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Elucidating clogging and breakage of colloids in porous microchannel

Research Project

Project/Area Number 21K14939
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 41030:Rural environmental engineering and planning-related
Research InstitutionUniversity of Tsukuba

Principal Investigator

Sugimoto Takuya  筑波大学, 生命環境系, 助教 (70899509)

Project Period (FY) 2021-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2023: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2022: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2021: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Keywords沈着 / コロイド / 輸送現象 / 流動現象 / 界面電気現象 / 凝集 / 破壊 / 界面動電現象 / 目詰まり
Outline of Research at the Start

土壌の透水性の低下は,微細なコロイド画分の剥離や移動と,それらの間隙内への集積による目詰まりに支配される.従来のカラム輸送実験では,間隙スケールでの土壌マトリクスへのコロイドの集積に伴う目詰まりや,目詰まり層からの剥離や再浮遊による破壊現象のダイナミクスを評価することは難しい.
本研究では,微細な間隙構造を有するマイクロ流路中の顕微鏡観察に基づいて目詰まり・破壊現象の評価系を構築する.間隙内の流動条件やコロイドの帯電・凝集特性に関する情報をレファレンスとしながら,目詰まりの形成-成長-破壊過程の支配因子を探索する.

Outline of Final Research Achievements

Clogging and breakdown phenomena caused by colloids in soil and aquatic environments can affect the dynamics and transport of chemicals through changes in soil permeability and erodibility. This study systematically elucidated these phenomena by: (1) constructing an experimental system for the formation and breakdown of clogs using microfluidic channels and acquiring experimental data, (2) assessing the charging and aggregation characteristics of colloids, and (3) conducting column transport experiments to evaluate macroscopic deposition rates and analyzing the results. Furthermore, simulations related to dense colloidal suspensions, which are experimentally similar to clogging, were employed to analyze the system, successfully achieving good agreement with the experimental data.

Academic Significance and Societal Importance of the Research Achievements

土壌中で起きているミクロとマクロなスケールの現象を接続し,体系的な理解と理論を深化させていくために,マイクロ流路を活用した直接観察系の構築と測定,帯電量評価の評価と凝集解析,マクロなカラム実験と解析を行い,学術的に新規な成果を得た。得られた成果は環境中のマイクロプラスチック動態,土中の微生物の動態や目詰まりなど,より発展的な課題への応用の基礎となる。

Report

(4 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (31 results)

All 2024 2023 2022 2021 Other

All Int'l Joint Research (1 results) Journal Article (12 results) (of which Peer Reviewed: 11 results,  Open Access: 1 results) Presentation (18 results) (of which Int'l Joint Research: 3 results,  Invited: 3 results)

  • [Int'l Joint Research] 国科温州研究院(中国)

    • Related Report
      2022 Research-status Report
  • [Journal Article] The Effect of Lysozyme on the Aggregation and Charging of Oxidized Carbon Nanohorn (CNHox) in Aqueous Solution2024

    • Author(s)
      Tian Zhengjian、Li Maolin、Sugimoto Takuya、Kobayashi Motoyoshi
    • Journal Title

      Applied Sciences

      Volume: 14 Issue: 6 Pages: 2645-2645

    • DOI

      10.3390/app14062645

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Effects of ionic valence on aggregation kinetics of colloidal particles with and without a mixing flow2023

    • Author(s)
      Gao Jiahui、Sugimoto Takuya、Kobayashi Motoyoshi
    • Journal Title

      Journal of Colloid and Interface Science

      Volume: 638 Pages: 733-742

    • DOI

      10.1016/j.jcis.2023.02.019

    • Related Report
      2023 Annual Research Report 2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Adsorption kinetics of polyacrylamide-based polyelectrolyte onto a single silica particle studied using microfluidics and optical tweezers2023

    • Author(s)
      Geonzon Lester C.、Kobayashi Motoyoshi、Sugimoto Takuya、Adachi Yasuhisa
    • Journal Title

      Journal of Colloid and Interface Science

      Volume: 630 Pages: 846-854

    • DOI

      10.1016/j.jcis.2022.10.067

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Climbing Colloidal Suspension2023

