)
      辻内亨, 安井久一, 小塚晃透, 砥綿篤哉
    • Journal Title

      Proceedings of Symposium on ULTRASONIC ELECTRONICS

      Volume: 31 Pages: 355-356

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] パルス超音波によるソノケミカル反応=高効率化に向けて=2010

    • Author(s)
      辻内亨
    • Journal Title

      超音波テクノ

      Volume: 22 Pages: 53-55

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Influence of surface active solute on ultrasonic waveform distortion in liquid containing air bubbles2009

    • Author(s)
      辻内亨、安井久一、Lee Yu-Ting Judy、小塚晃透、砥綿篤哉、飯田康夫
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY A

      Volume: 113 Issue: 31 Pages: 8893-8900

    • DOI

      10.1021/jp901898p

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Influence of surface active solute on ultrasonic waveform distortion in liquid containing air bubbles2009

    • Author(s)
      辻内亨、安井久一、Lee Yh-TingJudy、小塚晃透、砥綿篤哉、飯田康夫
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY A 113

      Pages: 8893-8900

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] On the influence of surface active solute on ultrasonic waveform distortion in liquid containing air bubbles2009

    • Author(s)
      辻内亨、安井久一、Lee Yh-TingJudy、小塚晃透、砥綿篤哉、飯田康夫
    • Journal Title

      Proceedings of Symposium on Ultrasonics Electronics 30

      Pages: 127-128

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] キャビテーション気泡の空間分布とソノケミカル反応効率の関係2009

    • Author(s)
      辻内亨
    • Journal Title

      非線形超音波研究会資料 II-14

      Pages: 1-2

    • Related Report
      2009 Annual Research Report
  • [Presentation] 溶存気体飽和度がソノルミネッセンス強度に与える影響(招待講演)2012

    • Author(s)
      辻内亨
    • Organizer
      日本ソノケミストリー学会第4回超音波とマイクロバブルの相互作用に関するシンポジウム
    • Place of Presentation
      名古屋駅前イノベーションハブ(名古屋)
    • Year and Date
      2012-01-20
    • Related Report
      2011 Final Research Report
  • [Presentation] 溶存気体飽和度がソノルミネッセンス強度に与える影響2012

    • Author(s)
      辻内亨
    • Organizer
      日本ソノケミストリー学会第4回超音波とマイクロバブルの相互作用に関するシンポジウム
    • Place of Presentation
      名古屋駅前イノベーションハブ(名古屋)(招待講演)
    • Year and Date
      2012-01-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] On the influence of degree of gas saturation on multibubble sonoluminescence intensity2011

    • Author(s)
      Toru Tuziuti, Kyuichi Yasui, Kazumi Kato
    • Organizer
      The 32nd Symposium on Ultrasonic Electronics (USE2011)
    • Place of Presentation
      京都大学(京都)
    • Year and Date
      2011-11-10
    • Related Report
      2011 Annual Research Report
  • [Presentation] Influence of particle addition on sonochemiluminescence intensity under pulsed ultrasound2010

    • Author(s)
      辻内亨, 安井久一, 小塚晃透, 砥綿篤哉
    • Organizer
      The 31st Symposium on Ultrasonics Electronics (USE2010)
    • Place of Presentation
      明治大学、東京
    • Year and Date
      2010-12-07
    • Related Report
      2010 Annual Research Report
  • [Presentation] On the influence of liquid-surface vibration on sonochemiluminescence2010

    • Author(s)
      辻内亨,安井久一,小塚晃透,砥綿篤哉
    • Organizer
      International Congress on Acoustics 2010
    • Place of Presentation
      シドニーコンベンションセンター、シドニー
    • Year and Date
      2010-08-25
    • Related Report
      2011 Final Research Report 2010 Annual Research Report
  • [Presentation] On the influence of surface active solute on ultrasonic waveform distortion inliquid containing air bubbles2009

    • Author(s)
      辻内亨、安井久一、Lee Yh-TingJudy、小塚晃透、砥綿篤哉、飯田康夫
    • Organizer
      The 30th Symposium on Ultrasonics Electronics
    • Place of Presentation
      京都
    • Year and Date
      2009-11-18
    • Related Report
      2009 Annual Research Report
  • [Presentation] キャビテーション気泡の空間分布とソノケミカル反応効率の関係2009

    • Author(s)
      辻内亨
    • Organizer
      日本非破壊検査協会非線形超音波研究会
    • Place of Presentation
      富山大学(富山)
    • Year and Date
      2009-08-10
    • Related Report
      2011 Final Research Report
  • [Presentation] キャビテーション気泡の空間分布とソノケミカル反応効率の関係(招待講演)2009

    • Author(s)
      辻内亨
    • Organizer
      日本非破壊検査協会 非線形超音波研究会
    • Place of Presentation
      富山大学
    • Year and Date
      2009-08-10
    • Related Report
      2009 Annual Research Report
  • [Remarks] 研究成果に関するwebページ

    • URL

      http://www.aist.go.jp/RRPDB/system/Koukai.Top

    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://www.aist.go.jp/RRPDB/system/Koukai.Top

    • Related Report
      2011 Annual Research Report

URL: 

Published: 2009-04-01   Modified: 2016-04-21  

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