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Fabrication of organic electronics based on fused organic semiconductors

Research Project

Project/Area Number 22550165
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Functional materials/Devices
Research InstitutionTokai University

Principal Investigator

KUNUGI Yoshihito  東海大学, 工学部, 教授 (90243518)

Project Period (FY) 2010-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2014: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2013: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2012: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2011: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2010: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Keywords有機トランジスタ / 有機半導体 / 有機デバイス / 半導体物性
Outline of Final Research Achievements

Organic semiconductors have attracted significant attention as a new class of electronic materials for organic field-effect transistors (OFETs), organic light-emitting diodes and organic solar cells. Particularly, OFETs have been intensively investigated for applications in organic integrated circuits for flexible active-matrix displays, radio frequency identification tags, and chemical and biological sensors, because of the merits of organic materials, such as low cost, flexibility, and easy fabrication. The charge carrier mobility is strongly influenced by the organic semiconductor layer, and therefore, great efforts have been made toward the development of various semiconducting small molecules and polymers.
In this work, I synthesized a series of 2,8-disubstituted chrysene, diphenyldinaphthofuran, and dinaphthothienothiophene derivatives as novel fused organic semiconductors, and applied them to organic thin-film and single-crystal transistors.

Report

(6 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (46 results)

All 2015 2014 2013 2012 2011 2010

All Journal Article (15 results) (of which Peer Reviewed: 15 results,  Acknowledgement Compliant: 2 results) Presentation (31 results) (of which Invited: 2 results)

  • [Journal Article] Organic Field-effect Transistors Based on Alkylphenyl-substituted Dinaphtho[2,1-b:2’,1’-f]thieno[3,2-b]thiophenes2015

    • Author(s)
      Y. KUNUGI, Y. FUJITA, M. TSUTSUI, and K. OKAMOTO
    • Journal Title

      Electrochemistry

      Volume: 83

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Synthesis of Conjugated D-A Polymers Bearing Bi(dithienogermole) as a New Donor Component and Their Applications to Polymer Solar Cells and Transistors2015

    • Author(s)
      J. OHSHITA, M. MIYAZAKI, M. NAKASHIMA, D. TANAKA, Y. OOYAMA, T. SASAKI, Y. KUNUGI, Y. MORIHARA
    • Journal Title

      RSC Advances

      Volume: 5 Issue: 17 Pages: 12686-12691

    • DOI

      10.1039/c4ra16749j

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication of Organic Single Crystal Transistors Based on 5,9-Diphenyldinaphtho[2,1-b:1’,2’-d]furan Derivatives2014

    • Author(s)
      Y. KUNUGI, A. MAEDA, T. ARAKAWA, and K. OKAMOTO
    • Journal Title

      Journal of Photopolymer Science and Technology

      Volume: 27 Pages: 317-320

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Multifunctional π-Expanded Macrocyclic Oligothiophene 6-Mers and Related Macrocyclic Oligomers2014

    • Author(s)
      Iyoda, M.; Tanaka, K.; Shimizu, H.; Hasegawa, M.; Nishinaga, T.; Nishiuchi, T.; Kunugi, Y.; Ishida, T.; Otani, H.; Sato, H.; Inukai, K.; Tahara, K.; Tobe, Y.
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 136 Issue: 6 Pages: 2389-2396

    • DOI

      10.1021/ja4101744

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Antiaromatic planar cyclooctatetraene: a strategy for ambipolar semiconductors in field effect transistors2013

    • Author(s)
      T. Nishinaga, T. Ohmae, K. Aita, M. Takase, M. Iyoda, T. Arai, Y. Kunugi
    • Journal Title

      Chem. Commun.

      Volume: 49 Issue: 47 Pages: 5354-5356

    • DOI

      10.1039/c3cc41764f

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Characteristics of Thin-Film Transistors Based on 2,8-Disubstituted Chrysene Derivatives with Polymer-Treated SiO<sub>2</sub> Dielectric Layers2013

    • Author(s)
      Y. KUNUGI, H. HOSHINO, H. OTSUKI and K. OKAMOTO
    • Journal Title

      Electrochemistry

      Volume: 81 Issue: 5 Pages: 402-404

    • DOI

      10.5796/electrochemistry.81.402

    • NAID

      10031152013

    • ISSN
      1344-3542, 2186-2451
    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis and Optical Properties of Organosiliconeoligothiophene Branched  Polymers2013

