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Preparation of composition-and valence-controlled BiFeO_3 thin films and investigation of leakage mechanism

Research Project

Project/Area Number 22656075
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeSingle-year Grants
Research Field Electronic materials/Electric materials
Research InstitutionUniversity of Hyogo

Principal Investigator

FUJISAWA Hironori  兵庫県立大学, 大学院・工学研究科, 准教授 (30285340)

Co-Investigator(Renkei-kenkyūsha) SHIMIZU Masaru  兵庫県立大学, 大学院・工学研究科, 教授 (30154305)
NAKASHIMA Seiji  兵庫県立大学, 大学院・工学研究科, 助教 (80552702)
Project Period (FY) 2010 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥3,510,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥210,000)
Fiscal Year 2011: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2010: ¥2,600,000 (Direct Cost: ¥2,600,000)
Keywordsビスマスフェライト / 絶縁性 / リーク電流 / 組成制御 / 価数制御 / BiFeO_3
Research Abstract

We investigated leakage mechanisms in composition-, valence-and domain structure-controlled epitaxial BiFeO_3 thin films prepared by dual ion beam sputtering. The leakage current was controlled by Poole-Frenkel emission independently of the composition ; AFM revealed the presence ofμm-sized local leakage spots with high conductivity. These results suggest that uniformity in composition and a large amount of charged traps can be the origin of a larger leakage than that in Pb-based ferroelectric thin films. Therefore, an improvement in composition uniformity and a decrease in charge traps will be indispensable to reduce the leakage in BiFeO_3 thin films.

Report

(3 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • Research Products

    (28 results)

All 2012 2011 2010

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (22 results)

  • [Journal Article] Growth of High Quality BiFeO_3 Thin Films by Dual Ion Beam Sputtering2011

    • Author(s)
      S. Nakashima, Y. Tsujita, S. Seto, H. Fujisawa, H. Nishioka, M. Kobune, M. Shimizu, J. M. Park, T. Kanashima, and M. Okuyama
    • Journal Title

      IEEE Proc. ISAF/PFM 2011

      Volume: - Pages: 168-171

    • DOI

      10.1109/isaf.2011.6014140

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of Epitaxial BiFeO_3 Thin Films Prepared by Ion Beam Sputtering2011

    • Author(s)
      S.Nakashima, Y.Tsujita, S.Kayahara, H.Fujisawa, J.M.Park, T.Kanashima, M.Okuyama, M.Shimizu
    • Journal Title

      Current Applied Physics

      Volume: 11 Issue: 3 Pages: 2556-2559

    • DOI

      10.1016/j.cap.2010.11.066

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Preparation of BiFeO_3 Thin Films on SrRuO_3/SrTiO_3(001) Substrate by Dual Ion Beam Sputtering Process2011

    • Author(s)
      S.Nakashima, H.Fujisawa, H.Suminaga, J.M.Park, H.Nishioka, M.Kobune, T.Kanashima, M.Okuyama, M.Shimizu
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 50 Issue: 9S2 Pages: 09NB01-09NB01

    • DOI

      10.1143/jjap.50.09nb01

    • Related Report
      2011 Annual Research Report 2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Structural and Ferroelectric Properties of Large c/a Phase Bismuth Ferrite Thin Films Prepared by Ion Beam Sputtering2011

    • Author(s)
      S. Nakashima, Y. Tsujita, H. Fujisawa, J. M. Park, T. Kanashima, M. Okuyama and M. Shimizu
    • Journal Title

      Mater. Res. Soc. Symp. Proc

      Volume: 1292

    • DOI

      10.1557/opl.2011.17

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of Epitaxial BiFeO_3 Thin Films Prepared by Ion Beam Sputtering2011

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Journal Title

      Current Applied Physics

      Volume: (印刷中 未定)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structural and Ferroelectric Properties of Large c/a Phase Bismuth Ferrite Thin Films Prepared by Ion Beam Sputtering2011

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Journal Title

      Mater.Res.Soc.Symp.Proc.

      Volume: 1292(オンラインのため該当無し)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] RFプレーナマグネトロンスパッタ法を用いたエピタキシャルBiFeO_3薄膜の作製2012

    • Author(s)
      高田祐介
    • Organizer
      平成24年(2012)春季第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2012-03-18
    • Related Report
      2011 Annual Research Report
  • [Presentation] デュアルイオンビームスパッタにより作製したBiFeO_3薄膜のドメイン構造と電気的特性2012

    • Author(s)
      中嶋誠二, 辻田陽介, 瀬戸翔太, 藤沢浩訓, 朴正敏, 金島岳, 小舟正文, 奥山雅則, 清水勝
    • Organizer
      第29回強誘電体応用会議講演予稿集
    • Place of Presentation
      コープイン京都
    • Related Report
      2011 Final Research Report
  • [Presentation] デュアルイオンビームスパッタにより作製したノンドープBiFeO_3薄膜のドメイン構造と強誘電ヒステリシスループ2011

