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Accelerated leaching of heavy metals from Landfilled municipal solid waste incineration bottom ash

Research Project

Project/Area Number 21760419
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Civil and environmental engineering
Research InstitutionKyushu University

Principal Investigator

TAKAHASHI Fumitake  Kyushu University, 工学研究院, 助教 (00414376)

Project Period (FY) 2009 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2010: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2009: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywords焼却灰 / 重金属 / 錯体形成 / 溶出 / 廃棄物再資源化 / 廃棄物処理 / 土木環境システム / 環境技術 / 環境調和型都市基盤整備・建築 / 溶出促進
Research Abstract

Assisted leaching mechanisms of heavy metals from landfilled municipal solid waste incineration bottom ash was investigated. Citric acid co-existed with urea had the largest effect on the complexation with heavy metals and promoted the leaching of some elements, in particular chromium, copper, iron, and phosphorus. Although fulvic acid generated in landfill site had great complexation capacity with copper cation, it was two orders of magnitude smaller than that of natural fulvic acid. The combination of pH-dependent leaching tests and sequential extraction tests indicated great difference between geochemical simulation results and leaching test results. This suggested that leaching mechanisms were not controlled by some dominant minerals. In addition, it is also concluded that leaching of heavy metals from bottom ash are very complex mechanisms, which consisted of dissolution, precipitation, and conversions of heavy metals to other geochemical forms during leaching.

Report

(3 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • Research Products

    (35 results)

All 2011 2010 2009 Other

All Journal Article (17 results) (of which Peer Reviewed: 7 results) Presentation (17 results) Remarks (1 results)

  • [Journal Article] Mineralogical characteriza-tion of municipal solid waste incineration bot-tom ash with an emphasis on heavy metal-bearing phases2011

    • Author(s)
      Y.WEI, T.SHIMAOKA, A.SAFFARZADEH, F.TAKAHASHI
    • Journal Title

      Journal of Hazardous Materials Vol.187(1-3)

      Pages: 534-543

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Metal Mobilization From Municipal Solid Wastes Incineration Bottom Ash Through Metal Complexation With Organic And Inorganic Ligands2010

    • Author(s)
      Takahashi Fumitake, Etoh Jiro, Shimaoka Ta-kayuki
    • Journal Title

      Journal of Material Cycles and Waste Management Vol.12(1)

      Pages: 1-9

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Copper complexation by fulvic acid generated in landfilled municipal solid wasete incineration residues2010

    • Author(s)
      F.TAKAHASHI, K.YOKOHATA, T.SHI-MAOKA
    • Journal Title

      Proceedings of Ko-rea-Japan Special Symposium : 14th Ko-rea-Japan Joint International Session, Korea Society of Waste Management

      Pages: 177-179

    • Related Report
      2010 Final Research Report
  • [Journal Article] The Solubility and Chemical Conver-sions of Lead Species in Insoluble Residues of Municipal Solid Waste Incineration Fly Ash During pH-dependent Leaching Test2010

    • Author(s)
      F.TAKAHASHI, T.KANOU, T.SHIMA-OKA
    • Journal Title

      Pro-ceedings of 4th International Conference of East Asia Environment Problems "EAEP2010"

      Pages: 255-260

    • Related Report
      2010 Final Research Report
  • [Journal Article] Weathering of MSWI Bottom Ash With Emphasis on the Evolution of Iron-rich Constituents2010

    • Author(s)
      Y.WEI, T.SHIMAOKA, A.SAF-FARAZADEH, F.TAKAHASHI
    • Journal Title

      Proceed-ings of 4th International Conference of East Asia Environment Problems "EAEP2010"

      Pages: 241-248

    • Related Report
      2010 Final Research Report
  • [Journal Article] Copper Complexation by Fulvic Acid Generated in Landfills from Municipal Solid Waste Incineration Residues2010

    • Author(s)
      K.YOKOHATA, F.TAKAHASHI, T.SHI-MAOKA
    • Journal Title

      Proceed-ings of International Symposium on Earth Science and Technology 2010

      Pages: 145-148

    • Related Report
      2010 Final Research Report
  • [Journal Article] Metal Mobilization From Municipal Solid Wastes Incineration Bottom Ash Through Metal Complexation With Organic And Inorganic Ligands2010

    • Author(s)
      Takahashi Fumitake, Etoh Jiro, Shimaoka Takayuki
    • Journal Title

      Journal of Material Cycles and Waste Management.

