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Hydrogen diffusion mechanism in ultra-thin Pd alloys by torsional oscillator

Research Project

Project/Area Number 21760025
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionTokyo Institute of Technology

Principal Investigator

AOKI Yuki  東京工業大学, 大学院・総合理工学研究科, 助教 (60514271)

Project Period (FY) 2009 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2011: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2010: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2009: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywords水素 / シリコン基板 / 透過 / 超薄膜 / 界面 / 吸着 / 拡散 / パラジウム / 昇温脱離 / 銀 / シリコン / 銀薄膜
Research Abstract

The technological innovation for improvement of the hydrogen storage efficiency is expected. In the viewpoint of the hydrogen absorption in the atomic level, the hydrogen molecule dissociatively adsorbs at the Pd top surface. Subsequently, the hydrogen atom diffuses into the bulk. During the diffusing process toward the bulk, the atomic hydrogen goes through the very near surface region, whose potential energy is drastically different than that of the bulk. Though this very near surface region is very narrow as 1 or 2 atom layers, every hydrogen atom stores into the bulk or releases to the vacuum via this region. Therefore, the investigation of the hydrogen adsorption or desorption mechanism at this peculiar very near surface region is a key for improvement of the hydrogen storage efficiency. This study focuses to the hydrogen adsorption or desorption mechanism at the very near surface region.

Report

(4 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (38 results)

All 2012 2011 2010 2009 Other

All Journal Article (19 results) (of which Peer Reviewed: 2 results) Presentation (18 results) Remarks (1 results)

  • [Journal Article] Quantum Interference of Rashba-type Spin-split Surface State Electrons2011

    • Author(s)
      H. Hirayama, Y. Aoki, and C. Kato
    • Journal Title

      Phys. Rev. Lett.

      Volume: 107

    • Related Report
      2011 Final Research Report
  • [Journal Article] Hydrogen chemisorption on Si(111)√<3>×√<3> R30-B passivated surface studied by thermal desorption and scanning tunneling microscopy2011

    • Author(s)
      Y. Aoki and H. Hirayama
    • Journal Title

      Surf. Sci.

      Volume: 605 Pages: 1394-1398

    • Related Report
      2011 Final Research Report
  • [Journal Article] Surface Majorana Cone of the Superfluid^3<He> B Phase2011

    • Author(s)
      S. Murakawa, Y. Wada, Y. Tamura, M. Wasai, M. Saitoh, Y. Aoki, R. Nomura, Y. Okuda, Y. Nagato, M. Yamamoto, S. Higashitani, and K. Nagai
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 80 Pages: 13602-13602

    • Related Report
      2011 Final Research Report
  • [Journal Article] Surface Andreev Bound States of the Superfluid^3<He> B Phase2011

    • Author(s)
      R. Nomura, S. Murakawa, Y. Wada, Y. Tamura, M. Wasai, K. Akiyama, M. Saitoh, Y. Aoki and Y. Okuda
    • Journal Title

      Physica E

      Volume: 43 Pages: 718-721

    • Related Report
      2011 Final Research Report
  • [Journal Article] Scanning Tunneling Microscope of Bi-induced Ag(111) Surface Structures2010

    • Author(s)
      C. Kato, Y. Aoki, and H. Hirayama
    • Journal Title

      Phys. Rev. B

      Volume: 82

    • Related Report
      2011 Final Research Report
  • [Journal Article] Spin Fluid Dynamics Observed by Magnetic Fountain Effect and Mechanical spin pumping effect in the ferromagnetic superfluid^3<He> A_1 Phase2010

    • Author(s)
      Y. Aoki, A. Yamaguchi, K. Suzuki, H. Ishimoto and H. Kojima
    • Journal Title

      Phys. Rev.

      Volume: 82

    • Related Report
      2011 Final Research Report
  • [Journal Article] H adsorption at Ag/Si interfaces in epitaxially grown Ag(111) films on Si(111) 7×7 substrates2010

    • Author(s)
      Y. Aoki, L. Shin, T. Sugimoto, H. Hirayama
    • Journal Title

      Surf. Sci.

