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Elucidation and coherent control of excitonic states of carbon nanotubes

Research Project

Project/Area Number 21760038
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Applied optics/Quantum optical engineering
Research InstitutionKyoto University

Principal Investigator

HIRORI Hideki  Kyoto University, 物質-細胞統合システム拠点, 助教 (00512469)

Project Period (FY) 2009 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2010: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2009: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywords非線形光学 / 応用光学・量子光工学 / 光源技術 / テラヘルツ/赤外材料・素子 / ナノ材料 / 光物性 / テラヘリツ / カーボンナノチューブ / 非線形分光 / 遠赤外分光 / THz分光 / 高強度テラヘルツ / 低次元半導体
Research Abstract

Aim of this study is to elucidate excitonic states of single-walled carbon nanotubes (SWNTs) and to develop coherent control technique with the excitonic states. For this purpose, (1) we established the method to generate single-cycle THz pulses with amplitudes with exceeding 1MV/cm electric field. (2) By developing a THz nonlinear spectroscopic method, we observe excitonic ionization under strong THz pulse with Stark effect and dynamical Frantz-Keldysh effect for both ZnSe and GaAs quantum wells. Furthermore, (3) we demonstrated for the first time that the number of carriers of GaAs quantum wells is enhanced 103 times more by irradiation of the THz pulse, eventually which leading a bright near-infrared luminescence. (4) For study THz response of single SWNTs, we developed the THz near-field microscope. With the developed THz spectroscopic technique we continue the experiment for the THz coherent control of excitonic states.

Report

(3 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • Research Products

    (40 results)

All 2011 2010 2009 Other

All Journal Article (14 results) (of which Peer Reviewed: 14 results) Presentation (18 results) Remarks (2 results) Patent(Industrial Property Rights) (6 results)

  • [Journal Article] Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO32011

    • Author(s)
      広理英基、土井厚志、ブランチャード・フランソワ、田中耕一郎
    • Journal Title

      Applied Physics Letters誌 98巻

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Real-time terahertz near-field microscope2011

    • Author(s)
      ブランチャード・フランソワ、土井厚志、田中智子、広理英基、田中秀明、角屋豊、田中耕一郎
    • Journal Title

      Optics Express誌 19巻

      Pages: 8277-8284

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO_32011

    • Author(s)
      H.Hirori, A.Doi, F.Blanchard, K.Tanaka
    • Journal Title

      App.Phys.Lett

      Volume: 98 Pages: 91106-91108

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Real-time terahertz near-field microscope2011

    • Author(s)
      F.Blanchard, A.Doi, T.Tanaka, H.Hirori, H.Tanaka, Y.Kadoya, K.Tanaka
    • Journal Title

      Opt.Express

      Volume: 19 Pages: 8277-8284

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Excitonic Interactions with Intense Terahertz Pulses in ZnSe/ZnMgSSe Multiple Quantum Wells2010

    • Author(s)
      広理英基、永井正也、田中耕一郎
    • Journal Title

      Physical Review B Rapid Comunications誌 81巻

      Pages: 81305-81308

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dynamical Franz-Keldysh Effect in GaAs/AlGaAs Multiple Quantum Wells Induced by Single-Cycle Terahertz Pulses2010

    • Author(s)
      篠北啓介、広理英基、永井正也、佐藤尚子、角屋豊、田中耕一郎
    • Journal Title

      Applied Physics Letters誌 97巻

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dynamical Franz-Keldysh effect in GaAs/AlGaAs multiple quantum wells induced by single-cycle terahertz pulses2010

    • Author(s)
      K.Shinokita, H.Hirori, M.Nagai, N.Satoh, Y.Kadoya, K.Tanaka
    • Journal Title

      App.Phys.Lett

      Volume: 97 Pages: 211902-211904

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Near-field THz imaging of free induction decay from a tyrosine crystal2010

    • Author(s)
      A.Doi, F.Blanchard, H.Hirori, K.Tanaka
    • Journal Title

      Opt.Express

      Volume: 18 Pages: 18419-18424

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Excitonic Interactions with Intense Terahertz Pulses in ZnSe/ZnMgSSe Multiple Quantum Wells2010

    • Author(s)
      Hideki Hirori, Masaya Nagai, Koichiro Tanaka
    • Journal Title

      Physical Review B誌(Rapid Communications) Vol.81

      Pages: 81305-81308

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Near-field THz imaging of free induction decay from a tyrosine crystal2009

    • Author(s)
      土井厚志、ブランチャード・フランソワ、広理英基、田中耕一郎
    • Journal Title

      Optics Express誌 18巻

      Pages: 18419-18424

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Radiative lifetimes and coherence lengths of one-dimensional excitons in single-walled carbon nanotubes2009

