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Understanding of the high-speed sintering mechanisms and improvement of the technical construction in the pulsed-current-sintering (PCS) processing

Research Project

Project/Area Number 22560675
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionNational Institute for Materials Science

Principal Investigator

MORITA Koji  独立行政法人物質・材料研究機構, 先端材料プロセスユニット, 主幹研究員 (20354186)

Co-Investigator(Renkei-kenkyūsha) KIM Byung-nam  独立行政法人物質・材料研究機構, 先端材料プロセスユニット, 主席研究員 (50254149)
SAKKA Yoshio  独立行政法人物質・材料研究機構, 先端材料プロセスユニット, ユニット長 (00354217)
Project Period (FY) 2010 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2012: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2011: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2010: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywordsパルス通電焼結 / 構造用セラミックス / スピネル / 透光性 / パルス通電焼結(PCS) / 酸化物セラミックス / 焼結機構 / パルス効果 / パルス通電焼結(PCS) / パルス通電焼結法 / 焼結 / 通電効果 / クリープ
Research Abstract

In order to achieve an advanced pulsed-current-sintering (PCS) technique, this work was performed to understand the sintering mechanisms and to clarify the effect of the sintering parameters, such as heating rate, sintering temperature, dwelling time, loading schedule and so on, on PCS processing of MgAl2O4 spinel. It is found that the sintering behavior changes sensitively with the parameters and dense fine-grained ceramics can be fabricated by carefully optimizing the parameters. Loading at high temperatures, for example, can attain high density spinel even at a high heating rate of 100°C/min, and hence, can save the total processing time.

Report

(4 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • Research Products

    (46 results)

All 2013 2012 2011 2010

All Journal Article (24 results) (of which Peer Reviewed: 23 results) Presentation (22 results) (of which Invited: 1 results)

  • [Journal Article] Development of high-strain-rate superplastic oxide ceramics based on flow mechanism2013

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, Y. Sakka and K. Hiraga
    • Journal Title

      Mat. Sci. Forum

      Volume: 735 Pages: 9-14

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of Loading Schedule on Densification of MgAl_2O_4 Spinel during Spark Plasma Sintering (SPS) Processing2012

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, H. Zhang, K. Hiraga and Y. Sakka
    • Journal Title

      J Eur. Ceram. Soc.,

      Volume: 32 Pages: 2303-2309

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of loading schedule during SPS processingfor attaining dense MgAl_2O_4 spinel poly-crystal2012

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, H.Zhang, K. Hiraga and Y. Sakka
    • Journal Title

      Journal of the Euro Ceramics Society

      Volume: vol.32 Issue: 10 Pages: 2303-2309

    • DOI

      10.1016/j.jeurceramsoc.2012.02.016

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 放電プラズマ焼結(SPS)装置を用いた透光性セラミックスの創製2012

    • Author(s)
      森田孝治、金炳男、吉田英弘、目義雄、平賀啓二郎
    • Journal Title

      マテリアルインテグレーション

      Volume: 25[10] Pages: 75-82

    • NAID

      130003388704

    • Related Report
      2012 Annual Research Report
  • [Journal Article] High-Pressure Spark Plasma Sintering of MgO-doped Transparent Alumina2012

    • Author(s)
      B. Kim, K. Hiraga, G. Salvatore, K. Morita, H. Yoshida, H. Zhang, Y. Sakka
    • Journal Title

      J. Ceram. Soc. Jpn.

      Volume: 120[3] Pages: 116-118

    • NAID

      130002067597

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Optical Properties and Microstructure of Nanocrystalline Cubic Zirconia Prepared by High-Pressure Spark Plasma Sintering2011

    • Author(s)
      H. Zhang, B.-N. Kim, K. Morita, H. Yoshida, J. Lim, K. Hiraga
    • Journal Title

      J. Am. Ceram. Soc.

      Volume: 94 Pages: 2981-2986

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Diffusive model of pore shrinkage in final-stage sintering under hydrostatic pressure2011

    • Author(s)
      B.-N. Kim, K. Hiraga, K. Morita, H. Yoshida and H. Zhang
    • Journal Title

      Acta Mater

      Volume: 59[10] Pages: 4079-4087

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Highly Infrared Transparent Nanometric Tetragonal Zirconia Prepared by High-Pressure Spark Plasma Sintering2011