    • Author(s)
      中嶋成二
    • Organizer
      第21回日本MRS学術シンポジウム
    • Place of Presentation
      横浜情報文化センター,波止場会館(神奈川県)
    • Year and Date
      2011-12-21
    • Related Report
      2011 Annual Research Report
  • [Presentation] Low Pressure Growth and Fully Saturated Hysteresis Loops of Epitaxial BiFeO_3 Thin Films Prepared by Dual Ion Beam Sputtering2011

    • Author(s)
      S. Nakashima, Y. Tsujita, H. Fujisawa, M. Kobune, H. Nishioka, J. M. Park, T. Kanashima, M. Okuyama and M. Shimizu
    • Organizer
      Mater. Res. Soc.
    • Place of Presentation
      Boston, Massachusetts, U. S. A.
    • Year and Date
      2011-11-30
    • Related Report
      2011 Final Research Report
  • [Presentation] Low Pressure Growth and Fully Saturated Hysteresis Loops of Epitaxial BiFeO_3 Thin Films Prepared by Dual Ion Beam Sputtering2011

    • Author(s)
      H.Fujisawa
    • Organizer
      Mater.Res.Soc.2011 Fall Meeting
    • Place of Presentation
      Boston, USA
    • Year and Date
      2011-11-30
    • Related Report
      2011 Annual Research Report
  • [Presentation] エピタキシャルPbTiO_3薄膜のリーク電流2011

    • Author(s)
      高田祐介
    • Organizer
      平成23年(2011)秋季第72回応用物理学会学術講演会
    • Place of Presentation
      山形大学(山形県)
    • Year and Date
      2011-09-01
    • Related Report
      2011 Annual Research Report
  • [Presentation] デュアルイオンビームスパッタ法を用いたBiFeO_3薄膜の作製(II)2011

    • Author(s)
      辻田陽介
    • Organizer
      平成23年(2011)秋季第72回応用物理学会学術講演会
    • Place of Presentation
      山形大学(山形県)
    • Year and Date
      2011-08-31
    • Related Report
      2011 Annual Research Report
  • [Presentation] STRUCTURAL AND FERROELECTRIC PROPERTIES OF BiFeO_3 THIN FILMS PREPARED BY DUAL ION BEAM SPUTTERING PROCESS2011

    • Author(s)
      S. Nakashima, H. Suminaga, Y. Tsujita, H. Fujisawa, M. Kobune, H. Nishioka, J. M. Park, T. Kanashima, M. Okuyama and M. Shimizu
    • Organizer
      The 20th IEEE International Symposium on Applications of Ferroelectrics/International Symposium on Piezoresponse Force Microscopy & Nanoscale Phenomena in Polar Materials
    • Place of Presentation
      Vancouver, Canada
    • Year and Date
      2011-07-25
    • Related Report
      2011 Final Research Report
  • [Presentation] STRUCTURAL AND FERROELECTRIC PROPERTIES OF BiFeO_3 THIN FILMS PREPARED BY DUAL ION BEAM SPUTTERING PROCESS2011

    • Author(s)
      S.Nakashima
    • Organizer
      Int.Symp.on Piezoresponse Force Microscopy & Nanoscale Phenomena in Polar Materials
    • Place of Presentation
      Vancouver, Canada
    • Year and Date
      2011-07-25
    • Related Report
      2011 Annual Research Report
  • [Presentation] デュアルイオンビームスパッタを用いたSrRuO_3/SrTiO_3基板上へのBiFeO_3薄膜の作製2011

    • Author(s)
      中嶋誠二, 住永寛幸, 辻田陽介, 藤沢浩訓, 小舟正文, 清水正文, 清水勝, 朴正敏, 金島岳, 奥山雅則
    • Organizer
      第28回強誘電体応用会議講演予稿集
    • Place of Presentation
      コープイン京都
    • Year and Date
      2011-05-27
    • Related Report
      2011 Final Research Report
  • [Presentation] デュアルイオンビームスパッタを用いたSrRuO_3/SrTiO_3基板上へのBiFeO_3薄膜の作製2011

    • Author(s)
      中嶋誠二
    • Organizer
      第28回強誘電体応用会議
    • Place of Presentation
      コープイン京都(京都府)
    • Year and Date
      2011-05-27
    • Related Report
      2011 Annual Research Report
  • [Presentation] デュアルイオンビームスパッタ法を用いたBiFeO_3薄膜の作製2011