    • Author(s)
      Kobayashi Motoyoshi、Sugimoto Takuya、Sato Shunsuke、Ishibashi Ryouichi
    • Journal Title

      Liquids

      Volume: 3 Issue: 1 Pages: 40-47

    • DOI

      10.3390/liquids3010004

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Colloidal Dispersion System2023

    • Author(s)
      杉本卓也、小林幹佳
    • Journal Title

      Oleoscience

      Volume: 23 Issue: 3 Pages: 153-158

    • DOI

      10.5650/oleoscience.23.153

    • ISSN
      1345-8949, 2187-3461
    • Related Report
      2022 Research-status Report
  • [Journal Article] Aggregation and charging of natural allophane particles in the presence of oxyanions2022

    • Author(s)
      Li Maolin、Sugimoto Takuya、Yamashita Yuji、Kobayashi Motoyoshi
    • Journal Title

      Colloids and Surfaces A: Physicochemical and Engineering Aspects

      Volume: 649 Pages: 129413-129413

    • DOI

      10.1016/j.colsurfa.2022.129413

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Effect of pH and electrolyte concentration on sol?gel state of semi-dilute aqueous cellulose nanofiber suspension: an interpretation based on angle-dependent DLVO theory2022

    • Author(s)
      Kobayashi Motoyoshi、Sato Yusuke、Sugimoto Takuya
    • Journal Title

      Colloid and Polymer Science

      Volume: 300 Issue: 8 Pages: 953-960

    • DOI

      10.1007/s00396-022-04999-7

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Interaction between silica particles with poly(ethylene oxide) studied using an optical tweezer: insignificant effect of poly(ethylene oxide) on long-range double layer interaction2022

    • Author(s)
      Geonzon Lester C.、Kobayashi Motoyoshi、Sugimoto Takuya、Adachi Yasuhisa
    • Journal Title

      Colloid and Polymer Science

      Volume: 300 Issue: 10 Pages: 1179-1186

    • DOI

      10.1007/s00396-022-05020-x

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] The comparison of adsorption kinetics of polystyrene particles with two polyelectrolytes near the isoelectric points2022

    • Author(s)
      Feng Lili、Duan Lifan、Zhuang Yiran、Sugimoto Takuya、Adachi Yasuhisa
    • Journal Title

      Colloids and Surfaces A: Physicochemical and Engineering Aspects

      Volume: 655 Pages: 130297-130297

    • DOI

      10.1016/j.colsurfa.2022.130297

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Heteroaggregation rate coefficients between oppositely charged particles in a mixing flow: Effect of surface charge density and salt concentration2022

    • Author(s)
      Sugimoto Takuya、Adachi Yasuhisa、Kobayashi Motoyoshi
    • Journal Title

      Colloids and Surfaces A: Physicochemical and Engineering Aspects

      Volume: 632 Pages: 127795-127795

    • DOI

      10.1016/j.colsurfa.2021.127795

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Study on the kinetics of adsorption of poly(ethylene oxide) onto a silica particle using optical tweezers and microfluidics2022

    • Author(s)
      Geonzon Lester C.、Kobayashi Motoyoshi、Sugimoto Takuya、Adachi Yasuhisa
    • Journal Title

      Colloids and Surfaces A: Physicochemical and Engineering Aspects

      Volume: 642 Pages: 128691-128691

    • DOI

      10.1016/j.colsurfa.2022.128691

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Inhibited nanobubble transport in a saturated porous medium: Effects of deposited colloidal particles2021

    • Author(s)
      Sugimoto Takuya、Hamamoto Shoichiro、Nishimura Taku
    • Journal Title

      Journal of Contaminant Hydrology

      Volume: 242 Pages: 103854-103854

    • DOI

      10.1016/j.jconhyd.2021.103854

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Presentation] Hetero-aggregation in the presence of multivalent ions2023