    • Author(s)
      宮内雄平、広理英基、松田一成、金光義彦
    • Journal Title

      Physical Review B Rapid Comunications誌 80巻

    • NAID

      120001682370

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Temporal decoupling of spin and crystallographic phase transitions in Fe (ptz) (6) (BF4) (2)2009

    • Author(s)
      渡邉浩、広理英基、モルナ・ガボア、ブゼク・アゼディン、田中耕一郎
    • Journal Title

      Physical Review B Rapid Comunications誌 79巻

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Radiative lifetimes and coherence lengths of one-dimensional excitons in single-walled carbon nanotubes2009

    • Author(s)
      Yuhei Miyauchi, Hideki Hirori, Kazunari Matsuda, Yoshihiko Kanemitsu
    • Journal Title

      Physical Review B誌(Rapid Communications) Vol.80

      Pages: 81410-81413

    • NAID

      120001682370

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temporal decoupling of spin and crystallographic phase transitions in Fe(ptz)6(BF4)22009

    • Author(s)
      Hiroshi Watanabe, Hideki Hirori, Gabor Molnar, Azzedine Bousseksou, Koichiro Tanaka
    • Journal Title

      Physical Review B誌(Rapid Communications) Vol.79

      Pages: 180405-180408

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] 1MV/cm超の高強度THzパルス照射下での半導体GaAsの光学応答2011

    • Author(s)
      篠北啓介
    • Organizer
      第66回日本物理学会年次大会
    • Place of Presentation
      新潟大学
    • Year and Date
      2011-03-27
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] 高強度テラヘルツ光パルス励起によるGaAs/AlGaAs多重量子井戸からの励起子発光の観測2011

    • Author(s)
      広理英基
    • Organizer
      第58回応用物理学関係連合講演会
    • Place of Presentation
      神奈川工科大学
    • Year and Date
      2011-03-25
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Terahertz nonlinear spectroscopy on single quantum dots2010

    • Author(s)
      広理英基
    • Organizer
      The 8th iCeMS International Synposium "Meso-Control of Functional Architectures"
    • Place of Presentation
      京都大学
    • Year and Date
      2010-11-11
    • Related Report
      2010 Final Research Report
  • [Presentation] Terahertz nonlinear spectroscopy on single quantum dots2010

    • Author(s)
      広理英基
    • Organizer
      The 8th iCeMS International Symposium "Meso-Control of Functional Architectures"
    • Place of Presentation
      京都大学
    • Year and Date
      2010-11-11
    • Related Report
      2010 Annual Research Report
  • [Presentation] Enhancement of THz field in a gap of dipole antenna2010

    • Author(s)
      田中秀明
    • Organizer
      The 35th International Conference on Infrared, Millimeter, and Terahertz Waves
    • Place of Presentation
      ローマ(イタリア)
    • Year and Date
      2010-09-08
    • Related Report
      2010 Final Research Report
  • [Presentation] Enhancement of THz field in a gap of dipole antenna2010

    • Author(s)
      Y.Kadoya
    • Organizer
      The 35^<th> International Conference on Infrared, Millimeter, and Terahertz Waves
    • Place of Presentation
      ローマ,イタリア
    • Year and Date
      2010-09-08
    • Related Report
      2010 Annual Research Report
  • [Presentation] Nonperturbative Excitonic Interaction with Intense THz Pulses in ZnSe/ZnMgSSe Multiple Quantum Wells2010

    • Author(s)
      広理英基
    • Organizer
      The Conference on Lasers and Electro-Optics and The Quantum Electronics and Laser Science conference (CLEO/QELS 2010)
    • Place of Presentation
      サンノゼ(アメリカ)
    • Year and Date
      2010-05-22
    • Related Report
      2010 Final Research Report
  • [Presentation] Nonperturbative Excitonic Interaction with Intense THz Pulses in ZnSe/ZnMgSSe Multiple Quantum Wells2010

    • Author(s)
      H.Hirori
    • Organizer
      The Conference on Lasers and Electro-Optics and The Quantum Electronics and Laser Science conference (CLEO/QELS 2010)
    • Place of Presentation
      サンノゼ,米国
    • Year and Date
      2010-05-22
    • Related Report
      2010 Annual Research Report
  • [Presentation] GaAs/AlGaAs多重量子井戸のテラヘルツ非線形分光2010

    • Author(s)
      篠北啓介、広理英基、角屋豊、田中耕一郎
    • Organizer
      日本物理学会 第65回年次大会
    • Place of Presentation
      岡山大学(岡山県)
    • Year and Date
      2010-03-21
    • Related Report
      2009 Annual Research Report
  • [Presentation] 酸化銅結晶の励起子吸収における高強度THzパルス照射効果2010