    • Author(s)
      H. Zhang, Z. Li, B.-N. Kim, K. Morita, H. Yoshida, K. Hiraga, Y. Sakka and J. Blendell
    • Journal Title

      J. Am. Ceram. Soc.

      Volume: 94[9] Pages: 2739-2741

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication of Transparent Yttria by High-Pressure Spark Plasma Sintering2011

    • Author(s)
      H. Zhang, B.-N. Kim, K. Morita, H. Yoshida, K. Hiraga, Y. Sakka and J. Ballato
    • Journal Title

      J. Am. Ceram. Soc.

      Volume: 94[10] Pages: 3206-3210

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Highly infrared transparentnanometric tetragonal zirconia preparedby high-pressure spark plasma sintering2011

    • Author(s)
      H. Zhang, Z. Li, B. Kim, K. Morita, H.Yoshida, K. Hiraga,Y. Sakka and J.Blendell
    • Journal Title

      Journal of the American Ceramic Society

      Volume: vol.94 Issue: 9 Pages: 2739-2741

    • DOI

      10.1111/j.1551-2916.2011.04680.x

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effect of sintering temperature on optical properties and microstructure of translucent zirconia prepared by high-pressure spark plasma sintering2011

    • Author(s)
      Haibin Zhang
    • Journal Title

      Sci.Tech.Adv.Mat.

      Volume: 12 Issue: 5 Pages: 55003-55001

    • DOI

      10.1088/1468-6996/12/5/055003

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication of Transparent Yttria by High-Pressure Spark Plasma Sintering2011

    • Author(s)
      H.Zhang
    • Journal Title

      Journal of the American Ceramics Society

      Volume: 94 Issue: 10 Pages: 3206-3210

    • DOI

      10.1111/j.1551-2916.2011.04789.x

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of Preheating of Powder Before Spark Plasma Sintering of Transparent MgAl2O4 Spinel2010

    • Author(s)
      B.-N. Kim, K. Morita, J.-H. Lim, K. Hiraga, H. Yoshida
    • Journal Title

      J. Am. Ceram. Soc.

      Volume: 93[8] Pages: 158-2160

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Light scattering in MgO-doped alumina fabricated by spark plasma sintering2010

    • Author(s)
      B.-N. Kim, K. Hiraga, K. Morita, H. Yoshida and Y. Kagawa
    • Journal Title

      Acta Mater

      Volume: 58[13] Pages: 4527-4535

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Densification behavior of a fine- grained MgAl_2O_4 spinel during spark plasma sintering (SPS)2010

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida and K. Hiraga
    • Journal Title

      Scripta Mater

      Volume: 63[6] Pages: 565-568

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Optimization of high-pressure sintering of transparent zirconia with nano-sized grains2010

    • Author(s)
      H. B. Zhang, B.-N. Kim, K. Morita, H. Yoshida, J.-H. Lim and K. Hiraga
    • Journal Title

      J. Alloy. Compd.

      Volume: 508[1] Pages: 196-199

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spark-Plasma-Sintering (SPS) Processing of High Strength Transparent MgAl2O4 Spinel Polycrystals2010

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, K. Hiraga
    • Journal Title

      PACRIM8 2009 Meeting, Ceram. Trans

      Volume: 212 Pages: 19-29

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] High-Strain-Rate Superplastic Flow Mechanism in ZrO2-30vol% Spinel Two-Phase Composite2010

    • Author(s)
      K. Morita, K. Hiraga, B.-N. Kim, H. Yoshida
    • Journal Title

      Key Eng. Mat.

      Volume: 433 Pages: 333-338

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Densification Behavior in Spark-Plasma-Sintering of MgAl2O4 Spinel2010

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, K. Hiraga
    • Journal Title

      Mat. Sci. Forum

      Volume: 654-656 Pages: 1986-1989

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Densification Behavior in Spark-Plasma-Sintering of MgAl_2O_4 Spinel2010

    • Author(s)
      Koji Morita, et al
    • Journal Title

      Mat.Sci.Forum

      Volume: 654-656 Pages: 1986-1989

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Densification behavior of a fine-grained MgAl_2O_4 spinel during spark plasma sintering (SPS)2010

    • Author(s)
      Koji Morita, et al
    • Journal Title

      Scripta Materialia

      Volume: 63 Pages: 565-568

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-Strain-Rate Superplastic Flow Mechanism in ZrO_2-30vol% Spinel Two-Phase Composite2010

    • Author(s)
      Koji Morita, et al
    • Journal Title

      Key Eng.Mat.

