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Functional Advancement of Aluminum-based Hydrogen Storage Materials-Elucidation and Promotion of Reaction Mechanism

Research Project

Project/Area Number 21760547
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Structural/Functional materials
Research InstitutionHigh Energy Accelerator Research Organization (2010)
Tohoku University (2009)

Principal Investigator

IKEDA Kazutaka  High Energy Accelerator Research Organization, 物質構造科学研究所, 特任准教授 (80451615)

Research Collaborator OHSHITA Hidetoshi  大学共同利用機関法人高エネルギー加速器研究機構, 物質構造科学研究所, 特任助教
OTOMO Toshiya  大学共同利用機関法人高エネルギー加速器研究機構, 物質構造科学研究所, 教授 (90270397)
SUZUYA Kentaro  独立行政法人日本原子力研究開発機構, J-PARCセンター, 研究主幹 (50354684)
MUTO Shunsuke  名古屋大学, 大学院・工学研究科, 教授 (20209985)
YUKAWA Hiroshi  名古屋大学, 大学院・工学研究科, 助教 (50293676)
SATO Toyoto  東北大学, 原子分子材料科学高等研究機構, 助教 (20455851)
SEMBOSHI Satoshi  東北大学, 金属材料研究所, 講師 (00364026)
LI Hai-Wen  東北大学, 金属材料研究所, 助教 (20505771)
OHOYAMA Kenji  東北大学, 金属材料研究所, 准教授 (60241569)
ORIMO Shin-ichi  東北大学, 金属材料研究所, 教授 (40284129)
Project Period (FY) 2009 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2010: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2009: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywords水素 / 水素化物 / 水素貯蔵 / エネルギー / 中性子 / アルミニウム / 熱的安定性 / 結晶構造 / ミリング / X線光電子分光 / 透過型電子顕微鏡 / 高輝度X線回折
Research Abstract

Functional advancement of aluminum-based hydrogen storage materials was studied. Synthesis conditions of aluminum hydrides, AlH_3, were optimized, and the crystal and surface structures, the thermodynamic stabilities, the hydrogen desorption properties and their correlations were investigated. We confirmed that the presence of amorphous Al_2O_3 andχ-Al_2O_3 on the surface may prevent the hydrogen desorption reaction of AlH_3, which can be promoted by milling process under the atmosphere control.

Report

(3 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • Research Products

    (28 results)

All 2011 2010 2009 Other

All Journal Article (15 results) (of which Peer Reviewed: 14 results) Presentation (9 results) Book (2 results) Remarks (2 results)

  • [Journal Article] Structural and hydrogen desorption properties of aluminum hydride2011

    • Author(s)
      K.Ikeda, H.Ohshita, N.Kaneko, J.Zhang, M.Yonemura, T.Otomo, K.Suzuya, H.Yukawa, M.Morinaga, H.W.Li, S.Semboshi, S.Orimo.
    • Journal Title

      Materials Transactions 52

    • NAID

      10028174826

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Structural and hydrogen desorption properties of aluminum hydride2011

    • Author(s)
      K.Ikeda, H.Ohshita, N.Kaneko, J.Zhang, M.Yonemura, T.Otomo, K.Suzuya, H.Yukawa, M.Morinaga, H.W.Li, S.Semboshi, S.Orimo
    • Journal Title

      Materials Transactions

      Volume: 52 Pages: 598-601

    • NAID

      10028174826

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Multimode hydriding/dehydriding reactions of CaPd2010

    • Author(s)
      K.Ikeda, N.Okuda, K.Ohoyama, H.-W.Li, H.T.Takeshita, T.Otomo, S.Orimo.
    • Journal Title

      Chemical Communications 46

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Surface changes on AlH_3 during the hydrogen desorption2010

    • Author(s)
      S.Kato, M.Bielmann, K.Ikeda, S.Orimo, A.Borgschulte, A.Zuttel.
    • Journal Title

      Applied Physics Letters 96

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Multimode hydriding/dehydriding reactions of CaPd2010

    • Author(s)
      K.Ikeda, N.Okuda, K.Ohoyama, H.W.Li, H.T.Takeshita, T.Otomo, S.Orimo
    • Journal Title

      Chemical Communications

      Volume: 46 Pages: 8380-8382

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Surface changes on AlH_3 during the hydrogen desorption2010

