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Development and Microscopic magnetic characterization of actinide layered compounds

Research Project

Project/Area Number 21750067
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Inorganic chemistry
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

SAKAI Hironori  独立行政法人日本原子力研究開発機構, 先端基礎研究センター, 研究員 (80370401)

Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2011: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2010: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2009: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Keywords無機固体化学 / アクチノイド化合物 / ランタノイド化合物 / 層状化合物 / 核磁気共鳴
Research Abstract

Single crystals of actinide layered compounds ThCuPO and UCuPO have been successfully grown by the chemical transport method. Using these single crystals, the crystal structures and chemical compositions have been evaluated. The measurements of resistivity, specific heat, and magnetization for UCuPO have revealed that the strong magnetic anisotropy causes from the localized 5f electrons of uranium and the metallic conductivity occurs mainly owing to the layers of copper and phosphorus. For comparison, the microscopic magnetism has been investigated in the strongly correlated electron systems CeCoIn_5(superconductor), CePt_2In_7(antiferromagnet), etc. by means of nuclear magnetic resonance technique.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (23 results)

All 2011 2010 2009 Other

All Journal Article (10 results) (of which Peer Reviewed: 10 results) Presentation (10 results) Remarks (3 results)

  • [Journal Article] Magnetic-Field-Induced Enhancements of Nuclear Spin-Lattice Relaxation Rates in the Heavy-Fermion Superconductor CeCoIn5 Using 59Co Nuclear Magnetic Resonance2011

    • Author(s)
      H. Sakai, S. E. Brown, S.-H. Baek, F. Ronning, E. D. Bauer and J. D. Thompson
    • Journal Title

      Physical Review Letters

      Volume: 107 Issue: 13

    • DOI

      10.1103/physrevlett.107.137001

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Stabilization of commensurate antiferromagnetism in CePt_2In_7 by pressure up to 2.4GPa.-^<115>In-NMR spectral study under zero field2011

    • Author(s)
      H.Sakai, S.Kambe, 他7名
    • Journal Title

      Phys.Rev.B

      Volume: 83 Issue: 14 Pages: 140408-140408

    • DOI

      10.1103/physrevb.83.140408

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropy of antiferromagnetic spin fluctuations in the heavy fermion superconductors of CeMIn_5 and PuMGa_5(M=Co, Rh)2010

    • Author(s)
      H. Sakai, S. Kambe, Y. Tokunaga, Y. Haga, S.-H. Baek, F. Ronning, E. D. Bauer and J. D. Thompson
    • Journal Title

      Mater. Res. Soc. Symp. Proc.

      Volume: 1264 Pages: 69-79

    • URL

      http://dx.doi.org/10.1557/PROC-1264-Z12-01

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic Spin Fluctuations and Superconductivity in "115" Heavy Fermion Compounds : C^^<59> o NMR Study in PuCoGa_52010

    • Author(s)
      S.-H. Baek, H. Sakai, E. D. Bauer, J. N. Mitchell, J. A. Kennison, F. Ronning and J. D. Thompson
    • Journal Title

      Physical Review Letters

      Volume: 105 Issue: 21

    • DOI

      10.1103/physrevlett.105.217002

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Crystal Structure and Physical Properties of Uranium. Copper Oxyphosphide UCuPO2010

    • Author(s)
      H. Sakai, N. Tateiwa, T. D. Matsuda, T. Sugai, E. Yamamoto and Y. Haga
    • Journal Title

      Journal of Physical Society of Japan

      Volume: 79 Issue: 7 Pages: 74721-74721

    • DOI

      10.1143/jpsj.79.074721

    • NAID

      40017205475

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Crystal Structure and Physical Properties of Uranium-Copper Oxyphosphide UCuPO2010

    • Author(s)
      Hironori Sakai, et al.
    • Journal Title

      Journal of Physical Society of Japan

      Volume: 79

    • NAID

      40017205475

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic Spin Fluctuations and Superconductivity in "115" Heavy Fermion Compounds : ^<59>Co NMR Study in PuCoGa_52010

    • Author(s)
      Seung-Ho Baek, et al.
    • Journal Title

      Physical Review Letters

      Volume: 105

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fully Gapped Superconductivity in {Ni}-Pnictide Superconductors BaNi_2As_2 and SrNi_2P_22010

    • Author(s)
      Nobuyuki Kurita, et al.
    • Journal Title

      Journal of Physics : Conference Series

      Volume: 273

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Possible Existence of Magnetic Polaron in Nearly Ferromagnetic Semiconductor &beta;-US<SUB>2</SUB>2009

    • Author(s)
      S. Ikeda, H. Sakai, N. Tateiwa, T. D. Matsuda, D. Aoki, Y. Homma, E. Yamamoto, A. Nakamura, Y. Shiokawa, Y. Ota, K. Sugiyama, M. Hagiwara, K. Kindo, K. Matsubayashi, M. Hedo, Y. Uwatoko, Y. Haga and Y. Onuki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 78 Issue: 11 Pages: 114704-114704

