Towards the three dimensional structural analysis of liquid by using x-ray free electron laser

• Project/Area Number: 21654050
• Research Category: Grant-in-Aid for Challenging Exploratory Research
• Allocation Type: Single-year Grants
• Research Field: Condensed matter physics II
• Research Institution: Kyoto University
• Principal Investigator: YAO Makoto 京都大学, 大学院・理学研究科, 教授 (70182293)
• Co-Investigator(Kenkyū-buntansha): NAGAYA Kiyonobu 京都大学, 大学院・理学研究科, 助教 (30273436) ; KAWAKITA Yukinobu 日本原子力研究開発機構, J-PARCセンター (50264015)
• Project Period (FY): 2009 – 2011
• Project Status: Completed (Fiscal Year 2011)
• Budget Amount: ¥3,370,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥270,000); Fiscal Year 2011: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000); Fiscal Year 2010: ¥800,000 (Direct Cost: ¥800,000); Fiscal Year 2009: ¥1,400,000 (Direct Cost: ¥1,400,000)
• Keywords: X線自由電子レーザー / ナノ液滴 / 室温イオン液体 / 液体構造解析 / 逆モンテカルロ法 / 自由電子レーザー / 液体の中距離構造 / 極紫外自由電子レーザー / 構造モデリング

Research Abstract

We have developed an experimental apparatus and an analysis method aiming at realization of the three-dimensional structural analysis of the liquid using X-ray free electron laser. We developed an electro-spray ionization apparatus for producing liquid droplet sample for XFEL experiments. We also estimated the sample damage caused by FEL using SCSS test accelerator. A structure analysis method in the real space based on the reverse Monte Carlo method was developed.