      Volume: 604 Pages: 420-423

    • Related Report
      2011 Final Research Report
  • [Journal Article] Superfluid transition of a^4<He> thin film pressurized by bulk liquid^3<He>2010

    • Author(s)
      M. Wasai, S. Murakawa, Y. Tamura, Y. Wada, Y. Aoki, R. Nomura, and Y. Okuda
    • Journal Title

      J. Low Temp. Phys.

      Volume: 158 Pages: 268-274

    • Related Report
      2011 Final Research Report
  • [Journal Article] Transverse acoustic impedance measurements for surface states of superfluid^3<He> A_1 and A_2 phases2010

    • Author(s)
      S. Murakawa, A. Yamaguchi, M. Arai. M. Wasai, Y. Aoki, H. Ishimoto, R. Nomura, and Y. Okuda
    • Journal Title

      J. Low Temp. Phys.

      Volume: 158 Pages: 141-146

    • Related Report
      2011 Final Research Report
  • [Journal Article] Observations on Non-Classical Behavior of Solid^4<He> with Compound Torsional Oscillator2010

    • Author(s)
      M. C. Keiderling, Y. Aoki, and H. Kojima
    • Journal Title

      25^<th> International Conference on Low Temperature Physics(LT25), J. Phys.: Conf. Ser.

      Volume: 150 Pages: 32040-32040

    • Related Report
      2011 Final Research Report
  • [Journal Article] Scanning Tunneling Microscope of Bi-induced Ag(111) Surface Structures2010

    • Author(s)
      C.Kato, Y.Aoki, H.Hirayama
    • Journal Title

      Physical Review B

      Volume: 82

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] H adsorption at Ag/Si interfaces in epitaxially grown Ag(111)films on Si(111)7x7 substrates2010

    • Author(s)
      Yuki Aoki, Lin Shi, Tadashi Sugimoto, Hiroyuki Hirayama
    • Journal Title

      Surface Science 604

      Pages: 420-423

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dislocation-induced Local Modulation of the Surface States of Ag(111) Thin Films on Si(111) 7×7 Substrates2009

    • Author(s)
      K. Sawa, Y. Aoki, and H. Hirayama
    • Journal Title

      Phys. Rev. Lett.

      Volume: 104

    • Related Report
      2011 Final Research Report
  • [Journal Article] New Anomaly in the Transverse Acoustic Impedance of Superfluid^3<He>-B with a Wall Coated by Several Layers of^4<He>2009

    • Author(s)
      S. Murakawa, Y. Tamura, Y. Wada, M. Wasai, M. Saitoh, Y. Aoki, R. Nomura, Y. Okuda, Y. Nagato, M. Yamamoto, S. Higashitani and K. Nagai
    • Journal Title

      Phys. Rev. Lett.

      Volume: 103

    • Related Report
      2011 Final Research Report
  • [Journal Article] Hydrogen desorption from 6H-SiC(0001) surfaces during graphitization2009

    • Author(s)
      Y. Aoki and H. Hirayama
    • Journal Title

      Appl. Phys. Lett.

      Volume: 95

    • NAID

      130004674169

    • Related Report
      2011 Final Research Report
  • [Journal Article] Spin pump for boosting spin polarization of superfluid^3<He> A_1 phase2009

    • Author(s)
      A. Yamaguchi, Y. Aoki, S. Murakawa, H. Ishimoto, and H. Kojima
    • Journal Title

      Phys. Rev. B

      Volume: 80

    • Related Report
      2011 Final Research Report
  • [Journal Article] Thickness Dependence of Shockley-type Surface States of Ag(111) Ultra-thin Films on Si(111) 7×7 Substrates2009

    • Author(s)
      K. Sawa, Y. Aoki, and H. Hirayama
    • Journal Title

      Phys. Rev. B

      Volume: 80 Pages: 35428-35428

    • Related Report
      2011 Final Research Report
  • [Journal Article] Magnetically induced spin flow and relaxation in superfluid^3<He> A_1"25^<th> International Conference on Low Temperature Physics(LT25)2009

    • Author(s)
      A. Yamaguchi, Y. Aoki, K. Suzuki, H. Ishimoto, and H. Kojima
    • Journal Title

      J. Phys.: Conf. Ser.

      Volume: 150 Pages: 32122-32122

    • Related Report
      2011 Final Research Report
  • [Journal Article] Transverse Acoustic Impedance of Normal Liquid^3<He> with^4<He> Coating"25^<th> International Conference on Low Temperature Physics(LT25)2009

    • Author(s)
      Y. Tamura, S. Murakawa, Y. Wada, M. Wasai, M. Saitoh, Y. Aoki, R. Nomura, and Y. Okuda
    • Journal Title

      J. Phys.: Conf. Ser.

      Volume: 150 Pages: 320106-320106

    • Related Report
      2011 Final Research Report
  • [Presentation] Ag(111)/Si(111)表面上にエピタキシャル成長させたPd(111)超薄膜における水素吸着2012

    • Author(s)
      中島翔、青木悠樹、平山博之
    • Organizer
      第67回日本物理学会年次大会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-25
    • Related Report
      2011 Annual Research Report
  • [Presentation] Pd(111)/Ag(111)/Si(111)における水素昇温脱離2012