    • Author(s)
      広理英基
    • Organizer
      日本物理学会第65回年次大会
    • Place of Presentation
      岡山大学(岡山県)
    • Year and Date
      2010-03-20
    • Related Report
      2010 Final Research Report
  • [Presentation] 酸化銅結晶の励起子吸収における高強度THzパルス照射効果2010

    • Author(s)
      広理英基, 中暢子, 永井正也, 田中耕一郎
    • Organizer
      日本物理学会 第65回年次大会
    • Place of Presentation
      岡山大学(岡山県)
    • Year and Date
      2010-03-20
    • Related Report
      2009 Annual Research Report
  • [Presentation] リアルタイムテラヘルツ近接場顕微鏡の開発2010

    • Author(s)
      広理英基
    • Organizer
      第57回応用物理学関係連合講演会
    • Place of Presentation
      東海大学湘南キャンパス
    • Year and Date
      2010-03-19
    • Related Report
      2010 Final Research Report
  • [Presentation] リアルタイムテラヘルツ近接場顕微鏡の開発2010

    • Author(s)
      広理英基, 土井厚志, 田中耕一郎
    • Organizer
      2010年春季第57回応用物理学関係連合講演会
    • Place of Presentation
      東海大学湘南キャンパス(神奈川県)
    • Year and Date
      2010-03-19
    • Related Report
      2009 Annual Research Report
  • [Presentation] ZnSe/ZnMgSSe多重量子井戸におけるバンド端近傍のTHz非線形光学応答2010

    • Author(s)
      広理英基
    • Organizer
      第57回応用物理学関係連合講演会
    • Place of Presentation
      東海大学湘南キャンパス
    • Year and Date
      2010-03-18
    • Related Report
      2010 Final Research Report
  • [Presentation] ZnSe/ZnMgSSe多重量子井戸におけるバンド端近傍のTHz非線形光学応答2010

    • Author(s)
      広理英基, 永井正也, 田中耕一郎
    • Organizer
      2010年春季第57回応用物理学関係連合講演会
    • Place of Presentation
      東海大学湘南キャンパス(神奈川県)
    • Year and Date
      2010-03-18
    • Related Report
      2009 Annual Research Report
  • [Presentation] Crossover of excitonic interaction with terahertz electric field from perturbative to nonperturbative regime2009

    • Author(s)
      H.Hirori, M.Nagai, K.Tanaka
    • Organizer
      The International Workshop on Terahertz Technology 2009
    • Place of Presentation
      大阪大学中ノ島センター(大阪府)
    • Year and Date
      2009-12-12
    • Related Report
      2009 Annual Research Report
  • [Presentation] GaAs/AlGaAs多重量子井戸のテラヘルツ分光2009

    • Author(s)
      篠北啓介
    • Organizer
      第20回光物性研究会
    • Place of Presentation
      大阪市立大学
    • Year and Date
      2009-12-11
    • Related Report
      2010 Final Research Report
  • [Presentation] GaAs/AlGaAs多重量子井戸のテラヘルツ分光2009

    • Author(s)
      篠北啓介, 広理英基, 永井正也, 佐藤尚子, 角屋豊, 田中耕一郎
    • Organizer
      第20回光物性研究会(2009)
    • Place of Presentation
      大阪市立大学(大阪府)
    • Year and Date
      2009-12-11
    • Related Report
      2009 Annual Research Report
  • [Remarks] 業績論文(1)(Applied Physics Letters誌、査読有、98巻、2011、091106-1-091106-3) Nature Photonics誌に注目論文として採択される[Nature Photonics 5, 250.251(2011)]

    • Related Report
      2010 Final Research Report
  • [Remarks] 業績論文(3)(Physical Review B Rapid Comunications誌、査読有、81巻,2010、81305-081308)編集者の注目論文として採択される(Editor's Suggestion)

    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 観察装置2009

    • Inventor(s)
      雙木満, 土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-09-29
    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 観察方法および観察装置2009

    • Inventor(s)
      土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-08-05
    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 観察方法、入射タイミング設定方法および観察装置2009

    • Inventor(s)
      土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-08-05
    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 観察装置2009

    • Inventor(s)
      雙木満, 土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-09-29
    • Related Report
      2009 Annual Research Report
  • [Patent(Industrial Property Rights)] 観察方法および観察装置2009

    • Inventor(s)
      土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-08-05
    • Related Report
      2009 Annual Research Report
  • [Patent(Industrial Property Rights)] 観察方法、入射タイミング設定方法および観察装置2009

    • Inventor(s)
      土井厚志, 田中耕一郎, 広理英基
    • Industrial Property Rights Holder
      オリンパス株式会社
    • Filing Date
      2009-08-05
    • Related Report
      2009 Annual Research Report

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Published: 2009-04-01   Modified: 2025-06-05  

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