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Direct observation of mantle-water reaction in subduction zone using neutron imaging

Research Project

Project/Area Number 21K18641
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 17:Earth and planetary science and related fields
Research InstitutionTohoku University

Principal Investigator

Sakamaki Tatsuya  東北大学, 理学研究科, 助教 (30630769)

Project Period (FY) 2021-07-09 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥6,240,000 (Direct Cost: ¥4,800,000、Indirect Cost: ¥1,440,000)
Fiscal Year 2023: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2022: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2021: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords中性子イメージング / 水 / 高圧 / 高温 / マントル / 水素
Outline of Research at the Start

水の惑星とも呼ばれる地球において、マントル-水反応は普遍的な現象であり、火山や地震なども含めた地球内部活動に多大に影響を及ぼす。マントル中での水の挙動を知ることは極めて重要であるため、本研究では特に重要な「プレートからマントルへの水の移動」と「マントルの水和」の2つに焦点を当てて研究を進める。
研究遂行のためには中性子イメージングの利用が不可欠であり、日本のような沈み込み帯の直下における地学現象の可視化を目指す極めて挑戦的な研究である。最終的にはマントルウェッジ周辺での流体の挙動と役割を解明する。

Outline of Final Research Achievements

Using neutron diffraction experiments, I succeeded in directly determining the structure of hydrous sodium silicate melts (including hydrogen positions), which was not possible by X-ray diffraction. I obtained structural data of silicate melts under pressure conditions up to 5 GPa, and I’m able to understand the pressure dependence of each bond. I found that the hydrogen-oxygen bond distance is sensitive to pressure and I concluded that pressure-induced polymerization occurs.
I constructed an experimental cell that can maintain stable high temperature and high pressure conditions for a long time, and succeeded in obtaining the neutron imaging under high temperature and high pressure conditions. I confirmed that there is a correlation between the amount of hydrogen and the intensity in the imaging (degree of absorption), which enables us to directly observe the distribution of hydrogen in the sample.

Academic Significance and Societal Importance of the Research Achievements

地球科学という観点に立つと、軽い元素を対象にした研究を避けることはできない。特に地球という惑星を考えた場合、「水」は極めて重要な物質である。そこで、水を研究する上で有効な中性子ビームを活用することに目を付けた。本研究で実現した地球内部を再現した高温高圧条件下における中性子イメージングは、世界的に見ても非常に珍しく、先導的な研究・技術である。高温高圧発生プレスと中性子イメージング技術を組み合わせた測定システムの構築・最適化は大きなブレイクスルーであり、他の研究テーマにも適用されることが期待される。つまり、高温高圧中性子イメージングを利用した今後の地球科学の発展にも繋がり、極めて波及効果が高い。

Report

(4 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • 2021 Research-status Report
  • Research Products

    (31 results)

All 2024 2023 2022 2021

All Journal Article (10 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 10 results,  Open Access: 7 results) Presentation (20 results) (of which Int'l Joint Research: 13 results,  Invited: 1 results) Book (1 results)

  • [Journal Article] Elastic wave velocity measurements of sodium aluminosilicate glass and melt at high pressure and temperature2024

    • Author(s)
      Takahashi Naoki、Sakamaki Tatsuya、Ikeda Osamu、Kakizawa Sho、Higo Yuji、Suzuki Akio
    • Journal Title

      Physics of the Earth and Planetary Interiors

      Volume: 350 Pages: 107167-107167

    • DOI

      10.1016/j.pepi.2024.107167

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Magnetic Spin-Flop Transition of ε-FeOOH at 8 GPa2023

    • Author(s)
      Ikeda Osamu、Sakamaki Tatsuya、Mitsui Takaya、Fujiwara Kosuke、McCammon Catherine A.、Suzuki Akio
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 92 Issue: 4 Pages: 043702-043702

    • DOI

      10.7566/jpsj.92.043702

    • Related Report
      2023 Annual Research Report 2022 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] A Molecular‐Scale Origin of Shear Thinning and Brittle Failure of Silicate Melt2023

    • Author(s)
      Okumura S.、Uesugi K.、Goto A.、Matsumoto K.、Sakamaki T.
    • Journal Title

      Geophysical Research Letters

      Volume: 50 Issue: 16

    • DOI

      10.1029/2023gl104083

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Molecular-scale structural changes of silicate melts under tension revealed by time-resolved X-ray diffraction2023

    • Author(s)
      Okumura Satoshi、Uesugi Kentaro、Goto Akio、Namiki Atsuko、Matsumoto Kazuhisa、Sakamaki Tatsuya
    • Journal Title

