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Construction of Production Base of Strain-Controlled Graphene Nanoribbon-Base Bio-Sensor for Detecting Multi-Molecules in Liquid

Research Project

Project/Area Number 21K18665
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 18:Mechanics of materials, production engineering, design engineering, and related fields
Research InstitutionTohoku University

Principal Investigator

Miura Hideo  東北大学, 工学研究科, 教授 (90361112)

Project Period (FY) 2021-07-09 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
Fiscal Year 2022: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2021: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywordsひずみ / グラフェン / 分子吸着 / バイオセンサ / 界面制御 / 歪み
Outline of Research at the Start

本研究ではグラフェンナノリボン表面の歪み状態を制御することで,特定の分子の吸着あるいは脱離特性を可逆的に変化させる技術を確立する.またグラフェンナノリボン表面に特定の分子吸着を制御する機能性分子と表面保護皮膜をコーティングし,気体あるいは液体中に存在する当該分子の選択的検出を可能とする基本技術も構築する.これにより,マルチ分子選択センサ開発に向けた歪み制御多機能バイオセンサ開発の基盤技術の構築を図る.

Outline of Final Research Achievements

The effect of substrate material and strain on the gas-molecule adsorption behavior of graphene was clarified quantitatively by applying the first principles calculation. It was found that the electronic band structure of graphene varied drastically from electron conduction type to hole conduction type as a strong function of the substrate material. In addition, the direct growth process of carbon nanotube on graphene was successfully developed. The grown CNT plays an important role as catalyst for improving the sensitivity of gas molecules. It was validated that the adsorption energy of NO2 gas molecule was improved under the application of uniaxial strain by 15 meV/1%-strain. These results clearly indicate the possibility of the development of multi-gas detecting sensor with high sensitivity and selectivity.

Academic Significance and Societal Importance of the Research Achievements

CNT-グラフェンハイブリッドセンサはグラフェン単体センサより約6倍の感度向上と約5倍の脱離速度を有することを実証し,センサの高性能化に向けた設計指針を構築できた.またグラフェンの電気抵抗率変化の歪み依存性をシリコンデバイス比約1000倍にまで向上させることもでき,超高感度歪みセンサへの応用可能性も示した.本研究成果の独創性や工学的有用性などは国内外の学会賞の受賞などでも評価されている.これにより危険環境中の有害物質検出や,人体の体液や血液中の目標分子の存在や濃度を高感度で定量的に検出可能なマルチ分子選択センサ開発に向けた歪み制御多機能バイオセンサ開発の基盤技術の構築ができたものと考えている.

Report

(3 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • Research Products

    (24 results)

All 2023 2022 2021 Other

All Int'l Joint Research (2 results) Journal Article (8 results) (of which Int'l Joint Research: 6 results,  Peer Reviewed: 8 results,  Open Access: 8 results) Presentation (12 results) (of which Int'l Joint Research: 9 results,  Invited: 2 results) Remarks (2 results)

  • [Int'l Joint Research] 清華大学/北京科学技術大学(中国)

    • Related Report
      2022 Annual Research Report
  • [Int'l Joint Research] 北京科学技術大学/清華大学(中国)

    • Related Report
      2021 Research-status Report
  • [Journal Article] Improvement of the Sensitivity and Selectivity of Gas Molecules of Graphene-base Gas Sensor with Carbon Nanotubes under the Application of Strain2023

    • Author(s)
      Yuto Hirose, Xiangyu Qiao, Wangyang Fu, Ken Suzuki, and Hideo Miura
    • Journal Title

      Proc. ASME IMECE2022

      Volume: 12

    • DOI

      10.1115/imece2022-95307

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Penta-graphene and phagraphene: thermal expansion, linear compressibility, and Poisson’s ratio2022

    • Author(s)
      Lei Wang, Ying Chen, Hideo Miura, Ken Suzuki and Cong Wang
    • Journal Title

      Journal of Physics: Condensed Matter

      Volume: 34 Issue: 50 Pages: 505301-505301

    • DOI

      10.1088/1361-648x/ac9c3e

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Tunable uniaxial, area, and volume negative thermal expansion in quartz-like and diamond-like metalorganic frameworks2022

    • Author(s)
      Lei Wang, Ying Chen, Hideo Miura, Ken Suzuki and Cong Wang
    • Journal Title

      Royal Society of Chemistry (RSC) Advances

      Volume: 12 Issue: 34 Pages: 21770-21779

    • DOI

      10.1039/d2ra03292a

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Strain-Induced Change in the Photonic Properties of Dumbbell-Shaped Graphene Nanoribbon Structures2022

    • Author(s)
      Goundar Jowesh Avisheik、Suzuki Ken、Miura Hideo
    • Journal Title

      Proc. of International Conference on Electronic Packaging

      Volume: - Pages: 81-82

    • DOI

      10.23919/icep55381.2022.9795457

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Strain-Induced Change of Adsorption Behaviour of Gas Molecules on Graphene Analyzed by Density Functional Method2022

    • Author(s)
      Yin Meng、Qiao Xiangyu、Zhang Qinqiang、Suzuki Ken、Wang Lei
    • Journal Title

