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Experimental verification of the validity of the semi-classicalapproximation for the decay dynamics on the complex potential

Research Project

Project/Area Number 22550008
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionSophia University (2012)
Tokyo Institute of Technology (2010-2011)

Principal Investigator

ODAGIRI Takeshi  上智大学, 理工学部, 准教授 (80282820)

Project Period (FY) 2010 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2012: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2011: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2010: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywords原子分子物理 / 2 電子励起分子 / 解離 / 対称性分離 / 飛行時間測定 / 崩壊ダイナミックス / 準安定原子 / 2電子励起分子 / 準安定水素原子 / 2電子励起分子 / 準安定水準 / 準安定水素
Research Abstract

Doubly excited states of molecular hydrogen decay mainly via autoionizations or neutral dissociations. The dynamics of the competitive decay is sometimes described by the semi-classical approximation. In the present study, we would like to experimentally verify the validity of the semi-classical approximation by measuring (i) a time-of-flight spectrum of the metastable atomic fragments, the H(2s) atoms, in photoexcitation of H_2 with the electronic symmetry and final state in neutral dissociation being resolved, and (ii) the cross sections for producing two H(2p) atoms as a function of the incident photon energy. The two experiments are expected to give comprehensive information about the decay dynamics, especially for the decay of the Q_2 doubly excite states of H_2. The development of the experiment (i) was about to finish. However, 2011 T?hoku earthquake unfortunately affected the operation of the KEK-PF ring and thus the study has not completed.

Report

(4 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (22 results)

All 2013 2012 2011 2010

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (16 results)

  • [Journal Article] Dynamics of entangled H(2p) pairgenerated in the photodissociation of H_22012

    • Author(s)
      T. Odagiri, T. Tanabe and N. Kouchi
    • Journal Title

      J. Phys.: Conf. Ser

      Volume: 388 Issue: 1 Pages: 12024-12024

    • DOI

      10.1088/1742-6596/388/1/012024

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Three-body neutraldissociations of a multiply excitedwater molecule around the doubleionization potential2012

    • Author(s)
      T. Odagiri, M. Nakano, T. Tanabe, Y.Kumagai, I. H Suzuki, M. Kitajima andN. Kouchi
    • Journal Title

      J. Phys. B:At. Mol. Opt. Phys

      Volume: 45 Pages: 215204-215204

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Three-body neutral dissociations of a multiply excited water molecule around the double ionization potential2012

    • Author(s)
      T. Odagiri
    • Journal Title

      J. Phys. B: At. Mol. Opt. Phys.

      Volume: 45 Issue: 21 Pages: 215204-215204

    • DOI

      10.1088/0953-4075/45/21/215204

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Formation of metastableatomic hydrogen in the 2s state fromsymmetry-resolved doubly excitedstates of molecular hydrogen2011

    • Author(s)
      T. Odagiri, Y. Kumagai, M. Nakano, T.Tanabe, I. H. Suzuki, M. Kitajima andN. Kouchi
    • Journal Title

      Phys.Rev

      Volume: 84[5] Issue: 5 Pages: 53401-53401

    • DOI

      10.1103/physreva.84.053401

    • Related Report
      2012 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A new spectroscopicmethod for resolving the electronicsymmetry properties of the highlyexcited molecules produced inphotoexcitation2010

    • Author(s)
      T. Odagiri, Y. Kumagai, T. Tanabe, M.Nakano, I. H. Suzuki, M. Kitajima, andN. Kouchi
    • Journal Title

      Rev. Sci. Instrum

      Volume: 81 Issue: 6 Pages: 63108-63108

    • DOI

      10.1063/1.3436653

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] A new spectroscopic method for resolving the electronic symmetry properties of the highly excited molecules produced in photoexcitation2010

    • Author(s)
      T.Odagiri, et al.
    • Journal Title

      Rev.Sci.Instrum

      Volume: 81

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] SB モードを利用した準安定原子検出による分子二電子励起状態ダイナミクスの研究2013

    • Author(s)
      熊谷嘉晃, 小田切丈, 田辺健彦, 中野元善, 仲西祐子, 向後陵子,穂坂綱一, 北島昌史, 河内宣之, 鈴木功
    • Organizer
      物構研サイエンスフェスタ,第30回 PF シンポジウム
    • Place of Presentation
      つくば国際会議場(つくば)
    • Related Report
      2012 Final Research Report
  • [Presentation] SB モードを利用した準安定原子検出による分子二電子励起状態ダイナミクスの研究2013

    • Author(s)
      熊谷嘉晃
    • Organizer
      物構研サイエンスフェスタ
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2012 Annual Research Report
  • [Presentation] Metastable hydrogen in the 2s state as a probe for dissociative doubly excited states of molecules2011

    • Author(s)
      Y.Kumagai
    • Organizer
      IMSS Symposium '11
    • Place of Presentation
      Tsukuba, Japan
    • Year and Date
      2011-12-06
    • Related Report
      2011 Annual Research Report
  • [Presentation] Generation and decay of an entangled atom pair through photodissociation of H_22011