    • Author(s)
      S.Kato, M.Bielmann, K.Ikeda, S.Orimo, A.Borgschulte, A.Zuttel
    • Journal Title

      Applied Physics Letters

      Volume: 96

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Surface changes on AlH3 during the hydrogen desorption2010

    • Author(s)
      S.Kato, M.Bielmann, K.Ikeda, S.Orimo, A.Borgschulte, A.Zuttel
    • Journal Title

      Applied Physics Letters 96

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dehydriding reaction of AlH_3 : in-situ microscopic observations combined with thermal and surface analyses2009

    • Author(s)
      K.Ikeda, S.Muto, K.Tatsumi, M.Menjo, S.Kato, M.Bielmann, A.Zuttel, C.M.Jensen, S.Orimo.
    • Journal Title

      Nanotechnology 20

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dehydriding process of α-AlH_3 observed by transmission electron microscopy and electron energy-loss spectroscopy2009

    • Author(s)
      S.Muto, K.Tatsumi, K.Ikeda, S.Orimo.
    • Journal Title

      Journal of Applied Physics 105

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dehydriding reaction of AlH_3 : in-situ microscopic observations combined with thermal and surface analyses2009

    • Author(s)
      K.Ikeda, S.Muto, K.Tatsumi, M.Menjo, S.Kato, M.Bielmann, A.Zuttel, C.M.Jensen, S.Orimo
    • Journal Title

      Nanotechnology 20

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dehydriding process of α-AlH_3 observed by transmission electron micros copy and electron energy-loss spectroscopy2009

    • Author(s)
      S.Muto, K.Tatsumi, K.Ikeda, S.Orimo
    • Journal Title

      Journal of Applied Physics 105

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Reversible hydriding/dehydriding properties of new Y_3Al_2 hydrides2009

    • Author(s)
      K.Ikeda, N.Watanabe, S.Kato, T.Sato, Y.Nakamori, S.Orimo
    • Journal Title

      Journal of Alloys and Compounds 471

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct dry syntheses and thermal analyses of a series of aluminum complex hydrides2009

    • Author(s)
      T.Sato, K.Ikeda, H.-W.Li, S.Orimo
    • Journal Title

      Materials Transactions 50

      Pages: 182-186

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Syntheses, crystal structures, and thermal analyses of solvent-free Ca(AlD_4)_2 and CaAlD_52009

    • Author(s)
      T.Sato, M.H.Sorby, K.Ikeda, S.Sato, B.C.Hauback, S.Orimo
    • Journal Title

      Journal of Alloys and Compounds 487

      Pages: 472-478

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 高密度水素貯蔵を目指した水素化物の材料設計と特性評価2009

    • Author(s)
      池田一貴, 李海文, 折茂慎一
    • Journal Title

      化学工業 60

      Pages: 51-55

    • Related Report
      2009 Annual Research Report
  • [Presentation] Synthesis, atomic structure and hydrogen storage properties of aluminum hydride2011

    • Author(s)
      K.Ikeda, S.Muto, T.Otomo, S.Orimo
    • Organizer
      Thermec'2011 International Conference on Processing & Manufacturing of Advanced Materials
    • Place of Presentation
      Quebec, Canada. (Invited)
    • Year and Date
      2011-08-01
    • Related Report
      2010 Final Research Report
  • [Presentation] Synthesis, atomic structure and hydrogen storage properties of aluminum hydride2011

    • Author(s)
      K.Ikeda, S.Muto, T.Otomo, S.Orimo
    • Organizer
      Thermec' 2011 International Conference on Processing & Manufacturing of Advanced Materials
    • Place of Presentation
      Quebec, Canada (発表確定)
    • Related Report
      2010 Annual Research Report
  • [Presentation] アルミニウム水素化物の脱水素化過程の解明2010

    • Author(s)
      池田一貴, 李海文, 折茂慎一, 巽一厳, 武藤俊介, 湯川宏, 森永正彦, 橋邦彦, 伊藤秀明, 兜森俊樹, S.Kato, M.Bielmann, A.Borgschulte, A.Zuttel
    • Organizer
      日本金属学会2010年春期(第146回)大会
    • Place of Presentation
      筑波大学(つくば市)
    • Year and Date
      2010-03-28
    • Related Report
      2009 Annual Research Report
  • [Presentation] Hydrogen Storage in Aluminum Hydride-from nano-characterization to semi-practical evaluation-2009