    • Author(s)
      J. OHSHITA, Y. TOMINAGA, D. TANAKA, T. MIZUMO, Y. FUJITA and Y. KUNUGI
    • Journal Title

      Journal of Organometallic Chemistry

      Volume: 736 Pages: 50-54

    • DOI

      10.1016/j.jorganchem.2013.03.007

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ambipolar Single Crystal Organic Field-effect Transistors Based on (4,4&rsquo;-Diphenyl)dinaphtho [2,1-b:2&rsquo;,1&rsquo;-f]thieno[3,2-b]thiophene2012

    • Author(s)
      Y. Kunugi
    • Journal Title

      Journal of Photopolymer Science and Technology

      Volume: 25 Issue: 3 Pages: 285-288

    • DOI

      10.2494/photopolymer.25.285

    • NAID

      130004833454

    • ISSN
      0914-9244, 1349-6336
    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Preparation, Hybrid Formation with Single-walled Carbon Nanotube, and Film Morphology of Pyrene-containing Polysiloxanes2012

    • Author(s)
      Z. Lu
    • Journal Title

      Composite Interfaces

      Volume: 19 Issue: 9 Pages: 573-581

    • DOI

      10.1080/15685543.2012.762866

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Single Crystal Organic Field-effect Transistors Based on 2,8-Diphenyl and Dinaphthyl Chrysenes2011

    • Author(s)
      Yoshihito Kunugi, Tatsuya Arai, Norihiro Kobayashi, Hiroyuki Otsuki, TohruNishinaga, Kazuo Okamoto
    • Journal Title

      Journal of Photopolymer Science and Technology

      Volume: 24 Issue: 3 Pages: 345-348

    • DOI

      10.2494/photopolymer.24.345

    • NAID

      130004464902

    • ISSN
      0914-9244, 1349-6336
    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis and Structural, Electronic, Optical and FET Properties of Thiophene-Pyrrole Mixed Hexamers End-Capped with Phenyl and Pentafluorophenyl Groups2011

    • Author(s)
      Tohru Nishinaga, Toshihiko Miyata, Masaki Tateno, Masahide Koizumi, Masayoshi Takase, Masahiko Iyoda, Norihiro Kobayashi, Yoshihito Kunugi
    • Journal Title

      J. Mater. Chem.

      Volume: 21 Issue: 38 Pages: 14959-14966

    • DOI

      10.1039/c1jm12966j

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Single Crystal Organic Field-effect Transistors Based on Dinaphthothienothiophene Isomers2010

    • Author(s)
      Y.Kunugi
    • Journal Title

      Journal of Photopolymer Science and Technology

      Volume: 23 Pages: 323-326

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 有機デバイスへの挑戦2010

    • Author(s)
      功刀義人
    • Journal Title

      Journal of the Society of Inorganic Materials, Japan

      Volume: 17 Pages: 182-187

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis of star-shaped molecules with pyrene-containing pi-conjugated units linked by an organosilicon core2010

    • Author(s)
      J.Ohshita
    • Journal Title

      Applied Organometallic Chemistry

      Volume: 24 Pages: 540-544

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of the Silicon Core Structures on the Hole Mobility of Star-shaped Oligothiophenes2010

    • Author(s)
      J.Ohshita
    • Journal Title

      Dalton Transactions

      Volume: 39 Pages: 9314-9320

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] Organic Thin-film Transistors based on Alkylsilylamine-treated SiO2 Dielectric Layers2015

    • Author(s)
      T. SASAKI, K. TANIGUCHI, H. ARASE, J. OHSHITA, and Y. KUNUGI
    • Organizer
      The International Conference on Materials for Advanced Technologies (ICMAT2015)
    • Place of Presentation
      Singapore(Singapore)
    • Year and Date
      2015-06-29 – 2015-07-03
    • Related Report
      2014 Annual Research Report
  • [Presentation] Organic Single-crystal Transistors based on Alkyl Substituted Diphenyl-dinaphtho [2,1-b:2’,1’f]thieno[3,2b]thiophen Derivatives2015

    • Author(s)
      T. ONOZUKA, A. MAEDA, H. OTUKI, K. OKAMOTO, and Y. KUNUGI
    • Organizer
      The International Conference on Materials for Advanced Technologies (ICMAT2015)
    • Place of Presentation
      Singapore(Singapore)
    • Year and Date
      2015-06-29 – 2015-07-03
    • Related Report
      2014 Annual Research Report
  • [Presentation] Characterization of Alkyl-substituted Picene Thin Films as Active Layers of Organic Field Effect Transistors2014