      Volume: 433 Pages: 333-338

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spark-Plasma-Sintering (SPS) Processing of High Strength Transparent MgAl_2O_4 Spinel Polycrystals2010

    • Author(s)
      Koji Morita, et al
    • Journal Title

      CERAMIC TRANSACTIONS

      Volume: 212 Pages: 19-29

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Densification Mechanism of MgAl2O4 Spinel during Spark-Plasma-Sintering2010

    • Author(s)
      Koji Morita, et al
    • Journal Title

      Advances in Science and Technology

      Volume: 63 Pages: 62-67

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] Fabrication of Transparent MgAl2O4 Spinel using Pulsed-Current-Sintering (PCS) Processing2013

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, Z. Zhang, Y. Sakka, K. Hiraga
    • Organizer
      Seminar in KIMS
    • Place of Presentation
      Changwon Korea
    • Year and Date
      2013-05-27
    • Related Report
      2012 Final Research Report
  • [Presentation] ジルコニアセラミックスの超塑性変形と高速化に関する研究2013

    • Author(s)
      森田孝治
    • Organizer
      日本金属学会2013春期大会
    • Place of Presentation
      東京理科大学
    • Year and Date
      2013-03-27
    • Related Report
      2012 Annual Research Report 2012 Final Research Report
  • [Presentation] Development of high-strain-rate superplastic oxide ceramics based on flow mechanism2012

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, Y. Sakka and K. Hiraga
    • Organizer
      ICSAM2012
    • Place of Presentation
      Albi Francs
    • Year and Date
      2012-07-04
    • Related Report
      2012 Final Research Report
  • [Presentation] Spark-plasma-sintering (SPS) processing for the synthesis of transparent MgAl_2O_4 spinel2012

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, Z. Zhang, Y. Sakka, K. Hiraga
    • Organizer
      CMCee2012
    • Place of Presentation
      Dresden Germany
    • Year and Date
      2012-05-21
    • Related Report
      2012 Final Research Report
  • [Presentation] Spark- Plasma-Sintering of Transparent MgAl_2O_4 Spinel2012

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, K. Hiraga, Y. Sakka
    • Organizer
      29th K-J Ceramics Seminar
    • Place of Presentation
      Daegu Korea
    • Related Report
      2012 Final Research Report
  • [Presentation] Spark-plasma-sintering (SPS) processing for the synthesis of transparent MgAl2O4 spinel2012

    • Author(s)
      Koji Morita
    • Organizer
      International Symposium on Ceramic Materials and Components for Energy and Environmental Applications (CMCee2012)
    • Place of Presentation
      Dresden, Germany
    • Related Report
      2012 Annual Research Report
  • [Presentation] Development of high-strain-rate superplastic oxide ceramics based on flow mechanism2012

    • Author(s)
      Koji Morita
    • Organizer
      11th International Conference on superplasticity in advanced materials (ICSAM2012)
    • Place of Presentation
      Albi, France
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Transparent materials obtained by SPS densification2011

    • Author(s)
      Koji Morita
    • Organizer
      2nd Int.Workshop on Spark Plasma Sintering
    • Place of Presentation
      Capbreton, France(Invited)
    • Year and Date
      2011-10-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] Fabrication of high-strength transparent MgAl2O4 by optimizing spark-plasma-sintering (SPS) conditions2011

    • Author(s)
      Koji Morita
    • Organizer
      International workshop on Field Assisted Sintering Technology (FAST)
    • Place of Presentation
      Penn State University, US(Invited)
    • Year and Date
      2011-08-24
    • Related Report
      2011 Annual Research Report
  • [Presentation] Effect of Loading Schedule during SPS Processing for Attaining Dense MgAl2O4 Spinel Polycrystal2011

    • Author(s)
      Koji Morita
    • Organizer
      12th Conf.of the Euro.Ceram.Soc.(ECerSXII)
    • Place of Presentation
      Stockholm, Sweden
    • Year and Date
      2011-06-22
    • Related Report
      2011 Annual Research Report
  • [Presentation] Transparent Materials Obtained by SPS Densification2011