    • DOI

      10.1143/jpsj.78.114704

    • NAID

      130005437242

    • ISSN
      0031-9015, 1347-4073
    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Possible Existence of Magnetic Polaron in Nearly Ferromagnetic Semiconductor β-US□2009

    • Author(s)
      Shugo Ikeda et al.
    • Journal Title

      Journal of Physical Society of Japan 78

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] Anisotropic Spin Fluctuations in the Heavy Fermion Systems : Nuclear Magnetic Resonance Study2011

    • Author(s)
      H. Sakai, H. Chudo, Y. Tokunaga, S. Kambe, Y. Haga, F. Ronning, E. D. Bauer, J. D. Thompson, Y. Homma, D. Aoki, Y. Nakano, F. Honda, R. Settai, Y. Onuki
    • Organizer
      TOKIMEKI2011 International Workshop on Heavy Fermions
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2011-11-24
    • Related Report
      2011 Final Research Report
  • [Presentation] Anisotropy of Spin Fluctuations in the Heavy Fermion Systems : Nuclear Magnetic Resonance Study2011

    • Author(s)
      Hironori Sakai, et al
    • Organizer
      TOKIMEKI2011 International Workshop on Heavy Fermions
    • Place of Presentation
      Osaka Univ., Japan(招待講演)
    • Year and Date
      2011-11-24
    • Related Report
      2011 Annual Research Report
  • [Presentation] 反強磁性体CePt_2In_7における単結晶試料を用いたNQR/NMR研究2011

    • Author(s)
      酒井宏典、徳永陽、神戸振作、H.-O. Lee、V. A. Sidorov、P. H. Tobash、F. Ronning、E. D. Bauer、J. D. Thompson
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-21
    • Related Report
      2011 Final Research Report
  • [Presentation] 反強磁性体CePt_2In_7における単結晶試料を用いたNQR/NMR研究(II)2011

    • Author(s)
      酒井宏典, 他
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-21
    • Related Report
      2011 Annual Research Report
  • [Presentation] ウラン元素を含むオキシニクタイドUCuPOの単結晶育成と物性2010

    • Author(s)
      酒井宏典、立岩尚之、松田達磨、菅井孝志、山本悦嗣、芳賀芳範
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-26
    • Related Report
      2011 Final Research Report
  • [Presentation] ウラン元素を含むオキシニクタイトUCuPOの単結晶育成と物性2010

    • Author(s)
      酒井宏典, 他
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] d波超伝導体CeCoIn_5におけるスピン揺らぎの異方性と関連物質の比較2010

    • Author(s)
      酒井宏典、徳永陽、神戸振作、芳賀芳範、S.-H. Baek、S. E. Brown、F. Ronning、E. D. Bauer、J. D. Thompson
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-24
    • Related Report
      2011 Final Research Report
  • [Presentation] d波超伝導体CeCoIn_5におけるスピン揺らぎの異方性と関連物質との比較2010

    • Author(s)
      酒井宏典, 他
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-24
    • Related Report
      2010 Annual Research Report
  • [Presentation] Anisotropy of antiferromagnetic spin fluctuations in the heavy fermion superconductors of CeMIn_5 and PuMGa_5(M=Co, Rh)2010

    • Author(s)
      H. Sakai, S. Kambe, Y. Tokunaga, Y. Haga, S.-H. Baek, F. Ronning, E. D. Bauer and J. D. Thompson
    • Organizer
      MRS Spring Meeting
    • Place of Presentation
      San Francisco, USA
    • Year and Date
      2010-04-09
    • Related Report
      2011 Final Research Report
  • [Presentation] Anisotropy of Antiferromagnetic Spin Fluctuations in the Heavy Fermion Superconductors of CeMIn_5 and PuMGa_5 (M=Co, Rh)2010

    • Author(s)
      Hironori Sakai, et al.
    • Organizer
      2010 MRS Spring Meeting
    • Place of Presentation
      San Francisco, USA(招待講演)
    • Year and Date
      2010-04-09
    • Related Report
      2010 Annual Research Report
  • [Remarks] ホームページ等(プレス発表)

    • URL

      http://www.jaea.go.jp/02/press2011/p11091501/index.html

    • Related Report
      2011 Final Research Report
  • [Remarks] ホームページ等(所属機関・研究グループホームページ)

    • URL

      http://asrc.jaea.go.jp/soshiki/gr/kambe-gr/index.html

    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://www.jaea.go.jp/02/press2011/p11091501/index.html

    • Related Report
      2011 Annual Research Report

URL: 

Published: 2009-04-01   Modified: 2016-04-21  

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