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Exploration of novel topological electric phenomena in frustrated magnets

Research Project

Project/Area Number 21K13871
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionThe University of Tokyo

Principal Investigator

Ueda Kentaro  東京大学, 大学院工学系研究科(工学部), 助教 (40835336)

Project Period (FY) 2021-04-01 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2022: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2021: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords強相関電子系 / 磁性 / トポロジカル電子系 / トポロジカル物質 / フラストレート磁性 / 磁気転移 / イリジウム酸化物 / トポロジカル電子状態 / 量子輸送現象
Outline of Research at the Start

本研究課題では、三次元フラストレーション格子であるパイロクロア型酸化物に着目し、局在スピンと遍歴電子の多彩な磁気相関がもたらす新奇トポロジカル電子物性の開拓・究明を目的とする。
従来の磁性トポロジカル絶縁体・半金属の研究の多くは、電子相関が比較的小さい金属間化合物を対象としてきた。フラストレーション格子磁性体に着目することで、以下の利点がある。(i)多様な磁性が生じるため、磁性トポロジカル電子状態について豊富な知見を得ることができる。(ii)外場による容易な相制御が期待できる。

Outline of Final Research Achievements

I have investigated topological electronic properties in frustrated pyrochlore oxides.
In the pyrochlore iridium oxide Pr2Ir2O7, I found spin-ice-like magnetic order and giant anomalous Hall effect. I also found a giant thermoelectric response in (Nd,Pr)2Ir2O7 in the vicinity of the metal-insulator transition. We discuss the relationship between the observed transport properties and the possible emergence of topological semimetallic states.
We succeeded in growing single crystals of Ca-doped pyrochlore molybdenum oxide Tb2Mo2O7. A filling-controlled metal-insulator transition was observed and the geometric Hall effect in the paramagnetic metallic state was investigated.

Academic Significance and Societal Importance of the Research Achievements

本課題では、磁性とトポロジカル電子の結合がもたらす新しい物性の開拓を目指した。本課題によって下記が期待される;(i)量子技術への応用が期待されているスピンアイス状態が遍歴系で実現することから、新しいメカニズムによる実現温度の向上や候補物質の拡大が見込まれる;(ii)外場によるトポロジカル電子状態・巨大熱電応答制御により、エナジーハーヴェスティングに有望な物質設計指針を示された;(iii)常磁性体での幾何学的ホール効果を発見したことから、ナノスケールのスピンによる創発電磁気学の学理構築への貢献が期待される。

Report

(3 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • Research Products

    (9 results)

All 2022 2021

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (6 results) (of which Int'l Joint Research: 1 results,  Invited: 1 results)

  • [Journal Article] Large magneto-thermoelectric effect on the verge of metal?insulator and topological transitionsin pyrochlore iridates2022

    • Author(s)
      Ueda Kentaro、Fujioka Jun、Kanazawa Naoya、Tokura Yoshinori
    • Journal Title

      APL Materials

      Volume: 10 Issue: 9 Pages: 091111-091111

    • DOI

      10.1063/5.0097460

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental signatures of a versatile Weyl semimetal in a pyrochlore iridate with spin-ice-like magnetic orders2022

    • Author(s)
      Ueda Kentaro、Ishizuka Hiroaki、Kriener Markus、Kitou Shunsuke、Maryenko Denis、Kawamura Minoru、Arima Taka-hisa、Kawasaki Masashi、Tokura Yoshinori
    • Journal Title

      Physical Review B

      Volume: 105 Issue: 16

    • DOI

      10.1103/physrevb.105.l161102

    • Related Report
      2022 Annual Research Report 2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Highly anisotropic geometrical Hall effect via <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>f</mml:mi><mml:mtext>?</mml:mtext><mml:mi>d</mml:mi></mml:mrow></mml:math> exchange fields in doped pyrochlore molybdates2022

    • Author(s)
      Fukuda Hikaru、Ueda Kentaro、Kaneko Yoshio、Kurihara Ryosuke、Miyake Atsushi、Karube Kosuke、Tokunaga Masashi、Taguchi Yasujiro、Tokura Yoshinori
    • Journal Title

      Physical Review B

      Volume: 106 Issue: 14 Pages: 144431-144431

    • DOI

      10.1103/physrevb.106.144431

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed
  • [Presentation] Field-anisotropic geometrical Hall effect via f-d exchange fields in doped pyrochlore molybdates2022

    • Author(s)
      H. Fukuda, K. Ueda, Y. Kaneko, R. Kurihara, A. Miyake, K. Karube, M. Tokunaga, Y. Taguchi, and Y. Tokura
    • Organizer
      American Physical Society March Meeting, March 2023
    • Related Report
      2022 Annual Research Report
  • [Presentation] Topology and correlation induced exotic transport phenomena in pyrochlore and half-Heusler compounds2022

    • Author(s)
      K. Ueda
    • Organizer
      Workshop on Topology in Magnetic Materials, Herzberg, Switzerland, November 2022
    • Related Report
      2022 Annual Research Report
    • Invited
  • [Presentation] Experimental signatures of versatile Weyl semimetal in pyrochlore iridate with spin-ice like magnetic orders2022

    • Author(s)
      5.K. Ueda, H. Ishizuka, M. Kriener, S. Kitou, D. maryenko, M. Kawamura, T.-h. Arima, M. Kawasaki, and Y. Tokura
    • Organizer
      American Physical Society March Meeting, March 2022
    • Related Report
      2022 Annual Research Report
  • [Presentation] パイロクロア型Pr2Ir2O7における磁気転移と異常ホール効果の制御2021

    • Author(s)
      上田健太郎, 石塚大晃,Markus Kriener, Denis Maryenko, 川村稔, 川﨑雅司, 十倉好紀
    • Organizer
      日本物理学会2021年秋季大会
    • Related Report
      2021 Research-status Report
  • [Presentation] Experimental signatures of a versatile Weyl semimetal in a pyrochlore iridate with spin-ice-like magnetic orders2021

    • Author(s)
      Kentaro Ueda, Hiroaki Ishizuka, Markus Kriener, Shunsuke Kitou, Denis Maryenko, Minoru Kawamura, Taka-hisa Arima, Masashi Kawasaki, Yoshinori Tokura
    • Organizer
      APS March meeting 2022
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] フィリング制御パイロクロア (Tb1-xCax)2Mo2O7における異方的幾何学的ホール効果2021

    • Author(s)
      福田光 、 上田健太郎 、 金子良夫 、 軽部皓介 、 栗原綾佑 、 三宅厚志 、 徳永将史 、 田口康二郎 、 十倉好紀
    • Organizer
      日本物理学会2022年春季大会
    • Related Report
      2021 Research-status Report

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Published: 2021-04-28   Modified: 2024-01-30  

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