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Spin Freezing Crossover and Cooper Pairing Symmetry in the Organic Strange Metal kappa-(ET)4Hg2.89Br8 and kappa-(ET)4Hg2.78Cl8

Research Project

Project/Area Number 21K13885
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionShibaura Institute of Technology

Principal Investigator

Dita PuspitaSari  芝浦工業大学, 工学部, 助教 (00821919)

Project Period (FY) 2021-04-01 – 2025-03-31
Project Status Granted (Fiscal Year 2023)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2024: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2023: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2022: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2021: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
KeywordsNon-Fermi liquid / Penetration depth / Knight shift / Cooper pair / Strange metal / Spin freezing / Quantum entanglement / strange metal / non-Fermi liquid / SYK model / Hubbard model / QCP / AdS/CFT correspondence
Outline of Research at the Start

The spin freezing crossover observed as a highly fluctuating spin in the metallic state and the Cooper pairing symmetry of two strange metal candidates known as a triangular lattice single-band Hubbard model system, k-(ET)4Hg2.89Br8 and k-(ET)4Hg2.78Cl8, will be studied by muon-spin relaxation.

Outline of Annual Research Achievements

We synthesized more samples twice the weight of last year sample of k-HgBr and k-HgCl to improve the signal-to-noise ratio. We performed transverse field muSR on k-HgBr sample for the penetration depth measurement in the parallel and perpendicular mode. The muSR measurement on k-HgCl for the spin diffusion measurement down to dilution-refrigerator temperature is continued.

Current Status of Research Progress
Current Status of Research Progress

2: Research has progressed on the whole more than it was originally planned.

Reason

The penetration depth measurement needs to be improved to get solid and complete data set, although an overview summary is being written up.
The spin diffusion measurement down to dilution-refrigerator temperature will be conducted in December 2024.

Strategy for Future Research Activity

2024: Writing up main papers and execute a continuation. A related project fund has been proposed and applied.

Report

(3 results)
  • 2023 Research-status Report
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (20 results)

All 2024 2023 2022 2021 Other

All Int'l Joint Research (4 results) Journal Article (3 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results) Presentation (13 results) (of which Int'l Joint Research: 9 results,  Invited: 3 results)

  • [Int'l Joint Research] ISIS Neutron and Muon Source(英国)

    • Related Report
      2023 Research-status Report
  • [Int'l Joint Research] TRIUMF(カナダ)

    • Related Report
      2023 Research-status Report
  • [Int'l Joint Research] TRIUMF(カナダ)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] ISIS(英国)

    • Related Report
      2022 Research-status Report
  • [Journal Article] Pressure effect in the metallic state of λ-(BETS)2GaCl42024

    • Author(s)
      Ueno Masaki、Tsutsumi Asako、Katsuoka Naoto、Sari Dita Puspita、Suzuki Takao、Ishii Yasuyuki
    • Journal Title

      Interactions

      Volume: 245 Issue: 1 Pages: 71-71

    • DOI

      10.1007/s10751-024-01909-x

    • Related Report
      2023 Research-status Report
  • [Journal Article] Magnetic Susceptibility Study of Hole-Doped Organic Metal κ-(ET)<sub>4</sub>Hg<sub>3-δ</sub>Cl<sub>8, </sub>δ=22% and κ-(ET)<sub>4</sub>Hg<sub>3-δ</sub>Br<sub>8, </sub>δ=11%2023

    • Author(s)
      Sari Dita Puspita、Widyaiswari Utami、Someya Yuta、Yamada Eiki、Taniguchi Hiromi、Watanabe Isao、Ishii Yasuyuki
    • Journal Title

      Solid State Phenomena

      Volume: 345 Pages: 47-52

    • DOI

      10.4028/p-1xerwq

    • Related Report
      2023 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Superconductivity nearby quantum critical region in hole-doped organic strange metal κ-(ET)<sub>4</sub>Hg<sub>3-δ</sub>Br<sub>8</sub>, δ=11%2023

    • Author(s)
      Sari D P、Kaito M、Someya Y、Widyaiswari U、Watanabe I、Taniguchi H、Ishii Y
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 2462 Issue: 1 Pages: 012061-012061

    • DOI

      10.1088/1742-6596/2462/1/012061

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Presentation] μSR Study of Hole-Doped Organic Metals: Superconductivity Nearby Quantum Spin Liquid States2023

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, A. E. Putri, E. Yamada, Y. Someya, A. Koda, Y. Ishii, F. L. Pratt, I. Watanabe, K. M. Kojima, and H. Taniguchi
    • Organizer
      Universiti Sains Malaysia (USM-RIKEN) International Conference on Advanced Sciences, Penang 2024
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Organic Superconductivity Nearby Quantum Criticality of a Magnetic Frustration2023