    • Author(s)
      T.Odagiri
    • Organizer
      International Symposium on (e,2e), Double Photoionization and Related Topics & 16th International Symposium on Polarization and Correlation in Electronic andAtomic Collisions
    • Place of Presentation
      Dublin, Ireland(招待講演)
    • Year and Date
      2011-08-05
    • Related Report
      2011 Annual Research Report
  • [Presentation] Metastable hydrogen in the 2s state as a probe for dissociative doubly excited states of molecules2011

    • Author(s)
      Y.Kumagai
    • Organizer
      XXVII International Conference on Photonic, Electronic and Atomic Collisions
    • Place of Presentation
      Belfast, Northern Ireland, UK
    • Year and Date
      2011-08-01
    • Related Report
      2011 Annual Research Report
  • [Presentation] 光解離H(2s)原子検出による2電子励起メタン、アンモニアの研究2011

    • Author(s)
      熊谷嘉晃
    • Organizer
      第28回PFシンポジウム
    • Place of Presentation
      つくば国際会議場
    • Year and Date
      2011-07-12
    • Related Report
      2011 Annual Research Report
  • [Presentation] The multiply excited states of molecules as probed by detection of meta stable H(2s) atoms produced in the photodissociation2011

    • Author(s)
      Y.Kumagai
    • Organizer
      第27回化学反応討論会
    • Place of Presentation
      東京工業大学
    • Year and Date
      2011-06-08
    • Related Report
      2011 Annual Research Report
  • [Presentation] Metastable hydrogen in the 2s state asa probe for dissociative doublyexcited states of molecules2011

    • Author(s)
      Y. Kumagai, T. Odagiri, T. Tanabe, M.Nakano, I. H Suzuki, N. Kouchi
    • Organizer
      IMSSSymposium
    • Place of Presentation
      Tsukuba,Japan
    • Related Report
      2012 Final Research Report
  • [Presentation] Generation and decay of anentangled atom pair throughphotodissociation of H_22011

    • Author(s)
      T. Odagiri
    • Organizer
      International Symposium on (e,2e),Double Photo-ionization and Related
    • Place of Presentation
      ublin, Ireland
    • Related Report
      2012 Final Research Report
  • [Presentation] Metastable hydrogen in the 2s state asa probe for dissociative doublyexcited states of molecules2011

    • Author(s)
      Y. Kumagai, T. Odagiri, T. Tanabe, M.Nakano, I. H Suzuki, N. Kouchi
    • Organizer
      XXVII International Conference on Photonic
    • Place of Presentation
      Belfast, NorthernIreland, UK
    • Related Report
      2012 Final Research Report
  • [Presentation] 光解離 H(2s)原子検出による 2 電子励起メタン、アンモニアの研究2011

    • Author(s)
      熊谷嘉晃, 小田切丈, 田邊健彦, 中野元善, 鈴木功, 河内宣之
    • Organizer
      第28回 PF シンポジウム
    • Place of Presentation
      つくば(つくば国際会議場)
    • Related Report
      2012 Final Research Report
  • [Presentation] The multiply excited states ofmolecules as probed by detection ofmetastable H(2s) atoms produced in thephotodissociation2011

    • Author(s)
      Y. Kumagai, T. Odagiri, T. Tanabe, M.Nakano, I. H. Suzuki, N. Kouchi
    • Organizer
      第27回化学反応討論会
    • Place of Presentation
      東京(東京工業大学 大岡山キャンパス)
    • Related Report
      2012 Final Research Report
  • [Presentation] メタン、アンモニア二電子励起状態からのH(2s)原子フラグメント生成2010

    • Author(s)
      熊谷嘉晃, 他
    • Organizer
      日本物理学会 平成22年度 秋季大会
    • Place of Presentation
      大阪府立大学中百舌鳥キャンパス
    • Year and Date
      2010-09-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] メタン、アンモニアの光解離による準安定水素原子生成2010

    • Author(s)
      熊谷嘉晃, 他
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪大学 豊中キャンパス
    • Year and Date
      2010-09-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] メタン、アンモニア二電子励起状態からの H(2s)原子フラグメント生成2010

    • Author(s)
      熊谷 嘉晃, 小田切 丈,田邊 健彦,中野元善,鈴木 功,河内 宣之
    • Organizer
      日本物理学会
    • Place of Presentation
      大阪
    • Related Report
      2012 Final Research Report
  • [Presentation] メタン、アンモニアの光解離による準安定水素原子生成2010

    • Author(s)
      熊谷 嘉晃, 小田切 丈,田邊 健彦,中野元善,鈴木 功,河内 宣之
    • Organizer
      第4回分子科学討論会
    • Place of Presentation
      大阪
    • Related Report
      2012 Final Research Report

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Published: 2010-08-23   Modified: 2019-07-29  

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