    • Author(s)
      Y. FUJITA, M. MONZAKI, K. OKAMOTO, Y. KUNUGI
    • Organizer
      2014 Material Research Society Fall Meeting
    • Place of Presentation
      Boston(USA)
    • Year and Date
      2014-11-30 – 2014-12-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] Organic Field-effect Transistors Based on Single-crystal Ribbons of Solution Processed Dialkyl DNTT Derivatives2014

    • Author(s)
      A. MAEDA, M. TSUTSUI, K. OKAMOTO, Y. KUNUGI
    • Organizer
      2014 Material Research Society Fall Meeting
    • Place of Presentation
      Boston(USA)
    • Year and Date
      2014-11-30 – 2014-12-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] Fabrication and Characterization of Field Effect Transistors Based on Asymmetric Chrysene Derivatives2014

    • Author(s)
      T. YOSHIDA, H. OTSUKI, K. OKAMOTO, Y. KUNUGI
    • Organizer
      2014 Material Research Society Fall Meeting
    • Place of Presentation
      Boston(USA)
    • Year and Date
      2014-11-30 – 2014-12-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] 有機半導体デバイス2014

    • Author(s)
      功刀義人
    • Organizer
      反応性・機能性材料シンポジウム
    • Place of Presentation
      東京工業大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] High Performance OFETs Based on Single-crystal Ribbons of Diphenylchrysene Derivatives2013

    • Author(s)
      A. MAEDA
    • Organizer
      The 4th German-Japanese Symposium on Electrosynthesis
    • Place of Presentation
      京都大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] Organic Semiconductors for Electronic Devices2013

    • Author(s)
      Y. KUNUGI
    • Organizer
      4th KMUTT-Tokai Joint Seminar on Advanced Engineering
    • Place of Presentation
      東海大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Characteristic of Thin Film Transistors Based on Alkylated Dinaphtho[2,1-b:2',1'-f]thieno[3,2-b]thiophenes2013

    • Author(s)
      Y. KOIKE
    • Organizer
      2013 International Symposium on Organic Reaction
    • Place of Presentation
      Taipei (Taiwan)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Characteristics of Single-crystal OFETs of Aromatic Heterocyclic Hydrocarbon, 21DNFU Derivatives2013

    • Author(s)
      T. ARAKAWA
    • Organizer
      7th International Conference on Materials for Advanced Technologies
    • Place of Presentation
      Suntec (singapore)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Picene単結晶を用いた有機トランジスタの特性2013

    • Author(s)
      荒川 哲平
    • Organizer
      日本化学会第93春季年会
    • Place of Presentation
      立命館大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] ジフェニルクリセン誘導体を用いた高移動度有機単結晶薄膜トランジスタの作製2013

    • Author(s)
      前田 采美
    • Organizer
      電気化学会第80回大会
    • Place of Presentation
      東北大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] π共役を拡張させた21DNTT誘導体の単結晶トランジスタ2012

    • Author(s)
      荒川哲平
    • Organizer
      電気化学会第79回大会
    • Place of Presentation
      アクトシティ浜松
    • Year and Date
      2012-03-29
    • Related Report
      2011 Annual Research Report
  • [Presentation] ジフェニルクリセン誘導体を用いた高性能OFET2012

    • Author(s)
      齋藤誠
    • Organizer
      日本化学会第92春季年会
    • Place of Presentation
      慶應義塾大学
    • Year and Date
      2012-03-27
    • Related Report
      2011 Annual Research Report
  • [Presentation] アルキル基を導入したジフェニルクリセンのOFET特性2012

    • Author(s)
      高橋義之
    • Organizer
      2012年春季第59回応用物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2012-03-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] Organic Field-effect Transistors Based on 2,8-Disubstituted Chrysene Derivatives2012

    • Author(s)
      Y. Takahashi
    • Organizer
      Vth International Conference on Molecular Materials
    • Place of Presentation
      AXA Convention Center, Barcelona, Spain
    • Related Report
      2012 Annual Research Report
  • [Presentation] Characterization of Single Crystal Organic Field-effect Transistors Based on 21DNTT Derivatives2012

