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Uptake of trace gas by tropospheric aerosol particles

Research Project

Project/Area Number 21710025
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Environmental dynamic analysis
Research InstitutionJapan Agency for Marine-Earth Science and Technology

Principal Investigator

TAKETANI Fumikazu  独立行政法人海洋研究開発機構, 地球環境変動領域, 研究員 (50377785)

Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2011: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2010: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2009: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Keywords不均一反応 / HO2ラジカル / エアロゾル粒子 / 取り込み係数 / 全球モデル / レーザー誘起蛍光法 / 湿度依存
Research Abstract

Uptake coefficients of HO2 radical with levoglucosan and dicarboxylic acids particles were measured. The results have the relative humidity dependence of determined uptake coefficients, suggesting water complex contribution for heterogeneous loss of HO2.We also carried out global chemical modeling using uptake coefficients of HO2 we have determined. Results suggested the potential importance of the heterogeneous reactions of HO2 radicals with aerosol particles in the areas with high aerosol loading for not only HO2 concentration, but other relevant species.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (15 results)

All 2012 2010 2009

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (12 results)

  • [Journal Article] Measurement of overall uptake coefficients for HO2 radicals by aerosol particles sampled from ambient air at Mts.2012

    • Author(s)
      F. Taketani, Y. Kanaya, P. Pochanart, Y. Liu, J. Li, K. Okuzawa, K. Kawamura, Z. Wang, and H. Akimoto
    • Journal Title

      Atmos. Chem. Phys. Discuss

      Volume: 12 Pages: 13787-13812

    • DOI

      10.5194/acpd-12-13787-2012

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Kinetics of HO2 Uptake in Levoglucosan and Polystyrene Latex Particles2010

    • Author(s)
      F. Taketani, Y. Kanaya, H. Akimoto
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 1 Issue: 11 Pages: 1701-1704

    • DOI

      10.1021/jz100478s

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Kinetics of HO2 Uptake in Levoglucosan and Polystyrene Latex Particles2010

    • Author(s)
      F.Taketani
    • Journal Title

      JOURNAL OF PHYSICAL CHEMISTRY LETTERS

      Volume: 1 Pages: 1701-1704

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] 大気エアロゾル粒子を利用したHO2ラジカル取り込み係数の測定2012

    • Author(s)
      竹谷文一、金谷有剛、秋元肇
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      神奈川県(慶応義塾大学)
    • Year and Date
      2012-03-25
    • Related Report
      2011 Final Research Report
  • [Presentation] 大気エアロゾル粒子を利用したHO2ラジカル取り込み係数の測定2012

    • Author(s)
      竹谷文一
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶応義塾大学(神奈川県)
    • Year and Date
      2012-03-25
    • Related Report
      2011 Annual Research Report
  • [Presentation] HO2ラジカルのジカルボン酸エアロゾル粒子との反応性測定2010

    • Author(s)
      竹谷文一、金谷有剛、秋元肇
    • Organizer
      第16回大気化学討論会
    • Place of Presentation
      東京(首都大学東京)
    • Year and Date
      2010-11-17
    • Related Report
      2011 Final Research Report
  • [Presentation] HO2ラジカルのジカルボン酸エアロゾル粒子との反応性測定2010

    • Author(s)
      竹谷文一
    • Organizer
      第16回大気化学討論会
    • Place of Presentation
      首都大学東京
    • Year and Date
      2010-11-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] Measurement of uptake coefficients of HO2 radical by dicarboxylic acid particles2010

    • Author(s)
      F. Taketani, Y. Kanaya, H. Akimoto
    • Organizer
      21st International Symposium Gas Kinetics
    • Place of Presentation
      Belgium(Leuven)
    • Year and Date
      2010-07-20
    • Related Report
      2011 Final Research Report
  • [Presentation] Measurement of uptake coefficients of HO2 radical by dicarboxylic acid partices2010

    • Author(s)
      Fumikazu Taketani
    • Organizer
      21st International Symposium Gas Kinetics
    • Place of Presentation
      Univ.of Leuven, Leuven, Belgium
    • Year and Date
      2010-07-20
    • Related Report
      2010 Annual Research Report
  • [Presentation] Measurement of Uptake Coefficients of HO2 Radical by Levoglucosan Particles2010

    • Author(s)
      竹谷文一、金谷有剛、秋元肇
    • Organizer
      第26回化学反応討論会
    • Place of Presentation
      広島(広島大学)
    • Year and Date
      2010-06-02
    • Related Report
      2011 Final Research Report
  • [Presentation] Measurement of Uptake Coefficients of HO2 Radical by Levoglucosan Particles2010

    • Author(s)
      竹谷文一
    • Organizer
      第26回化学反応討論会
    • Place of Presentation
      広島大学
    • Year and Date
      2010-06-02
    • Related Report
      2010 Annual Research Report
  • [Presentation] レーザー誘起蛍光法を利用したHO2ラジカルの大気エアロゾル粒子による消失過程の解明2009

    • Author(s)
      竹谷文一、金谷有剛、秋元肇
    • Organizer
      第50回大気環境学会
    • Place of Presentation
      神奈川県(慶応義塾大学)
    • Year and Date
      2009-09-16
    • Related Report
      2011 Final Research Report
  • [Presentation] レーザー誘起蛍光法を利用したHO2ラジカルの大気エアロゾル粒子による消失過程の解明2009

    • Author(s)
      竹谷文一
    • Organizer
      第50回大気環境学会
    • Place of Presentation
      横浜慶応大学
    • Year and Date
      2009-09-16
    • Related Report
      2009 Annual Research Report
  • [Presentation] Heterogeneous interaction of HO2 radicals with submicron aerosol particles2009

    • Author(s)
      F. Taketani, Y. Kanaya, H. Akimoto
    • Organizer
      The 30th International Symposium
    • Place of Presentation
      フィンランド(Wanha Kasino)
    • Year and Date
      2009-07-26
    • Related Report
      2011 Final Research Report
  • [Presentation] Heterogeneous interaction of HO2 radicals with submicron aerosol particles2009

    • Author(s)
      Fumikazu Taketani
    • Organizer
      The 30^<th> International Symposium on Free Radicals
    • Place of Presentation
      フィンランドWanha Kasino
    • Year and Date
      2009-07-26
    • Related Report
      2009 Annual Research Report

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Published: 2009-04-01   Modified: 2016-04-21  

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