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, A. E. Putri, E. Yamada, Y. Someya, A. Koda, Y. Ishii, F. L. Pratt, I. Watanabe, K. M. Kojima, and H. Taniguchi
    • Organizer
      The 1st Conference of Accelerator -Based Sciences and Technology CAST 2024, Jakarta 2024
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Introduction to the Muon Technique and Science2023

    • Author(s)
      D. P. Sari
    • Organizer
      ISIS Indonesia and Malaysia Webinar I Introduction to ISIS Neutron & Muon Source, ONLINE
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] μSR Study of Hole-Doped Organic Metals: Superconductivity Nearby Quantum Spin Liquid States2023

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, A. E. Putri, E. Yamada, Y. Someya, A. Koda, Y. Ishii, F. L. Pratt, I. Watanabe, K. M. Kojima, and H. Taniguchi
    • Organizer
      International Conference on Machine Learning, Kyoto 2023
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] μ+SR Knight Shift of the Hole-Doped Organic Metal kappa-(ET)4Hg2.78Cl82023

    • Author(s)
      D. P. Sari, Y. Cai, K. Kojima, I. Watanabe, H. Taniguchi, and Y. Ishii
    • Organizer
      International Conference Hyperfine Interactions 2023, Nara, November 2023
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] Superconductivity Nearby Quantum Spin Liquid States2023

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, A. E. Putri, E. Yamada, Y. Someya, A. Koda, Y. Ishii, F. L. Pratt, I. Watanabe, K. M. Kojima, and H. Taniguchi
    • Organizer
      International Long-term Workshop of Quantum Information, Quantum Matter, Quantum Gravity, Workshop number YITP-T-23-01, Kyoto
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] Superconductivity Nearby Quantum Spin Liquid States in Doped Organic Metal2022

    • Author(s)
      D. P. Sari, Y. Cai, M-V. deToro Sanchez, K. M. Kojima, I. Watanabe, Y. Ishii, and H. Taniguchi
    • Organizer
      The 13th International Conference on Materials and Mechanisms of Superconductivity (M2S 2022)
    • Related Report
      2022 Research-status Report
  • [Presentation] Superconductivity Nearby Quantum Critical Point in Hole-Doped Organic Strange Metal &#61547;-(ET)4Hg3-&#61540;Br82022

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, E. Yamada, M-V. deToro Sanchez, Y. Someya, A. Koda, K. M. Kojima, I. Watanabe, Y. Ishii, and H. Taniguchi
    • Organizer
      The 15th International Conference on Muon Spin Rotation, Relaxation and Resonance (muSR conference 2020)
    • Related Report
      2022 Research-status Report
  • [Presentation] μ+SR Study of κ-(ET)4Hg3-δBr8 (δ=0.11) and κ-(ET)4Hg3-δCl8 (δ=0.22) Part II2022

    • Author(s)
      D. P. Sari, Y. Cai, U. Widyaiswari, E. Yamada, M-V. deToro Sanchez, Y. Someya, A. Koda, K. M. Kojima, I. Watanabe, Y. Ishii, and H. Taniguchi
    • Organizer
      JPS Autumn Meeting 2022
    • Related Report
      2022 Research-status Report
  • [Presentation] μ+SR Study of κ-(ET)4Hg2.89Br8 and κ-(ET)4Hg2.78Cl82022

    • Author(s)
      4.1.15D. P. Sari, Y. Cai, U. Widyaiswari, E. Yamada, M-V. deToro Sanchez, Y. Someya, K. M. Kojima, I. Watanabe, H. Taniguchi and Y. Ishii
    • Organizer
      The 6th International Conference on Functional Materials Science (ICFMS 2022)
    • Related Report
      2022 Research-status Report
  • [Presentation] μ+SR Study of κ-(ET)4Hg3-δBr8 (δ=0.11) and κ-(ET)4Hg3-δCl8 (δ=0.22)2022

    • Author(s)
      Dita P. Sari, Y. Cai, M-V. deToro Sanchez, K. M. Kojima, I. Watanabe, A. Koda, Y. Ishii, H. Taniguchi
    • Organizer
      The 2022Annual 77th Japanese Physical Society Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Distorted Superconducting Nodal Line on Single Fermi Surface in Anisotropic Organic Superconductor λ-(BETS)2GaCl42021

    • Author(s)
      D. P. Sari, R. Asih, K. Hiraki, T. Nakano, Y. Nozue, A. D. Hillier, Y. Ishii, I. Watanabe
    • Organizer
      International Conference on Strongly Correlated Electron Systems 2020
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] μ+SR Study of an Organic Doped Spin-Liquid Candidate κ-(ET)4Hg3-δBr8 (δ=0.11)2021

    • Author(s)
      Dita P. Sari, Y. Cai, M-V. deToro Sanchez, K. M. Kojima, I. Watanabe, Y. Ishii, H. Taniguchi
    • Organizer
      Materials Research Meeting 2021
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research

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Published: 2021-04-28   Modified: 2024-12-25  

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