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Development and application of a holographic method for the analysis of interfaces with atomic resolution using X-ray CTR scattering

Research Project

Project/Area Number 22360018
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionThe University of Tokyo

Principal Investigator

TAKAHASHI Toshio  東京大学, 物性研究所, 教授 (20107395)

Co-Investigator(Kenkyū-buntansha) SHIRASAWA Tetsuro  東京大学, 物性研究所, 助教 (80451889)
Project Period (FY) 2010 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥19,370,000 (Direct Cost: ¥14,900,000、Indirect Cost: ¥4,470,000)
Fiscal Year 2012: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2011: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2010: ¥13,260,000 (Direct Cost: ¥10,200,000、Indirect Cost: ¥3,060,000)
KeywordsX線回折 / 表面・界面 / 位相問題 / ホログラフィ / 放射光 / 超薄膜 / トポロジカル絶縁体 / 結晶成長 / 放射線 / 直接法 / CTR散乱
Research Abstract

A new method for obtaining the interface structure of ultra-thin films on substrates from the analysis of X-Ray CTR scattering has been developed with a holographic method and iterative phase retrieval methods. In the method, inter-atomic layer distances, electron density and its distribution in each atomic layer are obtained for ultra-thin films on substrate. The results give valuable information on electronic states and crystal growth mechanisms.

Report

(4 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (53 results)

All 2013 2012 2011 2010 Other

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (46 results) (of which Invited: 4 results) Remarks (1 results)

  • [Journal Article] Structure of a Bi/Bi2Te3 heteroepitaxial film studied by x-ray crystal truncation rod scattering2013

    • Author(s)
      T.Shirasawa, J.Tsunoda, T.Hirahara and T.Takahashi
    • Journal Title

      Phys. Rev. B

      Volume: 87 Issue: 7 Pages: 75449-75449

    • DOI

      10.1103/physrevb.87.075449

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] A method for measuring the specular X-ray reflectivity with millisecond time resolution2013

    • Author(s)
      W.Voegeli1, T.Matsushita, E.Arakawa, T.Shirasawa, T.Takahashi and Y. F.Yano
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 425 Issue: 9 Pages: 092003-092003

    • DOI

      10.1088/1742-6596/425/9/092003

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] X線CTR散乱ホログラフィによる表面・界面原子イメージング2012

    • Author(s)
      白澤徹郎、高橋敏男
    • Journal Title

      X線結像光学ニューズレター

      Volume: 36 Pages: 5-7

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] 多波長同時分散型光学系を用いた結晶トランケーションロッド散乱プロファイルの迅速測定法の開発2012

    • Author(s)
      白澤徹郎、荒川悦雄、WolfgangVoegeli、高橋敏男、松下正
    • Journal Title

      放射光

      Volume: 25No.4 Pages: 229-237

    • NAID

      10030494792

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Interface of a Bi(001) film on Si(111)-7× 7 imaged by surface x-ray diffraction2011

    • Author(s)
      T.Shirasawa, M.Ohyama, W.Voegeli, and T.Takahashi
    • Journal Title

      Phys. Rev. B

      Volume: 84 Issue: 7

    • DOI

      10.1103/physrevb.84.075411

    • Related Report
      2012 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quick Measurement of Crystal TruncationRod Profiles in SimultaneousMulti-Wavelength Dispersive Mode2011

    • Author(s)
      T. Matsushita, T. Takahashi, T. Shirasawa, E. Arakawa, H. Toyokawa and H. Tajiri
    • Journal Title

      J. Appl. Phys.

      Volume: 110 Issue: 10

    • DOI

      10.1063/1.3661656

    • Related Report
      2012 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] 実験室特性X線源を用いた高速逆格子空間マッピング法の開発2013

    • Author(s)
      Voegel Wolfgang
    • Organizer
      第60回応用物理学会春季学術講演会
    • Place of Presentation
      神奈川工科大学
    • Year and Date
      2013-03-28
    • Related Report
      2012 Final Research Report
  • [Presentation] CuドープBi2Se3薄膜のX線CTR散乱法による構造解析2013