    • Author(s)
      青木悠樹、中島翔、平山博之
    • Organizer
      第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] Hydrogen chemisorption on Si(111)√<3>×√<3> R30°-B passivated surface2011

    • Author(s)
      Y. Aoki, and H. Hirayama
    • Organizer
      The 6th International Symposium on Surface Science(ISSS6)
    • Place of Presentation
      Tokyo, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] エピタキシャルグラフェン成長過程に及ぼすB原子の影響2011

    • Author(s)
      青木悠樹、小此木佑太、平山博之
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学
    • Related Report
      2011 Final Research Report
  • [Presentation] Ag/Si(111)7x7表面のAg/Si境界面に吸着した水素2010

    • Author(s)
      石林
    • Organizer
      第57回応用物理学関係連合講演会
    • Place of Presentation
      東海大学
    • Year and Date
      2010-03-18
    • Related Report
      2009 Annual Research Report
  • [Presentation] Ag/Si(111)√<3>×√<3> R30°-B界面における水素吸着2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      大阪府立大学
    • Related Report
      2011 Final Research Report
  • [Presentation] Si(111)√<3>×√<3> R30°-B表面における水素吸着2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      第71回応用物理学学術講演会
    • Place of Presentation
      長崎大学
    • Related Report
      2011 Final Research Report
  • [Presentation] H thermal desorption at Ag/Si(111)√<3>×√<3> R30°-B surface2010

    • Author(s)
      Y. Aoki, and H. Hirayama
    • Organizer
      18th International Vacuum Congress(IVC-18)
    • Place of Presentation
      Beijing, China
    • Related Report
      2011 Final Research Report
  • [Presentation] 水素吸着したSi(111)√<3>×√<3>-B表面における昇温脱離測定とSTM観察2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      日本物理学会第66回年次大会
    • Place of Presentation
      新潟大学
    • Related Report
      2011 Final Research Report
  • [Presentation] H thermal desorption Ag/Si(111)√<3x>√<3>R30°-B surface2010

    • Author(s)
      Y.Aoki, H.Hirayama
    • Organizer
      18^<th> International Vacuum Congress (IVC-18)
    • Place of Presentation
      Beijing, China
    • Related Report
      2010 Annual Research Report
  • [Presentation] 水素吸着したSi(111)√<3x>√<3>-B表面における昇温脱離測定とSTM観察2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      日本物理学会第66回年次大会
    • Place of Presentation
      新潟大学
    • Related Report
      2010 Annual Research Report
  • [Presentation] Ag/Si(111)√<3x>√<3>R30°-B表面における水素吸着2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      大阪府立大学
    • Related Report
      2010 Annual Research Report
  • [Presentation] Si(111)√<3x>√<3>R30°-B表面における水素吸着2010

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      第71回応用物理学学術講演会
    • Place of Presentation
      長崎大学
    • Related Report
      2010 Annual Research Report
  • [Presentation] Hydrogen desorption from ultra-thin Ag films on Si(111)substrates2009

    • Author(s)
      Yuki Aoki
    • Organizer
      The 10^<th> International Conference on Atomically Controlled Surfaces, Interface, and Nanostructures
    • Place of Presentation
      Granada, Spain
    • Year and Date
      2009-09-22
    • Related Report
      2009 Annual Research Report
  • [Presentation] Ag/Si(111)表面と水素原子の相互作用2009

    • Author(s)
      石林
    • Organizer
      第70回応用物理学学術講演会
    • Place of Presentation
      富山大学
    • Year and Date
      2009-09-09
    • Related Report
      2009 Annual Research Report
  • [Presentation] 6H-SiC(0001)再構成表面における水素脱離特性2009

    • Author(s)
      青木悠樹、平山博之
    • Organizer
      日本物理学会第64回年次大会
    • Place of Presentation
      熊本大学
    • Related Report
      2011 Final Research Report
  • [Presentation] Hydrogen desorption fromultra-thin Ag films on Si(111) substrates2009

    • Author(s)
      Y. Aoki, T. Sugimoto, L. Shi, and H. Hirayama
    • Organizer
      The 10th International Conference on Atomically Controlled Surfaces
    • Place of Presentation
      Granada, Spain
    • Related Report
      2011 Final Research Report
  • [Presentation] Ag/Si(111)上に吸着された水素原子の脱離特性II2009

    • Author(s)
      杉本匡、青木悠樹、平山博之
    • Organizer
      第56回応用物理学関係連合講演会
    • Place of Presentation
      筑波大学
    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://www.materia.titech.ac.jp/~hirayama/2009hirayamalabHP/

    • Related Report
      2011 Final Research Report

URL: 

Published: 2009-04-01   Modified: 2016-04-21  

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