Opto-spintronics in atomic-layer materials
| Project/Area Number |
21K13889
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| Research Category |
Grant-in-Aid for Early-Career Scientists
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| Allocation Type | Multi-year Fund |
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| Review Section |
Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
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| Research Institution | Institute of Physical and Chemical Research |
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Principal Investigator |
王 子謙 国立研究開発法人理化学研究所, 創発物性科学研究センター, 特別研究員 (00898934)
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| Project Period (FY) |
2021-04-01 – 2024-03-31
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| Project Status |
Completed (Fiscal Year 2023)
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| Budget Amount *help |
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2023: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2022: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2021: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
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| Keywords | Nonreciprocity / SHG / Domain contrast / vdW antiferromagnet / Symmetry / Magnon-sideband / Symmetry crossover / 2D materials / atomic-layer magnets / opto-spintronics / magneto-optical effects / harmonic generation / ultrafast spin dynamics |
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| Outline of Research at the Start |
In this study, light is used to visualize and manipulate the magnetic domains of emergent magnetic materials with a thickness of only a single or a few atomic layers (atomic-layer magnets), and to investigate the control of their magnetism on an ultrafast time scale.
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| Outline of Annual Research Achievements |
Nonreciprocal photonic responses play a crucial role in advanced photonics applications, ranging from from one-way window to quantum computing. In non-centrosymmetric antiferromagnets (AFMs), nonreciprocity can manifest through nonlinear optical effects like second-harmonic generation (SHG), featured by varying efficiencies for spin-reversal domains. So far, techniques harnessing nonreciprocity-driven domain contrast are limited, and effective and flexible control over such nonreciprocity remains largely unachieved. Moreover, a comprehensive roadmap for controlling these nonreciprocal photonic behaviors from a material symmetry perspective is lacking. Drawing insights from group theory, we experimentally demonstrated a general method to modulate SHG domain contrast and nonreciprocity, using a prototypical van der Waals layered AFM MnPS3 as proof of concept. Through targeted application of electric field, we effectively manipulated the interferences among multipole SHG sources inherent in the crystal, directly changing the nonreciprocity. This approach offers distinct advantages, including broad-band feasibility, rapid response governed by electric signals, minimal device complexity, and a wide choice of antiferromagnet materials. Additionally, we have compiled a detailed listing of applicable magnetic point groups and optimal electric field orientations, establishing a guiding framework for electrically controlling nonlinear optical nonreciprocity in AFMs.
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Report
(3 results)
Research Products
(11 results)