Research Products

• [Journal Article] Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser (2011)
  • Author(s): E. V. Gryzlova, Ri Ma, H. Fukuzawa, K. Motomura, A. Yamada, K. Ueda, A. N. Grum-Grzhimailo, N. M. Kabachnik, S. I. Strakhova, A. Rouz´ee, A. Hundermark, M. J. J. Vrakking, P. Johnsson, K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, M. Nagasono, K. Tono, T. Togashi, Y. Senba, H. Ohashi, M. Yabashi, and T. Ishikawa
  • Journal Title: Phys Rev Volume: A84 Pages: 63405-63405
  • Peer Reviewed
• [Journal Article] Second-order autocorrelation of XUV FEL pulses via time resolved two-photon single ionization of He (2011)
  • Author(s): R. Moshammer, Th. Pfeifer, A. Rudenko, Y. H. Jiang, L. Foucar, M. Kurka, K. U. Kuhnel, C. D. Schroter, J. Ullrich, O. Herrwerth, M. F. Kling, X.-J. Liu, K. Motomura, H. Fukuzawa, A. Yamada, K. Ueda, K. L. Ishikawa, K. Nagaya, H. Iwayama, A. Sugishima, Y. Mizoguchi, S. Yase, M. Yao, N. Saito, A. Belkacem, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togash
  • Journal Title: OPTICS EXPRESS Volume: Vol.19, Issue 22 Pages: 21698-21706
  • Peer Reviewed
• [Journal Article] Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser (2011)
  • Author(s): E.V.Gryzlova, M.Yao, 他22名
  • Journal Title: Phys Rev A Volume: 84 Issue: 6 Pages: 63405-63405
  • DOI: 10.1103/physreva.84.063405
  • Peer Reviewed
• [Journal Article] second-order autocorrelation of XUV FEL pulses via time resolved two-photon single ionization of He (2011)
  • Author(s): R.Moshammer, M.Yao, 他30名
  • Journal Title: OPTICS EXPRESS Volume: 19 Issue: 22 Pages: 21698-21706
  • DOI: 10.1364/oe.19.021698
  • Peer Reviewed
• [Journal Article] Metallic-like droplets produced by irradiating rare-gas clusters with free electron laser pulses (2011)
  • Author(s): M.Yao, K.Nagaya, H.Iwayama, H.Fukuzawa, K.Ueda, M.Nagasono, T.Ishikawa
  • Journal Title: Euro.Phys.J., Special Topics "Liquid and Amorphous metals : current trends and future perspectives" Volume: (印刷中)
  • Peer Reviewed
• [Journal Article] Coulomb explosion imaging of bromo-benzene and bromophenol molecules following Br K-shell ionization (2010)
  • Author(s): H Iwayama, K Nagaya, H Murakami, Y Ohmasa, M Yao
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 185207-185207
  • Peer Reviewed
• [Journal Article] Photoelectron spectroscopy of sequential three-photon double ionization of Ar irradiated by EUV free-electron laser pulses (2010)
  • Author(s): H Fukuzawa, E V Gryzlova, K Motomura, A Yamada, K Ueda, A N Grum-Grzhimailo, S I Strakhova, K Nagaya, A Sugishima, Y Mizoguchi, H Iwayama, M Yao, N Saito, P Piseri, T Mazza, M Devetta, M Coreno, M Nagasono, K Tono, M Yabashi, T Ishikawa, H Ohashi, H Kimura, T Togashi and Y Senba
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 111001-111001
  • Peer Reviewed
• [Journal Article] Ion-ion coincidence studies on multiple ionizations of N2 and O2 molecules irradiated by EUV free-electron laser pulses (2010)
  • Author(s): A. Yamada, H. Fukuzawa, K. Motomura, X.-J. Liu, L. Foucar, M. Kurka, M. Okunishi, K. Ueda, N. Saito, H. Iwayama, K. Nagaya, A. Sugishima, H. Murakami, M. Yao, A. Rudenko, K. U. Kuhnel, J. Ullrich, R. Feifel, A. Czasch, R. Dorner, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togashi
  • Journal Title: J. Chem. Phys. Volume: 132 Pages: 204305-204305
  • Peer Reviewed
• [Journal Article] Contact less measurements of charge migration within single molecules (2010)
  • Author(s): K. Nagaya, H. Iwayama, A. Sugishima, Y. Ohmasa, M. Yao
  • Journal Title: App. Phys. Lett. Volume: 96 Pages: 233101-233101
  • Peer Reviewed
• [Journal Article] Inhomogeneous charge redistribution in Xe clusters exposed to intense extreme ultraviolet free electron laser (2010)
  • Author(s): H. Iwayama, A. Sugishima, K. Nagaya, M. Yao, , H. Fukuzawa, K. Motomura, X.-J. Liu, A. Yamada, C. Wang, K. Ueda, N. Saito, M. Nagasono, K. Tono, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura, and T. Togashi
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 43 Pages: 161001-161001
  • Peer Reviewed
• [Journal Article] Coulomb explosion imaging of bromobenzene and bromophenol molecules following Br K-shell ionization (2010)
  • Author(s): H Iwayama, K Nagaya, H Murakami, Y Ohmasa, M Yao
  • Journal Title: J.Phys.B : At.Mol.Opt.Phys. Volume: 43 Issue: 18 Pages: 185207-185207
  • DOI: 10.1088/0953-4075/43/18/185207
  • Peer Reviewed
• [Journal Article] Inhomogeneous charge redistribution in Xe clusters exposed to intense extreme ultraviolet free electron laser (2010)
  • Author(s): H.Iwayama, A.Sugishima, K.Nagaya, M.Yao, et al.
  • Journal Title: J.Phys.B : At.Mol.Opt.Phys.Fast track Volume: 43 Pages: 161001-161001
  • Peer Reviewed
• [Journal Article] Dielectric permittivity of room temperature ionic liquids : A relation to the polar and non-polar domain structures (2010)
  • Author(s): M.Mizoshiri, T.Nagao, Y.Mizoguchi, M.Yao
  • Journal Title: J.Chem.Phys. Volume: 132 Pages: 164510-164510
  • Peer Reviewed
• [Journal Article] Multiple ionization of atomic argon irradiated by EUV free-electron laser pulses at 62 nm : evidence of sequential electron strip (2009)
  • Author(s): K. Motomura, H. Fukuzawa, L. Foucar, X.-J. Liu, G. Prumper, K. Ueda, N. Saito, H. Iwayama, K. Nagaya, H. Murakami, M. Yao, A. Belkacem, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi and H. Kimura
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys Volume: 42 Pages: 221003-221003
  • Peer Reviewed
• [Journal Article] Dissociation dynamics of C6H6 and C6H5F molecules following carbon 1s and fluorine 1s photoionization studied by 3D momentum imaging method (2009)