      Proc. ASME 2022 International Mechanical Engineering Congress and Exposition

      Volume: 9 Pages: 1-7

    • DOI

      10.1115/imece2022-94892

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Detachable Fine Bump Connection Using Multi-Walled Carbon-Nanotube Bundles for 3D Semiconductor Modules2022

    • Author(s)
      Masasuke Kobayashi, Ken Suzuki, Hideo Miura
    • Journal Title

      Micro- and Nano-Systems Engineering and Packaging

      Volume: 12

    • DOI

      10.1115/imece2021-70172

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Improvement in Photosensitivity of Dumbbell-Shaped Graphene Nanoribbon Structures by Using Asymmetric Metallization Technique2021

    • Author(s)
      Goundar Jowesh Avisheik、Xiangyu Qiao、Suzuki Ken、Miura Hideo
    • Journal Title

      International Mechanical Engineering Congress & Exposition (IMECE 2021), Proceedings,

      Volume: IMECE2021 Pages: 1-6

    • DOI

      10.1115/imece2021-69917

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Theoretical study on strain-controllable gradient Schottky barrier of dumbbell-shape graphene nanoribbon for highly sensitive strain sensors2021

    • Author(s)
      Qinqiang Zhang; Ken Suzuki; Hideo Miura
    • Journal Title

      Proc. of 2021 International Conference on Simulation of Semiconductor Processes and Devices (SISPAD)

      Volume: 2021 Pages: 171-174

    • DOI

      10.1109/sispad54002.2021.9592548

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Strain-Induced Change in the Photonic Properties of Dumbbell-Shaped Graphene Nanoribbon Structures2022

    • Author(s)
      Jowesh Avisheik Goundar
    • Organizer
      International Conference on Electronic Packaging
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Strain-induced Change of Adsorption Behaviour of Gas Molecules on Graphene: A first-principles Study2022

    • Author(s)
      Meng Yin
    • Organizer
      15th World Congress on Computational Mechanics (WCCM-XV)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Point Defect-Induced Variation of Electronic Properties and Reliability of Oxides for High Performance Devices2022

    • Author(s)
      Hideo MIURA
    • Organizer
      The 12th International Conference on High-Performance Ceramics
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] First-Principles Analysis on the Strain-Induced Variation of Adsorption Behavior of Gas Molecules on Graphene2022

    • Author(s)
      Meng Yin
    • Organizer
      ASME VVUQ2022: Verification, Validation, and Uncertainty Quantification Symposium
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Band-Gap Modulation of Dumbbell-Shaped Graphene Nanoribbon Structures by Application of Uniaxial Tensile Strain2022

    • Author(s)
      Jowesh Goundar
    • Organizer
      2nd International Conference on Diamond and Carbon Materials (ICDCM)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Substrate Material Effects on the Electronic Band Structure of Graphene and the Adsorption Properties of Gas Molecules on its Surface2022

    • Author(s)
      Kenryu Hasegawa
    • Organizer
      17th Asia-Pacific Conference on Fracture and Strength (APCFS2022)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 水分子吸着に伴うグラフェン電気抵抗変化挙動の基板材質依存性2022

    • Author(s)
      喬 向宇
    • Organizer
      第69回応用物理学会春季学術講演会
    • Related Report
      2021 Research-status Report
  • [Presentation] グラフェンの電子バンド構造に及ぼす基板材料の影響の第一原理解析2022

    • Author(s)
      長谷川堅隆
    • Organizer
      日本機械学会東北支部 東北学生会 第 52 回学生員卒業研究発表講演会
    • Related Report
      2021 Research-status Report
  • [Presentation] Strain Sensitivity of Electron Transport Properties of Dumbbell-Shape Graphene Nanoribbon and Its Application to Mobile Photovoltaic Devices2021

    • Author(s)
      Hideo Miura
    • Organizer
      3rd Global Summit on Physics 2021, Prague, Chez Republic
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Improvement in Photosensitivity of Dumbbell-Shaped Graphene Nanoribbon Structures by Using Asymmetric Metallization Technique2021

    • Author(s)
      Jowesh Avisheik Goundar
    • Organizer
      ASME International Mechanical Engineering Congress & Exposition (IMECE 2021)
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Presentation] グラフェン上ガス分子吸着脱離特性の歪み依存性に関する第一原理解析2021

    • Author(s)
      YIN MENG
    • Organizer
      日本機械学会 第34回計算力学講演会(CMD2021)
    • Related Report
      2021 Research-status Report
  • [Presentation] Strain-induced change of molecule adsorption on a graphene-base gas senor2021

    • Author(s)
      Xiangyu Qiao
    • Organizer
      2021 International Conference on Solid State Devices and Materials
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research
  • [Remarks] 三浦・鈴木研究室

    • URL

      http://www.miura.rift.mech.tohoku.ac.jp

    • Related Report
      2022 Annual Research Report
  • [Remarks] 東北大学 三浦・鈴木研究室

    • URL

      http://www.miura.rift.mech.tohoku.ac.jp

    • Related Report
      2021 Research-status Report

URL: 

Published: 2021-07-13   Modified: 2024-01-30  

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