    • Author(s)
      Takuya Sugimoto
    • Organizer
      China-Japan Seminar on Interfacial Progress and Control Measures of Combined Pollutants
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Effect of Lysozyme on the Aggregation and Charging of Oxidized Carbon Nanohorn (CNHox) in Aqueous Solution2023

    • Author(s)
      Tian Zhengjian; Li Maolin; Sugimoto Takuya; 小林 幹佳
    • Organizer
      2023年度土壌物理学会大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] アルミナビーズ充填カラム中におけるセルロースナノクリスタル粒子の沈着挙動2023

    • Author(s)
      杉本 卓也; 小林 幹佳
    • Organizer
      2023年度(第72回)農業農村工学会大会講演会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 振動下における高濃度の微粒子懸濁液の挙動について2023

    • Author(s)
      小林 幹佳; 杉本 卓也; 佐藤 駿介; 石橋 諒一
    • Organizer
      2023年度(第72回)農業農村工学会大会講演会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 振動下におけるシリカ微粒子と水の混合物の挙動2023

    • Author(s)
      小林 幹佳; 杉本 卓也; 佐藤 駿介; 石橋 諒一
    • Organizer
      第74回コロイドおよび界面化学討論会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 濃厚コロイド懸濁液のシアシックニングと電気二重層斥力の関係2023

    • Author(s)
      石橋 諒一; 杉本 卓也; 瀬戸 亮平; 小林 幹佳
    • Organizer
      第74回コロイドおよび界面化学討論会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 臨界凝集濃度への流れの効果2022

    • Author(s)
      杉本卓也,高家輝,小林幹佳
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] The effect of various oxyanions on the charging and aggregation of natural allophane particles2022

    • Author(s)
      Li Maolin, Sugimoto Takuya, Yamashita Yuji, Kobayashi Motoyoshi
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] Effect of lysozyme on the aggregation of oxidized carbon nanohorn (CNHox) in aqueous solution2022

    • Author(s)
      Tian Zhengjian, Sugimoto Takuya, Kobayashi Motoyoshi
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] Effects of counter-ionic valence on aggregation kinetics of colloidal particles with mixing flow2022

    • Author(s)
      Gao Jiahui, Sugimoto Takuya, Kobayashi Motoyoshi
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] シリカと水の濃厚分散系の挙動について2022

    • Author(s)
      小林 幹佳, 杉本 卓也, 佐藤 駿介, 石橋 諒一
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] 高濃度シリカ分散液のシェアシックニング2022

    • Author(s)
      石橋 諒一, 杉本 卓也, 小林 幹佳
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] 準希薄なセルロースナノクリスタル懸濁液のゾル-ゲル状態2022

    • Author(s)
      張 夕瑜, 杉本 卓也, 小林 幹佳
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] 振動下における濃厚懸濁液のクライミング現象2022

    • Author(s)
      杉本卓也, 佐藤 駿介, 石橋 諒一, 小林 幹佳
    • Organizer
      第10回ソフトマター研究会
    • Related Report
      2022 Research-status Report
  • [Presentation] 濃厚なシリカ-PEG懸濁液のシェアシックニング2022

    • Author(s)
      石橋 諒一, 杉本卓也, 小林 幹佳
    • Organizer
      第10回ソフトマター研究会
    • Related Report
      2022 Research-status Report
  • [Presentation] Effect of flow on critical coagulation concentration of colloidal microplastic particles2022

    • Author(s)
      Sugimoto Takuya
    • Organizer
      International Congress on Pure & Applied Chemistry Kota Kinabalu
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] コロイドの臨界凝集濃度:同種・異種粒子と流れの効果2022

    • Author(s)
      杉本 卓也
    • Organizer
      東京理科大学ウォーターフロンティア研究センター(WaTUS) 第7回イブニングセミナー
    • Related Report
      2022 Research-status Report
    • Invited
  • [Presentation] Heteroaggregation rates of oppositely charged colloidal particles in a mixing flow: effect of charge density2021

    • Author(s)
      Sugimoto Takuya, Kobayashi Motoyoshi
    • Organizer
      The 8th Asian Particle Technology Symposium
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research

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Published: 2021-04-28   Modified: 2025-01-30  

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