  • Author(s): K. Nagaya, H. Iwayama, M. Yao, J. Adachi, Y. Kimura, M. Yamazaki, A. Yagishita
  • Journal Title: J. Chem. Phys. Volume: 131 Pages: 114309-114309
  • Peer Reviewed
• [Journal Article] Frustration of direct photoionizations of Ar clusters in intense extreme ultraviolet pulses from a free electron laser (2009)
  • Author(s): K. Nagaya, M. Yao, H. Fukuzawa, X.-J. Liu, G. Prumper, M. Okunishi, K. Shimada, K. Ueda, T. Harada, M. Toyoda, M. Yanagihara, M. Yamamoto, K. Motomura, N. Saito, A. Rudenko, J. Ullrich, L. Foucar, A. Czasch, R. Dorner, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, and H. Kimura
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 42 Pages: 134019-134019
  • Peer Reviewed
• [Journal Article] Frustration of direct photoionizations of Ar clusters in intense extreme ultraviolet pulses from a free electron laser (2009)
  • Author(s): H Iwayama, K Nagaya, M Yao, et al.
  • Journal Title: J.Phys.B :At.Mol.Opt.Phys. 42 Pages: 134019-134019
  • Peer Reviewed
• [Journal Article] Ion momentum spectroscopy on multiple ionization of Xe clusters irradiated by EUV free-electron laser pulses (2009)
  • Author(s): H.Fukuzawa, H.Iwayama, K.Nagaya, M.Yao, K.Motomura, N.Saito, A.Rudenko, J.Ullrich, et al.
  • Journal Title: Physical Review A 79
  • Peer Reviewed
• [Presentation] ネオン・クラスターのEUV-FEL誘起イオン化のクロスオーバー (2012)
  • Author(s): 八瀬哲志、八尾誠, 他20名
  • Organizer: 第25回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 佐賀県鳥栖市民文化会館・中央公民館
  • Year and Date: 2012-01-09
• [Presentation] Brief introduction to the liquid state physics (2011)
  • Author(s): Makoto Yao
  • Organizer: JSPS-DFG Bilateral Seminar
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2011-10-10
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会秋季大会
  • Place of Presentation: 富山大学
  • Year and Date: 2011-09-24
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会 第66回年次大会
  • Place of Presentation: 新潟大学(招待講演)
  • Year and Date: 2011-03-25
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2011)
  • Author(s): K. Nagaya
  • Organizer: International workshop DyNano 2011 Structure and Dynamics of Nano-objects using short wavelength radiation
  • Place of Presentation: Kyoto, Japan
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会第66回年次大会
  • Place of Presentation: 新潟大学
• [Presentation] 動的光散乱法による複雑液体の表面張力波の研究 (2011)
  • Author(s): 大政義典, 八尾誠
  • Organizer: 文部科学省科学特別研究費補助金特定領域研究報告会特定領域研究ソフトマター物理研究会
  • Place of Presentation: 東京大学
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2011)
  • Author(s): Kiyonobu Nagaya
  • Organizer: International workshop DyNano2011
  • Place of Presentation: Kyoto, Japan
• [Presentation] イオン化におけるMore is Different (2010)
  • Author(s): 八尾誠
  • Organizer: Symposium on"Invitation to Integrated Complex System Sciences"
  • Place of Presentation: 京都大学理学研究科セミナーハウス
  • Year and Date: 2010-08-05
• [Presentation] Inhomogeneous chemical reaction fields (2010)
  • Author(s): M. Yao
  • Organizer: Workshop of Room Temperature Ionic Liquids in NDA
  • Place of Presentation: 防衛大学
  • Year and Date: 2010-07-21
• [Presentation] Inhomogeneous chemical reaction fields (2010)
  • Author(s): Makoto Yao
  • Organizer: Workshop of Room Temperature Ionic Liquids in NDA
  • Place of Presentation: 防衛大学(招待講演)
  • Year and Date: 2010-07-21
• [Presentation] International workshop DyNano2011" Structure and Dynamics of Nano-objects using short wavelength radiation" (2010)
  • Author(s): K. Nagaya, H. Iwayama and M. Yao, Kyoto U.
  • Organizer: Measurements of charge migration within single molecules using deep inner-core excitation combined with molecular imaging method
  • Place of Presentation: Kyoto, Japan
• [Presentation] Studies on Interaction of Clusters with Intense EUV-FEL Pulses at Spring 8 (2010)
  • Author(s): K. Nagaya
  • Organizer: International conference on many particle spectroscopy of atoms, molecules, clusters and surfaces(MPS2010)
  • Place of Presentation: Sendai, Japan
• [Presentation] Metallic-like droplets produced by irradiating rare-gas clusters with free electron laser pulses (2010)
  • Author(s): Makoto Yao
  • Organizer: 14th International Conference on Liquid and Amorphous Metals
  • Place of Presentation: Italy, Roma
• [Presentation] Self-organized charge redistribution in pure and mixed rare-gas clusters (2010)
  • Author(s): Makoto YAO
  • Organizer: International Workshop(DyNano-2010): Structure and Dynamics of Nano-objects using short wavelength radiation
  • Place of Presentation: France, Corsica
• [Presentation] Studies on Interaction of Clusters with Intense EUV-FEL Pulses at SPring8 (2010)
  • Author(s): Kiyonobu Nagaya
  • Organizer: International conference on many particle spectroscopy of atoms, molecules, clusters and surfaces
  • Place of Presentation: 仙台市(招待講演)
• [Presentation] ドメイン構造を有する室温イオン液体の誘電的性質 (2009)
  • Author(s): 溝尻誠, 長尾武奈, 溝口悠里, 八尾誠
  • Organizer: 日本物理学会 2009年秋季大会
  • Place of Presentation: 熊本大学 黒髪キャンパス
  • Year and Date: 2009-09-28
• [Presentation] INFLUENCES OF DOMAIN STRUCTURES ON THE BULK AND SURFACE DYNAMICS OF ROOM TEMPERATURE IONIC LIQUIDS (2009)
  • Author(s): 八尾誠
  • Organizer: 6th International Discussion Meeting on Relaxations in Complex Systems
  • Place of Presentation: ローマ大学 (イタリア)
  • Year and Date: 2009-08-31
• [Presentation] Cluster experiments at SCSS : present status and perspective
  • Author(s): K. Nagaya, Kyoto U.
  • Organizer: JSPS-DFG Bilateral Seminar
  • Place of Presentation: Kyoto, Japan
• [Book] 基礎物理学シリーズ11 現代物理学の世界 トップ研究者からのメッセージ12章 不規則系物理学 (2010)
  • Author(s): 八尾誠
  • Total Pages: 11
  • Publisher: 講談社