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Three-dimensional thermal diodes fabricated using selective bonding of transparent nanospheres

Research Project

Project/Area Number 21K18671
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 18:Mechanics of materials, production engineering, design engineering, and related fields
Research InstitutionNagaoka University of Technology

Principal Investigator

Mizoshiri Mizue  長岡技術科学大学, 工学研究科, 准教授 (70586594)

Co-Investigator(Kenkyū-buntansha) 石川 善恵  国立研究開発法人産業技術総合研究所, 材料・化学領域, 主任研究員 (20509129)
Project Period (FY) 2021-07-09 – 2023-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥6,370,000 (Direct Cost: ¥4,900,000、Indirect Cost: ¥1,470,000)
Fiscal Year 2022: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2021: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Keywords球状ナノ粒子 / レーザ微細加工 / 接合 / 還元 / Cu2O / 熱ダイオード
Outline of Research at the Start

本研究の目的は,申請者らがこれまでに発見したフェムト秒レーザパルス照射により透明なCu2O球状ナノ粒子が単層でCu薄膜上へ局所接合される新規現象を応用し,Cu2O球状ナノ粒子の局所接合・還元を用いた3次元熱ダイオードを創製することにある.具体的には,Cu・Cu2O球状ナノ粒子の3次元積層構造を作製し,Cu-Cu2O接合による熱整流作用を3次元的に利用する.特に,フェムト秒レーザを用いた選択還元接合は空間的・時間的熱マネージメントを必要とするプロセスであり,3次元熱ダイオードの熱整流特性の評価を通して,Cu2O微小球の接合還元現象の解明に挑戦する.

Outline of Final Research Achievements

Cu2O nanospheres, which were coated on various thin film metal substrates, were irradiated by near-infrared femtosecond laser pulses to investigate the bonding mechanism of single-layered and multi- and melted Cu2O nanospheres on the substrates. The minimum pulse energy of Cu2O nanosphere bonding on the thin film substrates such as Au, Cu, Cr, and Si materials were examined. On the other hand, the electric field intensity distributions and temperature distributions were calculated using electromagnetic filed analysis and heat transfer analysis. These results suggest that the local bonding was caused by the electromagnetic enhancement between Cu2O nanospheres and underlying metal thin films.

Academic Significance and Societal Importance of the Research Achievements

フェムト秒レーザパルス照射により透明なCu2O球状ナノ粒子が単層でCu薄膜上へ局所接合される新規現象を応用し,Cu2O球状ナノ粒子の局所接合・還元メカニズムを明らかにした.局所的な電場増強の光熱変換による接合の可能性を示唆する結果は熱の局所制御の知見として学術的意義があり,社会的には,還元焼結によるCuパターニング技術への応用が期待できる.

Report

(3 results)
  • 2022 Annual Research Report   Final Research Report ( PDF )
  • 2021 Research-status Report
  • Research Products

    (10 results)

All 2022 2021

All Journal Article (1 results) (of which Peer Reviewed: 1 results,  Open Access: 1 results) Presentation (9 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results)

  • [Journal Article] Bonding of single-layered Cu2O nanospheres on Cu substrates in irradiating near-infrared femtosecond laser pulses2022

    • Author(s)
      Shohei Murayama, Kien Vu Trung Nguyen, Masateru Anzai, Hideyuki Magara, Takahiro Nakamura and Mizue Mizoshiri
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: - Issue: SD Pages: SD1032-SD1032

    • DOI

      10.35848/1347-4065/ac54f1

    • Related Report
      2021 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Bonding Mechanism of Polydispersed Cu2O Nanospheres on Cu Thin Films by Irradiating Femtosecond Laser Pulses2022

    • Author(s)
      Mizue Mizoshiri, Masateru Anzai, Shohei Murayama, Kien Vu Trung Nguyen, Hideyuki Magara, Takahiro Nakamura
    • Organizer
      16th International Conference on Laser Ablation (COLA2021/2022)
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] フェムト秒レーザ多光子熱還元によるCu2O /NiO混合ナノ球インクを用いたCu-Ni合金の大気中描画2022

    • Author(s)
      NGUYEN VU TRUNG KIEN,小林 優希,Tran Duc Thuan,溝尻 瑞枝
    • Organizer
      第13回「マイクロ・ナノ工学シンポジウム」
    • Related Report
      2022 Annual Research Report
  • [Presentation] Direct writing of Cu-Ni alloy patterns fabricated by femtosecond laser multiphoton reductive sintering using Cu2O/NiO nanosphere mixed ink2022

    • Author(s)
      Kien Vu Trung Nguyen, Yuki Kobayashi, Thuan Duc Tran, Mizue Mizoshiri
    • Organizer
      7th STI-Gigaku 2022
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ポンプ・プローブ法を用いたCu2O球状ナノ粒子のフェムト秒レーザ局所接合の観測2022

    • Author(s)
      小林 優希,VU TRUNG KIEN NGUYEN,TRAN DUC THUAN,溝尻 瑞枝
    • Organizer
      日本機械学会北陸信越支部2023年合同講演会
    • Related Report
      2022 Annual Research Report
  • [Presentation] フェムト秒レーザーパルス照射によるCu2O微小球の局所加熱還元接合2022

    • Author(s)
      溝尻 瑞枝,村山 章平,NGUYEN VU TRUNG KIEN,安西 将輝,真柄 英之,中村 貴宏
    • Organizer
      レーザー学会学術講演会第42回年次大会
    • Related Report
      2021 Research-status Report
  • [Presentation] 3次元Cu微細造形に向けたCu2O球状ナノ粒子のフェムト秒レーザパルス誘起局所加熱接合"2022

    • Author(s)
      溝尻 瑞枝
    • Organizer
      第96回レーザ加工学会講演会
    • Related Report
      2021 Research-status Report
    • Invited
  • [Presentation] フェムト秒レーザパルス照射による多分散Cu2O球状ナノ粒子のCu薄膜上への還元接合2022

    • Author(s)
      安西 将輝,村山 章平,真柄 英之,中村 貴宏,溝尻 瑞枝
    • Organizer
      日本機械学会北陸信越支部2022年合同講演会
    • Related Report
      2021 Research-status Report
  • [Presentation] 3D微細造形のためのCu薄膜上へのCu2O微小球還元接合特性評価2021

    • Author(s)
      NGUYEN VU TRUNG KIEN,村山 章平, 安西 将輝,真柄 英之,中村 貴宏,溝尻 瑞枝
    • Organizer
      第12回「マイクロ・ナノ工学シンポジウム」
    • Related Report
      2021 Research-status Report
  • [Presentation] Consideration of the mechanism of single-layered Cu2O nanospheres bonded on metal substrates in irradiating near-infrared femtosecond laser pulses2021

    • Author(s)
      Shohei Murayama, Kien Vu Trung Nguyen, Masateru Anzai, Hideyuki Magara, Takahiro Nakamura, Mizue Mizoshiri
    • Organizer
      34tht International Microprocesses and Nanotechnology Conference (MNC2021)
    • Related Report
      2021 Research-status Report
    • Int'l Joint Research

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Published: 2021-07-13   Modified: 2024-01-30  

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