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Elucidation of mechanism for improving joining strength and durability of hybrid CFRTP by addition of nanofibers

Research Project

Project/Area Number 21K14060
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 18020:Manufacturing and production engineering-related
Research InstitutionFukuoka University (2022-2023)
Kanagawa University (2021)

Principal Investigator

Matsumoto Koki  福岡大学, 工学部, 助教 (50850070)

Project Period (FY) 2021-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2023: ¥520,000 (Direct Cost: ¥400,000、Indirect Cost: ¥120,000)
Fiscal Year 2022: ¥520,000 (Direct Cost: ¥400,000、Indirect Cost: ¥120,000)
Fiscal Year 2021: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords射出オーバーモールド成形 / 炭素繊維強化熱可塑性樹脂 / 接合強度 / カーボンナノチューブ / 伝熱 / 結晶化度 / 射出オーバーモールド / ナノ繊維 / 結晶特性 / ナノフィラー添加ハイブリッド複合材料 / 接合・界面
Outline of Research at the Start

本研究では,射出オーバーモールドによるテキスタイル複合材料と射出樹脂間の接合強度の高信頼化を目指し,接合界面部にナノ繊維添加樹脂フィルムを挟み,接合界面部をナノ繊維により直接強化することに取り組む.金型内流動の状態が接合部のナノ繊維の状態や樹脂結晶状態に影響を及ぼす点に着目し,プロセスの観点からナノ繊維添加による接合メカニズムを明らかにする.

Outline of Final Research Achievements

The joining strength of carbon fiber-reinforced thermoplastic (CFRTP) strongly depends on the interface temperature and pressure during the injection overmolding process. We attempted to strengthen the weld line by inserting the carbon nanotube (CNT)-reinforced polypropylene (PP) film at the interface. The objective of this research is to reveal the reinforcement effect of nanofiller against the joining strength.
We discussed the influence of CNT contents and the cooling rate of molding CFRTP substrate on the melting behavior of PP. The water-quench during the cooling of the heat-pressed substrate enables the reduction of the crystallinity of PP. Consequently, the joining strength was significantly improved. However, the effect of CNT addition on the joining strength was independent of the cooling rate. Thus, we revealed that the crystallinity reduction of PP at the surface of the substrate did not contribute to an increase in the joining strength by CNT addition.

Academic Significance and Societal Importance of the Research Achievements

これまで射出オーバーモールド成形の接合強度の発現には,圧力や温度等のパラメーターを中心に考察が進められてきた.本研究は新たに接合部の樹脂の結晶化度に着目し,結晶化度の低下が接合強度の向上に大きく寄与できる事を示した.また,結晶化度に寄らずCNTの接合部の補強効果が得られる事が示された.本研究成果を踏まえ,射出オーバーモールド成形において,接合界面部にナノ繊維を配置することで信頼性の高い接合強度の発現が可能となる.これらの成形部材はモビリティの軽量化が可能となり,二酸化炭素の排出量削減等に大きく貢献できる.

Report

(4 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (5 results)

All 2023 2022 2021

All Journal Article (2 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (3 results)

  • [Journal Article] Selective reinforcement of joining interface using nanofibers in single-lap joints of thermoplastic composites fabricated by the injection overmolding process: creep deformation behaviour2022

    • Author(s)
      Koki Matsumoto, Masaya Itabashi, Akira Kawasumi, Kenichi Takemura, Tatsuya Tanaka
    • Journal Title

      WIT Transactions on The Built Environment

      Volume: 209 Pages: 3-14

    • DOI

      10.2495/hpsu220011

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] The influence of the addition position of cellulose nanofibers on the crystalline and mechanical properties of carbon fiber-reinforced polypropylene composites2021

    • Author(s)
      Koki Matsumoto, Kenichi Takemura
    • Journal Title

      Composite Interfaces

      Volume: 29 Issue: 9 Pages: 1053-1070

    • DOI

      10.1080/09276440.2021.2007720

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Presentation] プレス成形の冷却速度が炭素繊維強化ポリプロピレンの結晶融解挙動に与える影響2023

    • Author(s)
      松本紘宜, 内藤優紀, 高倉健太郎, 森山茂章, 山辺純一郎
    • Organizer
      日本材料学会九州支部 第10回学術講演会
    • Related Report
      2023 Annual Research Report
  • [Presentation] ナノ繊維の選択的配置による炭素繊維強化ポリプロピレンの結晶特性のコントロール2021

    • Author(s)
      松本紘宜, 竹村兼一
    • Organizer
      第13回 自動車用途コンポジットシンポジウム
    • Related Report
      2021 Research-status Report
  • [Presentation] 射出オーバーモールド成形における被接合材表面の ポリマーの結晶状態と接合強度の関係2021

    • Author(s)
      松本紘宜, 板橋正弥, 竹村兼一
    • Organizer
      2021年度 JCOM若手ウェビナー
    • Related Report
      2021 Research-status Report

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Published: 2021-04-28   Modified: 2025-01-30  

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