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学
    • Year and Date
      2013-03-26
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] X線CTR散乱法によるトポロジカル絶縁体Bi2Se3超薄膜の構造解析2013

    • Author(s)
      杉木祐人
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学
    • Year and Date
      2013-03-26
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] X線CTR散乱法によるBi/Bi2Te3トポロジカル絶縁体薄膜の界面構造解析2013

    • Author(s)
      白澤徹郎
    • Organizer
      第30回PFシンポジウム
    • Place of Presentation
      つくば国際会議場
    • Year and Date
      2013-03-14
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] 結晶性ペンタセン絶縁体の表面X線回折法による構造解析2013

    • Author(s)
      白澤徹郎
    • Organizer
      第26回日本放射光学会年会
    • Place of Presentation
      名古屋大学
    • Year and Date
      2013-01-12
    • Related Report
      2012 Final Research Report
  • [Presentation] Atomic-layer-resolved imaging of epitaxially grown ultra thin films with X-ray CTR scattering2012

    • Author(s)
      高橋敏男
    • Organizer
      第8回放射光 表面科学研究部会顕微ナノ材料科学研究会合同シンポジウム
    • Place of Presentation
      慶応義塾大学
    • Year and Date
      2012-11-17
    • Related Report
      2012 Final Research Report
  • [Presentation] KEK低速陽電子回折研究およびPsビーム研究の新展開2012

    • Author(s)
      高橋敏男
    • Organizer
      陽電子回折への招待PF研究会
    • Place of Presentation
      高エネルギー加速器研究機構
    • Year and Date
      2012-10-04
    • Related Report
      2012 Final Research Report
  • [Presentation] A Molecular Arrangement of Pentacene in Ultra Thin Film Revealed by Surface2012

    • Author(s)
      白澤徹郎
    • Organizer
      第10回半導体表面に関する日露セミナー(JRSSS10)
    • Place of Presentation
      東京大学
    • Year and Date
      2012-09-26
    • Related Report
      2012 Final Research Report
  • [Presentation] Quick time-resolved X-ray reflectivity using an undulator source2012

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2012-09-18
    • Related Report
      2012 Final Research Report
  • [Presentation] 波長分散型X線CTR散乱法を用いたルチルTiO2(110)表面超親水化反応の時分割測定2012

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2012-09-18
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] Reconstruction of Atoms at Surface/interface by Using X-ray Crystal Truncation Rod Scattering2012

    • Author(s)
      高橋敏男
    • Organizer
      ISSP International Workshop on 3D Atomic Imaging at Nano-scale active sites in materials
    • Place of Presentation
      東京大学物性研究所
    • Year and Date
      2012-08-07
    • Related Report
      2012 Final Research Report
  • [Presentation] Molecular Arrangement of Pentacene Ultrathin Film Studied with Surface X-ray Scattering2012

    • Author(s)
      白澤徹郎
    • Organizer
      ISSP International Workshop on 3D Atomic Imaging at Nano-scale active sites in materials
    • Place of Presentation
      東京大学物性研究所
    • Year and Date
      2012-08-07
    • Related Report
      2012 Final Research Report
  • [Presentation] Structure of gold atomic chains on the Si(553) surface and their low-temperature structural changes2012

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      ISSP International Workshop on3D Atomic Imaging at Nano-scale activesites in materials
    • Place of Presentation
      東京大学物性研究所
    • Year and Date
      2012-08-07
    • Related Report
      2012 Final Research Report
  • [Presentation] Time-resolved X-ray CTR scattering measurement on the photo-induced hydorophilic transition of the TiO2(110) surface2012

    • Author(s)
      白澤徹郎
    • Organizer
      12th International Conference on Surface X-ray and Neutron Scattering (SXNS12)
    • Place of Presentation
      コルカタ(イ ンド)
    • Year and Date
      2012-07-26
    • Related Report
      2012 Final Research Report
  • [Presentation] Structure of gold atomic chains on the Si(553) surface and their Low-temperature structural changes2012