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, H. Zhang, K. Hiraga, Y. Sakka
    • Organizer
      2nd Int. Workshop on Spark Plasma Sintering
    • Place of Presentation
      Capbreton France
    • Related Report
      2012 Final Research Report
  • [Presentation] Diffusive Model of Pore Shrinkage in Final-Stage Sintering2011

    • Author(s)
      B.-N. Kim, K. Hiraga, K. Morita, H. Yoshida, H. Zhang
    • Organizer
      Sintering 2011
    • Place of Presentation
      Jeju Korea
    • Related Report
      2012 Final Research Report
  • [Presentation] Fabrication of high-strength transparent MgAl_ 2O_ 4 by optimizing spark-plasma-sintering (SPS) conditions2011

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, K. Hiraga, Y. Sakka
    • Organizer
      International workshop on Field Assisted Sintering Technology
    • Place of Presentation
      Pen State Univ. US
    • Related Report
      2012 Final Research Report
  • [Presentation] Grain-boundary-diffusion model of final-stage sintering under hydrostatic pressure2011

    • Author(s)
      B.-N. Kim, K. Hiraga, K. Morita, H. Yoshida, H. Zhang
    • Organizer
      12th Conf. of the European Ceramic Society
    • Place of Presentation
      Stockholm Sweden
    • Related Report
      2012 Final Research Report
  • [Presentation] 加圧下最終焼結段階における緻密化挙動の粒界拡散モデル2011

    • Author(s)
      金炳男, 平賀啓二郎, 森田孝治, 吉田英弘, 張海斌
    • Organizer
      日本セラミックス協会年会
    • Place of Presentation
      静岡大学
    • Related Report
      2012 Final Research Report
  • [Presentation] Microstructural Evolution of MgAl2O4 Spinel ceramics during Spark-Plasma-Sintering (SPS) Process2011

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, H. Zhang, K. Hiraga, Y. Sakka
    • Organizer
      European Symp. Current developments in TEM
    • Place of Presentation
      Freiberg Germany
    • Related Report
      2012 Final Research Report
  • [Presentation] Optimum Spark-Plasma-Sintering (SPS) Condition for Attaining Transparent MgAl_2O_4 Spinel Polycrystal2010

    • Author(s)
      Koji Morita
    • Organizer
      Materials Science and Engineering 2010 (MSE2010)
    • Place of Presentation
      Katrin Binner, Darmstadt(ドイツ)
    • Year and Date
      2010-08-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] Densification Behavior in Spark-Plasma-Sintering of MgAl_2O_4 Spinel2010

    • Author(s)
      Koji Morita
    • Organizer
      PRICM 7
    • Place of Presentation
      ケアンズコンベンションセンター(オーストラリア)
    • Year and Date
      2010-08-03
    • Related Report
      2010 Annual Research Report
  • [Presentation] High Temperature Flow Behavior of Textured α-Al_2O_3 Polycrystals2010

    • Author(s)
      Koji Morita
    • Organizer
      iib2010
    • Place of Presentation
      志摩観光ホテル(三重県)
    • Year and Date
      2010-06-29
    • Related Report
      2010 Annual Research Report
  • [Presentation] Densification Mechanism of MgAl_2O_4 Spinel during Spark-Plasma-Sintering2010

    • Author(s)
      Koji Morita
    • Organizer
      12th International Ceramics Congress (CIMTEC2010)
    • Place of Presentation
      Montecatini Terme(イタリア)
    • Year and Date
      2010-06-08
    • Related Report
      2010 Annual Research Report
  • [Presentation] 放電プラズマ焼結法により作成したMgO添加透明アルミナ2010

    • Author(s)
      B.-N. Kim, K. Hiraga, K. Morita, H. Yoshida, H. Zhang, J. Lim
    • Organizer
      27th K-J Ceramics Seminar
    • Place of Presentation
      Kurashiki Japan
    • Related Report
      2012 Final Research Report
  • [Presentation] Optimum Spark-Plasma-Sintering (SPS) Condition for Attaining Transparent MgAl2O4 Spinel Polycrystal2010

    • Author(s)
      K. Morita, B.-N. Kim, H. Yoshida, K. Hiraga
    • Organizer
      MSE2010
    • Place of Presentation
      Darmstadt Germany
    • Related Report
      2012 Final Research Report

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Published: 2010-08-23   Modified: 2019-07-29  

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