      Chemical Geology

      Volume: 621 Pages: 121372-121372

    • DOI

      10.1016/j.chemgeo.2023.121372

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Deuterium Content and Site Occupancy in Iron Sulfide at High Pressure and Temperature Determined Using In Situ Neutron Diffraction Measurements2023

    • Author(s)
      Abeykoon Sumith、Howard Christopher、Dominijanni Serena、Eberhard Lisa、Kurnosov Alexander、Frost Daniel J.、Ballaran Tiziana Boffa、Terasaki Hidenori、Sakamaki Tatsuya、Suzuki Akio、Ohtani Eiji、Sano‐Furukawa Asami、Abe Jun
    • Journal Title

      Journal of Geophysical Research: Solid Earth

      Volume: 128 Issue: 9

    • DOI

      10.1029/2023jb026710

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Density deficit of Earth’s core revealed by a multimegabar primary pressure scale2023

    • Author(s)
      Ikuta Daijo、Ohtani Eiji、Fukui Hiroshi、Sakamaki Tatsuya、Heid Rolf、Ishikawa Daisuke、Baron Alfred Q.?R.
    • Journal Title

      Science Advances

      Volume: 9 Issue: 36

    • DOI

      10.1126/sciadv.adh8706

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] High Pressure Melts2022

    • Author(s)
      Sakamaki Tatsuya、Ohtani Eiji
    • Journal Title

      Reviews in Mineralogy and Geochemistry

      Volume: 87 Issue: 1 Pages: 557-574

    • DOI

      10.2138/rmg.2022.87.11

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Structure of basaltic glass at pressures of up to 18 GPa2021

    • Author(s)
      Ohashi Tomonori、Sakamaki Tatsuya、Funakoshi Ken-ichi、Hattori Takanori、Hisano Naoki、Abe Jun、Suzuki Akio
    • Journal Title

      American Mineralogist

      Volume: in press Issue: 3 Pages: 325-335

    • DOI

      10.2138/am-2021-7742

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Phase transitions of ScOOH under high pressure2021

    • Author(s)
      Ito Yoshiaki、Ikeda Osamu、Ban Rintaro、Kubota Taito、Sakamaki Tatsuya、Kuribayashi Takahiro、Suzuki Akio
    • Journal Title

      High Pressure Research

      Volume: 41 Issue: 3 Pages: 275-289

    • DOI

      10.1080/08957959.2021.1964495

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Journal Article] Synchrotron Mossbauer spectroscopic and x-ray diffraction study of ferropericlase in the high-pressure range of the lower mantle region2021

    • Author(s)
      Hamada Maki、Kamada Seiji、Ohtani Eiji、Sakamaki Tatsuya、Mitsui Takaya、Masuda Ryo、Hirao Naohisa、Ohishi Yasuo、Akasaka Masahide
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 17 Pages: 1-9

    • DOI

      10.1103/physrevb.103.174108

    • Related Report
      2021 Research-status Report
    • Peer Reviewed
  • [Presentation] 放射光X線回折実験に基づく高圧下におけるCO2を含むナトリウムケイ酸塩メルトの構造解析2024

    • Author(s)
      早舩 紫野、坂巻 竜也、鈴木 昭夫
    • Organizer
      2023年度量子ビームサイエンスフェスタ
    • Related Report
      2023 Annual Research Report
  • [Presentation] 高圧下における水の定量評価:高圧中性子CT法の開発2024

    • Author(s)
      有馬 寛、服部 高典、佐野 亜沙美、町田 真一、阿部 淳、舟越 賢一、坂巻 竜也
    • Organizer
      2023年度量子ビームサイエンスフェスタ
    • Related Report
      2023 Annual Research Report
  • [Presentation] Neutron diffraction study of hydrous sodium silicate melt at high pressure and high temperature2023

    • Author(s)
      Tatsuya Sakamaki
    • Organizer
      Goldschmidt 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Effect of CO2 on the structure of sodium silicate melt at high pressure2023

    • Author(s)
      Shino Hayafune, Tatsuya Sakamaki, Tomonori Ohashi, Akio Suzuki
    • Organizer
      Japan Geoscience Union Meeting 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Elastic wave velocity measurement of a sodium aluminosilicate glass and melt at high pressure and high temperature2023