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      12th International Conference on Surface X-ray and Neutron Scattering(SXNS12)
    • Place of Presentation
      コ ルカタ(インド)
    • Year and Date
      2012-07-26
    • Related Report
      2012 Final Research Report
  • [Presentation] Quick Three-Dimensional Reciprocal Space Mapping in the Simultaneous Multi-Wavelength Dispersive Mode2012

    • Author(s)
      白澤徹郎
    • Organizer
      The 11th International Conference on Synchrotron Radiation Instrumentation
    • Place of Presentation
      リヨ ン(フランス)
    • Year and Date
      2012-07-10
    • Related Report
      2012 Final Research Report
  • [Presentation] 透過型off-Bragg条件におけるX線回折強度とビーム軌道2012

    • Author(s)
      高橋敏男
    • Organizer
      PF研究会シリコン単結晶:理想品質へのあくなき追求:半導体産業の米と放射光X線光学素子として
    • Place of Presentation
      高エネルギー加速器研究機構
    • Year and Date
      2012-05-27
    • Related Report
      2012 Final Research Report
  • [Presentation] Bi2Te3上のBi超薄膜の電子状態と表面構造解析2012

    • Author(s)
      平原徹
    • Organizer
      日本物理学会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-25
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] 表面X線回折法によるBi/Bi2Te3トポロジカル絶縁体界面の構造研究2012

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-24
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] X線CTR散乱法を用いた表面及び界面の原子イメージング2012

    • Author(s)
      高橋敏男
    • Organizer
      応用物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2012-03-15
    • Related Report
      2012 Final Research Report
  • [Presentation] 多波長同時分散型光学系を用いた迅速3次元逆格子空間マッピング2012

    • Author(s)
      白澤徹郎
    • Organizer
      応用物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2012-03-15
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] X線CTR散乱を用いた表面及び界面の原子イメージング2012

    • Author(s)
      高橋敏男
    • Organizer
      応用物理学会
    • Place of Presentation
      早稲田大学(招待講演)
    • Year and Date
      2012-03-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] ラウエケースのX線CTR散乱2011

    • Author(s)
      高橋敏男
    • Organizer
      日本物理学会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-23
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] 多波長同時分散型X線CTR散乱法の時分割測定への応用2011

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-23
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] X線CTR散乱法によるペンタセン超薄膜の界面構造2011

    • Author(s)
      大山真実
    • Organizer
      日本物理学会
    • Place of Presentation
      富山大学
    • Year and Date
      2011-09-21
    • Related Report
      2012 Final Research Report 2011 Annual Research Report
  • [Presentation] ペンタセン超薄膜のX線CTR散乱法による構造解析2011

    • Author(s)
      大山真実
    • Organizer
      日本物理学会
    • Place of Presentation
      新潟大学(学会は中止となったが発表は有効)
    • Related Report
      2010 Annual Research Report
  • [Presentation] Si(111)上のBi(001)超薄膜の界面構造解析2011

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      新潟大学(学会は中止となったが発表は有効)
    • Related Report
      2010 Annual Research Report
  • [Presentation] X線CTR散乱法によるPr1.1Ba1.9Cu3O7-δ/SrTiO界面構造解析2010

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-26
    • Related Report
      2012 Final Research Report
  • [Presentation] X線CTR散乱法によるPr1.1Ba1.9Cu3O7-δ/SrTiO3界面構造解析2010

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] 多波長同時分散光学系を用いたトランケーションロッドの測定III2010

    • Author(s)
      白澤徹郎
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-23
    • Related Report
      2012 Final Research Report 2010 Annual Research Report
  • [Presentation] Low temperature superstructure formation in gold atomic chains on high-index Si surface2010

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-23
    • Related Report
      2012 Final Research Report
  • [Presentation] Low temperature superstructure formation in gold atomic chains on high-index Si surfaces2010

    • Author(s)
      Wolfgang VOEGELI
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-23
    • Related Report
      2010 Annual Research Report
  • [Presentation] 透過型off-Bragg条件におけるX線回折強度とビーム軌道