    • Author(s)
      T. Arakawa
    • Organizer
      Vth International Conference on Molecular Materials
    • Place of Presentation
      AXA Convention Center, Barcelona, Spain
    • Related Report
      2012 Annual Research Report
  • [Presentation] Single-crystal Field-effect Transistors of 21DNTT Derivatives2012

    • Author(s)
      A. Maeda
    • Organizer
      PRiME 2012
    • Place of Presentation
      Hawaii Convention Center, Hawaii, USA
    • Related Report
      2012 Annual Research Report
  • [Presentation] Characterization of the Single Crystal Organic Field-effect Transistors Based on COTS Derivatives2011

    • Author(s)
      T.ARAI
    • Organizer
      ISOR10
    • Place of Presentation
      慶應義塾大学
    • Year and Date
      2011-11-23
    • Related Report
      2011 Annual Research Report
  • [Presentation] Charge Transport Properties of Bis(octyloxy)dinaphthothienothiophene Based OFETs2011

    • Author(s)
      H.HOSHINO
    • Organizer
      ISOR10
    • Place of Presentation
      慶應義塾大学
    • Year and Date
      2011-11-23
    • Related Report
      2011 Annual Research Report
  • [Presentation] ジフェニルクリセン誘導体のFET特性2011

    • Author(s)
      齊藤誠
    • Organizer
      日本化学会第5回関東支部大会
    • Place of Presentation
      東京農工大学
    • Year and Date
      2011-08-31
    • Related Report
      2011 Annual Research Report
  • [Presentation] ビスオクチルオキシジナフトチェノチオフェンを用いた有機トランジスタ特性2011

    • Author(s)
      星野光
    • Organizer
      日本化学会第5回関東支部大会
    • Place of Presentation
      東京農工大学
    • Year and Date
      2011-08-31
    • Related Report
      2011 Annual Research Report
  • [Presentation] Organic Field-effect Transistors based on 2,8-disubstitute d Chrysene Derivatives2011

    • Author(s)
      M.SAITO
    • Organizer
      ICMAT2011
    • Place of Presentation
      Singapore
    • Year and Date
      2011-06-28
    • Related Report
      2011 Annual Research Report
  • [Presentation] 芳香族基を導入したクリセン誘導体の有機単結晶トランジスタ特性2011

    • Author(s)
      荒井竜也
    • Organizer
      第28回フォトポリマーコンファレンス
    • Place of Presentation
      千葉大学
    • Year and Date
      2011-06-24
    • Related Report
      2011 Annual Research Report
  • [Presentation] 環状オリゴチオフェン四量体を用いた有機単結晶トランジスタの特性2011

    • Author(s)
      荒井竜也
    • Organizer
      電気化学会第78回大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2011-03-29
    • Related Report
      2010 Annual Research Report
  • [Presentation] アルコキシジナフトチエノチオフェンOFETのキャリア移動度と純度との相関2011

    • Author(s)
      星野光
    • Organizer
      電気化学会第78回大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2011-03-29
    • Related Report
      2010 Annual Research Report
  • [Presentation] ビスオクチルジフェニルクリセン誘導体のFET特性2011

    • Author(s)
      齊藤誠
    • Organizer
      日本化学会第91春季年会
    • Place of Presentation
      神奈川大学
    • Year and Date
      2011-03-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] π共役を拡張させたクリセン誘導体の有機単結晶トランジスタ特性2010

    • Author(s)
      荒井竜也
    • Organizer
      日本化学会第4回関東支部大会
    • Place of Presentation
      筑波大学
    • Year and Date
      2010-08-30
    • Related Report
      2010 Annual Research Report
  • [Presentation] Single Crystal Organic Field-effect Transistors Based on Chrysene Derivatives2010

    • Author(s)
      N.Kobayashi
    • Organizer
      International Conference on Science and Technology of Synthetic Metals 2010
    • Place of Presentation
      Kyoto International Conference Center
    • Year and Date
      2010-07-06
    • Related Report
      2010 Annual Research Report
  • [Presentation] ジナフトチエノチオフェン誘導体を用いた有機単結晶トランジスタ2010

    • Author(s)
      荒井竜也
    • Organizer
      第27回国際フォトポリマーコンファレンス
    • Place of Presentation
      千葉大学
    • Year and Date
      2010-06-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] 機能性有機材料における電子移動2010

    • Author(s)
      功刀義人
    • Organizer
      第6回有機電子移動化学若手の会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-06-24
    • Related Report
      2010 Annual Research Report

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Published: 2010-08-23   Modified: 2019-07-29  

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