    • Author(s)
      Naoki Takahashi, Tatsuya Sakamaki, Osamu Ikeda, Sho Kakizawa, Yuji Higo, Akio Suzuki
    • Organizer
      Japan Geoscience Union Meeting 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sound velocity measurement of B2 Fe-Ni-Si alloys at high pressure and high temperature2023

    • Author(s)
      Daijo Ikuta, Eiji Ohtani, Hiroshi Fukui, Tatsuya Sakamaki, Izumi Mashino, Daisuke Ishikawa, Alfred Q. R. Baron
    • Organizer
      Japan Geoscience Union Meeting 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 含水ケイ酸塩メルトの中性子回折構造解析と鉄メルトの中性子イメー ジング2023

    • Author(s)
      坂巻 竜也、大橋 智典、高橋 直生、服部 高典、有馬 寛、舟越 賢一
    • Organizer
      第64回 高圧討論会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 高温高圧下におけるナトリウムアルミノ珪酸塩ガラス・メルトの弾性波速度測定2023

    • Author(s)
      高橋 直生、坂巻 竜也、池田 理、 柿澤 翔、肥後 祐司、鈴木 昭夫
    • Organizer
      第64回 高圧討論会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Longitudinal wave velocity of sodium aluminosilicate melt at high pressure2022

    • Author(s)
      Sakamaki, T
    • Organizer
      Japan Geoscience Union Meeting 2022
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] H2O-induced melting at the uppermost lower mantle2022

    • Author(s)
      Sakamaki, T
    • Organizer
      Japan Geoscience Union Meeting 2022
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] Pressure-induced structural change of basaltic glass up to 18 GPa2022

    • Author(s)
      Ohashi, T., Sakamaki, T., Funakoshi, K., Hattori, T., Suzuki, A.
    • Organizer
      Japan Geoscience Union Meeting 2022
    • Related Report
      2022 Research-status Report
  • [Presentation] Density of Fe2O3-bearing magma under high pressure2022

    • Author(s)
      Ban, R., Sakamaki, T., Suzuki, A.
    • Organizer
      Japan Geoscience Union Meeting 2022
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] e-FeOOH の鉄スピン転移と弾性波速度2022

    • Author(s)
      池田 理、坂巻 竜也、福井 宏之、内山 裕士、三井 隆也、藤原 孝将、BARON Alfred、鈴木 昭夫
    • Organizer
      第63回高圧討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] 超高圧下における X 線非弾性散乱法による鉄合金およびレニウムの音速測定とその地球内部への適用2022

    • Author(s)
      大谷 栄治、生田 大穣、福井 宏、坂巻 竜也、増野 いづみ、境 毅、石川 大輔、BARON Alfred
    • Organizer
      第63回高圧討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] Viscosity of silicate melts under high pressures2021

    • Author(s)
      Sakamaki, T
    • Organizer
      Japan Geoscience Union Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Elastic wave velocity of silicate glasses at high pressure2021

    • Author(s)
      Sakamaki, T
    • Organizer
      Japan Geoscience Union Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Pressure-induced structural change of basaltic glass up to 18 GPa2021

    • Author(s)
      Ohashi, T., Sakamaki, T., Funakoshi, K., Hattori, T., Hisano, N., Abe, J., Suzuki, A.
    • Organizer
      Japan Geoscience Union Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Density of Fe2O3-bearing magma under high pressure2021

    • Author(s)
      Ban, R., Sakamaki, T., Suzuki
    • Organizer
      Japan Geoscience Union Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Elastic wave velocity of ε-FeOOH across the pressure-induced spin transition of iron2021

    • Author(s)
      Ikeda, O., Sakamaki, T., Fukui, H., Uchiyama, H., Baron, A.Q.R., Suzuki, A.
    • Organizer
      Japan Geoscience Union Meeting
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] Deuterium content and site occupancy in iron sulphide at high pressure and high temperature: Implications for the oxidation of early Earth’s mantle2021

    • Author(s)
      Abeykoon, S., Howard, C.M., Dominijanni, S., Eberhard, L., Frost, D.J., Ballaran, T.B., Kurnosov, A., Terasaki, H., Sakamaki, T., Suzuki, A., Ohtani, E., Sano-Furukawa, A., Abe, J.
    • Organizer
      Goldschmidt 2021
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Book] Static and Dynamic High Pressure Mineral Physics2022

    • Author(s)
      Yingwei Fei, Michael J. Walter
    • Total Pages
      418
    • Publisher
      Cambridge University Press
    • ISBN
      9781108479752
    • Related Report
      2022 Research-status Report

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Published: 2021-07-13   Modified: 2025-01-30  

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