    • Author(s)
      中嶋誠二, 藤沢浩訓, 他
    • Organizer
      平成23年春季第58回応用物理学関係連合講演会
    • Place of Presentation
      (講演予稿集DVD (震災のため講演会中止))
    • Year and Date
      2011-03-09
    • Related Report
      2010 Annual Research Report
  • [Presentation] SrRuO_3/SrTiO_3(100)上に作成した大きなc/a比を有するBiFeO_3薄膜の特性評価2010

    • Author(s)
      中嶋誠二, 藤沢浩訓, 他
    • Organizer
      第20回日本MRS学術シンポジウム
    • Place of Presentation
      横浜市開港記念会館・神奈川県
    • Year and Date
      2010-12-20
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structural and Ferroelectric Properties of Large c/a Phase Bismuth Ferrite Thin Films Prepared by Ion Beam Sputtering2010

    • Author(s)
      S. Nakashima, Y. Tsujita, H. Fujisawa, J. M. Park, T. Kanashima, M. Okuyama and M. Shimizu
    • Organizer
      Mater. Res. Soc
    • Place of Presentation
      Boston, Massachusetts, U. S. A.
    • Year and Date
      2010-11-29
    • Related Report
      2011 Final Research Report
  • [Presentation] Structural and Ferroelectric Properties of Large c/a Phase Bismuth Ferrite Thin Films Prepared by Ion Beam Sputtering2010

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Organizer
      Mater.Res.Soc.2010 Fall Meeting
    • Place of Presentation
      Hynes Convention Center・米国
    • Year and Date
      2010-11-29
    • Related Report
      2010 Annual Research Report
  • [Presentation] Characterization of Bismuth Ferrite Thin Films with Large c/a Axial Ratio Prepared by Ion Beam Sputtering2010

    • Author(s)
      S. Nakashima, Y. Tsujita, H. Fujisawa, M. Shimizu, J. M. Park, and T. Kanashima, and M. Okuyama
    • Organizer
      The 17th Workshop on Oxide Electronics
    • Place of Presentation
      Awaji Yume Butai, Japan
    • Year and Date
      2010-09-21
    • Related Report
      2011 Final Research Report
  • [Presentation] Characterization of Bismuth Ferrite Thin Films with Large c/a Axial Ratio Prepared by Ion Beam Sputtering2010

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Organizer
      The 17th Workshop on Oxide Electronics
    • Place of Presentation
      淡路夢舞台・兵庫県
    • Year and Date
      2010-09-21
    • Related Report
      2010 Annual Research Report
  • [Presentation] イオンビームスパッタ法を用いたBiFeO_3薄膜の作製とその評価(II)2010

    • Author(s)
      辻田陽介, 藤沢浩訓, 他
    • Organizer
      平成22年秋季第71回応用物理学会学術講演会
    • Place of Presentation
      長崎大学・長崎県
    • Year and Date
      2010-09-15
    • Related Report
      2010 Annual Research Report
  • [Presentation] Ferroelectric Properties of Epitaxial BiFeO_3 Thin Films Deposited by Ion Beam Sputtering2010

    • Author(s)
      Y. Tsujita, S. Nakashima, H. Fujisawa, J. M. Park, T. Kanashima, M. Okuyama and M. Shimizu
    • Organizer
      Japan-Korea Conference on Ferroelectrics(JKC-FE08)
    • Place of Presentation
      Himeji, Japan
    • Year and Date
      2010-08-05
    • Related Report
      2011 Final Research Report
  • [Presentation] Ferroelectric Properties of Epitaxial BiFeO_3 Thin Films Deposited by Ion Beam Sputtering2010

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Organizer
      The 8th Japan-Korea Conference on Ferroelectrics
    • Place of Presentation
      イーグレ姫路・兵庫県
    • Year and Date
      2010-08-05
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structural and Ferroelectric Properties of BiFeO_3 Thin Films Prepared by Ion Beam Sputtering Process2010

    • Author(s)
      S. Nakashima, Y. Tsujita, S. Kayahara, H. Fujisawa, J. M. Park, T. Kanashima, M. Okuyama, and M. Shimizu
    • Organizer
      The 7th Asian Meeting on Ferroelectricity and the 7th Asian Meeting on Electro Ceramics(AMF-AMEC-2010)
    • Place of Presentation
      Cheju, Korea
    • Year and Date
      2010-07-01
    • Related Report
      2011 Final Research Report
  • [Presentation] Structural and Ferroelectric Properties of BiFeO_3 Thin Films Prepared by Ion Beam Sputtering Process2010

    • Author(s)
      S.Nakashima, H.Fujisawa, et al.
    • Organizer
      The 7th Asian Meeting on Ferroelectricity and the 7th Asian Meeting on ElectroCeramics
    • Place of Presentation
      Ramada Plaza Jeju Hotel・韓国
    • Year and Date
      2010-07-01
    • Related Report
      2010 Annual Research Report

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Published: 2010-08-23   Modified: 2016-04-21  

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