      Volume: Vol.12 No.3 Pages: 1-9

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mineralogical characterization of municipal solid waste incineration bottom ash with an emphasis on heavy metal-bearing phases2010

    • Author(s)
      Yunmei WEI, Takayuki SHIMAOKA, Amirhomayoun SAFFARZ ADEH, Fumitake TAKAHASHI
    • Journal Title

      Journal of Hazardous Materials

      Volume: (Accepted)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Copper complexation by fulvic acid generated in landfilled municipal solid wasete incineration residues2010

    • Author(s)
      Fumitake TAKAHASHI, Kazuya YOKOHATA, Takayuki SHIMAOKA
    • Journal Title

      Proceedings of Korea-Japan Special Symposium : 14th Korea-Japan Joint International Session, Korea Society of Waste Management

      Pages: 177-179

    • Related Report
      2010 Annual Research Report
  • [Journal Article] The Solubility and Chemical Conversions of Lead Species in Insoluble Residues of Municipal Solid Waste Incineration Fly Ash During pH-dependent Leaching Test2010

    • Author(s)
      Fumitake TAKAHASHI, Takuma KANOU, Takayuki SHIMAOKA
    • Journal Title

      Proceedings of 4th International Conference of East Asia Environment Problems "EAEP2010"

      Pages: 255-260

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Weathering of MSWI Bottom Ash With Emphasis on the Evolution of Iron-rich Constituents2010

    • Author(s)
      Yunmei WEI, Takayuki SHIMAOKA, Amirhomayoun SAFFARA ZADEH, Fumitake TAKAHASHI
    • Journal Title

      Proceedings of 4th International Conference of East Asia Environment Problems "EAEP2010"

      Pages: 241-248

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Copper Complexation by Fulvic Acid Generated in Landfills from Municipal Solid Waste Incineration Residues2010

    • Author(s)
      Kazuya YOKOHATA, Fumitake TAKAHASHI, Takayuki SHIMAOKA
    • Journal Title

      Proceedings of International Symposium on Earth Science and Technology 2010

      Pages: 145-148

    • Related Report
      2010 Annual Research Report
  • [Journal Article] Metal Mobilization From Municipal Solid Wastes Incineration Bottom Ash Through Metal Complexation With Organic And Inorganic Ligands2010

    • Author(s)
      Takahashi Fumitake, Etoh Jiro, Shimaoka Takayuki
    • Journal Title

      Journal of Material Cycles and Waste Management (Accepted)

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] CO_2 sequestration capacity based on minera-logical composition of MSWI bottom ash and reactivity of Ca-containing minerals2009

    • Author(s)
      Y.WEI, T.SHIMAOKA, F.TAKAHASHI
    • Journal Title

      環境工学研究論文集 Vol.46

      Pages: 407-414

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] The weathe- ring of municipal solid waste incin-eration bottom ash evaluated by some weath-ering indices for natural rock profiles sug-gested in the mineralogy2009

    • Author(s)
      F.TAKAHASHI, T.SHIMAOKA
    • Journal Title

      Proceedings of 3rd International Conference of East Asia Envi-ronment Problems "EAEP2009"

      Pages: 62-68

    • Related Report
      2010 Final Research Report
  • [Journal Article] CO2 sequestration capacity based on mineralogical composition of MSWI bottom ash and reacitivity of Ca-contianing minerals2009

    • Author(s)
      Yunmei WEI, Takayuki SHIMAOKA, Fumitake TAKAHASHI
    • Journal Title

      環境工学研究論文集 46

      Pages: 407-414

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The weathering of municipal solid waste incineration bottom ash evaluated by some weathering indices for natural rock profiles suggested in the mineralogy2009

    • Author(s)
      Fumitake TAKAHASHI, Takayuki SHIMAOKA
    • Journal Title

      Proceedings of 3rd International Conference of East Asia Environment Problems "EAEP2009"

      Pages: 62-68

    • Related Report
      2009 Annual Research Report
  • [Presentation] 粘土鉱物への銅, フルボ酸およびその錯体物の吸着挙動2011

    • Author(s)
      横畑一也, 高橋史武, 島岡隆行
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      福岡
    • Year and Date
      2011-03-05
    • Related Report
      2010 Final Research Report
  • [Presentation] 飛灰中に存在する重金属の抽出に関する一考察2011

    • Author(s)
      村上考輝, 高橋史武, 島岡隆行
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      福岡
    • Year and Date
      2011-03-05
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] 粘土鉱物への銅,フルボ酸およびその錯体物の吸着挙動2011

    • Author(s)
      横畑一也, 高橋史武, 島岡隆行
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      福岡
    • Year and Date
      2011-03-05
    • Related Report
      2010 Annual Research Report
  • [Presentation] Copper Complexation by Fulvic Acid Generated in Landfills from Municipal Solid Waste Incineration Residues2010

    • Author(s)
      K.YOKOHATA, F.TAKAHASHI, T.SHI-MAOKA
    • Organizer
      Interna-tional Symposium on Earth Science and Technology 2010
    • Place of Presentation
      Fukuoka
    • Year and Date
      2010-12-07
    • Related Report
      2010 Final Research Report
  • [Presentation] Copper Complexation by Fulvic Acid Generated in Landfills from Municipal Solid Waste Incineration Residues2010

