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Opto-spintronics in atomic-layer materials

Research Project

Project/Area Number 21K13889
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

Wang Ziqian  国立研究開発法人理化学研究所, 創発物性科学研究センター, 特別研究員 (00898934)

Project Period (FY) 2021-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2023: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2022: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2021: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywordsvan der Waals materials / Magnetism / Symmetry / Nonlinear optics / Nonreciprocity / SHG / Domain contrast / vdW antiferromagnet / Magnon-sideband / Symmetry crossover / 2D materials / atomic-layer magnets / opto-spintronics / magneto-optical effects / harmonic generation / ultrafast spin dynamics
Outline of Research at the Start

In this study, light is used to visualize and manipulate the magnetic domains of emergent magnetic materials with a thickness of only a single or a few atomic layers (atomic-layer magnets), and to investigate the control of their magnetism on an ultrafast time scale.

Outline of Final Research Achievements

Two-dimensional (2D) van der Waals (vdW) magnets are a new class of materials with a layered structure that exhibit magnetism even when they are just a few atoms thick. These materials have unique features compared to conventional magnets, particularly their ability to be stacked into devices with only a few atomic layers. We conducted in-depth research on these 2D magnets, focusing on their structure, symmetry, and optical properties. Our work revealed an unusual atomic-scale structure in their thin layers that leads to unexpected changes in symmetry. We also discovered unique interactions between virtual particles in a 2D magnet, which have not been observed in traditional magnets. Additionally, we developed a method to control optical nonreciprocity, a property where the material responds differently to light when the direction of light propagation is reversed.

Academic Significance and Societal Importance of the Research Achievements

本研究では、新興の原子層磁性体の構造、対称性、光学特性に関する重要かつ新たな理解をもたらした。学術的には、この研究で得られた新しい知見は光スピントロニクスと低次元磁性の分野での開拓に基盤を提供していた。また、社会的には、この研究で実現した2D磁性体の新しい機能が、次世代の電子、磁気、光デバイスの開発に貢献していた。

Report

(4 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (11 results)

All 2024 2023 2022

All Journal Article (5 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 5 results,  Open Access: 3 results) Presentation (6 results) (of which Int'l Joint Research: 5 results)

  • [Journal Article] Giant Modulation of the Second Harmonic Generation by Magnetoelectricity in Two‐Dimensional Multiferroic CuCrP2S62024

    • Author(s)
      Aoki Shunta、Dong Yu、Wang Ziqian、Huang Xiang S.W.、Itahashi Yuki M.、Ogawa Naoki、Ideue Toshiya、Iwasa Yoshihiro
    • Journal Title

      Advanced Materials

      Volume: - Issue: 21 Pages: 2312781-2312781

    • DOI

      10.1002/adma.202312781

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Odd-parity multipole order in the spin-orbit coupled metallic pyrochlore Pb2Re2O7-δ2024

    • Author(s)
      Nakayama Yuki、Hirai Daigorou、Sagayama Hajime、Kojima Keita、Katayama Naoyuki、Lehmann Jannis、Wang Ziqian、Ogawa Naoki、Takenaka Koshi
    • Journal Title

      Physical Review Materials

      Volume: 8 Issue: 5 Pages: 055001-055001

    • DOI

      10.1103/physrevmaterials.8.055001

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Real-Space Observation of Ripple-Induced Symmetry Crossover in Ultrathin MnPS<sub>3</sub>2023

    • Author(s)
      Wang Ziqian、Gao Meng、Yu Tonghua、Zhou Siyuan、Xu Mingquan、Hirayama Motoaki、Arita Ryotaro、Shiomi Yuki、Zhou Wu、Ogawa Naoki
    • Journal Title

      ACS Nano

      Volume: 17 Issue: 3 Pages: 1916-1924

    • DOI

      10.1021/acsnano.2c04995

    • Related Report
      2023 Annual Research Report 2022 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Exciton-magnon splitting in the van der Waals antiferromagnet MnPS3 unveiled by second-harmonic generation2023

    • Author(s)
      Wang Ziqian、Zhang Xiao-Xiao、Shiomi Yuki、Arima Taka-hisa、Nagaosa Naoto、Tokura Yoshinori、Ogawa Naoki
    • Journal Title

      Physical Review Research

      Volume: 5 Issue: 4

    • DOI

      10.1103/physrevresearch.5.l042032

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Emergent zero-field anomalous Hall effect in a reconstructed rutile antiferromagnetic metal2023

    • Author(s)
      Wang Meng、Tanaka Katsuhiro、Sakai Shiro、Wang Ziqian、Deng Ke、Lyu Yingjie、Li Cong、Tian Di、Shen Shengchun、Ogawa Naoki、Kanazawa Naoya、Yu Pu、Arita Ryotaro、Kagawa Fumitaka
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 8240-8240

    • DOI

      10.1038/s41467-023-43962-0

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] Second harmonic generation from exciton-magnons in van der Waals antiferromagnet MnPS32023

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Taka-hisa. Arima, Naoto Nagaosa, Yoshinori Tokura, Naoki Ogawa
    • Organizer
      APS March Meeting
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Second harmonic generation from exciton-magnons in van der Waals antiferromagnet MnPS32023

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Taka-Hisa Arima, Naoto Nagaosa, Yoshinori Tokura, Naoki Ogawa
    • Organizer
      APS March Meeting
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] Electronic and magnetic excitations in van der Waals antiferromagnet MnPS3 probed by second-harmonic generation2022

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Akiko Kikkawa, Yasujiro Taguchi, Taka-Hisa Arima, Naoki Ogawa
    • Organizer
      The 29th International Conference on Low Temperature Physics (LT29)
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] Second-harmonic generation by electronic and magnetic excitation in van der Waals antiferromagnet MnPS32022

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Taka-Hisa Arima, Naoki Ogawa
    • Organizer
      The 15th Asia Pacific Physics Conference (APPC15)
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] Second-harmonic generation study of excitations in van der Waals antiferromagnet MnPS32022

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Taka-Hisa Arima, Naoki Ogawa
    • Organizer
      JPS 2022 Autumn Meeting
    • Related Report
      2022 Research-status Report
  • [Presentation] Revealing exciton-magnon correlation in van der Waals antiferromagnet MnPS3 by second harmonic generation spectroscopy2022

    • Author(s)
      Ziqian Wang, Yuki Shiomi, Taka-Hisa Arima, Naoto Nagaosa, Yoshinori Tokura, Naoki Ogawa
    • Organizer
      The 13th TOYOTA RIKEN International Workshop: Integrated Spectroscopy for Strong Electron Correlation - Theory, Computation and Experiment
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research

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Published: 2021-04-28   Modified: 2025-01-30  

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