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Study of photocatalysts for hydrogen production through photocatalytic steam reforming of methane at ambient temperature

Research Project

Project/Area Number 21560799
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Catalyst/Resource chemical process
Research InstitutionNagoya University

Principal Investigator

YOSHIDA Hisao  名古屋大学, 工学研究科, 准教授 (80273267)

Co-Investigator(Renkei-kenkyūsha) HIRANO Masanori  愛知工業大学, 工学部, 教授 (60267888)
YOSHIDA Tomoko  名古屋大学, エコトピア科学研究所, 准教授 (90283415)
SASAI Ryo  島根大学, 総合理工学研究科, 准教授 (60314051)
Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2011: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2010: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2009: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords太陽エネルギー / エネルギー変換 / 光触媒 / 水素 / メタン / 水 / 助触媒 / 水素生成 / 光エネルギー / 酸化ガリウム / チタン酸カルシウム
Research Abstract

We found a photocatalytic steam reforming of methane(PSRM) to produce hydrogen from water and methane as renewable resources, which can utilize solar energy. To develop active photocatalysts for the PSRM, we examined some photocatalysts and found several guidelines for the design of catalyst and the reaction system :(1) reaction condition suitable for the formation of surface intermediates,(2) semiconductor particles having less defects and high specific surface area,(3) doping and surface modification suitable for the semiconductors,(4) god junction between the semiconductor surface and the cocatalyst nanoparticles,(5) possible bifunctional cocatalyst, and(6) thermal acceleration.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (36 results)

All 2012 2011 2010 2009

All Journal Article (13 results) (of which Peer Reviewed: 13 results) Presentation (21 results) Book (2 results)

  • [Journal Article] Effect of doped zinc species on the photo catalytic activity of gallium oxide for hydrogen production2012

    • Author(s)
      K. Shimura, H. Yoshida
    • Journal Title

      Phys. Chem. Chem. Phys

      Volume: 14 Issue: 8 Pages: 2678-2684

    • DOI

      10.1039/c2cp23220k

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Heterogeneous photo catalytic hydrogen production from water and biomass derivatives2011

    • Author(s)
      K. Shimura, H. Yoshida
    • Journal Title

      Energy Environ. Sci

      Volume: 4 Issue: 7 Pages: 2467-2481

    • DOI

      10.1039/c1ee01120k

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Simultaneously photodeposited rhodium metal and oxide nanoparticles promoting photocatalytic hydrogen production2011

    • Author(s)
      K. Shimura, H. Kawai, T. Yoshida, H. Yoshida
    • Journal Title

      Chem. Commun.

      Volume: 47 Issue: 31 Pages: 8958-8960

    • DOI

      10.1039/c1cc12287h

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermal acceleration of electron migration in gallium oxide photocatalysts2011

    • Author(s)
      K. Shimura, K. Maeda, H. Yoshida
    • Journal Title

      J. Phys. Chem. C

      Volume: 115 Issue: 18 Pages: 9041-9047

    • DOI

      10.1021/jp110824n

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermal acceleration of electron migration in gallium oxide photocatalysts2011

    • Author(s)
      K Shimura, K Maeda, H Yoshida
    • Journal Title

      J Phys Chem.C

      Volume: 115(印刷中)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photocatalytic activation of water and methane over modified gallium oxide for hydrogen production2010

    • Author(s)
      K. Shimura, T. Yoshida, H. Yoshida
    • Journal Title

      J. Phys. Chem. C

      Volume: 114 Issue: 26 Pages: 11466-11474

    • DOI

      10.1021/jp1012126

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Preparation of gallium oxide photocatalysts for reduction of carbon dioxide2010

    • Author(s)
      H. Yoshida, K. Maeda
    • Journal Title

      Stud. Surf. Sci. Catal

      Volume: 175 Pages: 351-354

    • DOI

      10.1016/s0167-2991(10)75058-8

    • ISBN
      9780444536013
    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Preparation of calcium titanate photocatalysts for hydrogen production2010

    • Author(s)
      K. Shimura, H. Miyanaga, H. Yoshida
    • Journal Title

      Stud. Surf. Sci. Catal

      Volume: 175 Pages: 85-92

    • DOI

      10.1016/s0167-2991(10)75011-4

    • ISBN
      9780444536013
    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen production from water and methane over Pt-loaded calcium titanate photocatalyst2010

    • Author(s)
      K. Shimura, H. Yoshida
    • Journal Title

      Energy Environ. Sci

      Volume: 3 Issue: 5 Pages: 615-617

    • DOI

      10.1039/b922793h

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photocatalytic steam reforming of methane over sodium tantalate2010