    • Author(s)
      K.Ikeda, S.Orimo
    • Organizer
      Eighteenth International Symposium on Processing and Fabrication of Advanced Materials XVIII (PFAM XVIII)
    • Place of Presentation
      Sendai, Japan. (Invited)
    • Year and Date
      2009-12-12
    • Related Report
      2010 Final Research Report
  • [Presentation] Hydrogen Storage in Aluminum Hydride -from nano-characterization tosemi-practical evaluation-2009

    • Author(s)
      池田一貴, 折茂慎一
    • Organizer
      Eighteenth International Symposium on Processing and Fabrication of Advanced Materials XVIII(PFAMXVIII)
    • Place of Presentation
      東北大学(仙台市)
    • Year and Date
      2009-12-12
    • Related Report
      2009 Annual Research Report
  • [Presentation] Synthesis, properties and applications of aluminum hydride2009

    • Author(s)
      K.Ikeda, K.Tatsumi, S.Muto, S.Sato, M.Menjo, S.Kato, M.Bielmann, A.Zuttel, K.Hashi, H.Itoh, T.Kabutomori, C.M.Jensen, S.Orimo
    • Organizer
      Thermec'2009 International Conference on Processing&Manufacturing of Advanced Materials
    • Place of Presentation
      Berlin, Germany. (Invited)
    • Year and Date
      2009-08-27
    • Related Report
      2010 Final Research Report
  • [Presentation] Synthesis, properties and applications of aluminum hydride2009

    • Author(s)
      K.Ikeda, K.Tatsumi, S.Muto, S.Sato, M.Menjo, S.Kato, M.Bielmann, A.Zuttel, K.Hashi, H.Itoh, T.Kabutomori, C.M.Jensen, S.Orimo
    • Organizer
      Thermec' 2009 International Conference on PROCESSING & MANUFACTURING OF ADVANCED MATERIALS
    • Place of Presentation
      Berlin, Germany
    • Year and Date
      2009-08-27
    • Related Report
      2009 Annual Research Report
  • [Presentation] Hydrogen Storage in Aluminum Hydride2009

    • Author(s)
      K.Ikeda, M.Menjo, H.W.Li, S.Muto, K.Tatsumi, K.Hashi, H.Itoh, T.Kabutomori, S.Orimo
    • Organizer
      The Seventeenth Annual International Conference on Composites/Nano Engineering (ICCE-17)
    • Place of Presentation
      Honolulu, Hawaii, USA. (Invited)
    • Year and Date
      2009-07-28
    • Related Report
      2010 Final Research Report
  • [Presentation] Hydrogen Storage in Aluminum Hydride2009

    • Author(s)
      K.Ikeda, M.Menjo, H.W.Li, S.Muto, K.Tatsumi, K.Hashi, H.Itoh, T.Kabutomori, S.Orimo
    • Organizer
      The Seventeenth Annual International Conference on COMPOSITES/NANO ENGINEERING(ICCE-17)
    • Place of Presentation
      Honolulu, Hawaii, USA
    • Year and Date
      2009-07-28
    • Related Report
      2009 Annual Research Report
  • [Book] 水素製造・吸蔵・貯蔵・輸送材料と安全化("アルミニウム水素化物による水素貯蔵")2010

    • Author(s)
      池田一貴, 折茂慎一, 齋藤寛之, 町田晃彦, 片山芳則, 青木勝敏
    • Publisher
      サイエンス&テクノロジー
    • Related Report
      2010 Final Research Report
  • [Book] 水素製造・吸蔵・貯蔵・輸送材料と安全化2010

    • Author(s)
      池田一貴, 折茂慎一, 齋藤寛之, 町田晃彦, 片山芳則, 青木勝敏
    • Total Pages
      11
    • Publisher
      サイエンス&テクノロジー
    • Related Report
      2010 Annual Research Report
  • [Remarks] ホームページ等

    • URL

      http://www.kek.jp/imss/

    • Related Report
      2010 Final Research Report
  • [Remarks]

    • URL

      http://www.kek.jp/imss/

    • Related Report
      2010 Annual Research Report

URL: 

Published: 2009-04-01   Modified: 2016-04-21  

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