    • Author(s)
      高橋敏男
    • Organizer
      PF研究会「シリコン単結晶:理想品質へのあくなき追求:半導体産業の米と放射光X線光学素子として」
    • Place of Presentation
      高エネルギー加速器研究機構
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Quick Three-Dimensional Reciprocal Space Mapping in a the Simultaneous Multi-Wavelength Dispersive Mode

    • Author(s)
      白澤徹郎
    • Organizer
      The 11th International Conference on Synchrotron Radiation Instrumentation
    • Place of Presentation
      リヨン(フランス)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Time-resolved X-ray CTR scattering measurement on the photo-induced hydrophilic transition of the TiO2(110) surface

    • Author(s)
      白澤徹郎
    • Organizer
      12th International Conferance on Surface X-ray and Neutron Scattering (SXS12)
    • Place of Presentation
      コルカタ(インド)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Structure of gold atomic chains on the Si(553) surface and their low-temperature structural changes

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      12th International Conferance on Surface X-ray and Neutron Scattering (SXS12)
    • Place of Presentation
      コルカタ(インド)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Reconstruction of Atoms at Surface/interface by Using X-ray Crystal Truncation Rod Scattering

    • Author(s)
      高橋敏男
    • Organizer
      ISSP International Workshop on 3D Atomic Imaging at Nano-scale active sites in materials
    • Place of Presentation
      東京大学物性研究所
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Molecular Arrangement of Pentacene Ultrathin Film Studied with Surface X-ray Scattering

    • Author(s)
      白澤徹郎
    • Organizer
      ISSP International Workshop on 3D Atomic Imaging at Nano-scale active sites in materials
    • Place of Presentation
      東京大学物性研究所
    • Related Report
      2012 Annual Research Report
  • [Presentation] Structure of gold atomic chains on the Si(553) surface and their low-temperature structural changes

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      ISSP International Workshop on 3D Atomic Imaging at Nano-scale active sites in materials
    • Place of Presentation
      東京大学物性研究所
    • Related Report
      2012 Annual Research Report
  • [Presentation] Quick time-resolved X-ray reflectivity using an undulator source

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜国立大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] A Molecular Arrangement of Pentacene in UltraThin Film Revealed by Surface

    • Author(s)
      白澤徹郎
    • Organizer
      第10回半導体表面に関する日露セミナー(JRSSS10)
    • Place of Presentation
      東京大学本郷キャンパス
    • Related Report
      2012 Annual Research Report
  • [Presentation] 陽電子回折への期待

    • Author(s)
      高橋敏男
    • Organizer
      PF研究会「KEK低速陽電子実験施設における陽電子回折研究およびPsビーム研究の新展開
    • Place of Presentation
      高エネルギー加速器研究機構
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Atomic-layer-resolved imaging of epitaxially grown ultra thin films with X-ray CTR scattering

    • Author(s)
      高橋敏男
    • Organizer
      第8回放射光表面科学研究部会顕微ナノ材料科学研究会合同シンポジウム
    • Place of Presentation
      慶応義塾大学
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 結晶性ペンタセン超薄膜の表面X線回折法による構造解析

    • Author(s)
      白澤徹郎
    • Organizer
      第26回日本放射光学会年会
    • Place of Presentation
      名古屋大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] 多波長同時分散型X線CTR散乱法を用いたルチルTiO2(110)表面超親水化反応のその場観察

    • Author(s)
      白澤徹郎
    • Organizer
      第30回PFシンポジウム
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2012 Annual Research Report
  • [Presentation] 実験室特性X線源を用いた高速逆格子空間マッピング法の開発

    • Author(s)
      Voegeli Wolfgang
    • Organizer
      第60回応用物理学会春季学術講演会
    • Place of Presentation
      神奈川工科大学
    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://www.issp.u-tokyo.ac.jp/maincontents/organization/labs/takahashi_group.html

    • Related Report
      2012 Final Research Report

URL: 

Published: 2010-08-23   Modified: 2019-07-29  

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