    • Author(s)
      K. Shimura, S. Kato, T. Yoshida, H. Itoh, T. Hattori, H. Yoshida
    • Journal Title

      J. Phys. Chem. C

      Volume: 114 Issue: 8 Pages: 3493-3503

    • DOI

      10.1021/jp902761x

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen production from water and methane over Pt-loaded calcium titanate photocatalyst2010

    • Author(s)
      K Shimura, H Yosbida
    • Journal Title

      Energy Environ Sci

      Volume: 3 Pages: 615-617

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photocatalytic activation of water and methane over modified gallium oxide for hydrogen production2010

    • Author(s)
      K Shimura, T Yoshida, H Yoshida
    • Journal Title

      J.Phys Chem.C

      Volume: 114 Pages: 1146-11474

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photocatalytic steam reforming of methane over sodium tantalate2010

    • Author(s)
      K.Shimura, S.Kato, T.Yoshida, H.Itoh, T.Hattori, H.Yoshida
    • Journal Title

      J. Phys. Chem. C 114

      Pages: 3493-3503

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] チタン酸カリウム光触媒上のRh助触媒の構造解析2011

    • Author(s)
      吉田寿雄,志村勝也,吉田朋子
    • Organizer
      第14回XAFS討論会
    • Place of Presentation
      岡崎コンファレンスセンター(愛知県)
    • Year and Date
      2011-09-10
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] チタン酸カリウム光触媒上のRh助触媒の構造解析2011

    • Author(s)
      吉田寿雄,志村勝也,吉田朋子
    • Organizer
      第28回PFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県)
    • Year and Date
      2011-07-12
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] 常温メタン水蒸気改質反応に高活性なRh添加チタン酸カリウム光触媒2011

    • Author(s)
      吉田寿雄・志村勝也・吉田朋子
    • Organizer
      第30回光がかかわる触媒化学シンポジウム
    • Place of Presentation
      東京工業大学(東京都)
    • Year and Date
      2011-06-10
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] チタン酸塩を光触媒に用いた光触媒的水蒸気分解反応2011

    • Author(s)
      手島智輝,吉田寿雄
    • Organizer
      第11回グリーン・サステイナブルケミストリーシンポジウム
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2011-06-02
    • Related Report
      2011 Final Research Report
  • [Presentation] チタン酸塩を光触媒に用いた光触媒的水蒸気分解反応2011

    • Author(s)
      手島智輝, 吉田寿雄
    • Organizer
      第11回グリーン・サステイナブル ケミストリーシンポジウム
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2011-06-02
    • Related Report
      2011 Annual Research Report
  • [Presentation] Photo catalytic steam reforming of methane over Rh-loaded potassium titanate2010

    • Author(s)
      K. Shimura, M. Kawai, H. Yoshida
    • Organizer
      2010 International Chemical Congress of Pacific Basin Societies(PACIFICHEM 2010)
    • Place of Presentation
      Hawaii Convention Center, Honolulu, Hawaii, USA
    • Year and Date
      2010-12-16
    • Related Report
      2011 Final Research Report
  • [Presentation] Photocatalytic steam reforming of methane over Rh loaded potassium titanate2010

    • Author(s)
      K Shimura, M Kawai, H Yoshida
    • Organizer
      2010 International Chemicai Congress of Pacific Basin Societies (PACIFICHEM 2010)
    • Place of Presentation
      Hawaii Convention Center, Honolulu, Hawaii, USA
    • Year and Date
      2010-12-16
    • Related Report
      2010 Annual Research Report
  • [Presentation] Rh添加チタン酸カリウム光触媒によるメタン水蒸気改質反応2010

    • Author(s)
      志村勝也,河合宏将,吉田寿雄
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      山梨大学(山梨県)
    • Year and Date
      2010-09-17
    • Related Report
      2011 Final Research Report
  • [Presentation] Rh添加チタン酸カリウム光触媒によるメタン水蒸気改質反応2010

    • Author(s)
      志村勝也, 河合宏将, 吉田寿雄
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      山梨大学
    • Year and Date
      2010-09-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] Preparation of calcium titanate photo catalysts for hydrogen production2010

    • Author(s)
      K. Shimura, H. Miyanaga, H. Yoshida
    • Organizer
      10th International Symposium"Scientific Bases for the Preparation of Heterogeneous Catalysts"(PREPA10)
    • Place of Presentation
      Louvain-la-Neuve, Belgium
    • Year and Date
      2010-07-13
    • Related Report
      2011 Final Research Report
  • [Presentation] Preparation of calcium titanate photocatalysts for hydrogen production2010