    • Author(s)
      Kazuya YOKOHATA, Fumitake TAKAHASHI, Takayuki SHIMAOKA
    • Organizer
      International Symposium on Earth Science and Technology 2010
    • Place of Presentation
      Fukuoka
    • Year and Date
      2010-12-07
    • Related Report
      2010 Annual Research Report
  • [Presentation] 重金属と一般廃棄物焼却灰由来の腐植物質の錯体形成2010

    • Author(s)
      横畑一也, 高橋史武, 島岡隆行
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      熊本
    • Year and Date
      2010-03-06
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] 都市ごみ焼却飛灰中の化学形態および溶出のpH依存性に関する基礎研究2010

    • Author(s)
      叶琢磨, 高橋史武, 島岡隆行
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      熊本
    • Year and Date
      2010-03-06
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] 上海市の焼却残渣の基本性状および塩素測定方法の検討2010

    • Author(s)
      久良木暢, 高橋史武, 島岡隆行, 趙由才, 柴暁利
    • Organizer
      土木学会西部支部研究発表会
    • Place of Presentation
      熊本
    • Year and Date
      2010-03-06
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] Copper complexation by fulvic acid generated in landfilled municipal solid wasete incineration residues2010

    • Author(s)
      F.TAKAHASHI, K.YOKOHATA, T.SHI-MAOKA
    • Organizer
      Korea Society of Waste Management
    • Place of Presentation
      Daejeon
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Weathering of MSWI Bottom Ash With Emphasis on the Evolution of Iron-rich Con-stituents2010

    • Author(s)
      F.TAKAHASHI, T.KANOU, T.SHIMA-OKA
    • Organizer
      4th International Conference of East Asia Environment Problems "EAEP2010"
    • Place of Presentation
      Shanghai
    • Related Report
      2010 Final Research Report
  • [Presentation] Weathering of MSWI Bottom Ash With Emphasis on the Evolution of Iron-rich Constituents2010

    • Author(s)
      Y.WEI, T.SHIMAOKA, A.SAF-FARAZADEH, F.TAKAHASHI
    • Organizer
      4th Inter-national Conference of East Asia Environment Problems "EAEP2010"
    • Place of Presentation
      Shanghai
    • Related Report
      2010 Final Research Report
  • [Presentation] 一般廃棄物焼却灰由来の腐植物質と重金属の錯体形成に関する研究2010

    • Author(s)
      横畑一也, 高橋史武, 島岡隆行
    • Organizer
      土木学会年次学術講演会
    • Place of Presentation
      札幌
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] pH依存性試験に供した一般廃棄物焼却飛灰残渣中の鉛の化学形態変化と溶出性2010

    • Author(s)
      高橋史武, 叶琢磨, 島岡隆行
    • Organizer
      廃棄物資源循環学会研究発表会
    • Place of Presentation
      金沢
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Weathering of MSWI Bottom Ash With Emphasis on the Evolution of Iron-rich Constituents2010

    • Author(s)
      Fumitake TAKAHASHI, Takuma KANOU, Takayuki SHIMAOKA
    • Organizer
      4th International Conference of East Asia Environment Problems "EAEP2010"
    • Place of Presentation
      Shanghai
    • Related Report
      2010 Annual Research Report
  • [Presentation] The weath-ering of municipal solid waste incineration bottom ash evaluated by some weathering in-dices for natural rock profiles suggested in the mineralogy2009

    • Author(s)
      F.TAKAHASHI, T.SHIMAOKA
    • Organizer
      3rd International Conference of East Asia Environment Problems "EAEP2009"
    • Place of Presentation
      Fukuoka
    • Year and Date
      2009-12-03
    • Related Report
      2010 Final Research Report
  • [Presentation] The weathering of municipal solid waste incineration bottom ash evaluated by some weathering indices for natural rock profiles suggested in the mineralogy2009

    • Author(s)
      Fumitake TAKAHASHI, Takayuki SHIMAOKA
    • Organizer
      3rd International Conference of East Asia Environment Problems "EAEP2009"
    • Place of Presentation
      Fukuoka
    • Year and Date
      2009-12-03
    • Related Report
      2009 Annual Research Report
  • [Presentation] 埋立地における廃棄物焼却残渣の二酸化炭素吸収能の推定2009

    • Author(s)
      福井晋平, 高橋史武, 島岡隆行, Kevin Gardner
    • Organizer
      土木学会年次学術講演会
    • Place of Presentation
      福岡
    • Year and Date
      2009-09-03
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Remarks] ホームページ等

    • Related Report
      2010 Final Research Report

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Published: 2009-04-01   Modified: 2016-04-21  

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