    • Author(s)
      K Shimura, H Miyanaga, H Yoshida
    • Organizer
      10th International Symposium "Scientific Bases for the Preparatlon of Heterogeneous Catalysts' (PREPA10)
    • Place of Presentation
      Louvain la Neuve, Belgium
    • Year and Date
      2010-07-13
    • Related Report
      2010 Annual Research Report
  • [Presentation] 酸化ガリウム光触媒を用いたメタン水蒸気改質における熱的活性化機構2010

    • Author(s)
      志村勝也,吉田寿雄
    • Organizer
      第105回触媒討論会
    • Place of Presentation
      京都テルサ(京都府)
    • Year and Date
      2010-03-25
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] 酸化ガリウム光触媒上のRh助触媒の構造解析2010

    • Author(s)
      吉田寿雄,志村勝也
    • Organizer
      第27回PFシンポジウム
    • Place of Presentation
      つくば国際会議場(茨城県)
    • Year and Date
      2010-03-09
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] 酸化ガリウム光触媒による常温メタン水蒸気改質反応2010

    • Author(s)
      吉田寿雄
    • Organizer
      第8回太陽エネルギー化学研究センターシンポジウム
    • Place of Presentation
      大阪大学(大阪府)
    • Year and Date
      2010-02-03
    • Related Report
      2011 Final Research Report
  • [Presentation] 酸花ガリウム光触媒による常温メタン水蒸気改質反応2010

    • Author(s)
      吉田寿雄
    • Organizer
      第8回太陽エネルギー化学研究センターシンポジウム
    • Place of Presentation
      大阪大学(大阪府)
    • Year and Date
      2010-02-03
    • Related Report
      2009 Annual Research Report
  • [Presentation] Preparation of calcium titanate photo catalyst for hydrogen production from water and methane2009

    • Author(s)
      H. Miyanaga, K. Shimura, H. Yoshida
    • Organizer
      4th Japan-China Workshop on Environmental Catalysis and Eco-Materials
    • Place of Presentation
      名古屋大学(愛知県)
    • Year and Date
      2009-11-05
    • Related Report
      2011 Final Research Report
  • [Presentation] Preparation of calcium titanate photocatalyst for hydrogen production from water and methane2009

    • Author(s)
      H.Miyanaga, K.Shimura, H.Yoshida
    • Organizer
      4th Japan-China Workshop on Environmental Catalysis and Eco-Materials
    • Place of Presentation
      名古屋大学(愛知県)
    • Year and Date
      2009-11-05
    • Related Report
      2009 Annual Research Report
  • [Presentation] 常温メタン水蒸気改質における酸化ガリウム光触媒の活性支配因子2009

    • Author(s)
      志村勝也,吉田朋子,吉田寿雄
    • Organizer
      第104回触媒討論会
    • Place of Presentation
      フェニックスシーガイア・リゾート(宮崎県)
    • Year and Date
      2009-10-28
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] 水からの水素生成反応のためのチタン酸カルシウム光触媒の調製法の検討2009

    • Author(s)
      宮永啓世,志村勝也,吉田寿雄
    • Organizer
      第104回触媒討論会
    • Place of Presentation
      フェニックスシーガイア・リゾート(宮崎県)
    • Year and Date
      2009-10-27
    • Related Report
      2011 Final Research Report 2009 Annual Research Report
  • [Presentation] タンタル酸ナトリウム中にドープされたランタンのXAFSによる局所構造解析2009

    • Author(s)
      吉田寿雄,志村勝也,吉田朋子
    • Organizer
      第12回XAFS討論会
    • Place of Presentation
      おおわに山荘(青森県)
    • Year and Date
      2009-09-15
    • Related Report
      2011 Final Research Report
  • [Presentation] タンタル酸ナトリウム中にドープされたランタンの、XAFSによる局所構造解析2009

    • Author(s)
      吉田寿雄, 志村勝也, 吉田朋子
    • Organizer
      第12回XAFS討論会
    • Place of Presentation
      おおわに山荘(青森県)
    • Year and Date
      2009-09-15
    • Related Report
      2009 Annual Research Report
  • [Book] Photocatalytic hydrogen production from methane and water, Handbook of photocatalysts : preparation, structure and applications2009

    • Author(s)
      Hisao Yoshida
    • Publisher
      Nova Science Publishers
    • Related Report
      2011 Final Research Report
  • [Book] "Handbook of Photocatalysts : Preparation, Structure and Applications" Chapter 20 : Photocatalytic hydrogen production from methane and water2009

    • Author(s)
      Hisao Yoshida
    • Total Pages
      565
    • Publisher
      Nova Science Publishers, Inc.
    • Related Report
      2009 Annual Research Report

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Published: 2009-04-01   Modified: 2016-04-21  

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